We construct combined electric and magnetic field variables which independently represent energy flows in the forward and backward directions respectively, and use these to re-formulate Maxwell's equations. These variables enable us to not only judge the effect and significance of backward-travelling field components, but also to discard them when appropriate. They thereby have the potential to simplify numerical simulations, leading to potential speed gains of up to 100% over standard FDTD or PSSD simulations. We present results for various illustrative situations, including an example application to second harmonic generation in periodically poled lithium niobate. These field variables are also used to derive both envelope equations useful for narrow-band pulse propagation, and a second order wave equation. Alternative definitions are also presented.
I apply the method of characteristics to both bi-directional and uni-directional pulse propagation in dispersionless media containing nonlinearity of arbitrary order. The differing analytic predictions for the shocking distance quantify the effects of the uni-directional approximation used in many pulse propagation models. Results from numerical simulations support the theoretical predictions, and reveal the nature of the coupling between forward and backward waves.
I derive directional wave equations useful for pulses propagating in beam, rod, pipe, and disk geometries by using a cylindrical coordinate system; the scheme works equally well for either long multi-cycle or single-cycle ultrashort pulses. This is achieved by means of a factorization procedure that conveniently generates exact bi-directional and first order wave equations after the selection of propagation direction - either axial, radial, or even angular. I then discuss how to reduce these to a uni-directional form, and discuss the necessary approximation, which is essentially a paraxial app…
I calculate the limitations on the widely-used forward-only (uni-directional) propagation assumption by considering the effects of transverse effects (e.g. diffraction). The starting point is the scalar second order wave equation, and simple predictions are made which aim to clarify the forward-backward coupling limits on diffraction strength. The result is unsurprising, being based on the ratio of transverse and total wave vectors, but the intent is to present a derivation directly comparable to a recently published \emph{nonlinearity} constrained limits on the uni-directional approximation […
I derive unidirectional wave equations for fields propagating in materials with both electric and magnetic dispersion and nonlinearity. The derivation imposes no conditions on the pulse profile except that the material modulates the propagation slowly, that is, that loss, dispersion, and nonlinearity have only a small effect over the scale of a wavelength. It also allows a direct term-to-term comparison of the exact bidirectional theory with its approximate unidirectional counterpart.
I construct combined electric and magnetic field variables which independently represent energy flows in the forward and backward directions respectively, and use these to re-formulate Maxwell's equations. The emphasis is on detailed calculations, with a more general overview being published in Phys. Rev. A72 and arXiv. These directional variables enable us to not only judge the effect and significance of backward-travelling field components, but also to discard them when appropriate. They thereby have the potential to simplify numerical simulations, leading to potential speed gains of up to 1…
Propagation equations for optical pulses are needed to assist in describing applications in ever more extreme situations -- including those in metamaterials with linear and nonlinear magnetic responses. Here I show how to derive a single first order propagation equation using a minimum of approximations and a straightforward "factorization" mathematical scheme. The approach generates exact coupled bi-directional equations, after which it is clear that the description can be reduced to a single uni-directional first order wave equation by means of a simple "slow evolution" approximation, where …
I derive a temporally propagated uni-directional optical pulse equation valid in the few cycle limit. Temporal propagation is advantageous because it naturally preserves causality, unlike the competing spatially propagated models. The exact coupled bi-directional equations that this approach generates can be efficiently approximated down to a uni-directional form in cases where an optical pulse changes little over one optical cycle. They also permit a direct term-to-term comparison of the exact bi-directional theory with its corresponding approximate uni-directional theory. Notably, temporal p…
We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick" scheme) or a longer pulse sequence (a "chiral pulse train" scheme). In both cases, rotational control is achieved by varying the polarization of and the time delay between the consecutive laser pulses. Using the technique of polarization sensitive resonance-enhanced multi-photon ionization, we show that both methods produce significant rotational directiona…
I present an overview of pulse propagation methods used in nonlinear optics, covering both full-field and envelope-and-carrier methods. Both wideband and narrowband cases are discussed. Three basic forms are considered -- those based on (a) Maxwell's equations, (b) directional fields, and (c) the second order wave equation. While Maxwell's equations simulators are the most general, directional field methods can give significant computational and conceptual advantages. Factorizations of the second order wave equation complete the set by being the simplest to understand. One important conclusion…
We show that propagation of ultrashort (few-cycle) pulses in nonlinear Drude metamaterials with both electric and magnetic Kerr nonlinearities is described by coupled generalized Short Pulse Equations. The resulting system of equations generalizes to the case of metamaterials both the Short Pulse Equation and its vector generalizations which describe the few-cycle pulses in dielectric optical fibers beyond the slowly varying envelope approximation leading to the nonlinear Schroedinger equation.
In this paper we numerically study supercontinuum generation by pumping a silicon nitride waveguide, with two zero-dispersion wavelengths, with femtosecond pulses. The waveguide dispersion is designed so that the pump pulse is in the normal-dispersion regime. We show that because of self-phase modulation, the initial pulse broadens into the anomalous-dispersion regime, which is sandwiched between the two normal-dispersion regimes, and here a soliton is formed. The interaction of the soliton and the broadened pulse in the normal-dispersion regime causes additional spectral broadening through fo…
Unidirectional pulse propagation equations [UPPE, Phys. Rev. E 70, 036604 (2004)] have provided a theoretical underpinning for computer-aided investigations into dynamics of high-power ultrashort laser pulses and have been successfully utilized for almost a decade. Unfortunately, they are restricted to applications in bulk media or, with additional approximations, to simple waveguide geometries in which only a few guided modes can approximate the propagating waveform. The purpose of this work is to generalize the directional pulse propagation equations to structures characterized by strong ref…
The propagation of an electromagnetic pulse in a plasma is studied for pulse durations that are comparable to the plasma period. When the carrier frequency of the incident pulse is much higher than the plasma frequency, the pulse propagates without distortion at its group speed. When the carrier frequency is comparable to the plasma frequency, the pulse is distorted and leaves behind it an electromagnetic wake.
A parallel 2D+1 split-step Fourier method with Crank-Nicholson scheme running on multi-core shared memory architectures is developed to study the propagation of ultra-short high-intensity laser pulses in air. The parallel method achieves a near linear speed-up with results for the efficiency of more than 95% on a 24-core machine. This method is of great potential application in studying the long-distance propagation of the ultra-short high intensity laser pulses.
Forward and backward THz emission by ionizing two-color laser pulses in gas is investigated by means of a simple semi-analytical model based on Jefimenko's equation and rigorous Maxwell simulations in one and two dimensions. We find the emission in backward direction having a much smaller spectral bandwidth than in forward direction and explain this by interference effects. Forward THz radiation is generated predominantly at the ionization front and thus almost not affected by the opacity of the plasma, in excellent agreement with results obtained from a unidirectional pulse propagation model.
In this work, we perform a detailed review about the theoretical modeling of the optical propagation of ultra-short pulses in different scenarios of nonlinear optics. In particular, we focus our efforts on optical fibers and uniform media, with special attention on the white light continuum generation by using gases.
We review and extend the analogies between Gaussian pulse propagation and Gaussian beam diffraction. In addition to the well-known parallels between pulse dispersion in optical fiber and CW beam diffraction in free space, we review temporal lenses as a way to describe nonlinearities in the propagation equations, and then introduce further concepts that permit the description of pulse evolution in more complicated systems. These include the temporal equivalent of a spherical dielectric interface, which is used by way of example to derive design parameters used in a recent dispersion-mapped soli…
We report an asymmetric behavior of optical pulses during their propagation through a time-varying linear optical medium. The refractive index of the medium is considered to be varying with time and complex such that a sufficient amount of gain and loss is present to realize their effect on pulse propagation. We have exploited the universal formula for optical fields in time-varying media. Numerically simulated results reveal that pulses undergo opposite temporal shifts around their initial center position during their bi-directional propagation through the medium along with corresponding spec…
An effort was conducted to study temporal soliton pulse propagation in silicon nano-waveguides. These nonlinear phenomenas were studied both numerically and experimentally with phase-resolved Frequency Resolved Optical Gating. Soliton pulse broadening, as well as pulse splitting from two-photon absorption, was observed experimentally, and the simulations matched all of the experimental results. Further simulations with the validated model have demonstrated that compression can be observed in centimeter-length waveguides. This study has demonstrated the feasibility of self-sustaining soliton pu…
In this paper, the unidirectional pulse propagation equation generalized to structured media is derived. A fast modal transform linking the spatio-temporal representation of the field and its modal distribution is presented. This transform is used for solving the propagation equation by using a split-step algorithm. As an example, we present, to the best of our knowledge, the first numerical evidence of the generation of conical waves in highly multimodes waveguides.
The propagation of pulses through waveguides with subwavelength features, inhomogeneous transverse structure, and high index contrast cannot be described accurately using existing models in the presence of nonlinear effects. Here we report the development of a generalised full vectorial model of nonlinear pulse propagation and demonstrate that, unlike the standard pulse propagation formulation, the z-component of guided modes plays a key role for these new structures, and results in generalised definitions of the nonlinear coefficient $γ,$ $A_{eff}$, and mode orthognality. While new definition…
In this paper, the microwave pulse propagation transferred through a left-handed transmission line using Complementary Omega-Like Structures (COLS) loaded was studied. There was a stop band in transmission from 5.6GHz to 6.1GHz, and the anomalous dispersion was causes in this band. Negative group velocity corresponds to the case in which the peak of the pulse exited before the peak of the incident pulse had entered the sample. The negative group velocity reached (-0.27c~-1.85c).
Transient structural changes of Al$_2$O$_3$ on subatomic length scales following irradiation with an intense x-ray laser pulse (photon energy: 8.70 keV; pulse duration: 6 fs; fluence: 8$\times$10$^2$ J/cm$^{2}$) have been investigated by using an x-ray pump x-ray probe technique. The measurement reveals that aluminum and oxygen atoms remain in their original positions by $\sim$20 fs after the intensity maximum of the pump pulse, followed by directional atomic displacements at the fixed unit cell parameters. By comparing the experimental results and theoretical simulations, we interpret that el…
In this paper, we describe analytically the propagation of Airy-type pulses truncated by a finite-time aperture when second and third order dispersion effects are considered. The mathematical method presented here, based on the superposition of exponentially truncated Airy pulses, is very effective, allowing us to avoid the use of time-consuming numerical simulations. We analyze the behavior of the time truncated Ideal-Airy pulse and also the interesting case of a time truncated Airy pulse with a "defect" in its initial profile, which reveals the self-healing property of this kind of pulse sol…
Optical soliton pulses offer many applications within optical communication systems, but by definition a soliton is only subjected to second-order anomalous group-velocity-dispersion; an understanding of higher-order dispersion is necessary for practical implementation of soliton pulses. A numerical model of a waveguide was developed using the Nonlinear Schrodinger Equation, with parameters set to ensure the input pulse energy would be equal to the fundamental soliton energy. Higher-order group-velocity-dispersion was gradually increased, for various temporal widths and waveguide dispersions. …
This document contains my detailed calculation of the Generalised Few-cycle Envelope Approximation (GFEA) propagation equation reported and used in Phys. Rev. A (submitted) and its associated longer version at arXiv.org. This GFEA propagation equation is intended to be applicable to optical pulses only a few cycles long, a regime where the standard Slowly Varying Envelope Approximation (SVEA) fails.
I present a detailed derivation of wideband optical pulses interacting with a Raman transition in the kind of scheme currently used to generate the ultra broadband light fields needed to create ultrashort pulses. In contrast to the usual approach using separate field envelopes for the pump, Stokes, and anti-Stokes spectral lines, I use a single field envelope. This requires the inclusion of few-cycle corrections to the pulse propagation. The single-field model makes fewer approximations and is mathematically (and hence computationally) simpler, although it does require greater computational re…
We report time-resolved pulse self-steepening and temporal splitting in flint glass (SF11) in single-shot using broadband frequency-domain streak camera (B-FDSC). The broadband ($60$ nm) probe beam generated through a compact coverslip array provides $\sim 40$ fs temporal resolution. The experimental results support the theoretical model of pulse self-steepening and indicate that multiphoton ionization (MPI) initiates the pulse splitting process in glass. We perform a three-dimensional simulation to verify the experimental results.
Light responsive devices employing molecular photo-switches are interesting for displays and dynamic light filtering. In this work, polymeric microcavities embedding a layer of photochromic compound have been studied by means of the transfer matrix method. Different polymers, such as poly vinyl carbazole, poly styrene and cellulose acetate, have been used. A microcavity that includes random one-dimensional photonic structures sandwiching the photochromic layer has also been studied. Propagation of light pulses through the microcavities has been analysed.
Propagation of few-cycle laser pulses in optical fiber is investigated beyond the unidirectional approximation. Considered medium parameters include dispersion, Kerr and Raman nonlinearities. High intensities of ~10^10 kW/cm^2 lead to generation of the octave-spanning continuum. The error of the unidirectional approximation is seen in simulations as two pulses propagating forwards and backwards, both remain weak under the considered conditions. Direct analytical estimate of the error is derived and verified numerically. It can be applied to a priory justification of the unidirectional approach…
We consider pulse propagation in a linear anomalously dispersive medium where the group velocity exceeds the speed of light in vacuum (c) or even becomes negative. A signal velocity is defined operationally based on the optical signal-to-noise ratio, and is computed for cases appropriate to the recent experiment where such a negative group velocity was observed. It is found that quantum fluctuations limit the signal velocity to values less than c.
We analytically and numerically investigate the propagation of ultrashort tightly focused laser pulses in vacuum, with particular emphasis on Hermite-Gaussian and Laguerre-Gaussian modes. We revisit the Lax series approach for forward-propagating linearly-polarized laser pulses, in order to obtain Maxwell-consistent and symmetry-preserving analytical solutions for the propagation of all field components beyond the paraxial approximation in four-dimensional geometry (space and time). We demonstrate that our solution conserves the energy, which is set by the paraxial-level term of the series. Th…
Propagation of ultrashort light pulses in disordered multilayers is studied by using numerical simulations in time domain. We consider cases of instantaneous and noninstantaneous Kerr nonlinearities of the structure materials. The competitive nature of disorder and nonlinearity is revealed on the long and short timescales. We also pay special attention to the effect of pulse self-trapping in the photonic crystal with relaxing nonlinearity and show the dependence of this effect on the level of disorder. We believe that the results reported here will be useful not only in the field of optics but…
We consider propagation of light pulses detuned from the atomic resonance in a dense two-level medium and photonic structures with it. The large density of the medium is important to decrease spatial scale of such nonlinear effects as pulse compression, though it does not provide any fundamentally new phenomena as compared to dilute media. Frequency detuning decreases the effectivity of such nonlinear phenomena as pulse compression and dispersion spreading compensation as well. We propose simple logic gates based on interaction between two pulses in one-dimensional nonlinear photonic crystal. …
We investigate the interplay of diffraction and nonlinear effects during propagation of very short light pulses. Adapting the factorization approach to the problem at hand by keeping the transverse-derivative terms apart from the residual nonlinear contributions we derive an unidirectional propagation equation valid for weak dispersion and reducing to the slowly-evolving-wave-approximation for the case of paraxial rays. Comparison of numerical simulation results for the two equations shows pronounced differences when self-focusing plays important role. We devote special attention to modelling …
We model the process of ultra broadband light generation in which a pair of laser pulses separated by the Raman frequency drive a Raman transition. In contrast to the usual approach using separate field envelopes for the different frequency components, we treat the field as a single entity. This requires the inclusion of few-cycle corrections to the pulse propagation. Our single-field model makes fewer approximations and is mathematically (and hence computationally) simpler, although it does require greater computational resources to implement. The single-field theory reduces to the traditiona…
We experimentally studied intense femtosecond pulse filamentation and propagation in water for Gaussian, Laguerre-Gaussian, and Bessel-Gaussian incident beams. These different transverse modes for incident laser pulses were created from an initial Gaussian beam by using a computer generated hologram technique. We found that the length of the filament induced by the Bessel-Gaussian incident beam was longer than that for the other transverse modes under the conditions of the same peak intensity, pulse duration, and the size of the central part of the beam. To better understand the Bessel-Gaussia…
Study of photonic spin-orbital interactions, which involves control of the propagation and spatial distributions of light with the polarization of electromagnetic fields, is not only important at the fundamental level but also has significant implications for functional photonic applications that require active tuning of directional light propagation. Many of the experimental demonstrations have been attributed to the spin-momentum locking characteristic of evanescent waves. In this letter, we show another property of evanescent waves: the polarization dependent direction of the imaginary part…
The analysis of optical pulse generation by phase modulation of narrowband continuous-wave light, and subsequent propagation through a group-delay-dispersion circuit, is usually performed in terms of the so-called bunching parameter. This heuristic approach does not provide theoretical support for the electrooptic flat-top-pulse generation reported recently. Here, we perform a waveform synthesis in terms of the Fresnel images of the periodically phase-modulated input light. In particular, we demonstrate flat-top-pulse generation with a duty ratio of 50% at a quarter of the Talbot condition for…
Amplification/attenuation of light waves in artificial materials with a gain/loss modulation on the wavelength scale can be sensitive to the propagation direction. We give a numerical proof of the high anisotropy of the gain/loss in two dimensional periodic structures with square and rhombic lattice symmetry by solving the full set of Maxwell's equations using the finite difference time domain method. Anisotropy of amplification/attenuation leads to the narrowing of the angular spectrum of propagating radiation with wavevectors close to the edges of the first Brillouin Zone. The effect provide…
Propagation of a weak probe pulse through a $Λ$ system in a resonant gain configuration is investigated. We employ the control field intensity that permits the amplification of probe pulse during propagation, without instability at two photon resonance. Posterior to amplification, a broadened probe pulse is obtained, which retains its initial pulse shape and travels at the speed of light in vacuum, without experiencing any delay, absorption, and dispersion. The salient feature of this technique lies in the fact that in addition to preserving the initial pulse shape, it also ensures stable puls…
We develop a general method allowing one to construct the consistent theory of light pulse propagation through an atomic medium in arbitrary nonlinear regime with respect to the field strength, taking into account the light polarization, temporal (frequency) and spatial dispersions. The method is based on the reduced Maxwell equation, atomic density matrix formalism and adiabatic approximation. In order to demonstrate the efficiency of our method we investigate in detail the case of propagation of the polarization pulse under conditions of coherent population trapping in a medium of two-level …
We study the short pulse dynamics in the deterministic and stochastic environment in this thesis. The integrable short pulse equation is a modelling equation for ultra-short pulse propagation in the infrared range in the optical fibers. We investigate the numerical proof for the exact solitary solution of the short pulse equation. Moreover, we demonstrate that the short pulse solitons approximate the solution of the Maxwell equation numerically. Our numerical experiments prove the particle-like behaviour of the short pulse solitons. Furthermore, we derive a short pulse equation in the higher o…
We observe pulse delays of up to twenty times the input pulse duration when 200-ps laser pulses pass through a hot Rb 85 vapor cell. The pulse peak travels with a velocity equal to c/20, and the energy transmission is 5%. For pulses with linewidth greater than typical features in the atomic dispersion, pulse delay is predicted and observed for all center frequencies near resonance. Pulse advance is never observed. The measurements are in good agreement with a three-level linear-dispersion calculation. We are able to control the amount of delay by using a steady-state laser beam for optical pum…
Recent studies demonstrated the violation of reciprocity in optical processes in low-symmetry magnetic crystals. In these crystals the speed of light can be different for counter-propagating beams. Correspondingly, they can show strong directional anisotropies such as direction dependent absorption also called directional dichroism[S. Bordács et al., Nat. Phys. 8, 734 (2012); M. Saito et al., J. Phys. Soc. Jpn. 77, 013705 (2008)]. Based on symmetry considerations, we identify the magnetic point groups of materials which can host such directional anisotropies and also provide a list of possible…
Researchers claim to have observed superluminal (faster than light) propagation of a laser pulse in a gain medium by a new mechanism in which there is no distortion of the pulse [Nature, 406, 277 (2000)]. Our analysis shows that the observed mechanism is due to pulse distortion arising from a differential gain effect and should not be viewed as superluminal propagation.
Recent experiments on femtosecond pulses in water displayed long distance propagation analogous to that reported in air. We verify this phenomena numerically and show that the propagation is dynamic as opposed to self-guided. Furthermore, we demonstrate that the propagation can be interpreted as due to dynamic nonlinear X-waves whose robustness and role in long distance propagation is shown to follow from the interplay between nonlinearity and chromatic dispersion.
Pulsed Bessel beams of light propagating in free-space experience diffraction effects that resemble those of anomalous dispersion on pulse propagation. It is then shown that a pulsed Bessel beam in a normally dispersive material can remain diffraction- and dispersion-free due to mutual cancellation of diffraction and group velocity dispersion. The size of the Bessel transversal profile for localized transmission is determined by the dispersive properties of the material at the pulse carrier frequency.
In case of the nonlinear Schrödinger equation with designed group velocity dispersion, variable nonlinearity and gain/loss; we analytically demonstrate the phenomenon of chirp reversal crucial for pulse reproduction. Two different scenarios are exhibited, where the pulses experience identical dispersion profiles, but show entirely different propagation behavior. Exact expressions for dynamical quasi-solitons and soliton bound-states relevant for fiber communication are also exhibited.
Short description of the FORTRAN-codes for an analysis of the ultrashort pulse dynamics is presented. We consider: 1) the aberration-less approximation and the momentum method for the search of the single pulse stability regions in the laser with the soft-aperture Kerr-lens mode locking; 2) the distributed complex Ginzburg-Landau model for the same aim; 3) the generalized Schroedinger equation for the analysis of the femtosecond pulse propagation in the tapered and photonic crystal fibers.
We solve the problem of ultrashort pulse propagation in a two-level medium beyond the rotating-wave (RWA) and slowly-varying-envelope approximations. The method of solution is based on the Maxwell--Bloch equations represented in the form that allows one to switch between RWA and general (non-RWA) cases in the framework of a single numerical algorithm. Using this method, the effect of a subcycle pulse (containing less than a single period of field oscillations) on the two-level medium was analyzed. It is shown that for such short pulses, the clear breakdown of the area theorem occurs for the pu…
Pulse propagation is studied in an EIT medium with the control field having a periodically varying phase (chirp). Based both on numerical calculations and on an approximate approach neglecting absorption and nonadiabatic effects, it is shown that transparency occurs for probe pulses having a sufficiently narrow envelope and an appropriately suited chirp. For other chirped pulses the evolution of their spectra along a sample is studied. Using a projection method one can divide a pulse into a part for which the medium is transparent and a rest for which it is opaque.
We present a flexible, open-source Python package for the accurate simulation of the $z$-propagation dynamics of ultrashort optical pulses in nonlinear waveguides, especially valid for few-cycle pulses and their interaction. The simulation approach is based on unidirectional propagation equations for the analytic signal. The provided software allows to account for dispersion, attenuation, four-wave mixing processes including, e.g., third-harmonic generation, and features various models for the Raman response. The propagation equations are solved on a periodic temporal domain. For $z$-propagati…
We determine the linear optical susceptibility of a radiation pulse propagating through a mixture of a gas of atoms or molecules and a plasma. For a specific range of radiation and plasma frequencies, resonant generation of volume plasmons significantly amplifies the radiation intensity. The conditions for resonant amplification are derived from the dispersion relations in the mixture, and the amplification is demonstrated in a numerical simulation of pulse propagation.
We investigate the dynamics of a 10 fs light pulse propagating in a random medium by the direct solution of the 3D Maxwell equations. Our approach employs molecular dynamics to generate a distribution of spherical scatterers and a parallel finite-difference time-domain code for the vectorial wave propagation. We calculate the disorder-averaged energy velocity and the decay time of the transmitted pulse Versus the localization length for an increasing refractive index.
We study experimentally the propagation of nanosecond spin-wave pulses in microscopic waveguides made of nanometer-thick yttrium iron garnet films. For these studies, we use micro-focus Brillouin light scattering spectroscopy, which provides the possibility to observe propagation of the pulses with high spatial and temporal resolution. We show that, for most spin-wave frequencies, dispersion leads to broadening of the pulse by several times at propagation distances of 10 micrometers. However, for certain frequency interval, the dispersion broadening is suppressed almost completely resulting in…
