Neutral atom arrays are promising for large-scale quantum computing especially because it is possible to prepare large-scale qubit arrays. An unsolved issue is how to selectively excite one qubit deep in a 3D atomic array to Rydberg states. In this work, we show two methods for this purpose. The first method relies on a well-known result: in a dipole transition between two quantum states driven by two off-resonant fields of equal strength but opposite detunings $\pmΔ$, the transition is characterized by two counter-rotating Rabi frequencies $Ωe^{\pm iΔt}$~[or $\pmΩe^{\pm iΔt}$ if the two fields have a $π$-phase difference]. This pair of detuned fields lead to a time-dependent Rabi frequency $2Ω\cos(Δt)$~[or $2iΩ\sin(Δt)$], so that a full transition between the two levels is recovered. We show that when the two detuned fields are sent in different directions, one atom in a 3D optical lattice can be selectively addressed for Rydberg excitation, and when its state is restored, the state of any nontarget atoms irradiated in the light path is also restored. Moreover, we find that the Rydberg excitation by this method can significantly suppress the fundamental blockade error of a Rydberg gate, paving the way for a high-fidelity entangling gate with commonly used quasi-rectangular pulse that is easily obtained by pulse pickers. Along the way, we find a second method for single-site Rydberg addressing in 3D, where a selected target atom can be excited to Rydberg state while preserving the state of any nontarget atom due to a spin echo sequence. The capability to selectively address a target atom in 3D atomic arrays for Rydberg excitation makes it possible to design large-scale neutral-atom information processor based on Rydberg blockade.
We report on the selective addressing of an individual atom in a pair of single-atom microtraps separated by $3\;μ$m. Using a tunable light-shift, we render the selected atom off-resonant with a global Rydberg excitation laser which is resonant with the other atom, making it possible to selectively block this atom from being excited to the Rydberg state. Furthermore we demonstrate the controlled manipulation of a two-atom entangled state by using the addressing beam to induce a phase shift onto one component of the wave function of the system, transferring it to a dark state for the Rydberg ex…
Quantum gates and entanglement based on dipole-dipole interactions of neutral Rydberg atoms are relevant to both fundamental physics and quantum information science. The precision and robustness of the Rydberg-mediated entanglement protocols are the key factors limiting their applicability in experiments and near-future industry. There are various methods for generating entangling gates by exploring the Rydberg interactions of neutral atoms, each equipped with its own strengths and weaknesses. The basics and tricks in these protocols are reviewed, with specific attention paid to the achievable…
The performance of many control tasks with Rydberg atoms can be improved via suppression of the motion-induced dephasing between ground and Rydberg states of neutral atoms. The dephasing often occurs during the {\it gap} time when the atom is shelved in a Rydberg state before its deexcitation. By using laser fields to induce specific extra phase change to the Rydberg state during the gap time, it is possible to faithfully transfer the Rydberg state back to the ground state after the gap. Although the Rydberg state transitions back and forth between different eigenstates during the gap time, it…
The motion-induced dephasing is a severe problem that limits the accuracy of a quantum control process by using external laser fields in neutral Rydberg atoms. This dephasing is a major issue that limits the realizable fidelity of a quantum entangling gate with neutral atoms when there is a {\it gap} time for the Rydberg atom to drift freely. We find that such a dephasing can be largely suppressed by using a transition in a `V'-type dual-rail configuration. The left~(right) arm of this `V' represents a transition to a Rydberg state $|r_{1(2)}\rangle$ with a Rabi frequency $Ωe^{ikz}~(Ωe^{-ikz})…
Neutral atoms are promising for large-scale quantum computing, but accurate neutral-atom entanglement depends on large Rydberg interactions which strongly limit the interatomic distances. Via a phase accumulation in detuned Rabi cycles enabled by a Rydberg interaction of similar magnitude to the Rydberg Rabi frequency, we study a controlled-phase gate with an arbitrary phase and extend it to the controlled-NOT gate. The gates need only three steps for coupling one Rydberg state, depend on easily accessible van der Waals interaction that naturally arises between distant atoms, and have no rotat…
Hyperentanglement~(HE), the simultaneous entanglement between two particles in more than one degrees of freedom, is relevant to both fundamental physics and quantum technology. Previous study on HE has been focusing on photons. Here, we study HE in individual neutral atoms. In most alkaline-earth-like atoms with two valence electrons and a nonzero nuclear spin, there are two stable electronic states, the ground state and the long-lived clock state, which can define an electronic qubit. Meanwhile, their nuclear spin states can define a nuclear qubit. By the Rydberg blockade effect, we show that…
Experiments performed within the last year have demonstrated Rydberg state mediated quantum gates and deterministic entanglement between pairs of trapped neutral atoms. These experiments validate ten year old proposals for Rydberg mediated quantum logic, but are only the beginning of ongoing efforts to improve the fidelity of the results obtained and scale the experiments to larger numbers of qubits. We present here a summary of the results to date, along with a critical evaluation of the prospects for higher fidelity Rydberg gates.
Conditions to achieve an unusually strong Rydberg spin-exchange interaction are investigated and proposed as a means to generate pairwise entanglement and realize a SWAP-like quantum gate for neutral atoms. Ground-state entanglement is created by mapping entangled Rydberg states to ground states using optical techniques. A protocol involving SWAP gate and pairwise entanglement operations is predicted to create global entanglement of a chain of $N$ atoms in a time that is independent of $N$.
Exploring controllable interactions lies at the heart of quantum science. Neutral Rydberg atoms provide a versatile route toward flexible interactions between single quanta. Previous efforts mainly focused on the excitation annihilation~(EA) effect of the Rydberg blockade due to its robustness against interaction fluctuation. We study another effect of the Rydberg blockade, namely, the transition slow-down~(TSD). In TSD, a ground-Rydberg cycling in one atom slows down a Rydberg-involved state transition of a nearby atom, which is in contrast to EA that annihilates a presumed state transition. …
We demonstrate the first deterministic entanglement of two individually addressed neutral atoms using a Rydberg blockade mediated controlled-NOT gate. Parity oscillation measurements reveal an entanglement fidelity of $F=0.58\pm0.04$, which is above the entanglement threshold of $F=0.5$, without any correction for atom loss, and $F=0.71\pm0.05$ after correcting for background collisional losses. The fidelity results are shown to be in good agreement with a detailed error model.
We discuss a method for scaling a neutral atom Rydberg gate quantum processor to a large number of qubits. Limits are derived showing that the number of qubits that can be directly connected by entangling gates with errors at the $10^{-3}$ level using long range Rydberg interactions between sites in an optical lattice, without mechanical motion or swap chains, is about 500 in two dimensions and 7500 in three dimensions. A scaling factor of 60 at a smaller number of sites can be obtained using collective register encoding in the hyperfine ground states of the rare earth atom Holmium. We present…
Neutral atoms are building blocks of ground-up quantum many-body systems. Well-controlled and high-fidelity entangling gates are an essential component for realizing complex neutral atom architectures for quantum computing, quantum simulation, and measurement with precision better than the standard quantum limit. In this Letter we report the realization of a Mølmer-Sørensen unitary between two neutral atoms, based on adiabatic single-photon dressing to Rydberg levels. We show that this technique is highly robust to noise sources and experimental imperfections that have limited the fidelity of …
Alkaline-earth-like~(AEL) atoms with two valence electrons and a nonzero nuclear spin can be excited to Rydberg state for quantum computing. Typical AEL ground states possess no hyperfine splitting, but unfortunately a GHz-scale splitting seems necessary for Rydberg excitation. Though strong magnetic fields can induce a GHz-scale splitting, weak fields are desirable to avoid noise in experiments. Here, we provide two solutions to this outstanding challenge with realistic data of well-studied AEL isotopes. In the first theory, the two nuclear spin qubit states $|0\rangle$ and $|1\rangle$ are ex…
We present experimental results on two-qubit Rydberg blockade quantum gates and entanglement in a two-dimensional qubit array. Without post selection against atom loss we achieve a Bell state fidelity of $0.73\pm 0.05$, the highest value reported to date. The experiments are performed in an array of single Cs atom qubits with a site to site spacing of $3.8 ~ μ\rm m$. Using the standard protocol for a Rydberg blockade C$_Z$ gate together with single qubit operations we create Bell states and measure their fidelity using parity oscillations. We analyze the role of AC Stark shifts that occur when…
We report results of a ground-state entanglement protocol for a pair of Cs atoms separated by 6~$μ$m, combining the Rydberg blockade mechanism with a two-photon Raman transitions to prepare the $\vertΨ^+\rangle=(\vert 10\rangle+\vert 01\rangle)/\sqrt{2}$ Bell state with a loss-corrected fidelity of 0.81(5), equal to the best demonstrated fidelity for atoms trapped in optical tweezers but without the requirement for dynamically adjustable interatomic spacing. Qubit state coherence is also critical for quantum information applications, and we characterise both ground-state and ground-Rydberg dep…
One can implement fast two-qubit entangling gates by exploiting the Rydberg blockade. Although various theoretical schemes have been proposed, experimenters have not yet been able to demonstrate two-atom gates of high fidelity due to experimental constraints. We propose a novel scheme, which only uses a single Rydberg pulse illuminating both atoms, for the construction of neutral-atom controlled-phase gates. In contrast to the existing schemes, our approach is simpler to implement and requires neither individual addressing of atoms nor adiabatic procedures. With parameters estimated based on a…
We propose a cooling scheme to prepare stationary entanglement of neutral atoms in the Rydberg blockade regime by combination of periodically collective laser pumping and dissipation. In each cycle, the controlled unitary dynamics process can selectively pump atoms away from the non-target state while maintaining the target state unchanged. The subsequent dissipative process redistributes the populations of ground states through the engineered spontaneous emission. After a number of cycles, the system will be eventually stabilized into the desired steady state independent of the initial state.…
Compared with the idea of universal quantum computation, a direct synthesis of a multiqubit logic gate can greatly improve the efficiency of quantum information processing tasks. Here we propose an efficient scheme to implement a three-qubit controlled-not (Toffoli) gate of neutral atoms based on unconventional Rydberg pumping. By adjusting the strengths of Rabi frequencies of driving fields, the Toffoli gate can be achieved within one step, which is also insensitive to the fluctuation of the Rydberg-Rydberg interaction. Considering different atom alignments, we can obtain a high-fidelity Toff…
We demonstrate high fidelity two-qubit Rydberg blockade and entanglement in a two-dimensional qubit array. The qubit array is defined by a grid of blue detuned lines of light with 121 sites for trapping atomic qubits. Improved experimental methods have increased the observed Bell state fidelity to $F_{\rm Bell}=0.86(2)$. Accounting for errors in state preparation and measurement (SPAM) we infer a fidelity of $F_{\rm Bell}^{\rm -SPAM}=0.88$. Accounting for errors in single qubit operations we infer that a Bell state created with the Rydberg mediated $C_Z$ gate has a fidelity of $F_{\rm Bell}^{C…
Neutral atom array serves as an ideal platform to study the quantum logic gates, where intense efforts have been devoted to improve the two-qubit gate fidelity. We report our recent findings in constructing a different type of two-qubit controlled-PHASE quantum gate protocol with neutral atoms enabled by Rydberg blockade, which aims at both robustness and high-fidelity. It relies upon modulated driving pulse with specially tailored smooth waveform to gain appropriate phase accumulations for quantum gates. The major features include finishing gate operation within a single pulse, not necessaril…
Electromagnetically induced transparency (EIT) in atomic systems involving Rydberg states is known to be a sensitive probe of incident microwave (MW) fields, in particular those resonant with Rydberg-to-Rydberg transitions. Here we propose an intelligible analytical model of Rydberg atomic receiver's response to amplitude- (AM) and frequency-modulated (FM) signals, and compare it with experimental results: we present a setup that allows sending signals with either AM or FM and evaluating their efficiency with demodulation. Additionally, the setup reveals a new detection configuration, using al…
We report the generation of entanglement between two individual $^{87}$Rb atoms in hyperfine ground states $|F=1,M=1>$ and $|F=2,M=2>$ which are held in two optical tweezers separated by 4 $μ$m. Our scheme relies on the Rydberg blockade effect which prevents the simultaneous excitation of the two atoms to a Rydberg state. The entangled state is generated in about 200 ns using pulsed two-photon excitation. We quantify the entanglement by applying global Raman rotations on both atoms. We measure that 61% of the initial pairs of atoms are still present at the end of the entangling sequence. These…
While the Rydberg-blockade regime provides the natural setting for creating $W$-type entanglement with cold neutral atoms, it is demonstrated here that a scalable entanglement resource of this type can even be obtained under completely different physical circumstances. To be more precise, a special instance of twisted $W$ states -- namely, $π$-twisted ones -- can be engineered in one-dimensional arrays of cold neutral atoms with Rydberg-dressed resonant dipole-dipole interaction. In particular, it is shown here that this is possible even when a (dressed) Rydberg excitation is coupled to the mo…
Implementation of two-qubit Rydberg operations on neutral Rb-87 atoms in systems with different intermediate states
Moscow Institute of Physics and Technology (MIPT)（莫斯科物理技术学院）；Russian Quantum Center (RQC)（俄罗斯量子中心）；P. N. Lebedev Physical Institute (LPI)（列别捷夫物理研究所）；Quantum Technology Centre and Faculty of Physics, M. V. Lomonosov Moscow State University（莫斯科大学量子技术中心与物理系）；Technical University of Munich（慕尼黑工业大学）；Ludwig-Maximilians-Universität München（慕尼黑大学）
We study a scheme for implementing a controlled-Z (CZ) gate between two neutral-atom qubits based on the Rydberg blockade mechanism in a manner that is robust to errors caused by atomic motion. By employing adiabatic dressing of the ground electronic state, we can protect the gate from decoherence due to random phase errors that typically arise because of atomic thermal motion. In addition, the adiabatic protocol allows for a Doppler-free configuration that involves counterpropagating lasers in a $σ_+/σ_-$ orthogonal polarization geometry that further reduces motional errors due to Doppler shi…
Symmetric $C_Z$ gate for ultracold neutral atoms based on counterdiabatic driving at Rydberg excitation
Rzhanov Institute of Semiconductor Physics SB RAS（拉扎诺夫半导体物理研究所西伯利亚分院）；Novosibirsk State University（新西伯利亚国立大学）；Novosibirsk State Technical University（新西伯利亚国立技术大学）；Institute of Laser Physics SB RAS（激光物理研究所西伯利亚分院）；Division of Precision Measurement Physics, Wuhan Institute of Physics and Mathematics, Innovation Academy for Precision Measurement Science and Technology, Chinese Academy of Sciences（中国科学院精密测量科学与技术创新研究院武汉物理与数学研究所精密测量物理研究室）
Recently, the notion of two-qubit controlled phase gate via off-resonant modulated driving has been introduced into the neutral atom qubit platform, with respect to both single-photon and two-photon ground-Rydberg transitions. In order to reach a better performance practically, further developments are in need to overcome a few known limitations in previous discussions of this promising method. Here, we thoroughly analyze a variety of modulation styles for two-photon transitions, demonstrating the versatility of off-resonant modulated driving protocols. Furthermore, we show that it is possible…
Trapped Rydberg ions are a promising novel approach to quantum computing and simulations. They are envisaged to combine the exquisite control of trapped ion qubits with the fast two-qubit Rydberg gates already demonstrated in neutral atom experiments. Coherent Rydberg excitation is a key requirement for these gates. Here, we carry out the first coherent Rydberg excitation of an ion and perform a single-qubit Rydberg gate, thus demonstrating basic elements of a trapped Rydberg ion quantum computer.
Long range Rydberg blockade interactions have the potential for efficient implementation of quantum gates between multiple atoms. Here we present and analyze a protocol for implementation of a $k$-atom controlled NOT (C$_k$NOT) neutral atom gate. This gate can be implemented using sequential or simultaneous addressing of the control atoms which requires only $2k+3$ or 5 Rydberg $π$ pulses respectively. A detailed error analysis relevant for implementations based on alkali atom Rydberg states is provided which shows that gate errors less than 10% are possible for $k=35$.
We investigate the electronic structure of a triatomic Rydberg molecule formed by a Rydberg atom and two neutral ground-state atoms. Taking into account the $s$-wave and $p$-wave interactions we perform electronic structure calculations and analyze the adiabatic electronic potentials evolving from the Rb$(n=35, l\ge 3)$ Rydberg degenerate manifold. We hereby focus on three different classes of geometries of the Rydberg molecules, including symmetric, asymmetric and planar configurations. The metamorphosis of these potential energy surfaces in the presence of an external electric field is explo…
We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar molecule within the electron orbit in a Rydberg atom can either shift the Rydberg state, or form Rydberg molecule. Both the atomic shift and the Rydberg molecule states depend on the initial internal state of the polar molecule, resulting in molecular state dependent van der Waals or dipole-dipole interaction between Rydberg atoms. Rydberg atoms mediated in…
Neutral atom platform has become an attractive choice to study the science of quantum information and quantum simulation, where intense efforts have been devoted to the entangling processes between individual atoms. For the development of this area, two-qubit controlled-PHASE gate via Rydberg blockade is one of the most essential elements. Recent theoretical studies have suggested the advantages of introducing non-trivial waveform modulation into the gate protocol, which is anticipated to improve its performance towards the next stage. We report our recent experimental results in realizing a t…
Individual neutral atoms excited to Rydberg states are a promising platform for quantum simulation and quantum information processing. However, experimental progress to date has been limited by short coherence times and relatively low gate fidelities associated with such Rydberg excitations. We report progress towards high-fidelity quantum control of Rydberg atom qubits. Enabled by a reduction in laser phase noise, our approach yields a significant improvement in coherence properties of individual qubits. We further show that this high-fidelity control extends to the multi-particle case by pre…
Universal quantum gates and quantum error correction~(QEC) lie in the heart of quantum information science. Large-scale quantum computing depends on a universal set of quantum gates, in which some gates may be easily carried out, while others are hard with a certain physical system. There is a unique three-qubit quantum gate called the Deutsch gate~[$\mathbb{D}(θ)$], from which alone a circuit can be constructed so that any feasible quantum computing is attainable. As far as we know, however, $\mathbb{D}(θ)$ has not been demonstrated. Here we design an easily realizable $\mathbb{D}(θ)$ by usin…
We report on the local control of the transition frequency of a spin-$1/2$ encoded in two Rydberg levels of an individual atom by applying a state-selective light shift using an addressing beam. With this tool, we first study the spectrum of an elementary system of two spins, tuning it from a non-resonant to a resonant regime, where "bright" (superradiant) and "dark" (subradiant) states emerge. We observe the collective enhancement of the microwave coupling to the bright state. We then show that after preparing an initial single spin excitation and letting it hop due to the spin-exchange inter…
Anomalously enhanced lifetimes of low angular momentum Rydberg states in singly charged alkaline-earth metal ions
Institut für Theoretische Physik and Center for Integrated Quantum Science and Technology, Universität Tübingen（蒂宾根大学理论物理研究所与集成量子科学与技术中心）；School of Physics and Astronomy and Centre for the Mathematics and Theoretical Physics of Quantum Non-Equilibrium Systems, The University of Nottingham（诺丁汉大学物理与天文学学院及量子非平衡系统数学与理论物理中心）
Single neutral atoms trapped in optical tweezers and laser-coupled to Rydberg states provide a fast and flexible platform to generate configurable atomic arrays for quantum simulation. The platform is especially suited to study quantum spin systems in various geometries. However, for experiments requiring continuous trapping, inhomogeneous light shifts induced by the trapping potential and temperature broadening impose severe limitations. Here we show how Raman sideband cooling allows one to overcome those limitations, thus, preparing the stage for Rydberg dressing in tweezer arrays.
Quantum information processing based on Rydberg atoms emerged as a promising direction two decades ago. Recent experimental and theoretical progresses have shined exciting light on this avenue. In this concise review, we will briefly introduce the basics of Rydberg atoms and their recent applications in associated areas of neutral atom quantum computation and simulation. We shall also include related discussions on quantum optics with Rydberg atomic ensembles, which are increasingly used to explore quantum computation and quantum simulation with photons.
Neutral atom arrays have recently emerged as a promising platform for quantum information processing. One important remaining roadblock for the large-scale application of these systems is the ability to perform error-corrected quantum operations. To entangle the qubits in these systems, atoms are typically excited to Rydberg states, which could decay or give rise to various correlated errors that cannot be addressed directly through traditional methods of fault-tolerant quantum computation. In this work, we provide the first complete characterization of these sources of error in a neutral-atom…
We propose a protocol for sympathetically cooling neutral atoms without destroying the quantum information stored in their internal states. This is achieved by designing state-insensitive Rydberg interactions between the data-carrying atoms and cold auxiliary atoms. The resulting interactions give rise to an effective phonon coupling, which leads to the transfer of heat from the data atoms to the auxiliary atoms, where the latter can be cooled by conventional methods. This can be used to extend the lifetime of quantum storage based on neutral atoms and can have applications for long quantum co…
The multipartite Greenberger-Horne-Zeilinger (GHZ) states are indispensable elements for various quantum information processing tasks. Here we put forward two deterministic proposals to dissipatively prepare tripartite GHZ states in a neutral atom system. The first scheme can be considered as an extension of a recent work [T. M. Wintermantel, Y. Wang, G. Lochead, \textit{et al}, {Phys. Rev. Lett. \textbf{124}, 070503 (2020)}]. By virtue of the polychromatic driving fields and the engineered spontaneous emission, a multipartite GHZ state with odd numbers of atoms are generated with a high effic…
Expanding the Neutral Atom Gate Set: Native iSWAP and Exchange Gates from Dipolar Rydberg Interactions
Institute for Theoretical Physics, University of Innsbruck（因斯布鲁克大学理论物理研究所）；Parity Quantum Computing GmbH（Parity量子计算有限公司）；Parity Quantum Computing Germany GmbH（Parity量子计算德国有限公司）；Parity Quantum Computing France SAS（Parity量子计算法国股份有限公司）
We analyze neutral atom Rydberg $C_Z$ gates based on adiabatic pulses applied symmetrically to both atoms. Analysis with smooth pulse shapes and Cs atom parameters predicts the gates can create Bell states with fidelity ${\mathcal F}>0.999$ using adiabatic rapid passage (ARP) pulses. With globally optimized adiabatic pulse shapes, in a two-photon excitation process, we generate Bell states with fidelity ${\mathcal F}=0.997$. The analysis fully accounts for spontaneous emission from intermediate and Rydberg states, including the Rydberg lifetime in a room temperature environment, but does not i…
