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arXiv 2603.28186cond-mat.str-elcond-mat.mes-hallcond-mat.mtrl-sci
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一维电子系统中的Tomonaga-Luttinger液体与电荷密度波

Tomonaga-Luttinger liquid and charge-density wave in a quasi-one-dimensional material

Zhejiang University(浙江大学);Center for Correlated Matter and School of Physics, Zhejiang University(浙江大学关联物质中心及物理学院);School of Physics and Optoelectronic Engineering, Shandong University of Technology(山东理工大学物理与光电工程学院);Department of Applied Physics, Zhejiang University of Technology(浙江工业大学应用物理系);Department of Physics, Hong Kong University of Science and Technology(香港科技大学物理系);Department of Chemistry, Zhejiang University(浙江大学化学系);School of Physics, Hangzhou Normal University(杭州师范大学物理学院);Key Laboratory of Artificial Structures and Quantum Control, and Shanghai Center for Complex Physics, School of Physics and Astronomy, Shanghai Jiao Tong University(上海交通大学物理与天文学院人工结构与量子控制重点实验室及上海复杂系统物理研究中心);School of Information and Electrical Engineering, Hangzhou City University(杭州城市学院信息与电气工程学院);School of Physics and Optoelectronics, Xiangtan University(湘潭大学物理与光电工程学院);Institute of Fundamental and Transdisciplinary Research, and State Key Laboratory of Silicon and Advanced Semiconductor Materials, Zhejiang University(浙江大学基础与交叉研究院及硅材料与先进半导体材料国家重点实验室);Institue of Advanced Study in Physics, Zhejiang University(浙江大学物理学高等研究院)
Jing Li, Guo-Wei Yang, Bai-Zhuo Li, Yi Liu, Si-Qi Wu, Ji-Yong Liu, Jin-Ke Bao, Xiaoxian Yan, Hua-Xun Li, Jia-Xin Li, Jia-Lu Wang, Yun-Lei Sun, Yi-Ming Lu, Jia-Y… 展开作者

Jing Li, Guo-Wei Yang, Bai-Zhuo Li, Yi Liu, Si-Qi Wu, Ji-Yong Liu, Jin-Ke Bao, Xiaoxian Yan, Hua-Xun Li, Jia-Xin Li, Jia-Lu Wang, Yun-Lei Sun, Yi-Ming Lu, Jia-Yi Lu, Yi-Qiang Lin, Hui Xing, Chao Cao, Hao Jiang, Yang Liu, Guang-Han Cao, Hai-Qing Lin

AI总结:

研究发现了一种新的准一维材料Cs$_{1-δ}$Cr$_3$S$_3$,其同时表现出抗对立的CDW和TLL态,通过实验验证了CDW和TLL行为的存在,为一维系统中的新兴量子现象研究提供了新途径。

摘要:

在一维电子系统中,费米液体态因电子相互作用而崩溃,形成Tomonaga-Luttinger液体(TLL)态,或因Peierls不稳定性形成绝缘体电荷密度波(CDW)相。通常这两种现象互斥,但在真实材料中其共存仍不清楚。本文报告了一种新的准一维材料Cs$_{1-δ}$Cr$_3$S$_3$,意外表现出抗对立的CDW和TLL态。CDW态通过单元格内双键化和约250 meV的光学带隙得到证实。同时,TLL行为通过电导率测量和角分辨光电子能谱学证实,显示温度、偏压电压和电子能量的幂律缩放。能带结构计算揭示了围绕费米能级的孤立、线性色散的一维带。对于双键化的CDW相,1D费米面片位于布里渊区边界,因单元格内键对称性破坏而被打开。实验上,细微的Cs空位将费米能级移入线性色散的价带,使TLL行为的观察不破坏CDW有序。本工作确立了Cs$_{1-δ}$Cr$_3$S$_3$为一种稀有的材料平台,在其中对抗性的费米液体不稳定性共存并交织,为一维系统中的新兴量子现象研究开辟了新途径。

英文摘要:

In one-dimensional (1D) electron systems, the Fermi liquid state breaks down due either to electron interactions, which results in a Tomonaga-Luttinger liquid (TLL) state, or to Peierls instability, which leads to an insulating charge-density-wave (CDW) phase. In general, these two phenomena are mutually exclusive, and their coexistence remains elusive in real materials. Here, we report the discovery of a new quasi-1D material, Cs$_{1-δ}$Cr$_3$S$_3$, which unexpectedly exhibits coexistence of the antithetical CDW and TLL states. The CDW state is evidenced by the intra-unit-cell dimerization, and the opening of an optical band gap of $\sim$250 meV. Meanwhile, TLL behaviour is unambiguously demonstrated by the measurements of electrical transport and angle-resolved photoemission spectroscopy, which reveal a power-law scaling with temperature, bias voltage and electron energy. Band structure calculations reveal isolated, linearly dispersive, 1D bands around the Fermi level. For the dimerized CDW phase, the 1D Fermi-surface sheets located at the boundary of the Brillouin zone are gapped from intra-unit-cell bond symmetry breaking. Experimentally, subtle Cs vacancies shift the Fermi level into the linearly dispersive valence band, enabling the observation of TLL behaviour without interrupting the CDW order. This work establishes Cs$_{1-δ}$Cr$_3$S$_3$ as a rare material platform in which the antagonistic Fermi-liquid instabilities coexist and intertwine, opening new avenues for studying emergent quantum phenomena in 1D systems.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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