Alexios Beveratos, Sergei Kuehn, Rosa Brouri, Thierry Gacoin, Jean-Philippe Poizat, Philippe Grangier
备注：
7 pages, 10 figures, accepted to the special issue of the European Physical Journal D on "Quantum interference and cryptographic keys: novel physics and advancing technologies", proceedings of the conference QUICK 2001
We report on the realization of a stable solid state room temperature source for single photons. It is based on the fluorescence of a single nitrogen-vacancy (NV) color center in a diamond nanocrystal. Antibunching has been observed in the fluorescence light under both continuous and pulsed excitation. Our source delivers 2*10^4 single-photon pulses per second at an excitation repetition rate of 10 MHz. The number of two-photon pulses is reduced by a factor of five compared to strongly attenuated coherent sources.
We describe an efficient surface-passivated photonic crystal nanocavity laser, demonstrating room-temperature operation with 3-ps total pulse duration (detector response limited) and low-temperature operation with ultra-low-threshold near 9uW.
Single photon emitters are indispensable to photonic quantum technologies. Here we demonstrate waveform-controlled high-purity single photons from room-temperature colloidal quantum dots. The purity of the single photons does not vary with the excitation power, thereby allowing the generation rate to be increased without compromising the single-photon quality.
Quantum Key Distribution (QKD) allows the distribution of cryptographic keys between multiple users in an information-theoretic secure way, exploiting quantum physics. While current QKD systems are mainly based on attenuated laser pulses, deterministic single-photon sources could give concrete advantages in terms of secret key rate (SKR) and security owing to the negligible probability of multi-photon events. Here, we introduce and demonstrate a proof-of-concept QKD system exploiting a molecule-based single-photon source operating at room temperature and emitting at 785nm. With an estimated SK…
We report experimental generation of non-classically correlated photon pairs from collective emission in a room-temperature atomic vapor cell. The nonclassical feature of the emission is demonstrated by observing a violation of the Cauchy-Schwarz inequality. Each pair of correlated photons are separated by a controllable time delay up to 2 microseconds. This experiment demonstrates an important step towards the realization of the Duan-Lukin-Cirac-Zoller scheme for scalable long-distance quantum communication.
We report room temperature operation of telecom wavelength single-photon detectors for high bit rate quantum key distribution (QKD). Room temperature operation is achieved using InGaAs avalanche photodiodes integrated with electronics based on the self-differencing technique that increases avalanche discrimination sensitivity. Despite using room temperature detectors, we demonstrate QKD with record secure bit rates over a range of fiber lengths (e.g. 1.26 Mbit/s over 50 km). Furthermore, our results indicate that operating the detectors at room temperature increases the secure bit rate for sho…
Non-classical photon sources are a crucial resource for distributed quantum networks. Photons generated from matter systems with memory capability are particularly promising, as they can be integrated into a network where each source is used on-demand. Among all kinds of solid state and atomic quantum memories, room-temperature atomic vapours are especially attractive due to their robustness and potential scalability. To-date room-temperature photon sources have been limited either in their memory time or the purity of the photonic state. Here we demonstrate a single-photon source based on roo…
We study the average coincidence-count signal at the output of a two-mode squeezing device with $|N\rangle\otimes|α\rangle$ as the two input modes. We show that the input photon-number can be resolved from the average coincidence counts. In particular, we show jumps in the average coincidence-count signal as a function of input photon-number $N$. Therefore, we propose that such a device may be deployed as photon-number-resolving detector at room temperature with high efficiency.
Quantum memories capable of storing single photons are essential building blocks for quantum information processing, enabling the storage and transfer of quantum information over long distances. Devices operating at room temperature can be deployed on a large scale and integrated into existing photonic networks, but so far warm quantum memories have been susceptible to noise at the single photon level. This problem is circumvented in cold atomic ensembles, but these are bulky and technically complex. Here we demonstrate controllable, broadband and efficient storage and retrieval of weak cohere…
We report the realization of a solid-state triggered single-photon source with narrow emission in the near infrared at room temperature. It is based on the photoluminescence of a single nickel-nitrogen NE8 colour centre in a chemical vapour deposited diamond nanocrystal. Stable single-photon emission has been observed in the photoluminescence under both continuous-wave and pulsed excitations. The realization of this source represents a step forward in the application of diamond-based single-photon sources to Quantum Key Distribution (QKD) under practical operating conditions.
Photon number resolving monitoring is a practical light source monitoring scheme in QKD systems, which reduces the impacts from untrusted sources effectively. This scheme requires a single photon detector, normally working at low temperature to suppress its dark count rate. In this paper, we use a room-temperature detector and show that the dark count rate is irrelevant to the monitoring performance in our scheme, which can sufficiently relax requirements on the detector's working conditions as well as integration complexity, and this would be highly demanded for practical systems. Furthermore…
We experimentally demonstrate an integrated semiconductor ridge microcavity source of counterpropagating twin photons at room temperature in the telecom range. Based on parametric down conversion with a counterpropagating phase-matching, pump photons generate photon pairs with an efficiency of about 10^(-11) and a spectral linewidth of 0.3 nm for a 1mm long sample. The indistiguishability of the photons of the pair are measured via a two-photon interference experiment showing a visibility of 85%. This work opens a route towards new guided-wave semiconductor quantum devices.
Single-photon sources with high brightness and long coherence time are promising qubit candidates for quantum technology. To this end, interfacing emitters with high-finesse cavities is required, especially in the strong coupling regime, which so far has only been limited to cryogenic temperatures. Here, we experimentally demonstrate, at room temperature, strong coupling between a single photon emitter and a novel cavity based on optical bound states in the continuum. A remarkably large Rabi splitting of ~4 meV is achieved thanks to the combination of the narrow linewidth and large oscillator …
Photonics is a promising platform for quantum technologies. However, photon sources and two-photon gates currently only operate probabilistically. Large-scale photonic processing will therefore be impossible without a multiplexing strategy to actively select successful events. High time-bandwidth-product quantum memories - devices that store and retrieve single photons on-demand - provide an efficient remedy via active synchronisation. Here we interface a GHz-bandwidth heralded single-photon source and a room-temperature Raman memory with a time-bandwidth product exceeding 1000. We store heral…
We report the storage and retrieval of single photons, via a quantum memory, in the optical phonons of room-temperature bulk diamond. The THz-bandwidth heralded photons are generated by spontaneous parametric downconversion and mapped to phonons via a Raman transition, stored for a variable delay, and released on demand. The second-order correlation of the memory output is $g^{(2)}(0) = 0.65 \pm 0.07$, demonstrating preservation of non-classical photon statistics throughout storage and retrieval. The memory is low-noise, high-speed and broadly tunable; it therefore promises to be a versatile l…
The development of useful photon-photon interactions can trigger numerous breakthroughs in quantum information science, however this has remained a considerable challenge spanning several decades. Here we demonstrate the first room-temperature implementation of large phase shifts ($\approxπ$) on a single-photon level probe pulse (1.5us) triggered by a simultaneously-propagating few-photon-level signal field. This process is mediated by $Rb^{87}$ vapor in a double-$Λ$ atomic configuration. We use homodyne tomography to obtain the quadrature statistics of the phase-shifted quantum fields and per…
Future quantum photonic networks require coherent optical memories for synchronizing quantum sources and gates of probabilistic nature. We demonstrate a fast ladder memory (FLAME) mapping the optical field onto the superposition between electronic orbitals of rubidium vapor. Employing a ladder level-system of orbital transitions with nearly degenerate frequencies simultaneously enables high bandwidth, low noise, and long memory lifetime. We store and retrieve 1.7-ns-long pulses, containing 0.5 photons on average, and observe short-time external efficiency of 25%, memory lifetime (${1/e}$) of 8…
Large dynamic range room temperature photon number resolving (PNR) detectors can be very useful for measuring very low light intensities and for analyzing multiphoton quantum states. In this paper we present a PNR detector based on the up-conversion (UC) of telecom signal into visible wavelength and on its detection by a thermoelectrically cooled multi-pixel silicon avalanche photodiodode (APD), also known as Silicon Photon Multiplier (SiPM). An efficiency of 4% is attained and the poissonian statistics of input coherent states is maintained up to approximately 20 simultaneous detections. The …
Recent progress in nonlinear optical materials and microresonators has brought quantum computing with bulk optical nonlinearities into the realm of possibility. This platform is of great interest, not only because photonics is an obvious choice for quantum networks, but also because it may be the only feasible route to quantum information processing at room temperature. We introduce a paradigm for room-temperature photonic quantum logic that significantly simplifies the realization of various quantum circuits, and in particular, of error correction. It uses only the strongest available bulk no…
Nitrogen-vacancy (NV) centres in diamond are appealing nano-scale quantum sensors for temperature, strain, electric fields and, most notably, for magnetic fields. However, the cryogenic temperatures required for low-noise single-shot readout that have enabled the most sensitive NV-magnetometry reported to date, are impractical for key applications, e.g. biological sensing. Overcoming the noisy readout at room-temperature has until now demanded repeated collection of fluorescent photons, which increases the time-cost of the procedure thus reducing its sensitivity. Here we show how machine learn…
Efficient quantum memories will be an essential building block of large scale networked quantum systems and provide a link between flying photonic qubits and atomic or quasi-atomic local quantum processors. To provide a path to scalability avoidance of bulky, difficult to maintain systems such as high vacuum and low temperature cryogenics is imperative. Memory efficiencies above 50% are required to be operating above the quantum no-cloning limit. Such high efficiencies have only been achieved in systems with photon sources tailored to the memory bandwidth. In this paper we explore the combinat…
Quantum interfaces between photons and ensembles of atoms have emerged as powerful tools for quantum technologies. A major objective for such interfaces is high fidelity storage and retrieval of a photon in a collective quantum state of many atoms. This requires long-lived collective superposition states, which is typically achieved with immobilized atoms. Thermal atomic vapors, which present a simple and scalable resource, have, so far, only been used for continuous variable processing or for discrete variable processing on short time scales where atomic motion is negligible. We develop a the…
We report on a compact, simple and robust high brightness entangled photon source at room temperature. Based on a 30 mm long periodically poled potassium titanyl phosphate (PPKTP), the source produces non-collinear, type0 phase matched, degenerate photons at 810 nm with pair production rate as high 39.13 MHz per mW at room temperature. To the best of our knowledge, this is the highest photon pair rate generated using bulk crystals pump with continuous-wave laser. Combined with the inherently stable polarization Sagnac interferometer, the source produces entangled state violating the Bells ineq…
High-purity single photon sources (SPS) that can operate at room temperature are highly desirable for a myriad of applications, including quantum photonics and quantum key distribution. In this work, we realise an ultra-bright solid-state SPS based on an atomic defect in hexagonal boron nitride (hBN) integrated with a solid immersion lens (SIL). The SIL increases the source efficiency by a factor of six, and the integrated system is capable of producing over ten million single photons per second at room temperature. Our results are promising for practical applications of SPS in quantum communi…
Room-temperature (RT), on-chip deterministic generation of indistinguishable photons coupled to photonic integrated circuits is key for quantum photonic applications. Nevertheless, high indistinguishability (I) at RT is difficult to obtain due to the intrinsic dephasing of most deterministic single-photon sources (SPS). Here we present a numerical demonstration of the design and optimization of a hybrid slot-Bragg nanophotonic cavity that achieves theoretical near-unity I and high coupling efficiency (\b{eta}) at RT for a variety of singlephoton emitters. Our numerical simulations predict moda…
We present an optimal protocol to implement a room temperature Rydberg single photon source within an experimental setup based on micro cells filled with thermal vapor. The optimization of a pulsed four wave mixing scheme allows to double the effective Rydberg blockade radius as compared to a simple Gaussian pulse scheme, releasing some of the constrains on the geometry of the micro cells. The performance of the optimized protocol is improved by about 70% with respect to the standard protocol.
We experimentally demonstrate a real-time quantum random number generator by using a room-temperature single-photon emitter from the defect in a commercial gallium nitride wafer. Thanks to the brightness of our single photon emitter, the raw bit generation rate is ~1.8 MHz, and the unbiased bit generation rate is ~420 kHz after von Neumann's randomness extraction procedure. Our results show that commercial gallium nitride wafer has great potential for the development of integrated high-speed quantum random number generator devices.
The control of quantum correlations in solid state systems by means of material engineering is a broad avenue to be explored, since it makes possible steps toward the limits of quantum mechanics and the design of novel materials with applications on emerging quantum technologies. In this context, this Letter explores the potential of molecular magnets to be prototypes of materials for quantum information technology. More precisely, we engineered a material and from its geometric quantum discord we found significant quantum correlations up to 9540 K (even without entanglement); and, in addition…
In quantum optics, orbital angular momentum (OAM) is very promising to achieve high-dimensional quantum states due to the nature of infinite and discrete eigenvalue, which is quantized by the topological charge of l. Here, a heralded single-photon source with switchable OAM modes is proposed and demonstrated on silicon chip. At room-temperature, the heralded single photons with 11 OAM modes (l=2~6, -6~-1) have been successfully generated and switched through thermo-optical effect. We believe that such an integrated quantum source with multiple OAM modes and operating at room-temperature would …
We present and analyze a gated single photon avalanche detector using a sine gating scheme with a simple but effective low-pass filtering technique for fast low-noise single photon detection at telecom wavelength. The detector is characterized by 130 ps short gates applied with a frequency of 1.25 GHz, yields only 70 ps timing jitter and noise probabilities as low as 7E-7 per gate at 10% detection efficiency. We show that the detector is suitable for high rate quantum key distribution (QKD) and even at room temperature it could allow for QKD over distances larger than 25 km.
Single photon emitters (SPEs) are critical building blocks needed for quantum science and technology. For practical applications, large-scale room-temperature solid-state platforms are required. Color centers in layered hexagonal boron nitride (hBN) have recently been found to be ultra-bright and stable SPEs at room temperature. Yet, to scale up solid-state quantum information processing, large tuning range of single photon energy is demanded for wavelength division multiplexing quantum key distribution, where indistinguishability is not required, and for indistinguishable single-photon produc…
Heralded single-photon sources with on-demand readout are promising candidates for quantum repeaters enabling long-distance quantum communication. The need for scalability of such systems requires simple experimental solutions, thus favouring room-temperature systems. For quantum repeater applications, long delays between heralding and single-photon readout are crucial. Until now, this has been prevented in room-temperature atomic systems by fast decoherence due to thermal motion. Here we demonstrate efficient heralding and readout of single collective excitations created in warm caesium vapou…
We propose a compact high-intensity room-temperature source of entangled photons based on the efficient second-order process of two-photon spontaneous emission from electrically-pumped semiconductor quantum wells in a photonic microcavity. Two-photon emission rate in room-temperature semiconductor devices is determined solely by the carrier density, regardless of the residual one-photon emission. The microcavity selects two-photon emission for a specific signal and idler wavelengths and at a preferred direction without modifying the overall rate. Pair-generation rate in GaAs/AlGaAs quantum wel…
We propose a quantum repeater architecture that can operate under ambient conditions. Our proposal builds on recent progress towards non-cryogenic spin-photon interfaces based on nitrogen-vacancy centers, which have excellent spin coherence times even at room temperature, and optomechanics, which allows to avoid phonon-related decoherence and also allows the emitted photons to be in the telecom band. We apply the photon number decomposition method to quantify the fidelity and the efficiency of entanglement established between two remote electron spins. We describe how the entanglement can be s…
Narrowband single photons that couple well to atomic ensembles could prove essential for future quantum networks, but the efficient generation of such photons remains an outstanding challenge. We realize a spatially-multiplexed heralded source of single photons that are inherently compatible with the commonly employed D2 line of rubidium. Our source is based on four-wave mixing in hot rubidium vapor, requiring no laser cooling or optical cavities, and generates single photons with high rate and low noise. We use Hong-Ou-Mandel interference to verify the indistinguishability of the photons gene…
We describe a general analytical framework of a nanoplasmonic cavity-emitter system interacting with a dielectric photonic waveguide. Taking into account emitter quenching and dephasing, our model directly reveals the single photon extraction efficiency, $η$, as well as the indistinguishability, $I$, of photons coupled into the waveguide mode. Rather than minimizing the cavity modal volume, our analysis predicts an optimum modal volume to maximize $η$ that balances waveguide coupling and spontaneous emission rate enhancement. Surprisingly, our model predicts that near-unity indistinguishabilit…
We demonstrate the coupling of PbS quantum dot emission to photonic crystal cavities at room temperature. The cavities are defined in 33% Al, AlGaAs membranes on top of oxidized AlAs. Quantum dots were dissolved in Poly-methyl-methacrylate (PMMA) and spun on top of the cavities. Quantum dot emission is shown to map out the structure resonances, and may prove to be viable sources for room temperature cavity coupled single photon generation for quantum information processing applications. These results also indicate that such commercially available quantum dots can be used for passive structure …
We report on the control of the spontaneous emission dynamics from InAsP self-assembled quantum dots emitting in the telecommunications C-band and weakly coupled to the mode of a double heterostructure cavity etched on a suspended InP membrane at room temperature. The quality factor of the cavity mode is 44x10^3 with an ultra-low modal volume of the order of 1.2 lambda/n)^3, inducing an enhancement of the spontaneous emission rate of up a factor of 2.8 at 300 K.
We investigate the optical properties of Dibenzoterrylene (DBT) molecules in a spin-coated crystalline film of anthracence. By performing single molecule studies, we show that the dipole moments of the DBT molecules are oriented parallel to the plane of the film. Despite a film thickness of only 20 nm, we observe an exceptional photostability at room temperature and photon count rates around one million per second from a single molecule. These properties together with an emission wavelength around 800 nm make this system attractive for applications in nanophotonics and quantum optics.
One of the main challenges for future quantum information technologies is miniaturization and integration of high performance components in a single chip. In this context, electrically driven sources of non-classical states of light have a clear advantage over optically driven ones. Here we demonstrate the first electrically driven semiconductor source of photon pairs working at room temperature and telecom wavelength. The device is based on type-II intracavity Spontaneous Parametric Down-Conversion in an AlGaAs laser diode and generates pairs at 1.57 $μ$m. Time-correlation measurements of the…
Single-photon emitters are essential for enabling several emerging applications in quantum information technology, quantum sensing and quantum communication. Scalable photonic platforms capable of hosting intrinsic or directly embedded sources of single-photon emission are of particular interest for the realization of integrated quantum photonic circuits. Here, we report on the first-time observation of room-temperature single-photon emitters in silicon nitride (SiN) films grown on silicon dioxide substrates. As SiN has recently emerged as one of the most promising materials for integrated qua…
Highly efficient sources of indistinguishable single photons that can operate at room temperature would be very beneficial for many applications in quantum technology. We show that the implementation of such sources is a realistic goal using solid-state emitters and ultrasmall mode volume cavities. We derive and analyze an expression for photon indistinguishability that accounts for relevant detrimental effects, such as plasmon-induced quenching and pure-dephasing. We then provide the general cavity and emitter conditions required to achieve efficient indistinguishable photon emission, and als…
