We discuss advantages of using non-classical states of light for two aspects of optical imaging: creating of miniature images on photosensitive substrates, which constitutes the foundation for optical lithography, and imaging of micro objects. In both cases, the classical resolution limit given by the Rayleigh criterion is approximately a half of the optical wavelength. It has been shown, however, that by using multi-photon quantum states of the light field, and multi-photon sensitive material or detector, this limit can be surpassed. We give a rigorous quantum mechanical treatment of this problem, address some particularly widespread misconceptions and discuss the requirements for turning the research on quantum imaging into a practical technology.
In this article we try to describe the physics of a standard optical interferometer fed by "quantum" photons in terms of primitive, nevertheless accurate formulation. We derive explicit interferene patterns and show how they vary depending on the input photon state.
We use a parametric down-conversion source pumped by a short coherence-length continuous-wave (CW) diode laser to perform two-photon interferometry in an intermediate regime between the more familiar Franson-type experiments with a long coherence-length pump laser, and the short pulsed pump "time-bin" experiments pioneered by Gisin's group. The use of a time-bin-like Mach-Zehnder interferometer in the CW pumping beam induces coherence between certain two-photon amplitudes, while the CW nature of the experiment prevents the elimination of remaining incoherent ones. The experimental results high…
Sub-picosecond coincidence timing from nonlocal intensity interference of entangled photons allows quantum interferometry for plasmas. Using a warm plasma dispersion relation, we correlate phase measurement sensitivity with different plasma properties or physics mechanisms over 6 orders of magnitude. Due to $N^α$ ($α\leq -1/2$) scaling with the photon number $N$, quantum interferometry using entangled light can probe small signals in plasmas not previously accessible. As an example, it is predicted that plasmas will induce shifts to a Gaussian dip, a well-known quantum optics phenomenon that i…
Spin interferometry of the 4th order for independent polarized as well as unpolarized photons arriving simultaneously at a beam splitter and exhibiting spin correlation while leaving it, is formulated and discussed in the quantum approach. Beam splitter is recognized as a source of genuine singlet photon states. Also, typical nonclassical beating between photons taking part in the interference of the 4th order is given a polarization dependent explanation.
New methods are proposed to characterize the spectral-temporal distribution of single photons. The presented protocols take advantage of spectral filtering, frequency entanglement between two single photons the one of interest and a reference, followed by the generalized Hong, Ou and Mandel interferometer. The measurement of the coincidence probability in these different schemes reveals the chronocyclic Wigner, the pseudo-Wigner distribution and the spectrogram at the single-photon level.
Quantum phenomena such as entanglement can improve fundamental limits on the sensitivity of a measurement probe. In optical interferometry, a probe consisting of $N$ entangled photons provides up to a $\sqrt{N}$ enhancement in phase sensitivity compared to a classical probe of the same energy. Here, we employ high-gain parametric down-conversion sources and photon-number-resolving detectors to perform interferometry with heralded quantum probes of sizes up to $N=8$ (i.e. measuring up to 16-photon coincidences). Our probes are created by injecting heralded photon-number states into an interfero…
A polarized photon with well-defined orbital angular momentum that emerges from a Mach-Zehnder interferometer (MZI) is shown to circumvent wave-particle duality. Its polarization-resolved detection probability forms a non-sinusoidal interferometric pattern. For certain phase differences between the MZI arms, this pattern yields both reliable which-path information and high phase-sensitivity.
We report the experimental demonstration of four-photon quantum interference using telecom-wavelength photons. Realization of multi-photon quantum interference is essential to linear optics quantum information processing and measurement-based quantum computing. We have developed a source that efficiently emits photon pairs in a pure spectrotemporal mode at a telecom wavelength region, and have demonstrated the quantum interference exhibiting the reduced fringe intervals that correspond to the reduced de Broglie wavelength of up to the four photon `NOON' state. Our result should open a path to …
We solve the general problem of determining, through imaging, the three-dimensional positions of $N$ weak incoherent point-like emitters in an arbitrary spatial configuration. We show that a structured measurement strategy in which a linear interferometer feeds into an array of photo-detectors is always optimal for this estimation problem, in the sense that it saturates the quantum Cramér-Rao bound. We provide a method for the explicit construction of the optimal interferometer. Further explicit results for the quantum Fisher information and the optimal interferometer design that attains it ar…
We report the experimental observation of the nonlocal geometric phase in Hanbury Brown-Twiss polarized intensity interferometry. The experiment involves two independent, polar- ized, incoherent sources, illuminating two polarized detectors. Varying the relative polarization angle between the detectors introduces a geometric phase equal to half the solid angle on the Poincaré sphere traced out by a pair of single photons. Local measurements at either detector do not reveal the effect of the geometric phase, which appears only in the coincidence counts between the two detectors, showing a genui…
Recently a pair of experiments demonstrated a simulation of Abelian anyons in a spin network of single photons. The experiments were based on an Abelian discrete gauge theory spin lattice model of Kitaev. Here we describe how to use linear optics and single photons to simulate non-Abelian anyons. The scheme makes use of joint qutrit-qubit encoding of the spins and the resources required are three pairs of parametric down converted photons and 14 beam splitters.
We show how the entangled photons produced in parametric down conversion can be used to improve the sensitivity of a Sagnac interferometer. Two-photon and four-photon coincidences increases the sensitivity by a factor of two and four respectively. Our results apply to sources with arbitrary pumping and squeezing parameters.
The quantum measurement problem still finds no consensus. Nonlocal interferometry provides an unprecedented experimental probe by entangling two photons in the "measurement state" (MS). The experiments show that each photon "measures" the other; the resulting entanglement decoheres both photons; decoherence collapses both photons to unpredictable but definite outcomes; and the two-photon MS continues evolving coherently. Thus, contrary to common opinion, when a two-part system is in the MS, the outcomes actually observed at both subsystems are definite. Although standard quantum physics postul…
We propose a new experiment employing two independent sources of spin correlated photon pairs. Two photons from different unpolarized sources each pass through a polarizer to a detector. Although their trajectories never mix or cross they exhibit 4th-order-interference-like correlations when the other two photons interfere on a beam splitter even when the latter two do not pass any polarizers at all. A wave packet calculation shows that the experiment permits a very discriminatory test of hidden variable theories.
We theoretically investigate the phase sensitivity with parity detection on a Mach-Zehnder interferometer with a coherent state combined with a photon-added squeezed vacuum state. When the phase shift approaches zero, the squeezed vacuum state is indeed the optimal state within a constraint on the average number of photons. However, when the phase shift to be estimated slightly deviates from zero, the optimal state is neither the squeezed vacuum state nor the photon-subtracted squeezed vacuum state, but the photon-added squeezed vacuum state when they carry many photons. Finally, we show that …
We provide a compact full description of multiboson correlation measurements of arbitrary order N in passive linear interferometers with arbitrary input single-photon pure states. This allows us to physically analyze the novel problem of multiboson correlation sampling at the output of random linear interferometers. Our results also describe general multiboson correlation landscapes for an arbitrary number of input single photons and arbitrary interferometers. In particular, we use two different schemes to demonstrate, respectively, arbitrary-order quantum beat interference and 100% visibility…
Single-photon sources are a fundamental resource in quantum optics. The indistinguishability and purity of photons emitted from different sources are crucial (necessary, essential) properties for many quantum applications to ensure high-visibility interference between different sources. The state of a single-photon source is described by the modes occupied by the single light quanta. Thus the ability to determine the mode structure of a single-photon source provides a means to assess its quality, compare different sources, and provide feedback for source engineering. Here, we propose and demon…
A method for performing nonlocal interferometry using phase-entangled macroscopic coherent states is described. The required entanglement can be generated using weak nonlinearities while Bell's inequality can be violated using single photons as a probe. The entanglement is relatively robust against photon loss and Bell's inequality can be violated over a relatively large distance in optical fibers despite the fact that a large number of photons are absorbed in the process.
Many quantum advantages in metrology and communication arise from interferometric phenomena. Such phenomena can occur on ultrafast time scales, particularly when energy-time entangled photons are employed. These have been relatively unexplored as their observation necessitates time resolution much shorter than conventional photon counters. Integrating nonlinear optical gating with conventional photon counters can overcome this limitation and enable subpicosecond time resolution. Here, using this technique and a Franson interferometer, we demonstrate high-visibility quantum interference with tw…
Employing the time-dependent variational principle combined with the multiple Davydov $\mathrm{D}_2$ Ansatz, we investigate Landau-Zener (LZ) transitions in a qubit coupled to a photon mode with various initial photon states at zero temperature. Thanks to the multiple Davydov trial states, exact photonic dynamics taking place in the course of the LZ transition is also studied efficiently. With the qubit driven by a linear external field and the photon mode initialized with Schrödinger-cat states, asymptotic behavior of the transition probability beyond the rotating-wave approximation is uncove…
We propose a Heisenberg-limited quantum interferometer whose input is twin optical beams from which one or more photons have been indistinguishably subtracted. Such an interferometer can yield Heisenberg-limited performance while at the same time giving a direct fringe reading, unlike for the twin-beam input of the Holland-Burnett interferometer. We propose a feasible experimental realization using a photon-number correlated source, such as non-degenerate parametric down-conversion, and perform realistic analyses of performance in the presence of loss and detector inefficiency.
The archetypal quantum interferometry experiment yields an interference pattern that results from the indistinguishability of two spatiotemporal paths available to a photon or to a pair of entangled photons. A fundamental challenge in quantum interferometry is to perform such experiments with a higher number of paths, and over large distances. In particular, the distribution of such highly entangled states in long-haul optical fibers is one of the core concepts behind quantum information networks. We demonstrate that using indistinguishable frequency paths instead of spatiotemporal ones allows…
The minimum error of unbiased parameter estimation is quantified by the quantum Fisher information in accordance to the Cramér-Rao bound. We indicate that only superposed NOON states by simultaneous measurements can achieve the maximum quantum Fisher information with form $<\hat{N}^{2}>$ for a given photon number distribution by a POVM in linear two-path interferometer phase measurement. We present a series of specified superposed states with infinite quantum Fisher information but with finite average photon numbers. The advantage of this unbounded quantum Fisher information will be beneficial…
We analyze the spatial and temporal resolving power of two-photon intensity interferometry for the light emitting source in single bubble sonoluminescence (SBSL). We show that bubble sizes between several 10 nm and 3 um can be resolved by measuring the transverse correlation function, but that a direct determination of the flash duration via the longitudinal correlation function works only for SBSL pulses which are shorter than 0.1 ps. Larger pulse lengths can be determined indirectly from the intercept of the angular correlator at equal photon frequencies. The dynamics of the bubble is not ac…
A nonclassical feature of the fourth-order interference at a beam splitter, that genuine photon spin singlets are emitted in predetermined directions even when incident photons are unpolarized, has been used in a proposal for an experiment that imposes quantum spin correlation on truly independent photons. In the experiment, two photons from two such singlets interfere at a beam splitter, and as a result the other two photons - which nowhere interacted and whose paths nowhere crossed - exhibit a 100% correlation in polarization, even when no polarization has been measured in the first two phot…
We use a photon-number resolving detector to monitor the photon number distribution of the output of an interferometer, as a function of phase delay. As inputs we use coherent states with mean photon number up to seven. The postselection of a specific Fock (photon-number) state effectively induces high-order optical non-linearities. Following a scheme by Bentley and Boyd [S.J. Bentley and R.W. Boyd, Optics Express 12, 5735 (2004)] we explore this effect to demonstrate interference patterns a factor of five smaller than the Rayleigh limit.
Geometric phase may enable inherently fault-tolerant quantum computation. However, due to potential decoherence effects, it is important to understand how such phases arise for {\it mixed} input states. We report the first experiment to measure mixed-state geometric phases in optics, using a Mach-Zehnder interferometer, and polarization mixed states that are produced in two different ways: decohering pure states with birefringent elements; and producing a nonmaximally entangled state of two photons and tracing over one of them, a form of remote state preparation.
Passive optical interferometry with single photons injected into some input ports and vacuum into others is enriched by admitting polarization, thereby replacing the scalar electromagnetic description by a vector theory, with the recent triad phase being a celebrated example of this richness. On the other hand, incorporating polarization into interferometry is known to be equivalent to scalar theory if the number of channels is doubled. We show that passive multiphoton $m$ channel interferometry described by SU($m$) transformations is replaced by SU($2m$) interferometry if polarization is incl…
We present a new approach to engineering broadband sources of entangled photon pairs for quantum interferometry. The source is based on quasi-phase-matched spontaneous parametric down conversion in a titanium diffused periodically poled lithium niobate waveguide with a strongly-chirped poling period. The proposed non-standard asymmetric poling mitigates phase distortions associated with the process of chirping. Asymmetric poling significantly broadens the entangled source bandwidth while preserving high visibility quantum interferometric sensing.
Franson interferometry is a well-known quantum measurement technique for probing photon-pair frequency correlations that is often used to certify time-energy entanglement. We demonstrate the complementary technique in the time basis, called conjugate-Franson interferometry, that measures photon-pair arrival-time correlations, thus providing a valuable addition to the quantum toolbox. We obtain a conjugate-Franson interference visibility of $96\pm 1$% without background subtraction for entangled photon pairs generated by spontaneous parametric down-conversion. Our measured result surpasses the …
Imaging of surface adsorbed molecules is investigated as a novel detection method for matter wave interferometry with fluorescent particles. Mechanically magnified fluorescence imaging turns out to be an excellent tool for recording quantum interference patterns. It has a good sensitivity and yields patterns of high visibility. The spatial resolution of this technique is only determined by the Talbot gratings and can exceed the optical resolution limit by an order of magnitude. A unique advantage of this approach is its scalability: for certain classes of nano-sized objects, the detection sens…
Hong-Ou-Mandel interferometry takes advantage of the quantum nature of two-photon interference to increase the resolution of precision measurements of time-delays. Relying on few-photon probe states, this approach is applicable also in cases of extremely sensible samples and it achieves attosecond (nanometer path length) scale resolution, which is relevant to cell biology and two-dimensional materials. Here, we theoretically analyze how the precision of Hong-Ou-Mandel interferometers can be significantly improved by engineering the spectral distribution of two-photon probe states. In particula…
We present a versatile, high-brightness, guided-wave source of polarization entangled photons, emitted at a telecom wavelength. Photon-pairs are generated using an integrated type-0 nonlinear waveguide, and subsequently prepared in a polarization entangled state via a stabilized fiber interferometer. We show that the single photon emission wavelength can be tuned over more than 50 nm, whereas the single photon spectral bandwidth can be chosen at will over more than five orders of magnitude (from 25 MHz to 4 THz). Moreover, by performing entanglement analysis, we demonstrate a high degree of co…
Long-distance quantum communication relies on storing and retrieving photonic qubits in orthogonal field modes. The available degrees of freedom for photons are polarization, spatial-mode profile, and temporal/spectral profile. To date, methods exist for decomposing, manipulating, and analyzing photons into orthogonal polarization modes and spatial modes. Here we propose and theoretically verify the first highly efficient method to carry out analogous operations for temporally and spectrally overlapping, but field-orthogonal, temporal modes. The method relies on cascaded nonlinear-optical quan…
The working principles of linear optical quantum computing are based on photodetection, namely, projective measurements. The use of photodetection can provide efficient nonlinear interactions between photons at the single-photon level, which is technically problematic otherwise. We report an application of such a technique to prepare quantum correlations as an important resource for Heisenberg-limited optical interferometry, where the sensitivity of phase measurements can be improved beyond the usual shot-noise limit. Furthermore, using such nonlinearities, optical quantum nondemolition measur…
We examine two setups that reveal different operational implications of path-phase complementarity for single photons in a Mach-Zehnder interferometer (MZI). In both setups, the which-way (WW) information is recorded in the polarization state of the photon serving as a "flying which-way detector". In the "predictive" variant, using a {\em fixed} initial state, one obtains duality relation between the probability to correctly predict the outcome of either a which-way (WW) or which-phase (WP) measurement (equivalent to the conventional path-distinguishibility-visibility). In this setup, only one…
We review some recent experiments based upon multimode two-photon interference of photon pairs created by spontaneous parametric down-conversion. The new element provided by these experiments is the inclusion of the transverse spatial profiles of the pump, signal and idler fields. We discuss multimode Hong-Ou-Mandel interference, and show that the transverse profile of the pump beam can be manipulated in order to control two-photon interference. We present the basic theory and experimental results as well as several applications to the field of quantum information.
By engineering and manipulating quantum entanglement between incoming photons and experimental apparatus, we construct single-photon detectors which cannot distinguish between photons of very different wavelengths. These color erasure detectors enable a new kind of intensity interferometry, with potential applications in microscopy and astronomy. We demonstrate chromatic interferometry experimentally, observing robust interference using both coherent and incoherent photon sources.
The performance of photonic $N00N$ states, propagating in an attenuating medium, is analyzed with respect to phase estimation. It is shown that, for $N00N$ states propagating through a lossy medium, the Heisenberg limit is never achieved. It is also shown that, for a given value of $N$, a signal comprised of an attenuated separable state of $N$ photons will actually produce a better phase estimate than will a signal comprised of an equally attenuated $N00N$ state, unless the transmittance of the medium is very high. This is a consequence of the need to utilize measurement operators appropriate…
The propagation of polarized photons in optical media can be effectively modeled by means of quantum dynamical semigroups. These generalized time evolutions consistently describe phenomena leading to loss of phase coherence and dissipation originating from the interaction with a large, external environment. High sensitive experiments in the laboratory can provide stringent bounds on the fundamental energy scale that characterizes these non-standard effects.
We analyse the phase space representation of the optimal measurement of a phase shift in an interferometer with equal photon loss in both its arms. In the local phase estimation scenario with a fixed number of photons, we identify features of the spin Wigner function that warrant sub-shot noise precision, and discuss their sensitivity to losses. We derive the asymptotic form of an integral kernel describing the process of photon loss in the phase space in the limit of large photon numbers. The analytic form of this kernel allows one to assess the ultimate precision limit for a lossy interferom…
Implications of field quantization on Ramsey interferometry are discussed and general conditions for the occurrence of interference are obtained. Interferences do not occur if the fields in two Ramsey zones have precise number of photons. However in this case we show how two atom (like two photon) interferometry can be used to discern a variety of interference effects as the two independent Ramsey zones get entangled by the passage of first atom. Generation of various entangled states like |0,2>+|2,0> are discussed and in far off resonance case generation of entangled state of two coherent sta…
Optical interferometry has been a long-standing setup for characterization of quantum states of light. Both the linear and the nonlinear interferences can provide information about the light statistics an underlying detail of the light-matter interactions. Here we demonstrate how interferometric detection of nonlinear spectroscopic signals may be used to improve the measurement accuracy of matter susceptibilities. Light-matter interactions change the photon statistics of quantum light, which are encoded in the field correlation functions. Application is made to the Hong-Ou-Mandel two-photon in…
We propose a polarised intensity interferometry experiment, which measures the nonlocal Pancharatnam phase acquired by a pair of Hanbury Brown-Twiss photons. The setup involves two polarised thermal sources illuminating two polarised detectors. Varying the relative polarisation angle of the detectors introduces a two photon geometric phase. Local measurements at either detector do not reveal the effects of the phase, which is an optical analog of the multiparticle Aharonov-Bohm effect. The geometric phase sheds light on the three slit experiment and suggests ways of tuning entanglement.
The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of light has recently emerged as an essential means for quantum information science. Here we experimentally demonstrate a self-referencing technique to completely determine the pulse-mode structure of single photons by means of spectral shearing interferometry. We detail the calibration and resolution of the measurement and discuss challenges and critical require…
We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto experimentally easily accessible non-coincident single electron spectra. We analyze the interferometric signal in terms of a semi-analytical model which is validated by a numerical solution of the time-dependent two-electron Schrödinger equation in its full dimensionality.
Motivated by rapidly advancing capabilities for extensive nanoscale patterning of optical materials, I propose an approach to implementing photonic sequential logic that exploits circuit-scale phase coherence for efficient realizations of fundamental components such as a NAND-gate-with-fanout and a bistable latch. Kerr-nonlinear optical resonators are utilized in combination with interference effects to drive the binary logic. Quantum-optical input-output models are characterized numerically using design parameters that yield attojoule-scale energy separation between the latch states.
We observed two-photon phase super-resolution in an unbalanced Michelson interferometer with classical Gaussian laser pulses. Our work is a time-reversed version of a two-photon interference experiment using an unbalanced Michelson interferometer. A measured interferogram exhibits two-photon phase super-resolution with a high visibility of 97.9% \pm 0.4%. Its coherence length is about 22 times longer than that of the input laser pulses. It is a classical analogue to the large difference between the one- and two-photon coherence lengths of entangled photon pairs.
We obtain coincidence rates for passive optical interferometry by exploiting the permutational symmetries of partially distinguishable input photons, and our approach elucidates qualitative features of multi-photon coincidence landscapes. We treat the interferometer input as a product state of any number of photons in each input mode with photons distinguished by their arrival time. Detectors at the output of the interferometer count photons from each output mode over a long integration time. We generalize and prove the claim of Tillmann et al. [Phys. Rev. X 5 041015 (2015)] that coincidence r…
We develop a framework for solving the action of a three-channel passive optical interferometer on single-photon pulse inputs to each channel using SU(3) group-theoretic methods, which can be readily generalized to higher-order photon-coincidence experiments. We show that features of the coincidence plots vs relative time delays of photons yield information about permanents, immanants, and determinants of the interferometer SU(3) matrix.
We propose and implement a quantum procedure for enhancing the sensitivity with which one can determine the phase shift experienced by a weak light beam possessing thermal statistics in passing through an interferometer. Our procedure entails subtracting exactly one (which can be generalized to m) photons from the light field exiting an interferometer containing a phase-shifting element in one of its arms. As a consequence of the process of photon subtraction, and somewhat surprisingly, the mean photon number and signal-to-noise ratio of the resulting light field are thereby increased, leading…
