A coherent technique for the control of photon propagation in optically thick media and its application for quantum memories is discussed. Raman adiabatic passage with an externally controlled Stokes field can be used to transfer the quantum state of a light pulse (``flying'' qubit) to a collective spin-excitation (stationary qubit) and thereby slow down its propagation velocity to zero. The process is reversible and has a potential fidelity of unity without the necessity for strongly coupling resonators. A simple quasi-particle picture (dark-state polariton) of the transfer is presented. The analytic theory is supplemented with exact numerical solutions. Finally the influence of decoherence mechanisms on collective storage states, which are N-particle entangled states, is analyzed.
We report on a source of ultranarrow-band photon pairs generated by widely nondegenerate cavity-enhanced spontaneous down-conversion. The source is designed to be compatible with Pr3+ solid state quantum memories and telecommunication optical fibers, with signal and idler photons close to 606 nm and 1436 nm, respectively. Both photons have a spectral bandwidth around 2 MHz, matching the bandwidth of Pr3+ doped quantum memories. This source is ideally suited for long distance quantum communication architectures involving solid state quantum memories.
Storage time extension in photon echoes using optical deshelving via a robust spin state has been investigated for absorption-dependent optical leakage, where an incomplete population transfer, even by a πoptical pulse obviates the phase recovery condition of the deshelving. We analyze an optical depth-dependent echo leakage mechanism in the storage time extended photon echoes for the usage of optical deshelving to photon echo-based quantum memories.
We propose a quantum repeater protocol which builds on the well-known DLCZ protocol [L.M. Duan, M.D. Lukin, J.I. Cirac, and P. Zoller, Nature 414, 413 (2001)], but which uses photon pair sources in combination with memories that allow to store a large number of temporal modes. We suggest to realize such multi-mode memories based on the principle of photon echo, using solids doped with rare-earth ions. The use of multi-mode memories promises a speedup in entanglement generation by several orders of magnitude and a significant reduction in stability requirements compared to the DLCZ protocol.
A double rephasing photon echo is analyzed for inversion-free photon echo-based quantum memories using controlled Rabi flopping, where the Rabi flopping is used for phase control of atom coherence. Unlike the rephasing-caused pi-phase shift in a single rephasing scheme, the control Rabi flopping between the excited state and an auxiliary third state induces coherence inversion. Thus, the absorptive photon echo in a double rephasing scheme can be manipulated to be emissive via the controlled Rabi flopping. Here we present a quantum coherence control of atom phases in a double rephasing photon e…
We demonstrate a method for time gating the standard heralded continuous- wave (cw) spontaneous parametric down-converted (SPDC) single photon source by using pulsed pumping of the optical parametric oscillator (OPO) below threshold. The narrow bandwidth, high purity, high spectral brightness and the pseudo-deterministic character make the source highly suitable for light-atom interfaces with atomic memories.
Photonics offers a route to fast and distributed quantum computing in ambient conditions, provided that photon sources and logic gates can be operated deterministically. Quantum memories, capable of storing and re-emitting photons on demand, enable quasi-deterministic operations by synchronising stochastic events. We recently interfaced a Raman-type quantum memory with a travelling-wave heralded photon source. Here we discuss the trade-space for the spectral characteristics of such sources, and we present measurements of our source, which represents a practical compromise enabling passive stab…
Quantum memories for light, which allow the reversible transfer of quantum states between light and matter, are central to the development of quantum repeaters, quantum networks, and linear optics quantum computing. Significant progress has been reported in recent years, including the faithful transfer of quantum information from photons in pure and entangled qubit states. However, none of these demonstrations confirm that photons stored in and recalled from quantum memories remain suitable for two-photon interference measurements, such as C-NOT gates and Bell-state measurements, which constit…
The influence of decoherence on the fidelity of quantum memories for photonic qubits based on dark-state polaritons in atomic ensembles is discussed. It is shown that despite the large entanglement of the collective storage states corresponding to single photons or nonclassical states of light the sensitivity to decoherence does not scale with the number of atoms. This is due to the existence of equivalence classes of storage states corresponding to states with the same number of dark-state polariton excitations but arbitrary excitations in other polariton modes. Several decoherence processes …
Entangling quantum systems with different characteristics through the exchange of photons is a prerequisite for building future quantum networks. Proving the presence of entanglement between quantum memories for light working at different wavelengths furthers this goal. Here, we report on a series of experiments with a thulium-doped crystal, serving as a quantum memory for 794 nm photons, an erbium-doped fibre, serving as a quantum memory for telecommunication-wavelength photons at 1535 nm, and a source of photon pairs created via spontaneous parametric down-conversion. Characterizing the phot…
We report an experimental realization of a narrow-band polarization-entangled photon source with a linewidth of 9.6 MHz through cavity-enhanced spontaneous parametric down-conversion. This linewidth is comparable to the typical linewidth of atomic ensemble based quantum memories. Single-mode output is realized by setting a reasonable cavity length difference between different polarizations, using of temperature controlled etalons and actively stabilizing the cavity. The entangled property is characterized with quantum state tomography, giving a fidelity of 94% between our state and a maximally…
Quantum light-matter interfaces are at the heart of photonic quantum technologies. Quantum memories for photons, where non-classical states of photons are mapped onto stationary matter states and preserved for subsequent retrieval, are technical realizations enabled by exquisite control over interactions between light and matter. The ability of quantum memories to synchronize probabilistic events makes them a key component in quantum repeaters and quantum computation based on linear optics. This critical feature has motivated many groups to dedicate theoretical and experimental research to dev…
We report on a source of heralded narrowband (3MHz) single photons compatible with solid-state spin-wave quantum memories based on praseodymium doped crystals. Widely non-degenerate narrow-band photon pairs are generated using cavity enhanced down conversion. One photon from the pair is at telecom wavelengths and serves as heralding signal, while the heralded single photon is at 606nm, resonant with an optical transition in Pr:YSO. The source offers a heralding efficiency of 28% and a generation rate exceeding 2000 pairs/mW in a single-mode. The single photon nature of the heralded field is co…
We present a protocol to construct an arbitrary quantum circuit. The quantum bits (qubits) are encoded in polarisation states of single photons. They are stored in spatially separated dense media deposed in an optical cavity. Specific sequences of pulses address individually the storage media to encode the qubits and to implement a universal set of gates. The proposed protocol is decoherence-free in the sense that spontaneous emission and cavity damping are avoided. We discuss a coupling scheme for experimental implementation in Neon atoms.
We present a source of polarization-entangled photon pairs suitable for the implementation of long-distance quantum communication protocols using quantum memories. Photon pairs with wavelengths 883 nm and 1338 nm are produced by coherently pumping two periodically poled nonlinear waveguides embedded in the arms of a polarization interferometer. Subsequent spectral filtering reduces the bandwidth of the photons to 240 MHz. The bandwidth is well-matched to a quantum memory based on an Nd:YSO crystal, to which, in addition, the center frequency of the 883 nm photons is actively stabilized. A theo…
The sources, which generate atom-photon quantum correlations or entanglement based on quantum memory, are basic blocks for building quantum repeaters (QRs). For achieving highly entanglement-generation rates in ensemble-based QRs, spatial-, temporal- and spectral-multimode memories are needed. The previous temporal-multimode memories are based on rephrasing mechanisms in inhomogeneous-broadened media. Here, by applying a train of multi-direction write pulses into a homogeneous-broadened atomic ensemble to induce Duan-Lukin-Cirac-Zoller-like Raman processes, we prepare up to 19 pairs of modes, …
The ability to coherently convert the frequency and temporal waveform of single and entangled photons will be crucial to interconnect the various elements of future quantum information networks. Of particular importance in this context is the quantum frequency conversion of photons emitted by material systems able to store quantum information, so called quantum memories. There have been significant efforts to implement quantum frequency conversion using non linear crystals, with non classical light from broadband photon pair sources and solid state emitters. However, so far, solid state quantu…
Here we propose a solid-state quantum memory that does not require spectral holeburning, instead using strong rephasing pulses like traditional photon echo techniques. The memory uses external broadening fields to reduce the optical depth and so switch off the collective atom-light interaction when desired. The proposed memory should allow operation with reasonable efficiency in a much broader range of material systems, for instance Er3+ doped crystals which have a transition at 1.5 um. We present analytic theory supported by numerical calculations and initial experiments.
Quantum teleportation enables the deterministic exchange of qubits via lossy channels. While it is commonly believed that unconditional teleportation requires a preshared entangled qubit pair, here we demonstrate a protocol that is in principle unconditional and requires only a single photon as an ex-ante prepared resource. The photon successively interacts, first, with the receiver and then with the sender qubit memory. Its detection, followed by classical communication, heralds a successful teleportation. We teleport six mutually unbiased qubit states with average fidelity $\overline{\text{F…
Single photons are a vital resource for optical quantum information processing. Efficient and deterministic single photon sources do not yet exist, however. To date, experimental demonstrations of quantum processing primitives have been implemented using non-deterministic sources combined with heralding and/or postselection. Unfortunately, even for eight photons, the data rates are already so low as to make most experiments impracticable. It is well known that quantum memories, capable of storing photons until they are needed, are a potential solution to this `scaling catastrophe'. Here, we an…
We study the feasibility of meaningful proof-of-principle demonstrations of several quantum repeater protocols with photon (single-photon and photon-pair) sources and atomic-ensemble based quantum memories. We take into account non-unit memory efficiencies that decay exponentially with time, which complicates the calculation of repeater rates. We discuss implementations based on quantum dots, parametric down-conversion, rare-earth-ion doped crystals, and Rydberg atoms. Our results provide guidance for the near-term implementation of long-distance quantum repeater demonstrations, suggesting tha…
We analyze the two-photon linewidth of the recently proposed adiabatic transfer technique for ``stopping'' of light using electromagnetically induced transparency (EIT). We shown that a successful and reliable transfer of excitation from light to atoms and back can be achieved if the spectrum of the input probe pulse lies within the initial transparency window of EIT, and if the two-photon detuning $δ$ is less than the collective coupling strength (collective vacuum Rabi-frequency) $g\sqrt{N}$ divided by $\sqrt{γT}$, with $γ$ being the radiative decay rate, $N$ the effective number of atoms in…
Photon-echo based quantum memories use inhomogeneously broadened, optically thick ensembles of absorbers to store a weak optical signal and employ various protocols to rephase the atomic coherences for information retrieval. We study the application of two consecutive, frequency-chirped control pulses for coherence rephasing in an ensemble with a 'natural' inhomogeneous broadening. Although propagation effects distort the two control pulses differently, chirped pulses that drive adiabatic passage can rephase atomic coherences in an optically thick storage medium. Combined with spatial phase mi…
Attenuated laser pulses are often employed in place for single photons in order to test the efficiency of the elements of a quantum network. In this work we analyse theoretically the dynamics of storage of an attenuated light pulse (where the pulse intensity is at the single photon level) propagating along a transmission line and impinging on the mirror of a high finesse cavity. Storage is realised by the controlled transfer of the photonic excitations into a metastable state of an atom confined inside the cavity and occurs via a Raman transition with a suitably tailored laser pulse, which dri…
Quantum memories for optical and microwave photons provide key functionalities in quantum processing and communications. Here we propose a protocol well adapted to solid state ensemble based memories coupled to cavities. It is called Stark Echo Modulation Memory (SEMM), and allows large storage bandwidths and low noise. This is achieved in a echo like sequence combined with phase shifts induced by small electric fields through the linear Stark effect. We investigated the protocol for rare earth nuclear spins and found a high suppression of unwanted collective emissions that is compatible with …
Promising access to high-speed quantum networks relies on the creation of high-dimensional entangled memories that provide quantum communication with higher capacity of noisy quantum channels, thereby reducing the transmission time of information. Yet, the distribution of multidimensional entanglement between remote memory nodes is still faintly investigated. We propose an experimentally feasible protocol of deterministic generation of high-dimensional entanglement between distant multi-level atoms confined in high-finesse optical cavities and driven by laser pulses. Three-dimensional entangle…
A central challenge for many quantum technologies concerns the generation of large entangled states of individually addressable quantum memories. Here, we show that percolation theory allows the rapid production of arbitrarily large graph states by heralded photonic entanglement in a lattice of atomic memories. This approach can greatly reduce the time required to produce large cluster resource states for quantum information processing, including states required for universal one-way quantum computing. This reduction puts our architecture in an operational regime where demonstrated collection,…
Slowing/stopping the light travelling in free space with electromagnetically induced transparency to im- plement the optical quantum information processings and store information has been paid much attention in recent years. For the waveguide photons, here, we propose an approach to stop them with a controllable atomic cavity generated by a pair of atomic mirrors; one of them reflects the photon completely and an- other one with the adjustable reflected/transmitted probability of the photons. Based on the full quantum mechanical theory in real space, we show that the reflected/transmitted prob…
Quantum network has significant applications both practically and fundamentally. A hybrid architecture with photons and stationary nodes is highly promising. So far, experimental realizations are limited to two nodes with two photons. Going beyond state of the art by entangling many photons with many quantum nodes is highly appreciated. Here, we report an experiment realizing hybrid entanglement between three photons and three atomic-ensemble quantum memories. We make use of three similar setups, in each of which one pair of photon-memory entanglement with high overall efficiency is created vi…
Gravitational time dilation in quantum clock interferometry with entangled multi-photon states and quantum memories
Humboldt-Universität zu Berlin（柏林洪堡大学）；ZARM, Unversität Bremen（不来梅大学ZARM中心）；Vienna Center for Quantum Science and Technology, Atominstitut, TU Wien（维也纳量子科学与技术中心，原子物理研究所，维也纳工业大学）
Erbium dopants in crystals exhibit highly coherent optical transitions well suited for solid-state optical quantum memories operating in the telecom band. Here we demonstrate coupling of erbium dopant ions in yttrium orthosilicate to a photonic crystal cavity fabricated directly in the host crystal using focused ion beam milling. The coupling leads to reduction of the photoluminescence lifetime and enhancement of the optical depth in microns-long devices, which will enable on-chip quantum memories.
Modular quantum computing architectures require fast and efficient distribution of quantum information through propagating signals. Here we report rapid, on-demand quantum state transfer between two remote superconducting cavity quantum memories through traveling microwave photons. We demonstrate a quantum communication channel by deterministic transfer of quantum bits with 76% fidelity. Heralding on errors induced by experimental imperfection can improve this to 87% with a success probability of 0.87. By partial transfer of a microwave photon, we generate remote entanglement at a rate that ex…
We demonstrate a probabilistic entangling quantum gate between two distant trapped ytterbium ions. The gate is implemented between the hyperfine "clock" state atomic qubits and mediated by the interference of two emitted photons carrying frequency encoded qubits. Heralded by the coincidence detection of these two photons, the gate has an average fidelity of 90+-2%. This entangling gate together with single qubit operations is sufficient to generate large entangled cluster states for scalable quantum computing.
The use of multiplexed atomic quantum memories (MAQM) can significantly enhance the efficiency to establish entanglement in a quantum network. In the previous experiments, individual elements of a quantum network, such as the generation, storage and transmission of quantum entanglement have been demonstrated separately. Here we report an experiment to show the compatibility of these basic operations. Specifically, we generate photon-atom entanglement in a $6\times 5$ MAQM, convert the spin wave to time-bin photonic excitation after a controllable storage time, and then store and retrieve the p…
We demonstrate teleportation of quantum bits between two single atoms in distant laboratories. Using a time-resolved photonic Bell-state measurement, we achieve a teleportation fidelity of (88.0+/-1.5)%, largely determined by our entanglement fidelity. The low photon collection efficiency in free space is overcome by trapping each atom in an optical cavity. The resulting success probability of 0.1% is almost 5 orders of magnitude larger than in previous experiments with remote material qubits. It is mainly limited by photon propagation and detection losses and can be enhanced with a cavity-bas…
A quantum memory protocol of controlled ac Stark echoes (CASE) based on a double rephasing photon echo scheme via controlled Rabi flopping is proposed. A double rephasing scheme of photon echoes inherently satisfies the no-population inversion requirement for quantum memories, but the resultant absorptive echo has been a fundamental problem. In the present studies, firstly, the first echo in the double rephasing scheme is dynamically controlled not to affect the second echo by using unbalanced ac Stark shifts. Secondly, a control Rabi pulse coherently manipulates the second echo to be emissive…
Quantum error correction (QEC) is fundamental for quantum information processing but entails a substantial overhead of classically-controlled quantum operations, which can be architecturally cumbersome to accommodate. Here we discuss a novel approach to designing elementary QEC memory cells, in which all control operations are performed autonomously by an embedded optical feedback loop. Our approach is natural for nanophotonic implementations in which each qubit can be coupled to its own optical resonator, and our design for a memory cell based on the quantum bit-flip or phase-flip code requir…
An elementary quantum network operation involves storing a qubit state in an atomic quantum memory node, and then retrieving and transporting the information through a single photon excitation to a remote quantum memory node for further storage or analysis. Implementations of quantum network operations are thus conditioned on the ability to realize such matter-to-light and/or light-to-matter quantum state mappings. Here, we report generation, transmission, storage and retrieval of single quanta using two remote atomic ensembles. A single photon is generated from a cold atomic ensemble at Site …
Time-resolved photon detection can be used to generate entanglement between distinguishable photons. This technique can be extended to entangle quantum memories that emit photons with different frequencies and identical temporal profiles without the loss of entanglement rate or fidelity. We experimentally realize this process using remotely trapped $^{171}$Yb$^+$ ions where heralded entanglement is generated by interfering distinguishable photons. This technique may be necessary for future modular quantum systems and networks that are composed of heterogeneous qubits.
Optical approaches to quantum computation require the creation of multi-mode photonic quantum states in a controlled fashion. Here we experimentally demonstrate phase locking of two all-optical quantum memories, based on a concatenated cavity system with phase reference beams, for the time-controlled release of two-mode entangled single-photon states. The release time for each mode can be independently determined. The generated states are characterized by two-mode optical homodyne tomography. Entanglement and nonclassicality are preserved for release-time differences up to 400 ns, confirmed by…
High-visibility interference of photon echoes generated in spatially separated solid-state atomic ensembles is demonstrated. The solid state ensembles were LiNbO$_3$ waveguides doped with Erbium ions absorbing at 1.53 $μ$m. Bright coherent states of light in several temporal modes (up to 3) are stored and retrieved from the optical memories using two-pulse photon echoes. The stored and retrieved optical pulses, when combined at a beam splitter, show almost perfect interference, which demonstrates both phase preserving storage and indistinguishability of photon echoes from separate optical memo…
Quantum internet will enable a number of revolutionary applications. It relies on entanglement of remote quantum memories over long distances. Despite enormous progresses so far, the maximal physical separation achieved between two nodes is 1.3 km, and challenges for long distance remain. Here we make a significant step forward by entangling two atomic ensembles in one lab via photon transmission through metropolitan-scale fibers. We use cavity enhancement to create bright atom-photon entanglement, and harness quantum frequency conversion to shift the atomic wavelength to telecom. We realize e…
Quantum memories, capable of controllably storing and releasing a photon, are a crucial component for quantum computers and quantum communications. So far, quantum memories have operated with bandwidths that limit data rates to MHz. Here we report the coherent storage and retrieval of sub-nanosecond low intensity light pulses with spectral bandwidths exceeding 1 GHz in cesium vapor. The novel memory interaction takes place via a far off-resonant two-photon transition in which the memory bandwidth is dynamically generated by a strong control field. This allows for an increase in data rates by a…
We observe quantum, Hong-Ou-Mandel, interference of fields produced by two remote atomic memories. High-visibility interference is obtained by utilizing the finite atomic memory time in four-photon delayed coincidence measurements. Interference of fields from remote atomic memories is a crucial element in protocols for scalable generation of multi-node remote qubit entanglement.
Quantum memories are enabling devices for extending the reach of quantum key distribution (QKD) systems. The required specifications for memories are, however, often considered too demanding for available technologies. One can change this mindset by introducing memory-assisted measurement-device-independent QKD (MDI-QKD), which imposes less stringent conditions on the memory modules. It has been shown that, in the case of {\em fast} single-qubit memories, we can reach rates and distances not attainable by single no-memory QKD links. Single-qubit memories, such as single atoms or ions, have, cu…
A one-dimensional atom -- an atomic system coupled to a single optical mode -- is central for many applications in optical quantum technologies. Here we introduce an effective one-dimensional atom consisting of two interacting quantum emitters coupled to a cavity mode. The dipole-dipole interaction and cavity coupling gives rise to optical resonances of tunable bandwidth with a constant mode coupling. Such versatility, combined with a dynamical control of the system, opens the way to many applications. It can be used to generate single photon light pulses with continuous variable encoding in t…
