We study the dynamics of the cooling of a gas of caesium atoms in an optical lattice, both experimentally and with 1D full-quantum Monte Carlo simulations. We find that, contrary to the standard interpretation of the Sisyphus model, the cooling process does not work by a continuous decrease of the average kinetic energy of the atoms in the lattice. Instead, we show that the momentum of the atoms follows a bimodal distribution, the atoms being gradually transferred from a hot to a cold mode. We suggest that the cooling mechanism should be depicted in terms of a rate model, describing the transfer between the two modes along with the processes occurring within each mode.
Cooling molecular vibrations with shaped laser pulses: Optimal control theory exploiting the timescale separation between coherent excitation and spontaneous emission
Laser cooling of translational motion of small molecules is performed by addressing transitions that ensure spontaneous emission cannot cause net rotational excitation. This will not be possible once the rotational splitting becomes comparable to the operational excitation linewidth, as will occur for large molecules or wide bandwidth lasers. We show theoretically that in this regime, angular momentum transfer from red-detuned Doppler cooling light can also exert a damping torque on linear molecules, cooling rotation to the same Doppler limit (typically $\approx$ 500 $μ$K for molecules with $\…
We have designed and implemented a straightforward method to deterministically measure the temperature of the selected segment of a cold atom ensemble, and we have also developed an upgrade in the form of nondestructive thermometry. The essence is to monitor the thermal expansion of the targeted cold atoms after labeling them through manipulating the internal states, and the nondestructive property relies upon the nearly lossless detection via driving a cycling transition. For cold atoms subject to isotropic laser cooling, this method has the unique capability of addressing only the atoms on t…
We discuss the coupling of the motion of two ion species in separate Penning traps via a common tank circuit. The enhancement of the coupling assisted by the tank circuit is demonstrated by an avoided crossing behavior measurement of the motional modes of two coupled ions. We propose an intermittent laser cooling method for sympathetic cooling and provide a theoretical description. The technique enables tuning of the coupling strength between two ion species in separate traps and thus allows for efficient sympathetic cooling of an arbitrary type of single ion for high-precision Penning-trap ex…
We demonstrate phase locking of two ultraviolet laser sources by modulating a fundamental infrared laser with 4th-order sidebands using an electro-optic modulator and phase locking of one sideband to a second fundamental infrared laser. Subsequent sum frequency generation and second harmonic generation successfully translates the frequency offset to the ultraviolet domain. The phase lock at 139 GHz is confirmed through stimulated Raman transitions for thermometry of $^9$Be$^+$ ions confined in a cryogenic Penning trap. This technique might be used for sideband cooling of single $^9$Be$^+$ ions…
A recent progress on laser cooling of molecules is summarized. Since the development during 1980s for atomic species, laser cooling has been the very beginning step to cool and trap atoms for frontier research on quantum simulations, quantum sensing and precision measurements. Despite the complex internal structures of molecules, laser cooling of molecules have been realized with the deepened understanding of molecular structures and interaction between light and molecules. The development of laser technology over the last decades have also been a great aid for laser cooling of molecules becau…
We describe a compact and versatile multi-frequency laser system for laser-cooling potassium atoms, by frequency doubling a fiber-optic telecom beam ($\simeq 1534$ or $1540$~nm). Low-power fiber-based telecom lasers and components generate a single beam containing the cooling and repumper half frequencies, subsequently amplified by high-power amplifier. A final free-space SHG stage generates a single beam with typically 2.5 W at quasi-resonant frequencies ($\simeq 767$ or $770$~nm) with high-quality mode and ready for laser cooling. This allowed to trap up to $4\times10^9$ $^{41}$K atoms with …
We theoretically investigate the laser cooling of fermionic barium monofluoride (137BaF) molecules, which are promising candidates for precision studies of weak parity violation and nuclear anapole moments. This molecular species features two nuclear spins, resulting in a hyperfine structure that is considerably more complicated than the one found in the usual laser-cooled diatomics. We use optical Bloch equations and rate equations to show that optical cycling, sub-Doppler cooling and bichromatic forces can all be realized under realistically achievable experimental conditions.
Acetylene-based frequency stabilization of a laser system for potassium laser cooling
我们利用乙炔分子（$12$ C $_2$ H $_2$）的振转跃迁，在C波段光通信窗口的饱和吸收光谱的基础上，实现了钾原子激光冷却的激光稳频技术。我们确定并表征了几条分子线，由于高功率二次谐波产生（SHG）阶段，这些分子线可以解决钾D2（767 nm）和D1（770 nm）冷却跃迁中的每一个。我们成功地使用该激光系统冷却钾的$^{41}$ K同位素在2D-3D磁光阱设置。
We report on a scheme for laser cooling of $^{12}$C$_2$. We have calculated the branching ratios for cycling and repumping transitions and calculated the number of photon scatterings required to achieve deflection and laser cooling of a beam of $C_2$ molecules under realistic experimental conditions. Our results demonstrate that C$_2$ cooling using the Swan ($d^3Π_\text{g} \leftrightarrow a^3Π_\text{u}$) and Duck ($d^3Π_\text{g} \leftrightarrow c^3Σ_\text{u}^+$) bands is achievable via techniques similar to state-of-the-art molecular cooling experiments. The Phillips ($A^1Π_\text{u} \leftright…
Laser cooling exploits the physics of light scattering to cool atomic and molecular gases to close to absolute zero. It is the crucial initial step for essentially all atomic gas experiments in which Bose-Einstein condensation and, more generally, quantum degeneracy is reached. The ongoing development of laser-cooling methods has allowed more elements to be brought to quantum degeneracy, with each additional atomic species offering its own experimental opportunities. Improved methods are opening new avenues, for example, reaching Bose-Einstein condensation purely through laser cooling as well …
We demonstrate 1D simultaneous laser cooling of $^{87}$Rb and $^{85}$Rb atoms using an optical frequency comb. By adjusting the pulse repetition frequency and the offset frequency, the frequency comb spectrum is tuned to ensure that two distinct frequency comb modes are simultaneously red-detuned from the cooling transitions, one mode for each species. Starting from a pre-cooled cloud of $^{85,87}$Rb atoms at above-Doppler temperatures, we show simultaneous cooling of both species down to the Doppler temperature using two counter-propagating $σ$$^{+}$/$σ$$^{-}$-polarized beams from the frequen…
