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arXiv physics/0507061physics.optics
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飞秒w-3 w laser脉冲光四波混频的量子控制:相干交流斯塔克非线性光谱

Quantum control of optical four-wave mixing with femtosecond w-3w laser pulses: coherent ac Stark nonlinear spectroscopy

Carles Serrat

摘要:

在红外波段,两束超短锁相w-3 w激光脉冲在二能级系统中相干传输时产生的四波混频依赖于脉冲的相对相位。麦克斯韦-布洛赫方程的求解超出了驻波近似占场的频率,这是很大程度上从原子共振失谐。控制与5 w反斯托克斯拉曼分量的耦合效率的相对相位由系统中诱导的总ac斯塔克位移的符号确定,以这种方式,相位影响精确地消失,其中由于两个脉冲引起的ac斯塔克效应被补偿。这种基本的量子干涉效应可以作为非线性超快光谱技术的基础。

英文摘要:

The four-wave mixing produced with two ultrashort phase-locked w-3w laser pulses propagating coherently in a two-level system in the infrared spectral region is shown to depend on the pulses relative phase. The Maxwell-Bloch equations are solved beyond the rotating-wave approximation to account for field frequencies which are largely detuned from the atomic resonance. The relative phase dominating the efficiency of the coupling to the 5w anti-Stokes Raman component is determined by sign of the total ac Stark shift induced in the system, in such a way that the phase influence disappears precisely where the ac Stark effect due to both pulses is compensated. This fundamental quantum interference effect can be the basis for nonlinear ultrafast optical spectroscopy techniques.

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