Dielectric optical micro-resonators and micro-lasers represent a realization of a wave-chaotic system, where the lack of symmetry in the resonator shape leads to non-integrable ray dynamics. Modes of such resonators display a rich spatial structure, and cannot be classified through mode indices which would require additional constants of motion in the ray dynamics. Understanding and controlling the emission properties of such resonators requires the investigation of the correspondence between classical phase space structures of the ray motion inside the resonator and resonant solutions of the wave equations. We first discuss the breakdown of the conventional eikonal approximation in the short wavelength limit, and motivate the use of phase-space ray tracing and phase space distributions. Next, we introduce an efficient numerical method to calculate the quasi-bound modes of dielectric resonators, which requires only two diagonalizations per N states, where N is approximately equal to the number of half-wavelengths along the perimeter. The relationship between classical phase space structures and modes is displayed via the Husimi projection technique. Observables related to the emission pattern of the resonator are calculated with high efficiency.
Semiclassical multimode laser theory is extended to gas lasers with open two-dimensional resonators of arbitrary shape. The Doppler frequency shift of the linear-gain coefficient leads to an additional linear coupling between the modes, which, however, is shown to be negligible. The nonlinear laser equations simplify in the special case of wave-chaotic resonators. In the single-mode regime, the intensity of a chaotic laser, as a function of the mode frequency, displays a local minimum at the frequency of the atomic transition. The width of the minimum scales with the inhomogeneous linewidth, i…
We show the possibility of controlling the dynamical behavior of a single fiber ring (SFR) resonator system with the fiber being an amplified (gain) channel and the ring being attenuated (loss) nonlinear dielectric medium. Our model is based on the simple alterations in the parity time symmetric synthetic coupler structures proposed recently [A. Regensburger et al., Nature 488, 167 (2012)]. The system has been modeled using the transfer matrix formalism. We find that this results in a dynamically controllable algorithm for the chaotic dynamics inherent in the system. We have also shown the dep…
We study long-lived resonances (lowest-loss modes) in hexagonally shaped dielectric resonators in order to gain insight into the physics of a class of microcrystal lasers. Numerical results on resonance positions and lifetimes, near-field intensity patterns, far-field emission patterns, and effects of rounding of corners are presented. Most features are explained by a semiclassical approximation based on pseudointegrable ray dynamics and boundary waves. The semiclassical model is also relevant for other microlasers of polygonal geometry.
Metamaterials comprising assemblies of dielectric resonators have attracted much attention due to their low intrinsic loss and isotropic optical response. In particular, metasurfaces made from silicon dielectric resonators have shown desirable behaviors such as efficient nonlinear optical conversion, spectral filtering and advanced wave-front engineering. To further explore the potential of dielectric metamaterials, we present all-dielectric metamaterials fabricated from epitaxially grown III-V semiconductors that can exploit the high second-order optical susceptibilities of III-V semiconducto…
In this paper, we derive a model from Maxwell equations for the magnetic resonance of split-ring resonators. Using this model we revisit the scaling of split-ring resonators. Inspired by our model, we propose a new type of split-hybrid metal-dielectric ring resonator, of which the ring is made composed of moderately high index dielectric material (e.g. SiC, TiO2, ZnS) (for the major portion), while and metal (e.g. Ag) fills the gap. Such a new magnetic metamaterial is able to overcome the saturation problem of split-ring resonatorssaturation-free and therefore is able to operate at short wavel…
We demonstrate, for the first time, an all-dielectric metamaterial resonator in the mid-wave infrared based on high-index tellurium cubic inclusions. Dielectric resonators are desirable compared to conventional metallo-dielectric metamaterials at optical frequencies as they are largely angular invariant, free of ohmic loss, and easily integrated into three-dimensional volumes. With these low-loss, isotropic elements, disruptive optical metamaterial designs, such as wide-angle lenses and cloaks, can be more easily realized.
We measured the resonance spectra of two stadium-shaped dielectric microwave resonators and tested a semiclassical trace formula for chaotic dielectric resonators proposed by Bogomolny et al. [Phys. Rev. E 78, 056202 (2008)]. We found good qualitative agreement between the experimental data and the predictions of the trace formula. Deviations could be attributed to missing resonances in the measured spectra in accordance with previous experiments [Phys. Rev. E 81, 066215 (2010)]. The investigation of the numerical length spectrum showed good qualitative and reasonable quantitative agreement wi…
Recent progress in nanoscale optical physics is associated with the development of a new branch of nanophotonics exploring strong Mie resonances in dielectric nanoparticles with high refractive index. The high-index resonant dielectric nanostructures form building blocks for novel photonic metadevices with low losses and advanced functionalities. However, unlike extensively studied cavities in photonic crystals, such dielectric resonators demonstrate low quality factors (Q-factors). Here, we uncover a novel mechanism for achieving giant Q-factors of subwavelength nanoscale resonators by realiz…
We report emergence of saturation and chaotic spiking of optical power in a double ring resonator with balanced loss and gain, obeying the so-called parity-time symmetry. We have modeled the system using a discrete-time iterative equation known as the Ikeda Map. In the linear regime, evolution of optical power in the system shows power saturation behavior below the PT threshold and exponential blow-up above the PT threshold. We found that in the unbroken PT regime, optical power saturation occurs owing to the existence of stable stationary states, which lies on the surface of 4-dimensional hyp…
We introduce a practical dielectric metasurface design for microwave frequencies. The metasurface is made of an array of dielectric resonators held together by dielectric connections thus avoiding the need of a mechanical support in the form of a dielectric slab and the spurious multiple reflections that such a slab would generate. The proposed design can be used either for broadband metasurface applications or monochromatic wave transformations. The capabilities of the concept to manipulate the transmission phase and amplitude of the metasurface are supported by numerical and experimental res…
Creation of correlated photon pairs is one of the key topics in contemporary quantum optics. Here, we theoretically describe the generation of photon pairs in the process of spontaneous parametric down-conversion in a resonant spherical nanoparticle made of a dielectric material with bulk $χ^{(2)}$ nonlinearity. We pick the nanoparticle size that satisfies the condition of resonant eigenmodes described by Mie theory. We reveal that highly directional photon-pair generation can be observed utilising the nonlinear Kerker-type effect, and that this regime provides useful polarisation correlations…
We propose the construction of highly directional emission microlasers using two-dimensional high-index semiconductor waveguides as {\it open} resonators. The prototype waveguide is formed by two collinear leads connected to a cavity of certain shape. The proposed lasing mechanism requires that the shape of the cavity yield mixed chaotic ray dynamics so as to have the appropiate (phase space) resonance islands. These islands allow, via Heisenberg's uncertainty principle, the appearance of quasi bound states (QBS) which, in turn, propitiate the lasing mechanism. The energy values of the QBS are…
High-power and highly directional semiconductor cylinder-lasers based on an optical resonator with deformed cross section are reported. In the favorable directions of the far-field, a power increase of up to three orders of magnitude over the conventional circularly symmetric lasers was obtained. A "bow-tie"-shaped resonance is responsible for the improved performance of the lasers in the higher range of deformations, in contrast to "whispering-gallery"-type modes of circular and weakly deformed lasers. This resonator design, although demonstrated here in midinfrared quantum-cascade lasers, sh…
In this paper we describe a methodology for tailoring the design of metamaterial dielectric resonators, which represent a promising path toward low-loss metamaterials at optical frequencies. We first describe a procedure to decompose the far field scattered by subwavelength resonators in terms of multipolar field components, providing explicit expressions for the multipolar far fields. We apply this formulation to confirm that an isolated high-permittivity cube resonator possesses frequency separated electric and magnetic dipole resonances, as well as a magnetic quadrupole resonance in close p…
We measure strong magnetic field intensities in a subwavelength gap separating two dielectric resonators. This dimer magnetic antenna is characterized in the GHz spectral regime when considering three conditions of illumination. We detail the different magneto-electric couplings involved in the enhancement of the near magnetic field and derive the analytical expression of the magnetic field intensities. The results reported here in the GHz domain can be extended to other spectral domains since they are obtained with a dielectric permittivity 16 that can be observed in a very broad spectrum ran…
Nanometer-resolution 3D Tomographic and Vectorial Near-field Imaging in Dielectric Optical Resonators
State Key Laboratory of Surface Physics, Key Laboratory of Micro and Nano Photonic Structures (MOE), and Department of Physics, Fudan University（复旦大学表面物理国家重点实验室、微纳光子结构教育部重点实验室和物理系）；Shanghai Key Laboratory of Metasurfaces for Light Manipulation, Fudan University（复旦大学光调控超材料上海市重点实验室）
We investigated the frequency spectra and field distributions of a dielectric square resonator in a microwave experiment. Since such systems cannot be treated analytically, the experimental studies of their properties are indispensable. The momentum representation of the measured field distributions shows that all resonant modes are localized on specific classical tori of the square billiard. Based on these observations a semiclassical model was developed. It shows excellent agreement with all but a single class of measured field distributions that will be treated separately.
In this paper, we propose a novel design of dielectric laser-driven accelerator (DLA) utilizing evanescent electric field of racetrack ring resonator structures. Driven by laser light with the correctly designed optical phase window, sustained acceleration of electrons with controlled deflection is shown. Based on this design, we calculate an acceleration from 30 keV to 148.312 keV in 104.655 μm using a cascaded 11-stage racetrack ring resonators. This new idea poses a solution for on-chip integration of many DLA stages, while maintains high average accelerating gradients, providing a potentia…
We show that global lower bounds to the mode volume of a dielectric resonator can be computed via Lagrangian duality. State-of-the-art designs rely on sharp tips, but such structures appear to be highly sub-optimal at nanometer-scale feature sizes, and we demonstrate that computational inverse design offers orders-of-magnitude possible improvements. Our bound can be applied for geometries that are simultaneously resonant at multiple frequencies, for high-efficiency nonlinear-optics applications, and we identify the unavoidable penalties that must accompany such multiresonant structures.
The length spectra of flat three-dimensional dielectric resonators of circular shape were determined from a microwave experiment. They were compared to a semiclassical trace formula obtained within a two-dimensional model based on the effective index of refraction approximation and a good agreement was found. It was necessary to take into account the dispersion of the effective index of refraction for the two-dimensional approximation. Furthermore, small deviations between the experimental length spectrum and the trace formula prediction were attributed to the systematic error of the effective…
In this study, we used parallel plane mirror resonator analogy to design all-dielectric optical resonator that is performed with the objective-first inverse design algorithm. Confinement of the light is succeeded via predefined objective function to create symmetric mirror regions for the fundamental transverse-electric polarization mode. The algorithm creates bandgap in random structure to obtain resonance peak at the desired wavelength without any intuitive scanning of the parameter space. The first order mode is confined on the cavity region at pre-defined wavelength. The obtained structure…
The study of invisibility of an infinite dielectric rod with high refractive index is based on the two-dimensional Mie scattering problem, and it suggests strong suppression of scattering due to the Fano interference between spectrally broad nonresonant waves and narrow Mie-resonant modes. However, when the dielectric rod has a finite extension, it becomes a resonator supporting the Fabry-Perot modes which introduce additional scattering and eventually destroy the invisibility. Here we reveal that for shorter rods with modest values of the aspect ratio r/L (where r and L are the radius and len…
The ability to highly localize light with strong electric field enhancement is critical for enabling higher efficiency solar cells, light sources, and modulators. While deep subwavelength modes can be realized with plasmonic resonators, large losses in these metal structures preclude most practical applications. We developed an alternative approach to achieving subwavelength confinement that is not accompanied by inhibitive losses. We experimentally demonstrate a dielectric bowtie photonic crystal structure that supports mode volumes commensurate with plasmonic elements and quality factors tha…
Molecular optomechanics stems from the description of Raman scattering in the presence of an optical resonator using a cavity optomechanics formalism. We extend the molecular optomechanics formalism to the case of hybrid dielectric-plasmonic resonators, with multiple optical resonances and with both free-space and waveguide addressing. We demonstrate how the Raman enhancement is the product of a pump enhancement and a modified LDOS, that simply depend on the complex response functions of the hybrid system. The Fano lineshapes that result from hybridization of a broadband and narrowband modes a…
Existing methods for the localization of light at the nanoscale use either a structure with negative permittivity, by exploiting subwavelength plasmonic resonances, or a dielectric structure with a high refractive index, which reduces the wavelength. In this paper, we provide an alternative to these two methods based on a modification of the modes of dielectric resonators by means of an active medium. We show that an active medium can promote subwavelength light localization in the dielectric structure. We consider a dielectric layer of size substantially smaller than a half-wavelength of ligh…
We present a detailed experimental study of the symmetry properties and the momentum space representation of the field distributions of a dielectric square resonator as well as the comparison with a semiclassical model. The experiments have been performed with a flat ceramic microwave resonator. Both the resonance spectra and the field distributions were measured. The momentum space representations of the latter evidenced that the resonant states are each related to a specific classical torus, leading to the regular structure of the spectrum. Furthermore, they allow for a precise determination…
The recent realization of topological phases in insulators and superconductors has advanced the quest for robust quantum technologies. The prospects to implement the underlying topological features controllably has given incentive to explore optical platforms for analogous realizations. Here we realize a topologically induced defect state in a chain of dielectric microwave resonators and show that the functionality of the system can be enhanced by supplementing topological protection with non-hermitian symmetries that do not have an electronic counterpart. We draw on a characteristic topologic…
We conjecture that chaotic resonance modes in scattering systems are a product of a conditionally invariant measure from classical dynamics and universal exponentially distributed fluctuations. The multifractal structure of the first factor depends strongly on the lifetime of the mode and describes the average of modes with similar lifetime. The conjecture is supported for a dielectric cavity with chaotic ray dynamics at small wavelengths, in particular for experimentally relevant modes with longest lifetime. We explain scarring of the vast majority of modes along segments of rays based on mul…
Ensembles of nitrogen-vacancy (NV) color centers in diamond hold promise of ultraprecise magnetometery competing with SQUID detectors. By utilizing advantages of dielectric materials such as very low losses for electromagnetic field and therefore possibility to create high quality factor resonators with strong concentration of the field in it we implemented a dielectric resonator antenna for coherent manipulation of large ensemble of NV centers in diamond. We reached average Rabi frequency of 10 MHz in the volume of 7 cubic millimeters with standard deviation less than 1% at moderate pump powe…
Small perturbations in the dielectric environment around a high quality whispering gallery mode resonator usually lead to a frequency shift of the resonator modes directly proportional to the polarizability of the perturbation. Here, we report experimental observations of strong frequency shifts that can be opposite and even exceed the contribution of the perturbations' polarizability. The mode frequencies of a lithium niobate whispering gallery mode resonator are shifted using substrates of refractive indices ranging from 1.50 to 4.22. Both blue- and red-shifts are observed, as well as an inc…
In this paper, the chaotic ray dynamics inside dielectric cavities is described by the properties of an invariant chaotic saddle. I show that the localization of the far field emission in specific directions is related to the filamentary pattern of the saddle's unstable manifold, along which the energy inside the cavity is distributed. For cavities with mixed phase space, the chaotic saddle is divided in hyperbolic and non-hyperbolic components, related, respectively, to the intermediate exponential (t<t_c) and the asymptotic power-law (t>t_c) decay of the energy inside the cavity. The alignme…
Dielectric spheres of various sizes may sustain electromagnetic whispering-gallery modes resonating at optical frequencies with very narrow linewidths. Arbitrary small deviations from the spherical shape typically shift and broaden such resonances. Our goal is to determine these shifted and broadened resonances. A boundary-condition perturbation theory for the acoustic vibrations of nearly circular membranes was developed by Rayleigh more than a century ago. We extend this theory to describe the electromagnetic excitations of nearly spherical dielectric cavities. This approach permits us to av…
We consider eigenmodes of a ring resonator made of a circular dielectric waveguide. Taking into account the polarization corrections, which are responsible for the interaction of polarization and orbital properties of electromagnetic waves (spin-orbit interaction of photons), results in fine splitting of the levels of scalar approximation. The basic features of this fine structure of the levels are similar to that of electron levels in an atom. Namely: 1) sublevels of the fine structure are defined by an additional quantum number: product of helicity of the wave and its orbital moment; 2) for …
The quasi-bound modes localized on stable periodic ray orbits of dielectric micro-cavities are constructed in the short-wavelength limit using the parabolic equation method. These modes are shown to coexist with irregularly spaced "chaotic" modes for the generic case. The wavevector quantization rule for the quasi-bound modes is derived and given a simple physical interpretation in terms of Fresnel reflection; quasi-bound modes are explictly constructed and compared to numerical results. The effect of discrete symmetries of the resonator is analyzed and shown to give rise to quasi-degenerate m…
We discuss the statistical properties of lifetimes of electromagnetic eigenmodes in dielectric microresonators with fully chaotic ray dynamics. Using the example of a resonator of stadium geometry, we find that a recently proposed random-matrix model very well describes the lifetime statistics of long-lived resonances, provided that two effective parameters are appropriately renormalized. This renormalization is linked to the formation of anomalously short-lived resonances, a mechanism also known from the fractal Weyl law and the resonance trapping phenomenon.
We study lasing emission from asymmetric resonant cavity (ARC) GaN micro-lasers. By comparing far-field intensity patterns with images of the micro-laser we find that the lasing modes are concentrated on three-bounce unstable periodic ray orbits, i.e. the modes are scarred. The high-intensity emission directions of these scarred modes are completely different from those predicted by applying Snell's law to the ray orbit. This effect is due to the process of ``Fresnel filtering'' which occurs when a beam of finite angular spread is incident at the critical angle for total internal reflection.
A path within the parameter space of detuning and pump power is demonstrated in order to obtain a single cavity soliton (CS) with certainty in SiN microring resonators in the anomalous dispersion regime. Once the single CS state is reached, it is possible to continue a path to compress it, broadening the corresponding single free spectral range (FSR) Kerr frequency comb. The first step to achieve this goal is to identify the stable regions in the parameter space via numerical simulations of the Lugiato-Lefever equation (LLE). Later, using this identification, we define a path from the stable m…
Electromagnetic response of dielectric resonators with high refractive index is governed by optically induced electric and magnetic Mie resonances facilitating confinement of light with the amplitude enhancement. However, strong subwavelength trapping of light was associated traditionally only with plasmonic or epsilon-near-zero structures which however suffer from losses. Recently, an alternative localization mechanism was proposed to trap light in individual subwavelength optical resonators with a high quality factor in the regime of a supercavity mode. Here, we present the experimental obse…
The authors report on observation of Bragg confined mode in a hollow cylindrical dielectric cavity. A resonance was observed at 13.4 $GHz$ with an unloaded Q-factor of order $2\times10^5$, which is more than a factor of 6 above the dielectric loss limit. Previously such modes have only been realized from pure Transverse Electric modes with no azimuthal variations and only the $E_ϕ$ component. From rigorous numeric simulations it is shown that the mode is a hybrid mode with non-zero azimuthal variations and with dominant $E_r$ and $E_ϕ$ electric field components and $H_z$ magnetic field compone…
A comparative study of unloaded Q-factor measurements of a TE011 mode sapphire dielectric resonator with unloaded Q-factor value of 731,000 at a frequency of 10 GHz and temperature of 65 K using two best Q-factor measurement methods are presented. The Transmission (TMQF) and Reflection methods are based on relevant multi-frequency S-parameter measurements and circle fitting procedures to compute the unloaded Q-factor of the resonator. For accurate comparison of the methods a delay compensation procedure (introduced in the TMQF technique to remove delay due to non-calibrated cables) has been ap…
Optomechanical crystals provide coupling between phonons and photons by confining them to commensurate wavelength-scale dimensions. We present a new concept for designing optomechanical crystals capable of achieving unprecedented coupling rates by confining optical and mechanical waves to deep sub-wavelength dimensions. Our design is based on a dielectric bowtie unit cell with an effective optical/mechanical mode volume of $7.6 \times 10^{-3} {(λ/n_{\textrm{Si}})}^3$/$ 1.2 \times 10^{-3} {λ_{\textrm{mech}}}^3$. We present results from numerical modeling, indicating a single-photon optomechanic…
Dielectric resonators are open systems particularly interesting due to their wide range of applications in optics and photonics. In a recent paper [PRE, vol. 78, 056202 (2008)] the trace formula for both the smooth and the oscillating parts of the resonance density was proposed and checked for the circular cavity. The present paper deals with numerous shapes which would be integrable (square, rectangle, and ellipse), pseudo-integrable (pentagon) and chaotic (stadium), if the cavities were closed (billiard case). A good agreement is found between the theoretical predictions, the numerical simul…
The ultimate limits of performance for any classical optical system are set by sub-wavelength fluctuations within the host material, that may be frozen-in or even dynamically induced. The most common manifestation of such sub-wavelength disorder is Rayleigh light scattering, which is observed in nearly all wave-guiding technologies today and can lead to both irreversible radiative losses as well as undesirable intermodal coupling. While it has been shown that backscattering from disorder can be suppressed by breaking time-reversal symmetry in magneto-optic and topological insulator materials, …
We present a new approach to dielectric metasurface design that relies on a single resonator per unit cell and produces robust, high quality-factor Fano resonances. Our approach utilizes symmetry breaking of highly symmetric resonator geoemetries, such as cubes, to induce couplings between the otherwise orthogonal resonator modes. In particular, we design perturbations that couple "bright" dipole modes to "dark" dipole modes whose radiative decay is suppressed by local field effects in the array. Our approach is widely scalable from the near-infrared to radio frequencies. We first unravel the …
We develop a random-matrix model of two-dimensional dielectric resonators which combines internal wave chaos with the deterministic Fresnel laws for reflection and refraction at the interfaces. The model is used to investigate the statistics of the laser threshold and line width (lifetime and Petermann factor of the resonances) when the resonator is filled with an active medium. The laser threshold decreases for increasing refractive index $n$ and is smaller for TM polarization than for TE polarization, but is almost independent of the number of out-coupling modes $N$. The Petermann factor in …
Metasurfaces are engineered thin surfaces comprising two dimensional (2D) arrays of sub-wavelength spaced and sub-wavelength sized resonators. Metasurfaces can locally manipulate the amplitude, phase and polarization of light with high spatial resolution. In this study, we report numerical and experimental results of a vortex-beam-generating metasurface fabricated specifically for infrared (IR) and terahertz (THz) wavelengths. The designed metasurface consisted of a 2D array of dielectric cross-shaped resonators with spatially varying length, thereby providing desired spatially varying phase s…
Machine learning algorithms have opened a breach in the fortress of the prediction of high-dimensional chaotic systems. Their ability to find hidden correlations in data can be exploited to perform model-free forecasting of spatiotemporal chaos and extreme events. However, the extensive feature of these evolutions constitutes a critical limitation for full-size forecasting processes. Hence, the main challenge for forecasting relevant events is to establish the set of pertinent information. Here, we identify precursors from the transfer entropy of the system and a deep Long Short-Term Memory ne…
We present a novel design of optical micro-cavity where the optical energy resides primarily in free space, therefore is readily accessible to foreign objects such as atoms, molecules, mechanical resonators, etc. We describe the physics of these resonators, and propose a design method based on stochastic optimization. Cavity designs with diffraction-limited mode volumes and quality factors in the range of $10^4$--$10^6$ are presented. With a purely planar geometry, the cavity can be easily integrated on-chip using conventional micro- and nano- fabrication processes.
Printing technology based on plasmonic structures has many advantages over pigment based color printing such as high resolution, ultra-compact size and low power consumption. However, due to high losses and broad resonance behavior of metals in the visible spectrum, it becomes challenging to produce well-defined colors. Here, we investigate cross-shaped dielectric nanoresonators which enable high quality resonance in the visible spectral regime and, hence, high quality colors. We numerically predict and experimentally demonstrate that the proposed all-dielectric nanostructures exhibit high qua…
