We demonstrate 1D simultaneous laser cooling of $^{87}$Rb and $^{85}$Rb atoms using an optical frequency comb. By adjusting the pulse repetition frequency and the offset frequency, the frequency comb spectrum is tuned to ensure that two distinct frequency comb modes are simultaneously red-detuned from the cooling transitions, one mode for each species. Starting from a pre-cooled cloud of $^{85,87}$Rb atoms at above-Doppler temperatures, we show simultaneous cooling of both species down to the Doppler temperature using two counter-propagating $σ$$^{+}$/$σ$$^{-}$-polarized beams from the frequency comb. The results indicate that simultaneous dual-species frequency comb cooling does not affect the cooling characteristics of individual atomic species. The results of this work imply that several atomic species could be cooled simultaneously using a single frequency comb source. This comb-based multi-channel laser cooling could bring significant advances in multi-species atom interferometers for space applications and in the study of multi-species interactions.
We propose a new laser cooling method for atomic species whose level structure makes traditional laser cooling difficult. For instance, laser cooling of hydrogen requires single-frequency vacuum-ultraviolet light, while multielectron atoms need single-frequency light at many widely separated frequencies. These restrictions can be eased by laser cooling on two-photon transitions with ultrafast pulse trains. Laser cooling of hydrogen, antihydrogen, and many other species appears feasible, and extension of the technique to molecules may be possible.
We present measurements of resistive and sympathetic cooling of ion clouds confined in a Penning trap. For resistive cooling of a cloud consisting of one ion species, we observe a significant deviation from exponential cooling behavior which is explained by an energy-transfer model. The observed sympathetic cooling of simultaneously confined ion species shows a quadratic dependence on the ion charge state and is hence in agreement with expectations from the physics of dilute non-neutral plasmas.
We simultaneously trap ultracold lithium and cesium atoms in an optical dipole trap formed by the focus of a CO$_2$ laser and study the exchange of thermal energy between the gases. The cesium gas, which is optically cooled to $20 μ$K, efficiently decreases the temperature of the lithium gas through sympathetic cooling. The measured cross section for thermalizing $^{133}$Cs-$^7$Li collisions is $8 \times 10^{-12}$ cm$^2$, for both species in their lowest hyperfine ground state. Besides thermalization, we observe evaporation of lithium purely through elastic cesium-lithium collisions (sympathet…
Sympathetic cooling of trapped ions has become an indispensable tool for quantum information processing and precision spectroscopy. In the simplest situation a single Doppler-cooled ion sympathetically cools another ion which typically has a different mass. We analytically investigate the effect of the mass ratio of such an ion crystal on the achievable temperature limit in the presence of external heating. As an example, we show that cooling of a single Al+ with Be+, Mg+ and Ca+ ions provides similar results for heating rates typically observed in ion traps, whereas cooling ions with a larger…
We report the formation of a dual-species Bose-Einstein condensate of $^{87}$Rb and $^{133}$Cs in the same trapping potential. Our method exploits the efficient sympathetic cooling of $^{133}$Cs via elastic collisions with $^{87}$Rb, initially in a magnetic quadrupole trap and subsequently in a levitated optical trap. The two condensates each contain up to $2\times10^{4}$ atoms and exhibit a striking phase separation, revealing the mixture to be immiscible due to strong repulsive interspecies interactions. Sacrificing all the $^{87}$Rb during the cooling, we create single species $^{133}$Cs co…
Recent theoretical investigations have indicated that rapid optical cycling should be feasible in complex polyatomic molecules with diverse constituents, geometries and symmetries. However, as a composite molecular mass grows, so does the required number of photon scattering events necessary to decelerate and confine molecular beams using laser light. Utilizing coherent momentum exchange between light fields and molecules can suppress spontaneous emission and significantly reduce experimental complexity for slowing and trapping. Working with BaH as a test species, we have identified a robust, …
We report on the realization of a stable mixture of ultracold lithium and ytterbium atoms confined in a far-off-resonance optical dipole trap. We observe sympathetic cooling of 6Li by 174Yb and extract the s-wave scattering length magnitude |a6Li-174Yb| = (13 \pm 3)a0 from the rate of inter-species thermalization. Using forced evaporative cooling of 174Yb, we achieve reduction of the 6Li temperature to below the Fermi temperature, purely through inter-species sympathetic cooling.
We demonstrate key multi-qubit quantum logic primitives in a dual-species trapped-ion system based on $^{40}$Ca+ and $^{88}$Sr+ ions, using two optical qubits with quantum-logic-control frequencies in the red to near-infrared range. With all ionization, cooling, and control wavelengths in a wavelength band similar for the two species and centered in the visible, and with a favorable mass ratio for sympathetic cooling, this pair is a promising candidate for scalable quantum information processing. Same-species and dual-species two-qubit gates, based on the Moelmer-Soerensen interaction and perf…
We reported the realization of a $^{174}\mathrm{Yb}^+$-$^{113}\mathrm{Cd}^+$ bi-species Coulomb crystal comprising $^{174}\mathrm{Yb}^+$ ions as coolant and verified its potential for application as a $^{113}\mathrm{Cd}^+$ microwave frequency standard employing sympathetic cooling.The two species of massive ions stably trapped in a Paul trap make up this large two-component crystal. The $^{113}\mathrm{Cd}^+$ ions are trapped in the center, which reduces considerably RF heating and excess micromotion to which the $^{113}\mathrm{Cd}^+$ ions are subjected. Under this scheme, the uncertainty due t…
We discuss the coupling of the motion of two ion species in separate Penning traps via a common tank circuit. The enhancement of the coupling assisted by the tank circuit is demonstrated by an avoided crossing behavior measurement of the motional modes of two coupled ions. We propose an intermittent laser cooling method for sympathetic cooling and provide a theoretical description. The technique enables tuning of the coupling strength between two ion species in separate traps and thus allows for efficient sympathetic cooling of an arbitrary type of single ion for high-precision Penning-trap ex…
We theoretically investigate the laser cooling of fermionic barium monofluoride (137BaF) molecules, which are promising candidates for precision studies of weak parity violation and nuclear anapole moments. This molecular species features two nuclear spins, resulting in a hyperfine structure that is considerably more complicated than the one found in the usual laser-cooled diatomics. We use optical Bloch equations and rate equations to show that optical cycling, sub-Doppler cooling and bichromatic forces can all be realized under realistically achievable experimental conditions.
We report the 1-D cooling of $^{85}$Rb atoms using a velocity-dependent optical force based upon Ramsey matter-wave interferometry. Using stimulated Raman transitions between ground hyperfine states, 12 cycles of the interferometer sequence cool a freely-moving atom cloud from $21~μ$K to $3~μ$K. This pulsed analog of continuous-wave Doppler cooling is effective at temperatures down to the recoil limit; with augmentation pulses to increase the interferometer area, it should cool more quickly than conventional methods, and be more suitable for species that lack a closed radiative transition.
A recent progress on laser cooling of molecules is summarized. Since the development during 1980s for atomic species, laser cooling has been the very beginning step to cool and trap atoms for frontier research on quantum simulations, quantum sensing and precision measurements. Despite the complex internal structures of molecules, laser cooling of molecules have been realized with the deepened understanding of molecular structures and interaction between light and molecules. The development of laser technology over the last decades have also been a great aid for laser cooling of molecules becau…
We discuss cooling efficiency for different-species Fermi-Bose mixtures in magnetic traps. A better heat capacity matching between the two atomic species is achieved by a proper choice of the Bose cooler and the magnetically trappable hyperfine states of the mixture. When a partial spatial overlap between the two species is also taken into account, the deepest Fermi degeneracy is obtained for an optimal value of the trapping frequency ratio. This can be achieved by assisting the magnetic trap with a deconfining light beam, as shown in the case of fermionic 6Li mixed with 23Na, 87Rb, and 133Cs,…
Single-Photon Cooling (SPC), noted for its potential as a versatile method for cooling a variety of atomic species, has recently been demonstrated experimentally. In this paper, we study possible ways to improve the performance of SPC by applying it to atoms trapped inside a wedge billiard. The main feature of wedge billiard for atoms, also experimentally realized recently, is that the nature of atomic trajectories within it changes from stable periodic orbit to random chaotic motion with the change in wedge angle. We find that a high cooling efficiency is possible in this system with a relati…
We have studied the cooling dynamics, formation process and geometric structure of mesoscopic crystals of externally produced magnesium ions in a Penning trap. We present a cooling model and measurements for a combination of buffer gas cooling and laser cooling which has been found to reduce the ion kinetic energy by eight orders of magnitude from several hundreds of eV to micro-eV and below within seconds. With ion numbers of the order of 1000 to 100000, such cooling leads to the formation of ion Coulomb crystals which display a characteristic shell structure in agreement with theory of non-n…
We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic transition, it is most easily applicable to molecules with similar ground and excited potential energy surfaces, such that the vibrational state is usually unchanged during electronic relaxation. Compared with schemes that cool rotations by exciting vibrations, this approach achieves internal cooling on the orders-of- magnitude faster electronic decay times…
Cooling of particles to mK-temperatures is essential for a variety of experiments with trapped charged particles. However, many species of interest lack suitable electronic transitions for direct laser cooling. We study theoretically the remote sympathetic cooling of a single proton with laser-cooled $^9$Be$^+$ in a double-Penning-trap system. We investigate three different cooling schemes and find, based on analytical calculations and numerical simulations, that two of them are capable of achieving proton temperatures of about 10 mK with cooling times on the order of 10 s. In contrast, establ…
We present a realization of a magneto-optical trap of mercury atoms on the intercombination line. We report on trapping of all stable mercury isotopes. We characterize the effect of laser detuning, laser intensity, and gradient field on the trapping performance of our system. The atom number for the most abundant isotope Hg-202 is 50 million atoms. Moreover, we study the difference in cooling processes for bosonic and fermionic isotopes. We observe agreement with the Doppler cooling theory for the bosonic species and show sub-Doppler cooling for the fermionic species. We reach a phase space de…
We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler laser cooled in an optical molasses, to a temperature of 110(4) $μ$K. The temperatures and densities achieved here make CaOH a viable candidate for a wide variety of quantum science applications, including the creation of optical tweezer arrays of CaOH molecules. This work also suggests that laser cooling and magneto-optical trapping of many other polyatomi…
We present the simultaneous cooling and trapping of an isotopic mixture in a magneto-optical trap and we describe the transfer of the mixture into a conservative, far-off resonant dipole trap. The mixture is prepared with a new technique that applies to intermediate and heavy alkaline earth like atoms. In this work, 88Sr and 86Sr are simultaneously loaded first into the magneto-optical trap operated on the 1S0-3P1 spin-forbidden line at 689 nm, and then transferred into the dipole trap. We observe fast inter-species thermalization in the dipole trap which allows one to set a lower bound on the…
Hybrid traps for the simultaneous confinement of neutrals and ions have recently emerged as versatile tools for studying interactions between these species at very low temperatures. Such traps rely on the combination of different types of external fields for the confinement of either species raising the question of interactions between the individual traps. Here, the influence of a strongly inhomogeneous magnetic field used for trapping neutrals on the trapping and laser cooling of a single Ca$^+$ ion in a radiofrequency ion trap is studied theoretically using molecular-dynamics simulations ba…
We utilize the dark state in a Λ-type three-level system to cool an ensemble of 85Rb atoms in an optical lattice [Morigi et al., Phys. Rev. Lett. 85, 4458 (2000)]. The common suppression of the carrier transition of atoms with different vibrational frequencies allows them to reach a subrecoil temperature of 100 nK after being released from the optical lattice. A nearly zero vibrational quantum number is determined from the time-of-flight measurements and adiabatic expansion process. The features of sideband cooling are examined in various parameter spaces. Our results show that dark-state side…
A proposal for cooling the translational motion of optically levitated magnetic nanoparticles is presented. The theoretical cooling scheme involves the sympathetic cooling of a ferromagnetic YIG nanosphere with a spin-polarized atomic gas. Particle-atom cloud coupling is mediated through the magnetic dipole-dipole interaction. When the particle and atom oscillations are small compared to their separation, the interaction potential becomes dominantly linear which allows the particle to exchange energy with the $N$ atoms. While the atoms are continuously Doppler cooled, energy is able to be remo…
Laser cycling of resonances can remove entropy from a system via spontaneously emitted photons, with electronic resonances providing the fastest cooling timescales because of their rapid relaxation rates. Although atoms are routinely laser cooled, even simple molecules pose two interrelated challenges for cooling: every populated rotational-vibrational state requires a different laser frequency, and electronic relaxation generally excites vibrations. Here, we cool trapped AlH+ molecules to their ground rotational-vibrational quantum state using an electronically-exciting broadband laser to sim…
We realize a continuous guided beam of cold deuterated ammonia with a flux of 3e11 ND3 molecules/s and a continuous free-space beam of cold potassium with a flux of 1e16 K atoms/s. A novel feature of the buffer gas source used to produce these beams is cold neon, which, due to intermediate Knudsen number beam dynamics, produces a forward velocity and low-energy tail that is comparable to much colder helium-based sources. We expect this source to be trivially generalizable to a very wide range of atomic and molecular species with significant vapor pressure below 1000 K. This source has properti…
Laser cooling and trapping are central to modern atomic physics. The workhorse technique in cold-atom physics is the magneto-optical trap (MOT), which combines laser cooling with a restoring force from radiation pressure. For a variety of atomic species, MOTs can capture and cool large numbers of particles to ultracold temperatures (<1 mK); this has enabled the study of a wide range of phenomena from optical clocks to ultracold collisions whilst also serving as the ubiquitous starting point for further cooling into the regime of quantum degeneracy. Magneto-optical trapping of molecules could p…
We report direct laser cooling of a symmetric top molecule, reducing the transverse temperature of a beam of calcium monomethoxide (CaOCH$_3$) to $1.8\pm0.7$ mK while addressing two distinct nuclear spin isomers. These results open a path to efficient production of ultracold chiral molecules and conclusively demonstrate that by using proper rovibronic optical transitions, both photon cycling and laser cooling of complex molecules can be as efficient as for much simpler linear species.
We describe an experimental setup designed to produce ultracold trapped gas clouds of fermionic 6Li and bosonic 87Rb. This combination of alkali metals has the potential to reach deeper Fermi degeneracy with respect to other mixtures since it allows for improved heat capacity matching which optimizes sympathetic cooling efficiency. Atomic beams of the two species are independently produced and then decelerated by Zeeman slowers. The slowed atoms are collected into a magneto-optical trap and then transferred into a quadrupole magnetic trap. An ultracold Fermi gas with temperature in the 10^-3 T…
Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the creation of ultracold molecular gases using traditional methods (laser plus evaporative cooling) a challenge, in particular due to the spontaneous decay of molecules into dark states. We propose a way to circumvent this key bottleneck using an all-optical method for decelerating molecules using stimulated absorption and emission with a single ultrafast laser. We …
We demonstrate imaging of neutral atoms via the light scattered during continuous Raman sideband cooling. We detect single atoms trapped in optical tweezers while maintaining a significant motional ground-state fraction. The techniques presented provide a framework for single-atom resolved imaging of a broad class of atomic species.
We report on the first realization of sub-Doppler laser cooling of 39K atoms using degenerate 3D Raman sideband cooling. We take advantage of the well-resolved excited hyperfine states on the D1 optical transition to produce spin polarized samples with $1.4 \times 10^8$ atoms at temperatures of 1.8 $μ$K. The phase-space densities are $\geq 10^{-4}$, which significantly improves the initial conditions for a subsequent evaporative cooling step. The presented cooling technique using the D1 line can be adapted to other atomic species and is applicable to high-resolution imaging schemes in far off-…
We demonstrate a Magneto-Optical Trap (MOT) configuration which employs optical forces due to light scattering between electronically excited states of the atom. With the standard MOT laser beams propagating along the {\it x}- and {\it y}- directions, the laser beams along the {\it z}-direction are at a different wavelength that couples two sets of {\it excited} states. We demonstrate efficient cooling and trapping of cesium atoms in a vapor cell and sub-Doppler cooling on both the red and blue sides of the two-photon resonance. The technique demonstrated in this work may have applications in …
We present first indications of sympathetic cooling between two neutral, optically trapped atomic species. Lithium and cesium atoms are simultaneously stored in an optical dipole trap formed by the focus of a CO$_2$ laser, and allowed to interact for a given period of time. The temperature of the lithium gas is found to decrease when in thermal contact with cold cesium. The timescale of thermalization yields an estimate for the Li-Cs cross-section.
We demonstrate runaway evaporative cooling directly with a tightly confining optical dipole trap and achieve fast production of condensates of 1.5x10^5 87Rb atoms. Our scheme is characterized by an independent control of the optical trap confinement and depth, permitting forced evaporative cooling without reducing the trap stiffness. Although our configuration is particularly well suited to the case of 87Rb atoms in a 1565nm optical trap, where an efficient initial loading is possible, our scheme is general and should allow all-optical evaporative cooling at constant stiffness for most species…
Molecular overtone transitions provide optical frequency transitions sensitive to variation in the proton-to-electron mass ratio ($μ\equiv m_p/m_e$). However, robust molecular state preparation presents a challenge critical for achieving high precision. Here, we characterize infrared and optical-frequency broadband laser cooling schemes for TeH$^+$, a species with multiple electronic transitions amenable to sustained laser control. Using rate equations to simulate laser cooling population dynamics, we estimate the fractional sensitivity to $μ$ attainable using TeH$^+$. We find that laser cooli…
We present the first simultaneous trapping of two different ultracold atomic species in a conservative trap. Lithium and cesium atoms are stored in an optical dipole trap formed by the focus of a CO$_2$ laser. Techniques for loading both species of atoms are discussed and observations of elastic and inelastic collisions between the two species are presented. A model for sympathetic cooling of two species with strongly different mass in the presence of slow evaporation is developed. From the observed Cs-induced evaporation of Li atoms we estimate a cross section for cold elastic Li-Cs collision…
Motional ground state cooling and internal state preparation are important elements for quantum logic spectroscopy (QLS), a class of quantum information processing. Since QLS does not require the high gate fidelities usually associated with quantum computation and quantum simulation, it is possible to make simplifying choices in ion species and quantum protocols at the expense of some fidelity. Here, we report sideband cooling and motional state detection protocols for $^{138}$Ba$^+$ of sufficient fidelity for QLS without an extremely narrowband laser or the use of a species with hyperfine str…
We report a generally applicable computational and experimental approach to determine vibronic branching ratios in linear polyatomic molecules to the $10^{-5}$ level, including for nominally symmetry forbidden transitions. These methods are demonstrated in CaOH and YbOH, showing approximately two orders of magnitude improved sensitivity compared with the previous state of the art. Knowledge of branching ratios at this level is needed for the successful deep laser cooling of a broad range of molecular species.
Laser cooling exploits the physics of light scattering to cool atomic and molecular gases to close to absolute zero. It is the crucial initial step for essentially all atomic gas experiments in which Bose-Einstein condensation and, more generally, quantum degeneracy is reached. The ongoing development of laser-cooling methods has allowed more elements to be brought to quantum degeneracy, with each additional atomic species offering its own experimental opportunities. Improved methods are opening new avenues, for example, reaching Bose-Einstein condensation purely through laser cooling as well …
We explore the possibility of decelerating and Doppler cooling of an ensemble of two-level atoms by a coherent train of short, non-overlapping laser pulses. We develop a simple analytical model for dynamics of a two-level system driven by the resulting frequency comb field. We find that the effective scattering force mimics the underlying frequency comb structure. The force pattern depends strongly on the ratio of the atomic lifetime to the repetition time and pulse area. For example, in the limit of short lifetimes, the frequency peaks of the optical force wash out. We show that laser cooling…
We report the trapping of ultracold neutral $ \text{Rb}$ atoms and $ \text{Ba}^+ $ ions in a common optical potential in absence of any radiofrequency (RF) fields. We prepare $ \text{Ba}^+ $ at $ 370 ~ μK $ and demonstrate efficient sympathetic cooling by $100 ~ μK $ after one collision. Our approach is currently limited by the $ \text{Rb}$ density and related three-body losses, but it overcomes the fundamental limitation in RF traps set by RF-driven, micromotion-induced heating. It is applicable to a wide range of ion-atom species, and may enable novel ultracold chemistry experiments and comp…
Doppler and Sisyphus cooling of $^{174}$YbOH are achieved and studied. This polyatomic molecule has high sensitivity to physics beyond the Standard Model and represents a new class of species for future high-precision probes of new T-violating physics. The transverse temperature of the YbOH beam is reduced by nearly two orders of magnitude to $< 600 \, μ$K and the phase-space density is increased by a factor of $>6$ via Sisyphus cooling. We develop a full numerical model of the laser cooling of YbOH and find excellent agreement with the data. We project that laser cooling and magneto-optical t…
The unstable radium nucleus is appealing for probing new physics due to its high mass, octupole deformation and energy level structure. Ion traps, with long hold times and low particle numbers, are excellent for work with radioactive species, such as radium and radium-based molecular ions, where low activity, and hence low total numbers, is desirable. We address the challenges associated with the lack of stable isotopes in a tabletop experiment with a low-activity ($\sim 10 \ μ\mathrm{Ci}$) source where we laser-cool trapped radium ions. With a laser-cooled radium ion we measured the $7p\ ^2P_…
Laser cooling to sub-Doppler temperatures by optical molasses is thought to be inhibited in atoms with unresolved, near-degenerate hyperfine structure in the excited state. We demonstrate that such cooling is possible in one to three dimensions, not only near the standard D2 line for laser cooling, but over a range extending to the D1 line. Via a combination of Sisyphus cooling followed by adiabatic expansion, we reach temperatures as low as 40 μK, which corresponds to atomic velocities a factor of 2.6 above the limit imposed by a single photon recoil. Our method requires modest laser power at…
We report a detailed investigation on near-ground state cooling of one and two trapped atomic ions. We introduce a simple sideband cooling method for confined atoms and ions, using RF radiation applied to bare ionic states in a static magnetic field gradient, and demonstrate its application to ions confined at secular trap frequencies, $ω_z \approx 2π\times 117 $kHz. For a single \ybplus ion, the sideband cooling cycle reduces the average phonon number, $\left\langle\,n\,\right\rangle$ from the Doppler limit to $\left\langle\,n\,\right\rangle =$ 0.30(12). This is in agreement with the theoreti…
We report on the first realization of a two-species magneto-optical trap (MOT) for erbium and dysprosium. The MOT operates on an intercombination line for the respective species. Owing to the narrow-line character of such a cooling transition and the action of gravity, we demonstrate a novel trap geometry employing only five beams in orthogonal configuration. We observe that the mixture is cooled and trapped very efficiently, with up to \num{5e8} Er atoms and \num{e9} Dy atoms at temperatures of about $10\,μK$. Our results offer an ideal starting condition for the creation of a dipolar quantum…
The efficiency of laser-cooling relies on the existence of an almost closed optical-transition cycle in the energy spectrum of the considered species. In this respect rare-earth elements exhibit many transitions which are likely to induce noticeable leaks from the cooling cycle. In this work, to determine whether laser-cooling of singly-ionized erbium Er$^+$ is feasible, we have performed accurate electronic-structure calculations of energies and spontaneous-emission Einstein coefficients of Er$^+$, using a combination of \textit{ab initio} and least-square-fitting techniques. We identify five…
We experimentally demonstrate a variation on a Sisyphus cooling technique that was proposed for cooling antihydrogen. In our implementation, atoms are selectively excited to an electronic state whose energy is spatially modulated by an optical lattice, and the ensuing spontaneous decay completes one Sisyphus cooling cycle. We characterize the cooling efficiency of this technique on a continuous beam of Sr, and compare it with radiation pressure based laser cooling. We demonstrate that this technique provides similar atom number for lower end temperatures, provides additional cooling per scatte…
The term `laser cooling' is applied to the use of optical means to cool the motional energies of either atoms and molecules, or micromirrors. In the literature, these two strands are kept largely separate; both, however suffer from severe limitations. Laser cooling of atoms and molecules largely relies on the internal level structure of the species being cooled. As a result, only a small number of elements and a tiny number of molecules can be cooled this way. In the case of micromirrors, the problem lies in the engineering of micromirrors that need to satisfy a large number of constraints---t…
