Sources of spectrally engineered photonic states are a key resource in several quantum technologies. Of particular importance are the so-called factorizable biphoton states which possess no spectral entanglement and hence, are ideal for heralded generation of high-purity single photons. An essential prerequisite for generating these states through nonlinear frequency conversion is the control over the group indices of the photonic modes of the source. Here, we show that thin-film lithium niobate on insulator (LNOI) is an excellent platform for this purpose. We design and fabricate periodically poled ridge waveguides in LNOI to demonstrate group index engineering of its guided photonic modes and harness this control to experimentally realize on-chip group index matched type-II sum-frequency generation (SFG) and photon-pair creation through spontaneous parametric down-conversion (SPDC). Also, we numerically study the role of the top cladding layer in tuning the dispersion properties of the ridge waveguide structures and reveal a distinctive difference between the air and silica-clad designs which are currently among the two most common device cladding configurations in LNOI. We expect that these results will be relevant for various classical and quantum applications where dispersion control is crucial in tailoring the nonlinear response of the LNOI-based devices.
We demonstrate monolithically defined grating couplers in $Z$-cut lithium niobate on insulator for efficient vertical coupling between an optical fiber and a single mode waveguide. The grating couplers exhibit $\sim 44.6\%$/coupler and $\sim 19.4\%$/coupler coupling efficiency for TE and TM polarized light respectively. Taperless grating couplers are investigated to realize a more compact design.
We demonstrate efficient second harmonic generation in a quasi-phase-matched, high quality factor ($Q_0 \approx 5.3\times 10^5$) racetrack microresonator. The observed normalized conversion efficiency is about $3.8\%~mW^{-1}$.
Integrated Photonic Quantum Computing: From Silicon to Lithium Niobate
Tongji University（同济大学）；Shanghai University（上海大学）；National University of Singapore（新加坡国立大学）；Nanyang Technological University（南洋理工大学）；University of Bristol（布里斯托大学）；The Hong Kong Polytechnic University（香港理工大学）
Prospective integrated quantum optical technologies will combine nonlinear optics and components requiring cryogenic operating temperatures. Despite the prevalence of integrated platforms exploiting $χ^{(2)}$-nonlinearities for quantum optics, for example used for quantum state generation and frequency conversion, their material properties at low temperatures are largely unstudied. Here, we demonstrate the first second harmonic generation in a fiber-coupled lithium niobate waveguide at temperatures down to 4.4K. We observe a reproducible shift in the phase-matched pump wavelength within the te…
Existing nonlinear-optic implementations of pure, unfiltered heralded single-photon sources do not offer the scalability required for densely integrated quantum networks. Additionally, lithium niobate has hitherto been unsuitable for such use due to its material dispersion. We engineer the dispersion and the quasi-phasematching conditions of a waveguide in the rapidly emerging thin-film lithium niobate platform to generate spectrally separable photon pairs in the telecommunications band. Such photon pairs can be used as spectrally pure heralded single-photon sources in quantum networks. We est…
The absence of the single-photon nonlinearity has been a major roadblock in developing quantum photonic circuits at optical frequencies. In this paper, we demonstrate a periodically-poled thin film lithium niobate microring resonator (PPLNMR) that reaches 5,000,000%/W second harmonic conversion efficiency---almost 20-fold enhancement over the state-of-the-art---by accessing its largest $χ^{(2)}$ tensor component $d_{33}$ via quasi-phase matching. The corresponding single photon coupling rate $g/2π$ is estimated to be 1.2 MHz, which is an important milestone as it approaches the dissipation rat…
Squeezed light is a key quantum resource that enables quantum advantages for sensing, networking, and computing applications. The scalable generation and manipulation of squeezed light with integrated platforms are highly desired for the development of quantum technology with continuous variables. In this letter, we demonstrate squeezed light generation with thin-film lithium niobate integrated photonics. Para-metric down-conversion is realized with quasi-phase matching using ferroelectric domain engineering. With sub-wavelength mode confinement, efficient nonlinear processes can be observed w…
Quantum light sources in the mid-infrared (MIR) band play an important role in many applications, such as quantum sensing, quantum imaging, and quantum communication. However, there is still a lack of high-quality quantum light sources in the MIR band, such as the spectrally pure single-photon source. In this work, we present the generation of spectrally-pure state in an optimized poled lithium niobate crystal using a metaheuristic algorithm. In particular, we adopt the particle swarm optimization algorithm to optimize the duty cycle of the poling period of the lithium niobate crystal. With ou…
Chip-integrated nonlinear photonics holds the key for advanced optical information processing with superior performance and novel functionalities. Here, we present an optimally mode-matched, periodically poled lithium niobate nanowaveguide for efficient parametric frequency conversions on chip. Using a 4-mm nanowaveguide with subwavelength mode confinement, we demonstrate second harmonic generation with efficiency over $2200\%~W^{-1}cm^{-2}$, and broadband difference frequency generation with similar efficiency over a 4.5-THz spectral span. These allow us to generate correlated photon pairs ov…
We outline the design for a photonic crystal resonator made in a hybrid Silicon/Lithium Niobate material system. Using the index contrast between silicon and lithium niobate, it is possible to guide and confine photonic resonances in a thin film of silicon bonded on top of lithium niobate. Quality factors greater than $10^6$ at optical wavelength scale mode volumes are achievable. We show that patterning electrodes on such a system can yield an electro-optic coupling rate of 0.6 GHz/V (4 pm/V).
Lithium niobate is a multi-functional material, which has been regarded as one of the most promising platform for the multi-purpose optical components and photonic circuits. Targeting at the miniature optical components and systems, lithium niobate microstructures with feature sizes of several to hundreds of micrometers have been demonstrated, such as waveguides, photonic crystals, micro-cavities, and modulators, et al. In this paper, we presented subwavelength nanograting metasurfaces fabricated in a crystalline lithium niobate film, which hold the possibilities towards further shrinking the …
The integration of quantum emitters with integrated photonics enables complex quantum photonic circuits that are necessary for photonic implementation of quantum simulators, computers, and networks. Thin-film lithium niobate is an ideal material substrate for quantum photonics because it can tightly confine light in small waveguides and has a strong electro-optic effect that can switch and modulate single photons at low power and high speed. However, lithium niobite lacks efficient single-photon emitters, which are essential for scalable quantum photonic circuits. We demonstrate deterministic …
We demonstrate second harmonic generation of blue light on an integrated thin-film lithium niobate waveguide and observe a conversion efficiency of $η_0= 33000\%/\text{W-cm}^2$, significantly exceeding previous demonstrations.
We demonstrate efficient first-order quasi-phase-matched second-harmonic generation in a surface periodically poled Ti:indiffused lithium niobate waveguide; 6 mW of continuous-wave blue radiation (wavelength = 412.6 nm) was produced showing the potential of surface domain inversion for efficient nonlinear waveguide interactions.
Lithium Niobate (LN or just niobate) thin-film micro-photonic resonators have promising prospects in many applications including high efficiency electro-optic modulators, optomechanics and nonlinear optics. This paper presents free-standing thin-film lithium niobate photonic resonators on a silicon platform using MEMS fabrication technology. We fabricated a 35um radius niobate disk resonator that exhibits high intrinsic optical quality factor (Q) of 484,000. Exploiting the optomechanical interaction from the released free-standing structure and high optical Q, we were able to demonstrate acous…
Lithium Niobate on insulator (LNOI) photonics promises to combine the excellent nonlinear properties of Lithium Niobate with the high complexity achievable by high contrast waveguides. However, to date, fabrication challenges have resulted in high-loss and sidewall-angled waveguides, limiting its applicability. We report LNOI single mode waveguides with ultra low propagation loss of 0.4 dB/cm and sidewall angle of 75°. Our results open the route to a highly efficient photonic platform with applications ranging from high-speed telecommunication to quantum technology.
Many technologies in quantum photonics require cryogenic conditions to operate. However, the underlying platform behind active components such as switches, modulators and phase shifters must be compatible with these operating conditions. To address this, we demonstrate an electro-optic polarisation converter for 1550nm light at 0.8K in titanium in-diffused lithium niobate waveguides. To do so, we exploit the electro-optic properties of lithium niobate to convert between orthogonal polarisation modes with a fiber-to-fiber transmission >43%. We achieve a modulation depth of 23.6 +/-3.3dB and a c…
We demonstrate electro-optic tuning of an on-chip lithium niobate microresonator with integrated in-plane microelectrodes. First two metallic microelectrodes on the substrate were formed via femtosecond laser process. Then a high-Q lithium niobate microresonator located between the microelectrodes was fabricated by femtosecond laser direct writing accompanied by focused ion beam milling. Due to the efficient structure designing, high electro-optical tuning coefficient of 3.41 pm/V was observed.
We develop a chip-scale cavity optomechanical system in single-crystal lithium niobate that exhibits high optical quality factors and a large frequency-quality product as high as $3.6\times 10^{12}$ Hz at room temperature and atmosphere. The excellent optical and mechanical properties together with the strong optomechanical coupling allow us to efficiently excite the coherent regenerative optomechanical oscillation operating at 375.8 MHz with a threshold power of 174 ${\rm μW}$ in the air. The demonstrated lithium niobate optomechanical device enables great potential for achieving electro-opti…
Integrated thin-film lithium niobate platform has recently emerged as a promising candidate for next-generation, high-efficiency wavelength conversion systems that allow dense packaging and mass-production. Here we demonstrate efficient, phase-matched second harmonic generation in lithographically-defined thin-film lithium niobate waveguides with sub-micron dimensions. Both modal phase matching in fixed-width waveguides and quasi-phase matching in periodically grooved waveguides are theoretically proposed and experimentally demonstrated. Our low-loss (~ 3.0 dB/cm) nanowaveguides possess normal…
In this paper, we proposed and numerically demonstrated a giant enhancement up to 108 in both forward and backward propagation of the Second Harmonic Generation by combining the high-quality factor cavities of the Bound States in the Continuum and the excellent nonlinear optical crystal of lithium niobate. The enhancement factor is defined as the ratio of the second harmonic signal generated by the structure (lithium niobate membrane with Si grating) divided by the signal generated by lithium niobate membrane alone. Furthermore, a minimum interaction time of 350 ps is achieved despite the etch…
The lithium niobate integrated photonic platform has recently shown great promise in nonlinear optics on a chip scale. Here, we report second-harmonic generation in a high-Q lithium niobate microring resonator through modal phase matching, with a conversion efficiency of 1,500% W$^{-1}$. Our device also allows us to observe difference-frequency generation in the telecom band. Our work demonstrates the great potential of the lithium niobate integrated platform for nonlinear wavelength conversion with high efficiencies.
We report on backward second-harmonic-generation in bulk periodically poled congruent lithium niobate with a 3.2 microns period. A tunable continuous-wave Ti:sapphire laser allowed us exciting two resonant quasi-phase-matching orders in the backward configuration. The resonances were also resolved by temperature tuning and interpolated with standard theory to extract relevant information on the sample.
We demonstrate the integration of amorphous tungsten silicide superconducting nanowire single-photon detectors on titanium in-diffused lithium niobate waveguides. We show proof-of-principle detection of evanescently-coupled photons of 1550nm wavelength using bidirectional waveguide coupling for two orthogonal polarization directions. We investigate the internal detection efficiency as well as detector absorption using coupling-independent characterization measurements. Furthermore, we describe strategies to improve the yield and efficiency of these devices.
We demonstrate efficient multicycle terahertz pulse generation at 14.6 THz from large-area lithium niobate crystals by using high-energy (up to 2 J) femtosecond Ti:sapphire laser pulses. Such terahertz radiation is produced by phase-matched optical rectification in lithium niobate. Experimentally, we achieve maximal terahertz energy of 0.71 mJ with conversion efficiency of $\sim$0.04%. We also find that the effective interaction length for optimal terahertz conversion is fundamentally limited by terahertz absorption, laser pulse stretching by material dispersion, and terahertz-induced nonlinea…
We report an application of the tri-dimensional pseudo-spectral time domain algorithm, that solves with accuracy the nonlinear Maxwell's equations, to predict second harmonic generation in lithium niobate ridge-type waveguides with high index contrast. Characteristics of the nonlinear process such as conversion efficiency as well as impact of the multimode character of the waveguide are investigated as a function of the waveguide geometry in uniformly and periodically poled medium.
We show the proof-of-principle detection of light at 1550 nm coupled evanescently from a titanium in-diffused lithium niobate waveguide to a superconducting transition edge sensor. The coupling efficiency strongly depends on the polarization, the overlap between the evanescent field, and the detector structure. We experimentally demonstrate polarization sensitivity of this coupling as well as photon-number resolution of the integrated detector. The combination of transition edge sensors and lithium niobate waveguides can open the field for a variety of new quantum optics experiments.
Lithium Niobate (LN) is an important nonlinear optical material. Here we demonstrate LN microdisk resonators that feature optical quality factor ~ 100,000, realized using robust and scalable fabrication techniques, that operate over a wide wavelength range spanning visible and near infrared. Using our resonators, and leveraging LN's large second order optical nonlinearity, we demonstrate on-chip second harmonic generation with a conversion efficiency of 0.109 W-1.
Second harmonic generation is investigated in lithium niobate channels realized by proton exchange and quasi-phase-matched by surface periodic-poling. The reduction in conversion efficiency at high powers is interpreted in terms of multi-photon absorption via two-color terms, yielding an estimate of the dominating three-photon process.
Thin-film lithium niobate is an attractive integrated photonics platform due to its low optical loss and favorable optical nonlinear and electro-optic properties. However, in applications such as second harmonic generation, frequency comb generation, and microwave-to-optics conversion, the device performance is strongly impeded by the photorefractive effect inherent in thin-films. In this paper, we show that the dielectric cladding on lithium niobate microring resonator has a significant influence on the photorefractive effect. By removing the dielectric cladding layer, the photorefractive eff…
We demonstrate conversion of up to 4.5 GHz-frequency microwaves to 1500 nm-wavelength light using optomechanical interactions on suspended thin-film lithium niobate. Our method utilizes an interdigital transducer that drives a free-standing 100 $μ$m-long thin-film acoustic resonator to modulate light travelling in a Mach-Zehnder interferometer or racetrack cavity. Owing to the strong microwave-to-acoustic coupling offered by the transducer in conjunction with the strong photoelastic, piezoelectric, and electro-optic effects of lithium niobate, we achieve a half-wave voltage of $V_π$ = 4.6 V an…
Lithium niobate is an excellent photonic material with large $χ^2$ and $χ^3$ nonlinearities. Recent breakthroughs in nanofabrication technology have enabled ultralow-loss nanophotonic devices based on a lithium-niobate-on-insulator (LNOI) platform. Here we present an overview of recent developments in the LNOI platform for on-chip optical frequency comb generation. These devices could lead to new opportunities for integrated nonlinear photonic devices for classical and quantum photonic applications.
We demonstrate an ultralow loss monolithic integrated lithium niobate photonic platform consisting of dry-etched subwavelength waveguides. We show microring resonators with a quality factor of 10$^7$ and waveguides with propagation loss as low as 2.7 dB/m.
We demonstrate integration of an amorphous silicon photodetector with thin film lithium niobate photonic platform operating in the visible wavelength range. We present the details of the design, fabrication, integration and experimental characterization of this metal-semiconductor-metal photodetector that features responsivity of 22 mA/W to 37mA/W over the wide optical bandwidth spanning 635 nm to 850 nm wavelengths range.
Modern communication networks require high performance and scalable electro-optic modulators that convert electrical signals to optical signals at high speed. Existing lithium niobate modulators have excellent performance but are bulky and prohibitively expensive to scale up. Here we demonstrate scalable and high-performance nanophotonic electro-optic modulators made of single-crystalline lithium niobate microring resonators and micro-Mach-Zehnder interferometers. We show a half-wave electro-optic modulation efficiency of 1.8V$\cdot$cm and data rates up to 40 Gbps.
Lithium niobate on insulator (LNOI) waveguides, as an emerging technology, have proven to offer a promising platform for integrated optics, due to their strong optical confinement comparable to silicon on insulator (SOI) waveguides, while possessing the versatile properties of lithium niobate, such as high electro-optic coefficients. In this paper, we show that mode hybridization, a phenomenon widely found in vertically asymmetric waveguides, can be efficiently modulated in an LNOI ridge waveguide by electro-optic effect, leading to a polarization mode converter with 97% efficiency. Moreover, …
We report on two novel ways for patterning Lithium Niobate (LN) at submicronic scale by means of focused ion beam (FIB) bombardment. The first method consists of direct FIB milling on LiNbO3 and the second one is a combination of FIB milling on a deposited metallic layer and subsequent RIE (Reactive Ion Etching) etching. FIB images show in both cases homogeneous structures with well reproduced periodicity. These methods open the way to the fabrication of photonic crystals on LiNbO3 substrates.
We report on fabrication of crystalline lithium niobate microresonators with quality factors above 10^7 as measured around 770 nm wavelength. Our technique relies on femtosecond laser micromachining for patterning a mask coated on the lithium niobate on insulate (LNOI) into a microdisk, followed by a chemo-mechanical polishing process for transferring the disk-shaped pattern to the LNOI. Nonlinear processes including second harmonic generation and Raman scattering have been demonstrated in the fabricated microdisk.
Optical microresonators have recently attracted a growing attention in the photonics community. Their applications range from quantum electro-dynamics to sensors and filtering devices for optical telecommunication systems, where they are likely to become an essential building block. The integration of nonlinear and electro-optical properties in the resonators represents a very stimulating challenge, as it would incorporate new and more advanced functionality. Lithium niobate is an excellent candidate material, being an established choice for electro-optic and nonlinear optical applications. He…
High quality lithium niobate thin film microresonators provide an ideal platform for on-chip nonlinear optics applications. However, the phase matching condition for efficient parametric process sets a high requirement for fabrication control. Here we demonstrate a photonic molecular structure composed of two strongly coupled lithium niobate microdisks of different diameters fabricated using femtosecond laser micromachining and focused ion beam milling. With a continuous wave excitation, rich nonlinear optical processes including cascaded four-wave mixing and stimulated Raman scattering were o…
We report on fabrication of depressed cladding optical waveguides buried in lithium niobate crystal with shaped femtosecond laser pulses. Depressed cladding waveguides of variable mode-field sizes are fabricated by forming the four sides of the cladding using a slit-beam shaping technique. We show that the waveguides fabricated by our technique allows single-mode propagation of the light polarized in both vertical and horizontal directions.
We review measurements in the literature regarding Kerr nonlinearity of lithium niobate. Of particular interest is to separate the value of the electronic Kerr nonlinearity and the strength of the delayed Raman nonlinearity. The spectral shape of the Raman response in LN is discussed and we restrict ourselves to the case where the pump is polarized along the optical axis. This configuration is important for so-called type 0 noncritical interaction, which is used in QPM devices and in recent supercontinuum generation and few-cycle soliton compression experiments.
In this paper, by cascading several bichromatic photonic crystals we demonstrate that the quality factor can be much larger compared with that in an isolated cavity without increasing the total size of the device. We take lithium niobate photonic crystal as an example to illustrate that the simulated quality factor of the cascaded cavity can attain 10^5 with a 70° slant angle, which is an order of magnitude larger than that in isolated cavity. The device can be fabricated easily by current etching technique for lithium niobate. We have fabricated the proposed device experimentally including ho…
Erbium-doped lithium niobate high-Q microdisk cavities were fabricated in batches by UV exposure, inductively coupled plasma reactive ion etching and chemo-mechanical polishing. The stimulated emission at 1531.6 nm was observed under the pump of a narrow-band laser working at 974 nm in erbium-doped lithium niobate microdisk cavity with threshold down to 400 μW and a conversion efficiency of 3.1{\times}10^{-4} %, laying the foundation for the LNOI integrated light source research.
Much progress, both experimentally and theoretically, has recently been made towards optical frequency comb generation from continuously pumped second-order nonlinear systems. Here, we present the first observations towards finding an integrated solution for such a system, using a titanium indiffused lithium niobate waveguide resonator. These results are compared to recently developed theory for equivalent systems. The system is seen to exhibit strong instabilities, which require further investigation in order to fully determine the suitability of this platform for stable optical frequency com…
We demonstrate acousto-optic phase modulators in X-cut lithium niobate films on sapphire, detailing the dependence of the piezoelectric and optomechanical coupling coefficients on the crystal orientation. This new platform supports highly confined, strongly piezoelectric mechanical waves without suspensions, making it a promising candidate for broadband and efficient integrated acousto-optic devices, circuits, and systems.
We report intracavity Bragg scattering induced by photorefractive (PR) effect in high-Q lithium niobate (LN) ring resonators at cryogenic temperatures. We show that, when a cavity mode is strongly excited, the PR effect imprints a long-lived periodic space-charge field. This residual field in turn creates a refractive index modulation pattern that dramatically enhances the back scattering of an incoming probe light, and results in selective and reconfigurable mode splittings. This PR-induced Bragg scattering effect, despite being undesired for many applications, could be utilized to enable opt…
