We describe a method of selective generation and study of polarization moments of up to the highest rank $κ=2F$ possible for a quantum state with total angular momentum $F$. The technique is based on nonlinear magneto-optical rotation with frequency-modulated light. Various polarization moments are distinguished by the periodicity of light-polarization rotation induced by the atoms during Larmor precession and exhibit distinct light-intensity and frequency dependences. We apply the method to study polarization moments of $^{87}$Rb atoms contained in a vapor cell with antirelaxation coating. Distinct ultra-narrow (1-Hz wide) resonances, corresponding to different multipoles, appear in the magnetic-field dependence of the optical rotation. The use of the highest-multipole resonances has important applications in quantum and nonlinear optics and in magnetometry.
The possibility of achieving highly selective excitation of low metastable states of hydrogen and helium atoms by using short laser pulses with reasonable parameters is demonstrated theoretically. Interactions of atoms with the laser field are studied by solving the close-coupling equations without discretization. The parameters of laser pulses are calculated using different kinds of optimization procedures. For the excitation durations of hundreds of femtoseconds direct optimization of the parameters of one and two laser pulses with Gaussian envelopes is used to introduce a number of simple s…
We present an experimental and theoretical investigation of two-photon direct frequency-comb spectroscopy performed through velocity-selective excitation. In particular, we explore the effect of repetition rate on the $\textrm{5S}_{1/2}\rightarrow \textrm{5D}_{3/2, 5/2}$ two-photon transitions excited in a rubidium atomic vapor cell. The transitions occur via step-wise excitation through the $\textrm{5P}_{1/2, 3/2}$ states by use of the direct output of an optical frequency comb. Experiments were performed with two different frequency combs, one with a repetition rate of $\approx 925$ MHz and …
We propose here a few selective highly charged ions (HCIs), namely Ni$^{12+}$ and Cu$^{13+}$, Pd$^{12+}$ and Ag$^{13+}$, that not only promise to be very high accurate optical clocks below $10^{-19}$ uncertainties, but also offer quality factors larger than $10^{15}$ and yet possess simple atomic structures for the experimental set-up. Moreover, these ions have strong optical magnetic-dipole (M1) transitions than the previously proposed HCI clocks. They can be used for the cooling and detection techniques. To demonstrate the projected fractional uncertainties below $10^{-19}$ level, we have es…
We have studied the peculiarities of selective reflection from Rb vapor cell with thickness $L <$ 70 nm, which is over an order of magnitude smaller than the resonant wavelength for Rb atomic D$_1$ line $λ$ = 795 nm. A huge ($\approx$ 240 MHz) red shift and spectral broadening of reflection signal is recorded for $L =$ 40 nm caused by the atom-surface interaction. Also completely frequency resolved hyperfine Paschen-Back splitting of atomic transitions to four components for $^{87}$Rb and six components for $^{85}$Rb is recorded in strong magnetic field ($B >$ 2 kG).
We trap atoms in versatile two-dimensional (2D) arrays of optical potentials, prepare flexible 2D spin configurations, perform site-selective coherent manipulation, and demonstrate the implementation of simultaneous measurements of different system properties, such as dephasing and decoherence. This novel approach for the flexible manipulation of atomic quantum systems is based on the combination of 2D arrays of microlenses and 2D arrays of liquid crystal light modulators. It offers novel types of control for the investigation of quantum degenerate gases, quantum information processing, and qu…
We demonstrate novel implementations of high-precision optical magnetometers which allow for spatially-selective and spatially-resolved in situ measurements using cold atomic clouds. These are realised by using shaped dispersive probe beams combined with spatially-resolved balanced homodyne detection. Two magnetometer sequences are discussed: a vectorial magnetometer, which yields sensitivities two orders of magnitude better compared to a previous realisation and a Larmor magnetometer capable of measuring absolute magnetic fields. We characterise the dependence of single-shot precision on the …
We report on the selective addressing of an individual atom in a pair of single-atom microtraps separated by $3\;μ$m. Using a tunable light-shift, we render the selected atom off-resonant with a global Rydberg excitation laser which is resonant with the other atom, making it possible to selectively block this atom from being excited to the Rydberg state. Furthermore we demonstrate the controlled manipulation of a two-atom entangled state by using the addressing beam to induce a phase shift onto one component of the wave function of the system, transferring it to a dark state for the Rydberg ex…
Isotope-selective Ion Trapping via Sympathetic Cooling using a Surface-Electrode Trap with a Hole for Collimated Atomic Loading
Graduate School of Engineering Science, Osaka University（大阪大学工学研究科）；Institute for Integrated Radiation and Nuclear Science, Kyoto University（京都大学辐射核科学综合研究所）；National Institute of Information and Communications Technology（信息通信研究机构）；Center of Quantum Information and Quantum Biology, Osaka University（大阪大学量子信息与量子生物学中心）
We demonstrate that a method using the derivative of the selective reflection signal from a nanocell is a convenient and robust tool for atomic laser spectroscopy, achieving a nearly Doppler-free spectral resolution. The recorded linewidth of the signal from a potassium-filled cell, whose thickness $\ell$ lies in the range $350-500$ nm, is 18 times smaller than the Doppler linewidth ($\sim 900$ MHz full width at half maximum) of potassium atoms. We also show experimentally a sign oscillation of the reflected signal's derivative with a periodicity of $λ/2$ when $\ell$ varies from 190 to 1200~nm…
Decoupling of total electronic and nuclear spin moments of Cs atoms in external magnetic field for the case of atomic $D_1$ line, leading to onset of the hyperfine Paschen-Back regime has been studied theoretically and experimentally. Selective reflection of laser radiation from an interface of dielectric window and atomic vapor confined in a nanocell with 300 nm gap thickness was implemented for the experimental studies. The real time derivative of selective reflection signal with a frequency position coinciding with atomic transitions was used in measurements, providing $\sim$ 40 MHz spectra…
We study the fidelity of single qubit quantum gates performed with two-frequency laser fields that have a Gaussian or super Gaussian spatial mode. Numerical simulations are used to account for imperfections arising from atomic motion in an optical trap, spatially varying Stark shifts of the trapping and control beams, and transverse and axial misalignment of the control beams. Numerical results that account for the three dimensional distribution of control light show that a super Gaussian mode with intensity $I\sim e^{-2(r/w_0)^n}$ provides reduced sensitivity to atomic motion and beam misalig…
We implement a microscopic spin filter for cold fermionic atoms in a quantum point contact (QPC) and create fully spin-polarized currents while retaining conductance quantization. Key to our scheme is a near-resonant optical tweezer inducing a large effective Zeeman shift inside the QPC while its local character limits dissipation. We observe a renormalization of this shift due to interactions of a few atoms in the QPC. Our work represents the analog of an actual spintronic device and paves the way to studying the interplay between spin-splitting and interactions far from equilibrium.
We experimentally demonstrate robust selective excitation and attenuation of atomic Rydberg level populations in sodium vapor (Na I) using intense laser pulses in the strong field limit ($> 10^{12} W/cm^{2}$). The coherent control of the atomic population and related ionization channels is realized for intensities above the over-the-barrier ionization intensity. A qualitative model predicts that this strong field coherent control arises through the manifestation of a Freeman resonance.
In the annihilation of a positron with a bound atomic electron, the virtual gamma photon created may excite the atomic nucleus. We put forward this effect as a spectroscopic tool for an energy-selective excitation of nuclear transitions. This scheme can efficiently populate nuclear levels of arbitrary multipolarities in the MeV regime, including monopole transitions and giant resonances. In certain cases, it may have a higher cross sections than the conventionally used Coulomb excitation.
In the presence of Earth gravity and gravity-gradient forces, centrifugal and Coriolis forces caused by the Earth rotation, the phase of the time-domain atom interferometers is calculated with accuracy up to the terms proportional to the fourth degree of the time separation between pulses. We considered double-loop atom interferometers and found appropriate condition to eliminate their sensitivity to acceleration to get atomic gyroscope, or to eliminate the sensitivity to rotation to increase accuracy of the atomic gravimeter. Consequent use of these interferometers allows one to measure all c…
We report on a method of light-shift engineering where an auxiliary laser is used to tune the atomic transition frequency. The technique is used to selectively load a specific region of an optical lattice. The results are explained by calculating the differential light-shift of each hyperfine state. We conclude that the remarkable spatial selectivity of light-shift engineering using an auxiliary laser provides a powerful technique to prepare ultra-cold trapped atoms for experiments on quantum gases and quantum information processing.
Selective laser addressing of a single atom or atomic ion qubit can be improved using narrowband composite pulse sequences. We describe a Lie-algebraic technique to generalize known narrowband sequences and introduce new sequences related by dilation and rotation of sequence generators. Our method improves known narrowband sequences by decreasing both the pulse time and the residual error. Finally, we experimentally demonstrate these composite sequences using $^{40}$Ca$^+$ ions trapped in a surface-electrode ion trap.
A central goal within quantum optics is to realize efficient interactions between photons and atoms. A fundamental limit in nearly all applications based on such systems arises from spontaneous emission, in which photons are absorbed by atoms and then re-scattered into undesired channels. In typical treatments of atomic ensembles, it is assumed that this re-scattering occurs independently, and at a rate given by a single isolated atom, which in turn gives rise to standard limits of fidelity in applications such as quantum memories or quantum gates. However, this assumption can be violated. In …
We demonstrate arbitrary coherent addressing of individual neutral atoms in a $5\times 5\times 5$ array formed by an optical lattice. Addressing is accomplished using rapidly reconfigurable crossed laser beams to selectively ac Stark shift target atoms, so that only target atoms are resonant with state-changing microwaves. The effect of these targeted single qubit gates on the quantum information stored in non-targeted atoms is smaller than $3\times 10^{-3}$ in state fidelity. This is an important step along the path of converting the scalability promise of neutral atoms into reality.
Anisotropy of atomic states is characterized by population differences and coherences between Zeeman sublevels. It can be efficiently created and probed via resonant interactions with light, the technique which is at the heart of modern atomic clocks and magnetometers. Recently, nonlinear magneto-optical techniques have been developed for selective production and detection of higher polarization moments, hexadecapole and hexacontatetrapole, in the ground states of the alkali atoms. Extension of these techniques into the range of geomagnetic fields is important for practical applications. This …
We simulate collisions between two atoms, which move in an optical lattice under the dipole-dipole interaction. The model describes simultaneously the two basic dynamical processes, namely the Sisyphus cooling of single atoms, and the light-induced inelastic collisions between them. We consider the J=1/2 -> J=3/2 laser cooling transition for Cs, Rb and Na. We find that the hotter atoms in a thermal sample are selectively lost or heated by the collisions, which modifies the steady state distribution of atomic velocities, reminiscent of the evaporative cooling process.
Methods to manipulate the individual constituents of an ultracold quantum gas mixture are essential tools for a number of applications, for example the direct quantum simulation of impurity physics. We investigate a scheme in which species-selective control is achieved using magnetic potentials dressed with multiple radiofrequencies, exploiting the different Landé g-factors of the constituent atomic species. We describe a mixture dressed with two frequencies, where atoms are confined in harmonic potentials with a controllable degree of overlap between the two atomic species. This is then exten…
We present a compact $^{87}$Rb atomic source for high precision dual atom interferometers. The source is based on a double-stage magneto-optical trap (MOT) design, consisting of a 2-dimensional (2D)-MOT for efficient loading of a 3D-MOT. The accumulated atoms are precisely launched in a horizontal moving molasses. Our setup generates a high atomic flux ($>10^{10}$ atoms/s) with precise and flexibly tunable atomic trajectories as required for high resolution Sagnac atom interferometry. We characterize the performance of the source with respect to the relevant parameters of the launched atoms, i…
We apply optical pumping to prepare the lithium beam of our atom interferometer in a single hyperfine-Zeeman sublevel: we use two components of the D1-line for pumping the 7Li atoms in a dark state F,mF=+2 (or -2) sublevel. The optical pumping efficiency has been characterized by two techniques: state-selective laser atom deflection or magnetic dephasing of the atom interferometer signals. The first technique has not achieved a high sensitivity, because of a limited signal to noise ratio, but magnetic dephasing signals have shown that about 95% of the population has been transferred in the aim…
Rydberg spin waves are optically excited in a quasi-one-dimensional atomic sample of Rb atoms. Pair-wise spin-wave correlations are observed by a spatially selective transfer of the quantum state onto a light field and photoelectric correlation measurements of the light. The correlations are interpreted in terms of the dephasing of multiply-excited spin waves by long-range Rydberg interactions.
Neutral atom arrays are promising for large-scale quantum computing especially because it is possible to prepare large-scale qubit arrays. An unsolved issue is how to selectively excite one qubit deep in a 3D atomic array to Rydberg states. In this work, we show two methods for this purpose. The first method relies on a well-known result: in a dipole transition between two quantum states driven by two off-resonant fields of equal strength but opposite detunings $\pmΔ$, the transition is characterized by two counter-rotating Rabi frequencies $Ωe^{\pm iΔt}$~[or $\pmΩe^{\pm iΔt}$ if the two field…
We present a new and efficient implementation of Raman cooling of trapped atoms. It uses Raman pulses with an appropriate frequency chirp to realize a velocity selective excitation through a rapid adiabatic passage. This method allows to address in a single pulse a large number of non zero atomic velocity classes and it produces a nearly unity transfer efficiency. We demonstrate this cooling method using cesium atoms in a far-detuned crossed dipole trap. Three-dimensional cooling of $1 \times 10^{5}$ atoms down to $2 μ$K is performed in 100 ms. In this preliminary experiment the final atomic d…
Site-selective preparation of two-dimensional dipolar quantum gases in an optical beat-note lattice
Institut für Quantenoptik und Quanteninformation (IQOQI), Österreichische Akademie der Wissenschaften（奥地利科学院量子光学与量子信息研究所）；Institut für Experimentalphysik, Universität Innsbruck（因斯布鲁克大学实验物理系）
The two-photon transition $5S-5P-5D$ in rubidium vapor is investigated by detecting the fluorescence from the $6P_{3/2}$ state when the atomic system is excited by the combined action of a cw diode laser and a train of ultrashort pulses. The cw-laser plays a role as a velocity-selective filter and allows for a spectroscopy over a large spectral range including the $5D_{3/2}$ and $5D_{5/2}$ states. For a counterpropagating beam configuration, the response of each atomic velocity group is well characterized within the Doppler profile, and the excited hyperfine levels are clearly resolved. The co…
State selective field ionization detection techniques in physics require a specific progression through a complicated atomic state space to optimize state selectivity and overall efficiency. For large principle quantum number n, the theoretical models become computationally intractable and any results are often rendered irrelevant by small deviations from ideal experimental conditions, for example external electromagnetic fields. Several different proposals for quantum information processing rely heavily upon the quality of these detectors. In this paper, we show a proof of principle that it i…
A simple scheme is presented for realizing robust optically controlled quantum gates for scalable atomic quantum processors by driving the qubits with optical standing waves. Atoms localized close to the antinodes of the standing wave can realize phase-controlled quantum operations that are potentially more than an order of magnitude less sensitive to the local optical phase and atomic motion than corresponding travelling wave configurations. The scheme is compatible with robust optimal control techniques and spatial qubit addressing in atomic arrays to realize phase controlled operations with…
Polarization-selective quantum cooperative response in dual-species atom arrays
Institute of Optics and Electronics, Chinese Academy of Sciences（中国科学院光电技术研究所）；College of Materials Science and Opto-Electronic Technology, University of Chinese Academy of Sciences（中国科学院大学材料科学与光电技术学院）
Measurement-based quantum computing relies on the rapid creation of large-scale entanglement in a register of stable qubits. Atomic arrays are well suited to store quantum information, and entanglement can be created using highly-excited Rydberg states. Typically, isolating pairs during gate operation is difficult because Rydberg interactions feature long tails at large distances. Here, we engineer distance-selective interactions that are strongly peaked in distance through off-resonant laser coupling of molecular potentials between Rydberg atom pairs. Employing quantum gas microscopy, we veri…
This article proposes the first discrete-time implementation of Rydberg quantum walk in multi-dimensional spatial space that could ideally simulate different classes of topological insulators. Using distance-selective exchange-interaction between Rydberg excited atoms in an atomic array with dual lattice-constants, the new setup operates both coined and coin-less models of discrete-time quantum walk (DTQW). Here, complicated coupling tessellations are performed by a global laser that exclusively excites the site at the anti-blockade region. The long-range interaction provides a new feature of …
