Efficient synchronization of single photons that are compatible with narrowband atomic transitions is an outstanding challenge, which could prove essential for photonic quantum information processing. Here we report on the synchronization of independently-generated single photons using a room-temperature atomic quantum memory. The photon source and the memory are interconnected by fibers and employ the same ladder-level atomic scheme. We store and retrieve the heralded single photons with end-to-end efficiency of $η_\text{e2e}=25\%$ and final anti-bunching of $g^{(2)}_\text{h}=0.023$. Our synchronization process results in over tenfold increase in the photon-pair coincidence rate, reaching a rate of more than $1000$ detected synchronized photon pairs per second. The indistinguishability of the synchronized photons is verified by a Hong-Ou-Mandel interference measurement.
Phase synchronization refers to a kind of collective phenomenon that the phase difference between two or more systems is locked, and it has widely been investigated between systems with the identical physical properties, such as the synchronization between mechanical oscillators and the synchronization between atomic ensembles. Here, we investigate the synchronization behavior between the mechanical oscillator and the atomic ensemble, the systems with different physical properties, and observe a novel synchronization phenomenon, i.e., the phase sum, instead of phase difference, is locked. We r…
Synchronization phenomena have been recently reported in the quantum realm at atomic level due to collective dissipation. In this work we propose a dimer lattice of trapped atoms realizing a dissipative spin model where quantum synchronization occurs instead in presence of local dissipation. Atoms synchronization is enabled by the inhomogeneity of staggered local losses in the lattice and is favored by an increase of spins detuning. A comprehensive approach to quantum synchronization based on different measures considered in the literature allows to identify the main features of different sync…
Future quantum photonic networks require coherent optical memories for synchronizing quantum sources and gates of probabilistic nature. We demonstrate a fast ladder memory (FLAME) mapping the optical field onto the superposition between electronic orbitals of rubidium vapor. Employing a ladder level-system of orbital transitions with nearly degenerate frequencies simultaneously enables high bandwidth, low noise, and long memory lifetime. We store and retrieve 1.7-ns-long pulses, containing 0.5 photons on average, and observe short-time external efficiency of 25%, memory lifetime (${1/e}$) of 8…
Large-scale array of squeezed light and synchronization using atomic vapor
Fudan University（复旦大学）；Shanghai Institute of Technical Physics, Chinese Academy of Sciences（中国科学院上海技术物理研究所）；Weizmann Institute of Science（魏茨曼科学研究所）；Shanxi University（山西大学）
A clock steps a computer through a cycle of phases. For the propagation of logical symbols from one computer to another, each computer must mesh its phases with arrivals of symbols from other computers. Even the best atomic clocks drift unforeseeably in frequency and phase; feedback steers them toward aiming points that depend on a chosen wave function and on hypotheses about signal propagation. A wave function, always under-determined by evidence, requires a guess. Guessed wave functions are coded into computers that steer atomic clocks in frequency and position---clocks that step computers t…
Experiments have reported the entanglement of two spatially separated macroscopic atomic ensembles at room temperature (Krauter et al 2011 Phys. Rev. Lett. 107 080503; Julsgaard et al 2001 Nature 413 400). We show how an Einstein-Podolsky-Rosen (EPR) paradox is realizable with this experiment. Our proposed test involves violation of an inferred Heisenberg uncertainty principle, which is a sufficient condition for an EPR paradox. This is a stronger test of nonlocality than entanglement. Our proposal would enable the first definitive confirmation of quantum EPR paradox correlations between two m…
Superradiant lasers based on atomic ensembles exhibiting ultra-narrow optical transitions can emit light of unprecedented spectral purity and may serve as active atomic clocks. We consider two frequency-detuned active atomic clocks, which are coupled in a cascaded setup, i.e. as master & slave lasers, and study the synchronization of the slave to the master clock. In a setup where both atomic ensembles are coupled to a common cavity mode such synchronization phenomena have been predicted by Xu et al. [Phys. Rev. Lett. 113, 154101 (2014)] and experimentally observed by Weiner et al. [arXiv:1503…
We analyse a novel squeezing and entangling mechanism which is due to correlated Stokes and anti-Stokes photon forward scattering in a multi-level atom vapour. Following the proposal we present an experimental demonstration of 3.5 dB pulsed frequency nondegenerate squeezed (quadrature entangled) state of light using room temperature caesium vapour. The source is very robust and requires only a few milliwatts of laser power. The squeezed state is generated in the same spatial mode as the local oscillator and in a single temporal mode. The two entangled modes are separated by twice the Zeeman fr…
We study the time evolution of two coupled many-body quantum systems one of which is assumed to be Bose condensed. Specifically, we consider two ultracold atomic clouds populating each two localized single-particle states, i.e. a two-component Bosonic Josephson junction. The cold atoms cloud can retain its coherence when coupled to the condensate and displays synchronization with the latter, differing from usual entrainment. We term this effect among the ultracold and the condensed clouds as {\it hybrid synchronization}. The onset of synchronization, which we observe in the evolution of averag…
We predict synchronization of the chaotic dynamics of two atomic ensembles coupled to a heavily damped optical cavity mode. The atoms are dissipated collectively through this mode and pumped incoherently to achieve a macroscopic population of the cavity photons. Even though the dynamics of each ensemble are chaotic, their motions repeat one another. In our system, chaos first emerges via quasiperiodicity and then synchronizes. We identify the signatures of synchronized chaos, chaos, and quasiperiodicity in the experimentally observable power spectra of the light emitted by the cavity.
We present an experimental demonstration of the Hamiltonian manipulation in light-atom interface in Raman-type warm rubidium-87 vapor atomic memory. By adjusting the detuning of the driving beam we varied the relative contributions of the Stokes and anti-Stokes scattering to the process of four-wave mixing which reads out a spatially multimode state of atomic memory. We measured the temporal evolution of the readout fields and the spatial intensity correlations between write-in and readout as a function of detuning with the use of an intensified camera. The correlation maps enabled us to resol…
Advanced quantum technologies, such as quantum simulation, computation, and metrology are thriving for the implementation of large-scale configurations of identical quantum systems. Sets of atoms and molecules have the advantage of having identical intrinsic properties but need to be placed in identical environments as well. In this work, we present a strong suppression of dephasing effects and a significant increase of the coherence time for ensembles of neutral atoms in arrays of optical traps. Compensation of the differential Stark shift caused by the optical trapping potential is achieved …
Distributed g(2) Retrieval with Atomic Clocks: Eliminating Conventional Sync Protocols
Department of Physics & Astronomy, University of Tennessee, Knoxville（田纳西大学诺克斯维尔分校物理与天文学系）；Department of Physics & Astronomy, University of Tennessee, Chattanooga（田纳西大学查塔努加分校物理与天文学系）；UTC Quantum Center, University of Tennessee, Chattanooga（田纳西大学查塔努加分校UTC量子中心）
We report on the use of parametric excitation to coherently manipulate the collective spin state of an atomic vapour at room temperature. Signatures of the parametric excitation are detected in the ground-state spin evolution. These include the excitation spectrum of the atomic coherences, which contains resonances at frequencies characteristic of the parametric process. The amplitudes of the signal quadratures show amplification and attenuation, and their noise distribution is characterized by a strong asymmetry, similarly to those observed in mechanical oscillators. The parametric excitation…
Quantum memories capable of storing single photons are essential building blocks for quantum information processing, enabling the storage and transfer of quantum information over long distances. Devices operating at room temperature can be deployed on a large scale and integrated into existing photonic networks, but so far warm quantum memories have been susceptible to noise at the single photon level. This problem is circumvented in cold atomic ensembles, but these are bulky and technically complex. Here we demonstrate controllable, broadband and efficient storage and retrieval of weak cohere…
We report the experimental observation of Coherent Population Oscillation (CPO) based light storage in an atomic vapor cell at room temperature. Using the ultranarrow CPO between the ground levels of a $Λ$ system selected by polarization in metastable $^4$He, such a light storage is experimentally shown to be phase preserving. As it does not involve any atomic coherences it has the advantage of being robust to dephasing effects such as small magnetic field inhomogeneities. The storage time is limited by the population lifetime of the ground states of the $Λ$ system.
We demonstrate coherent storage and retrieval of pulsed light using the atomic frequency comb quantum memory protocol in a room temperature alkali vapour. We utilise velocity-selective optical pumping to prepare multiple velocity classes in the $F=4$ hyperfine ground state of caesium. The frequency spacing of the classes is chosen to coincide with the $F'=4 - F'=5$ hyperfine splitting of the $6^2$P$_{3/2}$ excited state resulting in a broadband periodic absorbing structure consisting of two usually Doppler-broadened optical transitions. Weak coherent states of duration $2\,\mathrm{ns}$ are map…
We sense the motion of a trapped atomic ion using a sequence of state-dependent ultrafast momentum kicks. We use this atom interferometer to characterize a nearly-pure quantum state with $n=1$ phonon and accurately measure thermal states ranging from near the zero-point energy to $\bar{n}\sim 10^4$, with the possibility of extending at least 100 times higher in energy. The complete energy range of this method spans from the ground state to far outside of the Lamb-Dicke regime, where atomic motion is greater than the optical wavelength. Apart from thermometry, these interferometric techniques a…
The Stark shift due to blackbody radiation (BBR) is the key factor limiting the performance of many atomic frequency standards, with the BBR environment inside the clock apparatus being difficult to characterize at a high level of precision. Here we demonstrate an in-vacuum radiation shield that furnishes a uniform, well-characterized BBR environment for the atoms in an ytterbium optical lattice clock. Operated at room temperature, this shield enables specification of the BBR environment to a corresponding fractional clock uncertainty contribution of $5.5 \times 10^{-19}$. Combined with uncert…
Establishing quantum entanglement between individual nodes is crucial for building large-scale quantum networks, enabling secure quantum communication, distributed quantum computing, enhanced quantum metrology and fundamental tests of quantum mechanics. However, the shared entanglements have been merely observed in either extremely low-temperature or well-isolated systems, which limits the quantum networks for the real-life applications. Here, we report the realization of heralding quantum entanglement between two atomic ensembles at room temperature, where each of them contains billions of mo…
We analyse the dynamics leading to radiative cooling of an atomic ensemble confined inside an optical cavity when the atomic dipolar transitions are incoherently pumped and can synchronize. Our study is performed in the semiclassical regime and assumes that cavity decay is the largest rate in the system dynamics. We identify three regimes characterising the cooling. At first hot atoms are individually cooled by the cavity friction forces. After this stage, the atoms' center-of-mass motion is further cooled by the coupling to the internal degrees of freedom while the dipoles synchronize. In the…
Efficient quantum memories will be an essential building block of large scale networked quantum systems and provide a link between flying photonic qubits and atomic or quasi-atomic local quantum processors. To provide a path to scalability avoidance of bulky, difficult to maintain systems such as high vacuum and low temperature cryogenics is imperative. Memory efficiencies above 50% are required to be operating above the quantum no-cloning limit. Such high efficiencies have only been achieved in systems with photon sources tailored to the memory bandwidth. In this paper we explore the combinat…
We analyze the origin and properties of the chaotic dynamics of two atomic ensembles in a driven-dissipative experimental setup, where they are collectively damped by a bad cavity mode and incoherently pumped by a Raman laser. Starting from the mean-field equations, we explain the emergence of chaos by way of quasiperiodicity -- presence of two or more incommensurate frequencies. This is known as the Ruelle-Takens-Newhouse route to chaos. The equations of motion have a $\mathbb{Z}_{2}$-symmetry with respect to the interchange of the two ensembles. However, some of the attractors of these equat…
Non-classical photon sources are a crucial resource for distributed quantum networks. Photons generated from matter systems with memory capability are particularly promising, as they can be integrated into a network where each source is used on-demand. Among all kinds of solid state and atomic quantum memories, room-temperature atomic vapours are especially attractive due to their robustness and potential scalability. To-date room-temperature photon sources have been limited either in their memory time or the purity of the photonic state. Here we demonstrate a single-photon source based on roo…
Here we show an ultra-low noise regime of operation in a simple quantum memory in warm Rb atomic vapor. By modelling the quantum dynamics of four-level room temperature atoms, we achieve fidelities >90% for single-photon level polarization qubits, clearly surpassing any classical strategy exploiting the non-unitary memory efficiency. This is the first time such important threshold has been crossed with a room temperature device. Additionally we also show novel experimental techniques capable of producing fidelities close to unity. Our results demonstrate the potential of simple, resource-moder…
Light storage, the controlled and reversible mapping of photons onto long-lived states of matter [1], enables memory capability in optical quantum networks [2-6]. Prominent storage media are warm alkali gases due to their strong optical coupling and long-lived spin states [7,8]. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds [9,10]. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. Th…
We consider the single photon transistor in coupled cavity system of resonators interacting with multilevel superconducting artificial atom simultaneously. Effective single mode transformation is used for the diagonalization of the the hamiltonian and impedance matching in terms of the normal modes. Storage and transmission of the incident field are described by the interactions between the cavities controlling the atomic transitions of lowest lying states. Rabi splitting of vacuum induced multiphoton transitions is considered in input/output relations by the quadrature operators in the absenc…
Two-dimensional transition metal di-chalcogenide semiconductors provide unique possibilities to investigate strongly confined excitonic physics and a plasmonic platform integrable to such materials constitutes a hybrid system that can be of interest to enable manipulation of their cumulative optical properties. Here we report tuning of excitonic emission from monolayer WSe2, mechanically exfoliated on top of a periodic two dimensional plasmonic array of elliptical gold (Au) nanodiscs. By exploiting the polarization-dependent nature of plasmonic resonance of the nano plasmonic array (NPA), the …
Quantum synchronization in atom-cavity coupled systems
Indian Association for the Cultivation of Science（印度科学培养印度协会）；Indian Institute of Technology, Kanpur（坎普尔印度理工学院）；TCG Centres of Research and Education in Science and Technology（TCG科学技术研究与教育中心）
An optical quantum memory is a stationary device that is capable of storing and recreating photonic qubits with a higher fidelity than any classical device. Thus far, these two requirements have been fulfilled in systems based on cold atoms and cryogenically cooled crystals. Here, we report a room-temperature quantum memory capable of storing arbitrary polarization qubits with a signal-to-background ratio higher than 1 and an average fidelity clearly surpassing the classical limit for weak laser pulses containing 1.6 photons on average. Our results prove that a common vapor cell can reach the …
Here we use a slow light quantum light-matter interface at room temperature to implement an analog simulator of complex relativistic and topological physics. We have realized the famous Jackiw-Rebbi model (JR), the celebrated first example where relativity meets topology. Our system is based upon interacting dark state polaritons (DSP's) created by storing light in a rubidium vapor using a dual-tripod atomic system. The DSP's temporal evolution emulates the physics of Dirac spinors and is engineered to follow the JR regime by using a linear magnetic field gradient. We also probe the obtained t…
Realization of practical terahertz wireless communications still faces many challenges. The receiver with high sensitivity is important for THz wireless communications. Here we demonstrate a terahertz receiver based on the cesium Rydberg atoms in a room-temperature vapor cell. The minimum detectable THz electric field is calibrated. With this receiver, the phase-sensitive conversion of amplitude-modulated or frequency-modulated terahertz waves into optical signals is performed. The results show that the atomic receiver has many advantages due to its quantum properties. Especially, the long dis…
Germanium has emerged as an exceptionally promising material for spintronics and quantum information applications, with significant fundamental advantages over silicon. However, efforts to create atomic-scale devices using donor atoms as qubits have largely focussed on phosphorus in silicon. Positioning phosphorus in silicon with atomic-scale precision requires a thermal incorporation anneal, but the low success rate for this step has been shown to be a fundamental limitation prohibiting the scale-up to large-scale devices. Here, we present a comprehensive study of arsine (AsH$_3$) on the germ…
Motivated by the spin self-rephasing recently observed in an atomic clock, we introduce a simple dynamical model to study the competition between dephasing and synchronization. Two spins $S$ are taken to be initially parallel and in the plane perpendicular to an inhomogeneous magnetic field $Δ$ that tends to dephase them. In addition, the spins are coupled by exchange interaction $J$ that tries to keep them locked. The analytical solution of the classical dynamics shows that, there is a phase transition to a synchronized regime for sufficiently large exchange interaction $J>Δ$ compared to the …
It is well known that ultranarrow electromagnetically induced transparency (EIT) resonances can be observed in atomic gases at room temperature. We report here the experimental observation of another type of ultranarrow resonances, as narrow as the EIT ones, in a Λ-system selected by light polarization in metastable 4He at room temperature. It is shown to be due to coherent population oscillations in an open two-level system (TLS). For perpendicular linearly polarized coupling and probe beams, this system can be considered as two coupled open TLSs, in which the ground state populations exhibit…
Quantum memories are a crucial technology for enabling large-scale quantum networks through synchronisation of probabilistic operations. Such networks impose strict requirements on quantum memory, such as storage time, retrieval efficiency, bandwidth, and scalability. On- and off-resonant ladder protocols on warm atomic vapour platforms are promising candidates, combining efficient high-bandwidth operation with low-noise on-demand retrieval. However, their storage time is severely limited by motion-induced dephasing caused by the broad velocity distribution of atoms comprising the vapour. In t…
The concept of measure synchronization between two coupled quantum many-body systems is presented. In general terms we consider two quantum many-body systems whose dynamics gets coupled through the contact particle-particle interaction. This coupling is shown to produce measure synchronization, a generalization of synchrony to a large class of systems which takes place in absence of dissipation. We find that in quantum measure synchronization, the many-body quantum properties for the two subsystems, e.g. condensed fractions and particle fluctuations, behave in a coordinated way. To illustrate …
Quantum memory capable of storage and retrieval of flying photons on demand is crucial for developing quantum information technologies. However, the devices needed for long-distance links are quite different from those envisioned for local processing. Here, we present the first hybrid quantum memory enabled network by demonstrating the interconnection and simultaneous operation of two types of quantum memory: an atomic-ensemble-based memory and an all-optical loop memory. The former generates and stores single atomic excitations that can then be converted to single photons; and the latter maps…
Both classical and quantum dynamics of the synchronization between two nonlinear mechanical modes scattered from Bose-Einstein condensates (BECs) by the standing-wave laser beam are comparatively investigated. As the ultra-low dissipations of the momentum modes in the atomic BECs, the synchronized dynamics are studied in a framework of closed-system theory in order to track down both the classical and the quantum synchronizations from an angle of quantum control. The classical synchronization and the relevant dynamics of measure synchronization, the quantum synchronization and two different ty…
We report a photon shot-noise-limited (SNL) optical magnetometer based on amplitude modulated optical rotation using a room-temperature $^{85}$Rb vapor in a cell with anti-relaxation coating. The instrument achieves a room-temperature sensitivity of $70$ fT/$\sqrt{\mathrm{Hz}}$ at $7.6$ $μ$T. Experimental scaling of noise with optical power, in agreement with theoretical predictions, confirms the SNL behaviour from $5$ $μ$T to $75$ $μ$T. The combination of best-in-class sensitivity and SNL operation makes the system a promising candidate for application of squeezed light to a state-of-the-art …
High-purity single photon sources (SPS) that can operate at room temperature are highly desirable for a myriad of applications, including quantum photonics and quantum key distribution. In this work, we realise an ultra-bright solid-state SPS based on an atomic defect in hexagonal boron nitride (hBN) integrated with a solid immersion lens (SIL). The SIL increases the source efficiency by a factor of six, and the integrated system is capable of producing over ten million single photons per second at room temperature. Our results are promising for practical applications of SPS in quantum communi…
We demonstrate trapping of electrons in a millimeter-sized quadrupole Paul trap driven at 1.6~GHz in a room-temperature ultra-high vacuum setup. Cold electrons are introduced into the trap by ionization of atomic calcium via Rydberg states and stay confined by microwave and static electric fields for several tens of milliseconds. A fraction of these electrons remain trapped longer and show no measurable loss for measurement times up to a second. Electronic excitation of the motion reveals secular frequencies which can be tuned over a range of several tens to hundreds of MHz. Operating a simila…
An atomic magnetometer operated with elliptically polarized light is investigated theoretically and experimentally. To explore the potential of this magnetometric configuration, the analytical form of the outgoing signal is derived. Parameters that significantly influence the performance are optimized, which lead to a sensitivity of 300 $\rm fT/\sqrt{Hz}$ at 45 $^{\circ}$C with a 2$\times$2$\times2$ cm uncoated Rb vapor cell. It is remarkable that a sensitivity of 690 $\rm fT/\sqrt{Hz}$ is achieved at room temperature of 24 $^{\circ}$C, which is improved by an order of magnitude compared with …
Electrically controllable quantum coherence in quantum dot clusters and arrays based on graphene stripes with zigzag atomic edges (ZZ-stripes) is studied using the Dirac equation and S-matrix technique. We find that respective multiqubit circuits promise stable operation up to room temperatures when the coherence time is prolonged up by a few orders of magnitude through the intrinsic spectral narrowing owing to electron transport between at bands in adjacent sections. Respectively, the coupling of qubits to a noisy environment is diminished, while the inelastic electron-phonon scattering is su…
Macroscopic ensembles of radiating dipoles are ubiquitous in the physical and natural sciences. In the classical limit the dipoles can be described as damped-driven oscillators, which are able to spontaneously synchronize and collectively lock their phases. Here we investigate the correspond- ing phenomenon in the quantum regime with arrays of quantized two-level systems coupled via long-range and anisotropic dipolar interactions. Our calculations demonstrate that the dipoles may overcome the decoherence induced by quantum fluctuations and inhomogeneous couplings and evolve to a synchronized s…
