We report the observation of correlated photon pairs generated by spontaneous parametric down-conversion in a quasi-phase matched KTiOPO4 nonlinear waveguide. The highest ratio of coincidence to single photon count rates observed in the 830 nm wavelength region exceeds 18%. This makes nonlinear waveguides a promising source of correlated photons for metrology and quantum information processing applications. We also discuss possibilities of controlling the spatial characteristics of the down-converted photons produced in multimode waveguide structures.
We present a study of the propagation of higher-order spatial modes in a waveguided parametric down-conversion photon pair source. Observing the multimode photon pair spectrum from a periodically poled KTiOPO$_4$ waveguide allowed us to isolate individual spatial modes through their distinctive spectral properties. We have measured directly the spatial distribution of each mode of the photon pairs, confirming the findings of our waveguide model, and demonstrated by coincidence measurements that the total parity of the modes is conserved in the nonlinear interaction. Furthermore, we show that w…
We report generation of near-infrared photon pairs in fundamental spatial modes via type-II spontaneous parametric down-conversion in a periodically poled potassium titanyl phosphate (KTiOPO4) nonlinear waveguide supporting multiple transverse modes. This demonstrates experimentally a versatile scheme for controlling the spatial characteristics of the produced nonclassical light based on exploitation of intermodal dispersion. The down-converted photons are characterized by the measurement of the beam quality factors in the heralded regime.
The propagation of several spatial modes has a significant impact on the structure of the emission from parametric down-conversion in a nonlinear waveguide. This manifests itself not only in the spatial correlations of the photon pairs but also, due to new phase-matching conditions, in the output spectrum, radically altering the degree of entanglement within each pair. Here we investigate both theoretically and experimentally the results of higher-order spatial-mode propagation in nonlinear waveguides. We derive conditions for the creation of pairs in these modes and present observations of hi…
Parametric down-conversion (PDC) offers the possibility to control the fabrication of non-Gaussian states such as Fock states. However, in conventional PDC sources energy and momentum conservation introduce strict frequency and photon number correlations, which impact the fidelity of the prepared state. In our work we optimize the preparation of single-photon Fock states from the emission of waveguided PDC via spectral filtering. We study the effect of correlations via photon number resolving detection and quantum interference. Our measurements show how the reduction of mixedness due to filter…
Low-noise, tunable wavelength-conversion through non-degenerate four-wave mixing Bragg scattering in SiNx waveguides is experimentally demonstrated. Finite element method simulations of waveguide dispersion are used with the split-step Fourier method to predict device performance, and indicate a strong dependence of the conversion efficiency on phase matching, which is controlled by the waveguide geometry. Two 1550 nm wavelength band pulsed pumps are used to achieve tunable conversion of a 980 nm signal over a range of 5 nm with a peak conversion efficiency of \approx 5 %. The demonstrated Bra…
Photonic crystals create dramatic new possibilities for nonlinear optics. Line defects are shown to support modes suitable for the production of pairs of photons by the material's second order nonlinearity even if the phase-matching conditions cannot be satisfied in the bulk. These structures offer the flexibility to achieve specific dispersion characteristics and potentially very high brightness. In this work, two phase matching schemes are identified and analyzed regarding their dispersive properties.
We report on the demonstration of correlated photon pair generation in quasi-phase-matched superlattice AlGaAs waveguides with a high coincidence-to-accidental ratio (CAR); with a continuous (CW) pump, the observed CAR (>100) is more than two order of magnitudes improvement over previously reported spontaneous down conversion (SPDC) schemes in AlGaAs waveguides with a pulsed pump.
We propose to use the integrated aluminum nitride waveguide with engineered width variation to achieve optical frequency conversion based on $χ^{(2)}$ nonlinear effect on a photonic chip. We show that in an adiabatically tapered waveguide, the frequency conversion has a much broader bandwidth and the efficiency within the bandwidth is almost constant, which is favorable for short pulses. We demonstrate both analytically and numerically an "area law" for the frequency conversion, i.e. the product of bandwidth and efficiency is conserved as long as peak conversion efficiency does not saturate. T…
High-efficiency photon-pair production is a long-sought-after goal for many optical quantum technologies, and coherent photon conversion processes are promising candidates for achieving this. We show theoretically how to control coherent conversion between a narrow-band pump photon and broadband photon pairs in nonlinear optical waveguides by tailoring frequency dispersion for broadband quantum frequency mixing. We reveal that complete deterministic conversion as well as pump-photon revival can be achieved at a finite propagation distance. We also find that high conversion efficiencies can be …
High dimensional quantum states are of fundamental interest for quantum information processing. They give access to large Hilbert spaces and, in turn, enable the encoding of quantum information on multiple modes. One method to create such quantum states is parametric down-conversion (PDC) in waveguide arrays (WGAs) which allows for the creation of highly entangled photon-pairs in controlled, easily accessible spatial modes, with unique spectral properties. In this paper we examine both theoretically and experimentally the PDC process in a lithium niobate WGA. We measure the spatial and spectra…
Phase-Selected Efficient Single-Photon Frequency Conversion via Local Fano Resonance in a Two-Giant-Atom Waveguide-QED System
Key Laboratory of Opto-electronic Control and Detection Technology of University of Hunan Province, and College of Physics and Electronic Engineering, Hengyang Normal University（衡阳师范学院光电控制与检测技术湖南省重点实验室及物理与电子工程学院）；Key Laboratory of Low Dimensional Quantum Structures and Quantum Control of Ministry of Education，Hunan Normal University（湖南师范大学教育部低维量子结构与量子控制重点实验室）
We analyze the process of simultaneous photon pair generation and quantum walks realized by spontaneous parametric down conversion of a pump beam in a quadratic nonlinear waveguide array. We demonstrate that this flexible platform allows for creating quantum states with different spatial correlations. In particular, we predict that the output photon correlations can be switched from photon bunching to antibunching controlled entirely classically by varying the temperature of the array or the spatial profile of the pump beam.
Modal phase matching (MPM) is a widely used phase matching technique in Al$_x$Ga$_{1-x}$As and other $χ^{(2)}$ nonlinear waveguides for efficient wavelength conversions. The use of a non-fundamental spatial mode compensates the material dispersion but also reduces the spatial overlap of the three interacting waves and therefore limits the conversion efficiency. In this work, we develop a technique to increase the nonlinear overlap by modifying the material nonlinearity, instead of the traditional method of optimizing the modal field profiles. This could eliminate the limiting factor of low spa…
We demonstrate quantum walks of correlated photons in a 2D network of directly laser written waveguides coupled in a 'swiss cross' arrangement. The correlated detection events show high-visibility quantum interference and unique composite behaviour: strong correlation and independence of the quantum walkers, between and within the planes of the cross. Violations of a classically defined inequality, for photons injected in the same plane and in orthogonal planes, reveal non-classical behaviour in a non-planar structure.
Counter-propagating parametric conversion processes in non-linear bulk crystals have been shown to feature unique properties for efficient narrowband frequency conversion. In quantum optics, the generation of photon pairs with a counter-propagating parametric down-conversion process (PDC) in a waveguide, where signal and idler photons propagate in opposite directions, offers unique material-independent engineering capabilities. However, realizing counter-propagating PDC necessitates quasi-phase-matching (QPM) with extremely short poling periods. Here, we report on the generation of counter-pro…
We report 10-ps correlated photon pair generation in periodically-poled reverse-proton-exchange lithium niobate waveguides with integrated mode demultiplexer at a wavelength of 1.5-um and a clock of 10 GHz. Using superconducting single photon detectors, we observed a coincidence to accidental count ratio (CAR) as high as 4000. The developed photon-pair source may find broad application in quantum information systems as well as quantum entanglement experiments.
We show that two-photon transport is strongly correlated in one-dimensional waveguide coupled to a two-level system. The exact S-matrix is constructed using a generalized Bethe-Ansatz technique. We show that the scattering eigenstates of this system include a two-photon bound state that passes through the two-level system as a composite single particle. Also, the two-level system can induce effective attractive or repulsive interactions in space for photons. This general procedure can be applied to the Anderson model as well.
We report the characterization of correlated photon pairs generated in dispersion-engineered silicon slow-light photonic crystal waveguides pumped by picosecond pulses. We found that taking advantage of the 15 nm flat-band slow-light window (vg ~ c/30) the bandwidth for correlated photon-pair generation in 96 and 196 \mum long waveguides was at least 11.2 nm; while a 396 \mum long waveguide reduced the bandwidth to 8 nm (only half of the slow-light bandwidth due to the increased impact of phase matching in a longer waveguide). The key metrics for a photon-pair source: coincidence to accidental…
We report measurements of two-photon interference using a cw-pumped type-II spontaneous parametric down-conversion source based on a multimode perodically poled potassium titanyl phosphate waveguide. We have used the recently demonstrated technique of controlling the spatial characteristics of the down-conversion process via intermodal dispersion to generate photon pairs in fundamental transverse modes, thus ensuring their spatial indistinguishability. Good spatial overlap of photon modes within pairs has been verified using the Hong-Ou-Mandel interferometer and the preparation of polarization…
Photon-pair sources based on thin film lithium niobate on insulator technology have a great potential for integrated optical quantum information processing. We report on such a source of correlated twin-photon pairs generated by spontaneous parametric down conversion in a silicon nitride (SiN) rib loaded thin film periodically poled lithium niobate (LN) waveguide. The generated photon pairs have a wavelength centred at 1560\,nm compatible with present telecom infrastructure, a large bandwidth (21\,THz) and a brightness of $\sim 2.5\times 10^5$\,pairs/s/mW/GHz. The photons are correlated and ex…
We explore theoretically the feasibility of using frequency conversion by sum- or difference-frequency generation, enabled by three- wave-mixing, for selectively multiplexing orthogonal input waveforms that overlap in time and frequency. Such a process would enable a drop device for use in a transparent optical network using temporally orthogonal waveforms to encode different channels. We model the process using coupled-mode equations appropriate for wave mixing in a uniform second- order nonlinear optical medium pumped by a strong laser pulse. We find Green functions describing the process, a…
Full control over the spatio-temporal structure of quantum states of light is an important goal in quantum optics, to generate for instance single-mode quantum pulses or to encode information on multiple modes, enhancing channel capacities. Quantum light pulses feature an inherent, rich spectral broadband-mode structure. In recent years, exploring the use of integrated optics as well as source-engineering has led to a deep understanding of the pulse-mode structure of guided quantum states of light. In addition, several groups have started to investigate the manipulation of quantum states by me…
We investigate the transport properties of two photons inside a one-dimensional waveguide side-coupled to a single-mode nonlinear cavity. The cavity is filled with a nonlinear Kerr medium. Based on the Laplace transform method, we present analytic solution of quantum states of the transmitted and reflected two photons, which are initially prepared in a Lorentzian wave packet. The solution reveals how quantum correlation between the two photons emerge after the scattering by the nonlinear cavity. In particular, we show that the output wave function of the two photons in position space can be lo…
We report on a highly efficient waveguide resonator device for the production of 775 nm light using a titanium indiffused LiNbO3waveguide resonator. When scanning the resonance the device produces up to 110 mW of second harmonic power with 140 mW incident on the device - an external conversion efficiency of 75 %. The cavity length is also locked, using a Pound-Drever-Hall type locking scheme, involving feedback to either the cavity temperature or the laser frequency. With laser frequency feedback a stable output power of approximately 28 mW from a 52 mW pump is seen over one hour.
High-efficient and high-purity photon sources are highly desired for quantum information processing. We report the design of a chip-scale hybrid SixNy and thin film periodically-poled lithium niobate waveguide for generating high-purity type-II spontaneous parametric down conversion (SPDC) photons in telecommunication band. The modeled second harmonic generation efficiency of 225% W^(-1)*cm^(-2) is obtained at 1560nm. Joint spectral analysis is performed to estimate the frequency correlation of SPDC photons, yielding intrinsic purity with up to 95.17%. The generation rate of these high-purity …
We report on the implementation of quantum frequency conversion (QFC) between infrared (IR) and ultraviolet (UV) wavelengths by using single-stage upconversion in a periodically poled KTP waveguide. Due to the monolithic waveguide design, we manage to transfer a telecommunication band input photon to the wavelength of the ionic dipole transition of Yb${}^{+}$ at 369.5 nm. The external (internal) conversion efficiency is around 5\% (10\%). The high energy pump used in this converter introduces a spontaneous parametric downconversion (SPDC) process, which is a cause for noise in the UV mode. Usi…
Quantum frequency conversion (QFC) in nonlinear optical media is a powerful tool for temporal-mode selective manipulation of light. Recent attempts at achieving high mode selectivities and/or fidelities have had to resort to multi-dimensional optimization schemes to determine the system's natural Schmidt modes. Certain combinations of relative-group velocities between the relevant frequency bands, medium length, and temporal pulse widths have been known to achieve good selectivities (exceeding 80%) for temporal modes that are nearly identical to pump pulse shapes, even for high conversion effi…
We propose a novel scheme to generate polarization entanglement from spatially-correlated photon pairs. We experimentally realized a scheme by means of a spatial correlation effect in a spontaneous parametric down-conversion and a modified Michelson interferometer. The scheme we propose in this paper can be interpreted as a conversion process from spatial correlation to polarization entanglement.
We demonstrate photon-pair generation in a reverse proton exchanged waveguide fabricated on a periodically poled magnesium doped stoichiometric lithium tantalate substrate. Detected pairs are generated via a cascaded second order nonlinear process where a pump laser at wavelength of 1.55 $μ$m is first doubled in frequency by second harmonic generation and subsequently downconverted around the same spectral region. Pairs are detected at a rate of 42 per second with a coincidence to accidental ratio of 0.7. This cascaded pair generation process is similar to four-wave-mixing where two pump photo…
We analyze spontaneous parametric down-conversion in various experimentally feasible 1D quadratic nonlinear waveguide arrays, with emphasis on the relationship between the lattice's topological invariants and the biphoton correlations. Nontrivial topology results in a nontrivial "winding" of the array's Bloch waves, which introduces additional selection rules for the generation of biphotons. These selection rules are in addition to, and independent of existing control using the pump beam's spatial profile and phase matching conditions. In finite lattices, nontrivial topology produces single ph…
Entangled photons are pivotal elements in emerging quantum information technologies. While several schemes are available for the production of entangled photons, they typically require the assistance of cumbersome optical elements to couple them to other components involved in logic operations. Here, we introduce a scheme by which entangled photon pairs are directly generated as guided mode states in optical waveguides. The scheme relies on the intrinsic nonlinearity of the waveguide material, circumventing the use of bulky optical components. Specifically, we consider an optical fiber under n…
We report on an integrated non-degenerate narrowband photon pair source produced at 890 nm and 1320nm via type II parametric down-conversion in a periodically poled waveguide with high-reflective dielectric mirrors deposited on the waveguide end faces. The conversion spectrum consists of three clusters and only 3 to 4 longitudinal modes with about 150 MHz bandwidth in each cluster. The high conversion efficiency in the waveguide, together with the spectral clustering in the double resonator, leads to a high brightness of $3\times10^3~$pairs/(s$\cdot$mW$\cdot$MHz). The compact and rugged monoli…
We analyze theoretically spontaneous parametric down-conversion in a multimode nonlinear waveguide as a source of entangled pairs of spatial qubits, realized as superpositions of a photon in two orthogonal transverse modes of the waveguide. It is shown that by exploiting intermodal dispersion, down-conversion into the relevant pairs of spatial modes can be selected by spectral filtering, which also provides means to fine-tune the properties of the generated entangled state. We also discuss an inverting interferometer detecting the spatial parity of the input beam as a versatile tool to charact…
The ability to coherently convert the frequency and temporal waveform of single and entangled photons will be crucial to interconnect the various elements of future quantum information networks. Of particular importance in this context is the quantum frequency conversion of photons emitted by material systems able to store quantum information, so called quantum memories. There have been significant efforts to implement quantum frequency conversion using non linear crystals, with non classical light from broadband photon pair sources and solid state emitters. However, so far, solid state quantu…
Sources of spectrally engineered photonic states are a key resource in several quantum technologies. Of particular importance are the so-called factorizable biphoton states which possess no spectral entanglement and hence, are ideal for heralded generation of high-purity single photons. An essential prerequisite for generating these states through nonlinear frequency conversion is the control over the group indices of the photonic modes of the source. Here, we show that thin-film lithium niobate on insulator (LNOI) is an excellent platform for this purpose. We design and fabricate periodically…
A new method for generating entangled photons with controllable frequency correlation via spontaneous parametric down-conversion (SPDC) is presented. The method entails initiating counter-propagating SPDC in a single-mode nonlinear waveguide by pumping with a pulsed beam perpendicular to the waveguide. The method offers several advantages over other schemes, including the ability to generate frequency-correlated photon pairs regardless of the dispersion characteristics of the system. Numerical evidence demonstrates the improvement provided by this source in the special case of frequency-correl…
Many technologies in quantum photonics require cryogenic conditions to operate. However, the underlying platform behind active components such as switches, modulators and phase shifters must be compatible with these operating conditions. To address this, we demonstrate an electro-optic polarisation converter for 1550nm light at 0.8K in titanium in-diffused lithium niobate waveguides. To do so, we exploit the electro-optic properties of lithium niobate to convert between orthogonal polarisation modes with a fiber-to-fiber transmission >43%. We achieve a modulation depth of 23.6 +/-3.3dB and a c…
Systems of atoms coupled to a single or few waveguide modes provide a testbed for physically and practically interesting interference effects. We consider the dynamics of a pair of atoms, approximated as two-level quantum emitters, coupled to a linear guided mode. In particular, we analyze the evolution of an initial state in which both atoms are excited, which is expected to decay into an asymptotic two-photon state. We investigate the lifetime of the initial configuration and the properties of the asymptotic photon correlations, and analyze the probability that the two photons are emitted in…
We report an experiment demonstrating quantum frequency conversion of weak light pulses compatible with atomic quantum memories to telecommunication wavelengths. We use a PPLN nonlinear waveguide to convert weak coherent states at the single photon level with a duration of 30ns from a wavelength of 780nm to 1552nm. We measure a maximal waveguide internal (external) conversion efficiency eta_int = 0.41 (eta_ext = 0.25), and we show that the signal to noise ratio (SNR) is good enough to reduce the input photon number below 1. In addition, we show that the noise generated by the pump beam in the …
We study modal characteristics of a customized ridge waveguide in Lithium Niobate designed to generate twin photons at telecom wavelength. A quantum analysis of SPDC predicts the possible down conversion processes and optimizes the input beam parameters for fundamental mode emission. Further, a Joint Spectral Amplitude (JSA) analysis ensures the generation of signal/idler at 1550 nm in the customized LN waveguide. A calculation of the parametric down conversion (PDC) signal power shows a dependence of L^(3/2) for a waveguide compared to a linear dependence in case of bulk crystal.
We study the spectral properties of Spontaneous Parametric Down Conversion in a periodically poled waveguided structure of KTP crystal pumped by ultra-short pulses. Our theoretical analysis reveals a strongly multimode and asymmetric structure of the two-photon spectral amplitude for type-II SPDC. Experimental evidence, based on Hong-Ou-Mandel polarization interference with narrowband filtering, confirms this result.
We demonstrate the generation of quantum-correlated photon pairs from a Si photonic-crystal coupled-resonator optical waveguide. A slow-light supermode realized by the collective resonance of high-Q and small-mode-volume photonic-crystal cavities successfully enhanced the efficiency of the spontaneous four-wave mixing process. The generation rate of photon pairs was improved by two orders of magnitude compared with that of a photonic-crystal line defect waveguide without a slow-light effect.
In this paper, we propose a method for the generation of higher dimensional modal entanglement through type II spontaneous parametric down conversion process using a three waveguide directional coupler in a periodically poled lithium niobate substrate. We show that by a proper design, it is possible to achieve an output state of two photons occupying three different spatial modes. The advantage of using such waveguide structure is its flexibility and the design space availability to achieve desired characteristics of the photon pairs generated in the down conversion process
In this paper, we begin with a model of a $Λ$-type atom whose both transitions are chirally coupled to a waveguide and then extend the model to its giant-atom version. We investigate the single-photon scatterings of the giant-atom model in both the Markovian and non-Markovian regimes. It is shown that the chiral atom-waveguide couplings enable nonreciprocal, reflectionless, and efficient frequency conversion, while the giant-atom structure introduces intriguing interference effects to the scattering behaviors, such as ultra-narrow scattering windows. The chiral giant-atom model exhibits quite …
We report on energy-time and time-bin entangled photon-pair sources based on a periodically poled lithium niobate (PPLN) waveguide. Degenerate twin photons at 1314 nm wavelength are created by spontaneous parametric down-conversion and coupled into standard telecom fibers. Our PPLN waveguide features a very high conversion efficiency of about 10^(-6), roughly 4 orders of magnitude more than that obtained employing bulk crystals. Even if using low power laser diodes, this engenders a significant probability for creating two pairs at a time - an important advantage for some quantum communication…
We report experimental determination of the phase-matching function for type-II three-wave mixing in a periodically poled KTiOPO_4 waveguide in the 792-815 nm spectral region. The measurement was performed by sum-frequency generation of spectrally tuned fundamental components. Strong dependence of the observed signal on the excited spatial modes in the waveguide has been observed and fully interpreted. These results indicate a route to employ the waveguide for spontaneous parametric down-conversion producing photon pairs in well-defined spatial modes.
We report the first (to our knowledge) observation of correlated photon emission in hydrogenated amorphous- silicon waveguides. We compare this to photon generation in crystalline silicon waveguides with the same geome- try. In particular, we show that amorphous silicon has a higher nonlinearity and competes with crystalline silicon in spite of higher loss.
This work proposes and analyses a novel approach for the generation of separable (quantum uncorrelated) photon pairs based on spontaneous parametric down-conversion in Bragg reflection waveguides composed of semiconductor AlGaN layers. This platform allows the removal of any spectral correlation between paired photons that propagate in different spatial modes. The photons can be designed to show equal or different spectra by tuning the structural parameters and hence the dispersion of the waveguide.
