Quantum correlations and fluctuations in the pulsed light produced by a synchronously pumped optical parametric oscillator below its oscillation threshold
V. A. Averchenko, Yu. M. Golubev, C. Fabre, N. Treps
We present a simple quantum theory for the pulsed light generated by a synchronously pumped optical parametric oscillator (SPOPO) in the degenerate case where the signal and idler trains of pulses coincide, below threshold and neglecting all dispersion effects. Our main goal is to precise in the obtained quantum effects, which ones are identical to the c.w. case and which ones are specific to the SPOPO. We demonstrate in particular that the temporal correlations have interesting peculiarities: the quantum fluctuations at different times within the same pulse turn out to be totally not correlated, whereas they are correlated between nearby pulses at times that are placed in the same position relative to the centre of the pulses. The number of significantly correlated pulses is of the order of cavity finesse. We show also that there is perfect squeezing at noise frequencies multiple of the pulse repetition frequency when one approaches the threshold from below on the signal field quadrature measured by a balanced homodyne detection with a local oscillator of very short duration compared to the SPOPO pulse length.
Quantum models for synchronously pumped type I optical parametric oscillators (SPOPO) are presented. The study of the dynamics of SPOPOs, which typically involves millions of coupled signal longitudinal modes, is significantly simplified when one considers the ?supermodes?, which are independent linear superpositions of all the signal modes diagonalizing the parametric interaction. In terms of these supermodes the SPOPO dynamics becomes that of about a hundred of independent, single mode degenerate OPOs, each of them being a squeezer. One derives a general expression for the squeezing spectrum…
We perform the quantum analysis of the light emitted by a synchronously pumped optical parametric oscillator operating in the above threshold regime, i.e. when the peak power of pulsed pumping exceeds the threshold of continuous generation. We show that both regimes (below and above threshold) are realized at different times within each pulse of the signal field. We show that the quantum fluctuations of signal and pump pulses are correlated between nearby pulses at times that are placed in the same position relative to the center of the pulses, whereas fluctuations are totally not correlated a…
We present in this paper a general model for determining the quantum properties of the light generated by a synchronously pumped optical parametric oscillator (SPOPO) operating below threshold. This model considers time and frequency on an equal footing, which allows us to find new quantum properties, related for example to the carrier envelope offset (CEO) phase, and to consider situations that are close to real experiments. We show that, in addition to multimode squeezing in the so-called 'supermodes', the system exhibits quadrature entanglement between frequency combs of opposite CEO phases…
We report the generation of polarization-entangled photons by femtosecond-pulse-pumped spontaneous parametric down-conversion in a cascade of two type-I crystals. Highly entangled pulsed states were obtained by introducing a temporal delay between the two orthogonal polarization components of the pump field. They exhibited high-visibility quantum interference and a large concurrence value, without the need of post-selection using narrow-bandwidth-spectral filters. The results are well explained by the theory which incorporates the space-time dependence of interfering two-photon amplitudes if d…
Photon pairs, highly entangled in polarization have been generated under femtosecond laser pulse excitation by a type I crystal source, operating in a single arm interferometric scheme. The relevant effects of temporal walk-off existing in these conditions between the ordinary and extraordinary photons were experimentally investigated. By introducing a suitable temporal compensation between the two orthogonal polarization components highly entangled pulsed states were obtained.
We study the spectral properties of Spontaneous Parametric Down Conversion in a periodically poled waveguided structure of KTP crystal pumped by ultra-short pulses. Our theoretical analysis reveals a strongly multimode and asymmetric structure of the two-photon spectral amplitude for type-II SPDC. Experimental evidence, based on Hong-Ou-Mandel polarization interference with narrowband filtering, confirms this result.
We present theoretical and experimental study of preparing maximally entangled two-photon polarization states, or Bell states, using femtosecond pulse pumped spontaneous parametric down-conversion (SPDC). First, we show how the inherent distinguishability in femtosecond pulse pumped type-II SPDC can be removed by using an interferometric technique without spectral and amplitude post-selection. We then analyze the recently introduced Bell state preparation scheme using type-I SPDC. Theoretically, both methods offer the same results, however, type-I SPDC provides experimentally superior methods …
A pulsed source of energy-time entangled photon pairs pumped by a standard laser diode is proposed and demonstrated. The basic states can be distinguished by their time of arrival. This greatly simplifies the realization of 2-photon quantum cryptography, Bell state analyzers, quantum teleportation, dense coding, entanglement swapping, GHZ-states sources, etc. Moreover the entanglement is well protected during photon propagation in telecom optical fibers, opening the door to few-photon applications of quantum communication over long distances.
We report a novel Bell state preparation experiment. High-purity Bell states are prepared by using femtosecond pulse pumped \emph{nondegenerate} collinear spontaneous parametric down-conversion. The use of femtosecond pump pulse {\em does not} result in reduction of quantum interference visibility in our scheme in which post-selection of amplitudes and other traditional mechanisms, such as, using thin nonlinear crystals or narrow-band spectral filters are not used. Another distinct feature of this scheme is that the pump, the signal, and the idler wavelengths are all distinguishable, which is …
We discuss the concept of characteristic squeezing modes applied to a travelling-wave optical parametric amplifier pumped by an ultrashort pulse. The characteristic modes undergo decoupled single-mode squeezing transformations, and therefore they form a useful basis to describe the evolution of the entire multimode system. This provides an elegant and intuitive picture of quantum statistical properties of parametric fluorescence. We analyse the efficiency of detecting quadrature squeezing, and present results of numerical calculations for a realistic nonlinear medium.
We have developed the full theory of a synchronously pumped type I optical parametric oscillator (SPOPO). We derive expressions for the oscillation threshold and the characteristics of the generated mode-locked signal beam. We calculate the output quantum fluctuations of the device, and find that, in the degenerate case (coincident signal and idler set of frequencies), perfect squeezing is obtained when one approaches threshold from below for a well defined "super-mode', or frequency comb, consisting of a coherent linear superposition of signal modes of different frequencies which are resonant…
Using the Bogoliubov transformation in multi-frequency modes to describe the evolution of the non-degenerate signal and idler twin beams, we theoretically investigate the quantum noise properties of the pulse pumped high gain fiber optical parametric amplifiers (FOPA). The results show that the noise figure of the FOPA is generally greater than the 3 dB quantum limit unless the joint spectral function is factorable and the spectrum of the input signal well matches the gain spectrum in the signal band. However, the intensity difference noise of the twin beams, which weakly depends on the joint …
The quantum state of the photon pair generated from type-II spontaneous parametric down-conversion pumped by a ultrafast laser pulse exhibits strong decoherence in its polarization entanglement, an effect which can be attributed to the clock effect of the pump pulse or, equivalently, to distinguishing spectral information in the two-photon state. Here, we propose novel temporal and spectral engineering techniques to eliminate these detrimental decoherence effects. The temporal engineering of the two-photon wavefunction results in a universal Bell-state synthesizer that is independent of the ch…
In this article, we employ multimode radiation of a synchronously pumped optical parametric oscillator (SPOPO) to build a cluster state through a conversion on the base of quantum memory cell. We demonstrate that by choosing an appropriate driving field we can ensure the effective writing of the only one supermode from the entire set of the SPOPO squeezed supermodes. Further, by changing the driving field profile at the readout, we convert the time profile of the retrieved signal while maintaining its quantum state. We demonstrate the possibilities of using the presented scheme by the example …
We demonstrate pulsed operation of a bidirectionally pumped polarization Sagnac interferometric down-conversion source and its generation of narrowband, high-visibility polarization-entangled photons. Driven by a narrowband, mode-locked pump at 390.35 nm, the phase-stable Sagnac source with a type-II phase-matched periodically poled KTiOPO$_4$ crystal is capable of producing 0.01 entangled pair per pulse in a 0.15-nm bandwidth centered at 780.7 nm with 1 mW of average pump power at a repetition rate of 31.1 MHz. We have achieved a mean photon-pair generation rate of as high as 0.7 pair per pul…
We present a detailed analysis of the multimode quantum state embedded in an optical frequency comb generated by a Synchronously Pumped Optical Parametric Oscillator (SPOPO). The full covariance matrix of the state is obtained with homodyne detection where the local oscillator is spectrally controlled with pulse shaping techniques. The resulting matrix reveals genuine multipartite entanglement. Additionally, the beam is comprised of several independent eigenmodes that correspond to specific pulse shapes. The experimental data is confirmed with numerical simulations. Finally, the potential to c…
The ability to generate mode-engineered single photons to interface with disparate quantum systems is of importance for building a quantum network. Here we report on the generation of a pulsed, heralded single photon source with a sub-GHz spectral bandwidth that couples to indium arsenide quantum dots centered at 942 nm. The source is built with a type-II PPKTP down-conversion crystal embedded in a semi-confocal optical cavity and pumped with a 76 MHz repetition rate pulsed laser to emit collinear, polarization-correlated photon pairs resonant with a single quantum dot. In order to demonstrate…
Polarization-sensitive quantum optical coherence tomography (PS-QOCT) makes use of a Type-II twin-photon light source for carrying out optical sectioning with polarization sensitivity. A BBO nonlinear optical crystal pumped by a Ti:sapphire psec-pulsed laser is used to confirm the theoretical underpinnings of this imaging paradigm. PS-QOCT offers even-order dispersion cancellation with simultaneous access to the group-velocity dispersion characteristics of the interstitial medium between the reflecting surfaces of the sample.
The sensitivity of the displacement transducer pumped with a train of high-intensity laser pulses is estimated. Due to the multicomponent character of the pump a consideration of transformations of the signal and the noises between optical modes plays an important role in estimation of the potential sensitivity. An expression for the minimal detectable external classical force resembles those for the continuous wave pumping with substitution of the laser power by a time averaged power of pulsed laser. Possible scheme for back action noise compensation for such transducers is considered. For fu…
We have theoretically investigated the possibility of using any of several continuous-variable Bell-type inequalities - for which the dichotomic measurements are achieved with coarse-grained quadrature (homodyne) measurements - in a multi-party configuration where each participant is given a section, in the frequency domain, of the output of an optical parametric oscillator which has been synchronously-pumped with a frequency comb. Such light sources are undergoing intense study due to their novel properties, including the potential for production of light entangled in many hundreds of physica…
Pulsed pumped four-wave mixing process via $χ^{(3)}$ non-linearity in optical fiber can generate optical pulses with continuous variable quantum correlation. However, pair-wise correlation of the generated pulses in this system has not been studied. Here we report a time-domain measurement of an intensity difference squeezed state generated in fiber. With a fast response differential detection system, we show the generated twin-beam pulses are pair-wisely correlated, and -3.8 dB (-8.1 dB after detection losses correction) intensity difference squeezing degree is measured in time-domain. Our re…
Broadly speaking, this thesis is about nonlinear optics, quantum mechanics, and computing. More specifically, it covers four main topics: Coherent LQG Control, Free-Carrier Oscillations, Optical Ising Machines and Pulsed OPO Dynamics. Tying them all together is a theory of open quantum systems called the SLH model, which I introduce in Chapters 1-2. The SLH model is a general framework for open quantum systems that interact through bosonic fields, and is the basis for the quantum circuit theory developed in the text. Coherent LQG control is discussed in Chapters 3-4, where I demonstrate that c…
Pulse-resolved post-generation phase control of squeezed light at 93 MHz with a bulk lithium-niobate modulator
Università degli Studi di Milano（米兰大学）；Istituto Nazionale di Fisica Nucleare, Sezione di Milano（意大利国家核物理研究所米兰分部）；Istituto di Fotonica e Nanotecnologie - CNR（光子与纳米技术研究所-意大利国家研究委员会）
In this paper, we examined a possibility of preservation of a substantially multimode radiation in a single cell of quantum memory. As a light source we considered a synchronously pumped optical parametric oscillator (SPOPO). As it was shown in [1-4], SPOPO radiation has a large number of the correlated modes making it attractive for the purposes of the quantum communication and computing. We showed that these correlations can be mapped on the longitudinal spin waves of the memory cell and be restored later in the readout light. The efficiencies of the writing and readout depend on the mode st…
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables, for example in cluster state computation. They can be generated either by mixing different squeezed light sources using linear optical operations, or directly in a multimode optical device. In parallel, frequency combs are perfect tools for high precision metrological applications and for quantum time transfer. Synchronously Pumped Optical Parametric Oscillators (SPOPOs) have been theoretically shown to produce multimode non-classical frequency combs. In this paper, we present the…
Dephasing processes significantly impact the performance of deterministic single-photon sources. Dephasing broadens the spectral line and suppresses the indistinguishability of the emitted photons, which is undesirable for many applications, primarily for quantum computing. We consider a light emitted by a two-level system with a pulsed incoherent pump in the presence of the spectral filter. The spectral filter allows control of the second-order autocorrelation function, indistinguishability, and quantum yield. We show that narrow spectral filters can increase the indistinguishability of the e…
The response of a SERF atomic magnetometer to a repetitive short-pulsed pump was investigated. Quantum sub-resonances at a repetition rate of $1/n$ of the Larmor frequency of the magnetic field inside the shield are experimentally observed and theoretically explained. This is a type of synchronization phenomenon. Investigations in single alkali atoms cells as well as mixed alkali atoms of K and Rb are presented. In the later, one species is pumped while the probe is on the other specie polarized by spin exchange. The effect of spin destruction, spin exchange and collisions are studied in order…
Synchronously pumped optical parametric oscillators (SPOPOs) are optical cavities containing a nonlinear crystal capable of down-converting a frequency comb to lower frequencies. These have received a lot of attention lately, because their intrinsic multimode nature makes them compact sources of quantum correlated light with promising applications in modern quantum information technologies. In this work we show that SPOPOs are also capable of accessing the challenging but interesting regime where spontaneous symmetry breaking plays a crucial role in the quantum properties of the emitted light,…
We describe a fiber Raman amplifier for nanosecond and sub-nanosecond pulses centered around 1260 nm. The amplification takes place inside a 4.5-m-long polarization-maintaining phosphorus-doped fiber, pumped at 1080 nm by 3-ns-long pulses with a repetition rate of 200 kHz and up to 1.75 kW peak power. The input seed pulses are of sub-mW peak-power and minimal duration of 0.25 ns, carved off a continuous-wave laser with sub-MHz linewidth. We obtain linearly-polarized output pulses with peak-powers of up to 1.4 kW, corresponding to peak-power conversion efficiency of over 80%. An ultrahigh small…
Optical quantum technologies such as quantum sensing, quantum cryptography and quantum computation all utilize properties of non-classical light, such as precise photon-number and entangled photon-pair states, to surpass technologies based on the classical light. A common route for obtaining heralded single photons is spontaneous four-wave mixing in optical fibers, allowing for a well-defined spatial mode, for high efficiency integration into optical fiber networks. These fibers are typically pumped using large, commercial, pulsed lasers requiring high-power (~10 W) pump lasers and are limited…
True random number generators (RNGs) are desirable for applications ranging from cryptogra- phy to computer simulations. Quantum phenomena prove to be attractive for physical RNGs due to their fundamental randomness and immunity to attack [1]- [5]. Optical parametric down conversion is an essential element in most quantum optical experiments including optical squeezing [9], and generation of entangled photons [10]. In an optical parametric oscillator (OPO), photons generated through spontaneous down conversion of the pump initiate the oscillation in the absence of other inputs [11, 12]. This q…
