A Search for Variations of Fundamental Constants using Atomic Fountain Clocks
H. Marion, F. Pereira Dos Santos, M. Abgrall, S. Zhang, Y. Sortais, S. Bize, I. Maksimovic, D. Calonico, J. Gruenert, C. Mandache, P. Lemonde, G. Santarelli, Ph… 展开作者
H. Marion, F. Pereira Dos Santos, M. Abgrall, S. Zhang, Y. Sortais, S. Bize, I. Maksimovic, D. Calonico, J. Gruenert, C. Mandache, P. Lemonde, G. Santarelli, Ph. Laurent, A. Clairon, C. Salomon
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4 pages, 3 figures, 1 table submitted to Phys. Rev. Lett
Over five years we have compared the hyperfine frequencies of 133Cs and 87Rb atoms in their electronic ground state using several laser cooled 133Cs and 87Rb atomic fountains with an accuracy of ~10^{-15}. These measurements set a stringent upper bound to a possible fractional time variation of the ratio between the two frequencies : (d/dt)ln(nu_Rb/nu_Cs)=(0.2 +/- 7.0)*10^{-16} yr^{-1} (1 sigma uncertainty). The same limit applies to a possible variation of the quantity (mu_Rb/mu_Cs)*alpha^{-0.44}, which involves the ratio of nuclear magnetic moments and the fine structure constant.
A caesium fountain clock is operated utilizing a microwave oscillator that derives its frequency stability from a stable laser by means of a fiber-laser femtosecond frequency comb. This oscillator is based on the technology developed for optical clocks and replaces the quartz based microwave oscillator commonly used in fountain clocks. As a result, a significant decrease of the frequency instability of the fountain clock is obtained, reaching 0.74E-14 at 100 s averaging time. We could demonstrate that for a significant range of detected atom numbers the instability is limited by quantum projec…
We have observed that the collisional frequency shift in primary caesium fountain clocks varies with the clock state population composition and, in particular, is zero for a given fraction of the |F = 4, mF = 0> atoms, depending on the initial cloud parameters. We present a theoretical model explaining our observations. The possibility of the collisional shift cancellation implies an improvement in the performance of caesium fountain standards and a simplification in their operation. Our results also have implications for test operation of fountains at multiple pi/2 pulse areas.
A cesium atomic fountain clock is under development at Huazhong University of Science and Technology (HUST) in China. In this paper, we describe the construction of the entire fountain clock system and report the preliminary results. A frequency stability of $2.5\times 10^{-13} τ^{-1/2}$ has been achieved by inter-comparison with a hydrogen maser, and the factors limiting the frequency stability are also discussed.
We report the evaluation of the second order Zeeman shift in the continuous atomic fountain clock FoCS-2. Because of the continuous operation and of its geometrical constraints, the methods used in pulsed fountains are not applicable. We use here time-resolved Zeeman spectroscopy to probe the magnetic field profile in the clock. The pulses of ac magnetic excitation allow us to spatially resolve the Zeeman frequency and to evaluate the Zeeman shift with a relative uncertainty smaller than 10E-16.
We report the operation of a dual Rb/Cs atomic fountain clock. 133Cs and 87Rb atoms are cooled, launched, and detected simultaneously in LNE-SYRTE's FO2 double fountain. The dual clock operation occurs with no degradation of either the stability or the accuracy. We describe the key features for achieving such a simultaneous operation. We also report on the results of the first Rb/Cs frequency measurement campaign performed with FO2 in this dual atom clock configuration, including a new determination of the absolute 87Rb hyperfine frequency.
An ensemble of rubidium atomic fountain clocks has been put into operation at the U.S. Naval Observatory (USNO). These fountains are used as continuous clocks in the manner of commercial cesium beams and hydrogen masers for the purpose of improved timing applications. Four fountains have been in operation for more than two years and are included in the ensemble used to generate the USNO master clock. Individual fountain performance is characterized by a white-frequency noise level below $2\times 10^{-13}$ and fractional-frequency stability routinely reaching the low $10^{-16}$s. The highest pe…
We performed an absolute frequency measurement of the $^1S_{0}$-$^3P_{0}$ transition in $^{87}$Sr with a fractional uncertainty of $1.2 \times 10^{-15}$, which is less than one third that of our previous measurement. A caesium fountain atomic clock was used as a transfer oscillator to reduce the uncertainty of the link between a strontium optical lattice clock and the SI second. The absolute value of the transition frequency is 429 228 004 229 873.56(49) Hz.
We demonstrate agreement between measurements and ab initio calculations of the frequency shifts caused by distributed cavity phase variations in the microwave cavity of a primary atomic fountain clock. Experimental verification of the finite element models of the cavities gives the first quantitative evaluation of this leading uncertainty and allows it to be reduced to delta nu / nu = 8.4\times10^-17. Applying these experimental techniques to clocks with improved microwave cavities will yield negligible distributed cavity phase uncertainties, less than \pm1\times10^-17.
We describe an optical frequency stabilization scheme of a microwave oscillator that is used for the interrogation of primary caesium fountain clocks. Because of its superior phase noise properties, this scheme, which is based on an ultrastable laser and a femtosecond laser frequency comb, overcomes the frequency instability limitations of fountain clocks given by the previously utilized quartz-oscillator-based frequency synthesis. The presented scheme combines the transfer of the short-term frequency instability of an optical cavity and the long-term frequency instability of a hydrogen maser …
In this article, we report on the work done with the LNE-SYRTE atomic clock ensemble during the last 10 years. We cover progress made in atomic fountains and in their application to timekeeping. We also cover the development of optical lattice clocks based on strontium and on mercury. We report on tests of fundamental physical laws made with these highly accurate atomic clocks. We also report on work relevant to a future possible redefinition of the SI second.
We present experimental work for improved atom loading in the optical molasses of a caesium fountain clock, employing a low-velocity intense source of atoms (LVIS) [Lu et al., Phys. Rev. Lett. 77, 3331 (1996)], which we modified by adding a "dark" state pump laser. With this modification the atom source has a mean flux of $4 \times 10^{8}$ atoms/s at a mean atom velocity of $8.6$ m/s. Compared to fountain operation using background gas loading, we achieved a significant increase of the loaded and detected atom number by a factor of 40. Operating the fountain clock with a total number of detect…
The fundamental limits of atomic fountains as operational clocks are considered. Four rubidium fountains in operation at the U.S. Naval Observatory for over 5.5 years have demonstrated unprecedented long-term stability for continuously running clocks [1,2]. With only these rubidium fountains, a post-processed timescale can be created that demonstrates superior long-term performance to any individual clock by compensating for occasional frequency steps. By comparing to the world's primary standards we demonstrate instability of this rubidium fountain timescale reaching the mid $10^{-17}$'s and …
Improvements of the systematic uncertainty, frequency instability, and long-term reliability of the two caesium fountain primary frequency standards CSF1 and CSF2 at PTB (Physikalisch-Technische Bundesanstalt) are described. We have further investigated many of the systematic effects and made a number of modifications of the fountains. With an optically stabilized microwave oscillator, the quantum projection noise limited frequency instabilities are improved to $7.2 \times 10^{-14} (τ/1\,\mathrm{s})^{-1/2}$ for CSF1 and $2.5 \times 10^{-14} (τ/1\,\mathrm{s})^{-1/2}$ for CSF2 at high atom densi…
We describe a new method to determine the position of the atomic cloud during its interaction with the microwave field in the cavity of a fountain clock. The positional information is extracted from the spectrum of the F=3,mF=0 to F=4,mF=-1 hyperfine transition, which shows a position dependent asymmetry when the magnetic C-field is tilted by a few degrees with respect to the cavity axis. Analysis of this spectral asymmetry provides the horizontal center-of-mass position for the ensemble of atoms contributing to frequency measurements. With an uncertainty on the order of 0.1 mm, the obtained i…
We demonstrate the use of a fiber-based femtosecond laser locked onto an ultra-stable optical cavity to generate a low-noise microwave reference signal. Comparison with both a liquid Helium cryogenic sapphire oscillator (CSO) and a Ti:Sapphire-based optical frequency comb system exhibit a stability about $3\times10^{-15}$ between 1 s and 10 s. The microwave signal from the fiber system is used to perform Ramsey spectroscopy in a state-of-the-art Cesium fountain clock. The resulting clock system is compared to the CSO and exhibits a stability of $3.5\times10^{-14}τ^{-1/2}$. Our continuously ope…
We present a trajectory dynamically tracing compensation method to smooth the spatial fluctuation of the static magnetic field (C-field) that provides a quantization axis in the fountain clock. The C-field coil current is point-to-point adjusted in accordance to the atoms experienced magnetic field along the flight trajectory. A homogeneous field with a 0.2 nT uncertainty is realized compared to 5 nT under the static magnetic field with constant current during the Ramsey interrogation. The corresponding uncertainty associated with the second-order Zeeman shift that we calculate is improved by …
We stabilise a microwave oscillator at 9.6 GHz to an optical clock laser at 344 THz by using a fibre-based femtosecond laser frequency comb as a transfer oscillator. With a second frequency comb we measure independently the instability of the microwave source with respect to another optical clock laser frequency at 456 THz. The total fractional frequency instability of this optic-to-microwave and microwave-to-optic conversion resulted in an Allan deviation sigma_y, of sigma_y=1.2E-14 at 1 s averaging time (band width 50 kHz). The residual phase noise density is -97 dBc/Hz at 10 Hz offset from …
Four rubidium fountains at the U.S. Naval Observatory (USNO) have been in operation for 4.5 years. Each fountain has demonstrated periods of stability marked by Total or Theo deviation below 10^-16. Occasional frequency changes, on order of 1.5 times per year per fountain, introduce deviations from white-frequency noise behavior. Averaged together, the four fountains form an ensemble with a white-frequency noise level of 10^-13 and excellent long-term stability as compared to the primary frequency standards contributing to TAI. Progress on using the clocks at USNO for improving limits on coupl…
We report on the development and phase noise performance of a 9.1926 GHz microwave frequency synthesizer to be used as the local oscillator for a Cs fountain clock. It is based on frequency multiplication and synthesis from an ultralow phase noise 5 MHz Oven Controlled Crystal Oscillator (OCXO) and 100 MHz Voltage Controlled Crystal Oscillator (VCXO).The key component of the frequency multiplication is a non-linear transmission-line (NLTL) used as a frequency comb generator. The phase noise of the synthesizer is improved by carefully optimizing the input power, the input and output impedances …
We give an overview of the work done with the Laboratoire National de Métrologie et d'Essais-Systèmes de Référence Temps-Espace (LNE-SYRTE) fountain ensemble during the last five years. After a description of the clock ensemble, comprising three fountains, FO1, FO2, and FOM, and the newest developments, we review recent studies of several systematic frequency shifts. This includes the distributed cavity phase shift, which we evaluate for the FO1 and FOM fountains, applying the techniques of our recent work on FO2. We also report calculations of the microwave lensing frequency shift for the thr…
An improved measurement of the electron electric dipole moment (EDM) appears feasible using ground-state alkali atoms in an atomic fountain in which a strong electric field, which couples to a conceivable electron dipole moment (EDM), is applied perpendicular to the fountain axis. In a practical fountain, the ratio of the atomic tensor Stark shift to the Zeeman shift is a facto mu~100. We expand the complete time evolution operator in inverse powers of this ratio; complete results are presented for atoms of total spin F=3, 4, and 5. For a specific set of entangled hyperfine sublevels (coherent…
In precision metrology the determination of the Newtonian gravity constant $G$ represents a real problem, since its history is plagued by huge unknown discrepancies between a large number of independent experiments. In this paper we propose a novel experimental setup for measuring $G$ with a relative accuracy of $10^{-5}$ using a standard cold atomic fountain and matter wave interferometry. We discuss in details the major sources of systematic errors, providing also the expected statistical uncertainty. Feasibility of determining $G$ at a level of $10^{-6}$ level is also discussed.
Ramsey fringes observed in an atomic fountain are formed by the superposition of the individual atomic signals. Due to the atomic beam residual temperature, the atoms have slightly different trajectories and thus are exposed to a different average magnetic field, and a velocity dependent Ramsey interaction time. As a consequence, both the velocity distribution and magnetic field profile are imprinted in the Ramsey fringes observed on Zeeman sensitive microwave transitions. In this work, we perform a Fourier analysis of the measured Ramsey signals to retrieve both the time averaged magnetic fie…
We used a Cs atomic fountain frequency standard to measure the Stark shift on the ground state hyperfine transiton frequency in cesium (9.2 GHz) due to the electric field generated by the blackbody radiation. The measures relative shift at 300 K is -1.43(11)e-14 and agrees with our theoretical evaluation -1.49(07)e-14. This value differs from the currently accepted one -1.69(04)e-14. The difference has a significant implication on the accuracy of frequency standards, in clocks comparison, and in a variety of high precision physics tests such as the time stability of fundamental constants.
This paper describes advances in microwave frequency standards using laser-cooled atoms at BNM-SYRTE. First, recent improvements of the $^{133}$Cs and $^{87}$Rb atomic fountains are described. Thanks to the routine use of a cryogenic sapphire oscillator as an ultra-stable local frequency reference, a fountain frequency instability of $1.6\times 10^{-14}τ^{-1/2}$ where $τ$ is the measurement time in seconds is measured. The second advance is a powerful method to control the frequency shift due to cold collisions. These two advances lead to a frequency stability of $2\times 10^{-16}$ at $50,000s…
The short-term stability of passive atomic frequency standards, especially in pulsed operation, is often limited by local oscillator noise via intermodulation effects. We present an experimental demonstration of the intermodulation effect on the frequency stability of a continuous atomic fountain clock where, under normal operating conditions, it is usually too small to observe. To achieve this, we deliberately degrade the phase stability of the microwave field interrogating the clock transition. We measure the frequency stability of the locked, commercial-grade local oscillator, for two modul…
We report on the first absolute transition frequency measurement at the 10^{-15} level with a single, laser-cooled 40Ca+ ion in a linear Paul trap. For this measurement, a frequency comb is referenced to the transportable Cs atomic fountain clock of LNE-SYRTE and is used to measure the S1/2-D5/2 electric-quadrupole transition frequency. After the correction of systematic shifts, the clock transition frequency f_Ca+ = 411 042 129 776 393.2 (1.0) Hz is obtained, which corresponds to a fractional uncertainty within a factor of three of the Cs standard. Future improvements are expected to lead to …
We demonstrate launching of laser-cooled Yb atoms in a cold atomic fountain. Atoms in a collimated thermal beam are first cooled and captured in a magneto-optic trap (MOT) operating on the strongly-allowed ${^1S}_0 \rightarrow {^1P}_1$ transition at 399~nm (blue line). They are then transferred to a MOT on the weakly-allowed ${^1S}_0 \rightarrow {^3P}_1$ transition at 556~nm (green line). Cold atoms from the green MOT are launched against gravity at a velocity of around 2.5~m/s using a pair of green beams. We trap more than $10^7$ atoms in the blue MOT and transfer up to 70\% into the green MO…
We propose a method of joint interrogation in a single atom interferometer which overcomes the dead time between consecutive measurements in standard cold atomic fountains. The joint operation enables for a faster averaging of the Dick effect associated with the local oscillator noise in clocks and with vibration noise in cold atom inertial sensors. Such an operation allows achieving the lowest stability limit due to atom shot noise. We demonstrate a multiple joint operation in which up to five clouds of atoms are interrogated simultaneously in a single setup. The essential feature of multiple…
We report tests of local position invariance based on measurements of the ratio of the ground state hyperfine frequencies of 133Cs and 87Rb in laser-cooled atomic fountain clocks. Measurements extending over 14 years set a stringent limit to a possible variation with time of this ratio: d ln(nu_Rb/nu_Cs)/dt=(-1.39 +/- 0.91)x 10-16 yr-1. This improves by a factor of 7.7 over our previous report (H. Marion et al., Phys. Rev. Lett. 90, 150801 (2003)). Our measurements also set the first limit to a fractional variation of the Rb/Cs ratio with gravitational potential at the level of c^2 d ln(nu_Rb/…
One of the main limitations of cesium atomic fountains has been the cold collision frequency shift. By using a method based on a transfer of population by adiabatic passage allowing to prepare cold atomic samples with a well defined ratio of atomic density as well as atom number the collisional shift is controlled at the 10E-3 of its value. A calibration of Zeeman sub-states contribution to the clock shift as a function of the field has been performed. Feshbach resonances have been observed for the first time at very low magnetic field and with a very good resolution. A Monte Carlo simulation …
Progress in realizing the SI second had multiple technological impacts and enabled to further constraint theoretical models in fundamental physics. Caesium microwave fountains, realizing best the second according to its current definition with a relative uncertainty of 2-4x10^(-16), have already been superseded by atomic clocks referenced to an optical transition, both more stable and more accurate. Are we ready for a new definition of the second? Here we present an important step in this direction: our system of five clocks connects with an unprecedented consistency the optical and the microw…
The environmental perturbation on atoms is the key factor restricting the performance of atomic frequency standards, especially in long term scale. In this letter, we demonstrate a real-time noise distinguish operation of atomic clocks. The operation improves the statistical uncertainty by about an order of magnitude of our fountain clock which is deteriorated previously by extra noises. The frequency offset bring by the extra noise is also corrected. The experiment proves the real-time noise distinguish operation can reduce the contribution of ambient noises and improve the uncertainty limit …
A microwave atomic clock scheme based on Rb and Cs atoms trapped in optical lattice with magic wavelength for clock transition is proposed. The ac Stark shift of clock transition due to trapping laser can be canceled at some specific laser wavelengths. Comparing with in fountain clock, the cavity related shifts, the collision shift, and the Doppler effect are eliminated or suppressed dramatically in atomic clock when the magic optical lattice is exploited. By carefully analyzing various sources of clock uncertainty, we conclude that a microwave atomic clock with an accuracy of better than $2\t…
We report on a new experiment that tests for a violation of Lorentz invariance (LI), by searching for a dependence of atomic transition frequencies on the orientation of the spin of the involved states (Hughes-Drever type experiment). The atomic frequencies are measured using a laser cooled $^{133}$Cs atomic fountain clock, operating on a particular combination of Zeeman substates. We analyze the results within the framework of the Lorentz violating standard model extension (SME), where our experiment is sensitive to a largely unexplored region of the SME parameter space, corresponding to firs…
We use an atomic fountain clock to measure quantum scattering phase shifts precisely through a series of narrow, low-field Feshbach resonances at average collision energies below $1\,μ$K. Our low spread in collision energy yields phase variations of order $\pm π/2$ for target atoms in several $F,m_F$ states. We compare them to a theoretical model and establish the accuracy of the measurements and the theoretical uncertainties from the fitted potential. We find overall excellent agreement, with small statistically significant differences that remain unexplained.
A review is given of the implications of the absence of an intrinsic notion of instantaneous 3-space, so that a clock synchronization convention has to be introduced, for relativistic theories.
In atomic systems, clock states feature a zero projection of the total angular momentum and thus a low sensitivity to magnetic fields. This makes them widely used for metrological applications like atomic fountains or gravimeters. Here, we show that a mixture of two such non-magnetic states still display magnetic dipole-dipole interactions. Using high resolution spectroscopy of a planar gas of $^{87}$Rb atoms with a controlled in-plane shape, we explore the effective isotropic and extensive character of these interactions and demonstrate their tunability. Our measurements set strong constraint…
In this paper we report the evaluation of an optical lattice clock based on neutral mercury down to a relative uncertainty of $1.7\times 10^{-16}$. Comparing this characterized frequency standard to a Cs atomic fountain we determine the absolute frequency of the $^1S_0 \rightarrow \phantom{}^3P_0$ transition of $^{199}$Hg as $ν_{\mathrm{Hg}} = 1 128\,575\,290\,808\,154.62\,$Hz $\pm\,0.19\,$Hz (statistical) $\pm\,0.38\,$Hz (systematic), limited solely by the realization of the SI second. Furthermore, by comparing the mercury optical lattice clock to a Rb atomic fountain, we determine for the fi…
To date, no framework combining quantum field theory and general relativity and hence unifying all four fundamental interactions, exists. Violations of the Einstein's equivalence principle (EEP), being the foundation of general relativity, may hold the key to a theory of quantum gravity. The universality of free fall (UFF), which is one of the three pillars of the EEP, has been extensively tested with classical bodies. Quantum tests of the UFF, e.g. by exploiting matter wave interferometry, allow for complementary sets of test masses, orders of magnitude larger test mass coherence lengths and …
The cosmological applications of atomic clocks so far have been limited to searches of the uniform-in-time drift of fundamental constants. In this paper, we point out that a transient in time change of fundamental constants can be induced by dark matter objects that have large spatial extent, and are built from light non-Standard Model fields. The stability of this type of dark matter can be dictated by the topological reasons. We point out that correlated networks of atomic clocks, some of them already in existence, can be used as a powerful tool to search for the topological defect dark matt…
We calculate the dependence of the nuclear magnetic moments on the quark masses including the spin-spin interaction effects and obtain limits on the variation of the fine structure constant $α$ and $(m_q/Λ_{QCD})$ using recent atomic clock experiments examining hyperfine transitions in H, Rb, Cs, Yb$^+$ and Hg$^+$ and the optical transition in H, Hg$^+$ and Yb$^+$ .
We have measured the absolute frequency of the optical lattice clock based on $^{87}$Sr at PTB with an uncertainty of $3.9\times 10^{-16}$ using two caesium fountain clocks. This is close to the accuracy of today's best realizations of the SI second. The absolute frequency of the 5s$^2$ $^1$S$_0$-5s5p $^3$P$_0$ transition in $^{87}$Sr is 429,228,004,229,873.13(17) Hz. Our result is in excellent agreement with recent measurements performed in different laboratories worldwide. We improved the total systematic uncertainty of our Sr frequency standard by a factor of five and reach $3\times 10^{-17…
We present the latest developments in the field of atomic clocks and their applications in metrology and fundamental physics. In the light of recent advents in the accuracy of optical clocks, we present an introduction to the relativistic modelization of frequency transfer and a detailed review of chronometric geodesy.
We perform calculations of the dependence of nuclear magnetic moments on quark masses and obtain limits on the variation of m_q/Lambda_{QCD} from recent atomic clock experiments with hyperfine transitions in H, Rb, Cs, Hg+ and optical transtion in Hg+.
We consider a free massive particle inside a box which is dragged by Rindler observers. Admitting that the particle obeys the Klein-Gordon equation, we find the frequencies of the stationary states of this system. Transitions between the stationary states are employed to set a standard frequency for a toy atomic clock. Comparing the energy spectrum of the accelerated system with the energy spectrum of an identical system in an inertial frame, we determine the influence of the instantaneous acceleration on the rate of atomic clocks. We argue that our result does not violate the clock hypothesis…
We analyze possible effects of the dark matter environment on the atomic clock stability measurements. The dark matter is assumed to exist in a form of waves of ultralight scalar fields or in a form of topological defects (monopoles and strings). We identify dark matter signal signatures in clock Allan deviation plots that can be used to constrain the dark matter coupling to the Standard Model fields. The existing data on the Al+/Hg+ clock comparison are used to put new limits on the dilaton dark matter in the region of masses m > 10^{-15} eV. We also estimate the sensitivities of future atomi…
We search for ultralight scalar dark matter candidates that induce oscillations of the fine structure constant, the electron and quark masses, and the quantum chromodynamics energy scale with frequency comparison data between an $^{171}$Yb optical lattice clock and a $^{133}$Cs fountain microwave clock that span 298 days with an uptime of 15.4 $\%$. New limits on the couplings of the scalar dark matter to electrons and gluons in the mass range from $10^{-22}$ eV/$c^{2}$ to $10^{-20}$ eV/$c^{2}$ are set, assuming that each of these couplings is the dominant source of the modulation in the frequ…
Dark Matter could potentially manifest itself in the form of asymmetric dark stars. In this paper we entertain the possibility of probing such asymmetric bosonic dark matter stars by the use of atomic clocks. If the dark sector connects to the standard model sector via a Higgs or photon portal, the interior of boson stars that are in a Bose-Einstein condensate state can change the values of physical constants that control the timing of atomic clock devices. Dilute asymmetric dark matter boson stars passing through the Earth can induce frequency shifts that can be observed in separated Earth ba…
