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arXiv 2604.04789quant-phcond-mat.other
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四阶对称脉冲序列用于超越理想脉冲近似之外的鲁棒量子控制

Quadrature-Symmetric PulsePol for Robust Quantum Control Beyond the Ideal Pulse Approximation

Center for Quantum and Topological Systems, New York University Abu Dhabi(纽约大学阿布扎比分校量子与拓扑系统中心);Interdisciplinary Nanoscience Center (iNANO) and Department of Chemistry, Aarhus University(奥胡斯大学跨学科纳米科学中心(iNANO)和化学系);Indian Institute of Science Education and Research, Bhopal(印度科学教育研究所博帕尔分校);Tata Institute of Fundamental Research Hyderabad(泰姬玛哈底拉基础研究所海得拉巴分所);Department of Chemistry, New York University Abu Dhabi(纽约大学阿布扎比分校化学系)

Mayur Jhamnani, Venkata SubbaRao Redrouthu, Jose P. Carvalho, Ethan Feldman, Anders B. Nielsen, Phani Kumar, Niels Chr. Nielsen, P. K. Madhu, Asif Equbal

AI总结:

本文提出Q-PulsePol方案,通过恢复四阶对称性提升核自旋在固体中的固态超极化效率,克服有限脉冲效应,实现鲁棒的量子控制。

摘要:

四阶对称脉冲序列用于超越理想脉冲近似之外的鲁棒量子控制。本文提出Q-PulsePol方案,通过恢复四阶对称性提升核自旋在固体中的固态超极化效率,克服有限脉冲效应,实现鲁棒的量子控制。PulsePol是一种巧妙设计的基于脉冲序列的量子控制方案,能够实现电子与核自旋之间的极化转移,例如在氮化物空位(NV)中心中。然而,之前的PulsePol分析假设了非常强的、近理想的瞬时微波脉冲,这在更高磁场下很少能实现。我们重新审视了在有限脉冲约束下的PulsePol方案,发现其性能因有限脉冲效应而显著下降。通过双模傅里叶理论,我们识别出导致保真度下降的对称性破坏机制。通过相位调整,我们重新建立了相互作用框架下的自旋哈密顿量的正确对称性,从而得到一种称为Q-PulsePol的序列,其中“Q”反映了恢复的四阶对称性。我们的结果展示了对有限脉冲效应的鲁棒性以及极化转移效率的提高,确立了Q-PulsePol作为通过单模(零量子或双量子)转移实现固体中核自旋固态超极化的实用且可靠的方案。这项工作将理想化的量子控制与现实的脉冲工程联系起来,建立了用于基于自旋的量子控制协议的设计规则。

英文摘要:

PulsePol is an elegantly designed pulse-sequence-based quantum control scheme that enables polarization transfer between electron and nuclear spins, for example, in nitrogen-vacancy (NV) centers. However, previous analyses of PulsePol assumed very strong, near-ideal, instantaneous microwave pulses, which is rarely achievable at higher magnetic fields. We revisit the PulsePol scheme under finite-pulse constraints and show that its performance significantly degrades due to finite-pulse effects. Using bimodal Floquet theory, we identify the symmetry-breaking mechanism responsible for this deterioration in fidelity. By phase adjustment, we reestablish the proper symmetry of the interaction-frame spin Hamiltonian, leading to a sequence called Q-PulsePol, where "Q" reflects the restored quadrature symmetry. Our results demonstrate robustness to finite-pulse effects and improved polarization transfer efficiency, establishing Q-PulsePol as a practical and reliable scheme for bulk hyperpolarization of nuclear spins in solids using a single-mode (zero-quantum or double-quantum) transfer. This work bridges idealized quantum control with realistic pulse engineering, establishing design rules for spin-based quantum control protocols.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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