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arXiv 2602.21729physics.optics
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迈向磁电偶极发射的极化路由:通过介电超材料

Towards Polarization Routing of Magnetic and Electric Dipolar Emission with Dielectric Metasurfaces

Friedrich Schiller University Jena(耶拿弗里德里希·席勒大学);Australian National University(澳大利亚国立大学)

Marijn Rikers, Ayesheh Bashiri, Katsuya Tanaka, Ángela Barreda, Duk-Yong Choi, Thomas Pertsch, Isabelle Staude

AI总结:

通过介电超材料实现电和磁偶极发射的极化路由,利用极化工程化光子局域密度态增强特定极化通道的发射

摘要:

我们研究了与铕(III)的磁偶极和电偶极跃迁相关的发射极化特性,该研究结合了各向异性介电超材料,并利用极化工程化的电和磁光子局部密度态。超材料由位于SiO₂基底上、嵌入PMMA薄膜中的Mie共振椭圆形a-Si:H双极组成,其中包含Eu(TTA)₃。基于互易原理,设计目的是在610nm处实现双极间隙的最大电场增强(610nm处的磁场增强用于590nm),以在x-极化(y-极化)的垂直入射光下,选择性增强电偶极(磁偶极)发射至x-极化(y-极化)发射通道。制备的发光超材料的动量解析光谱和后焦点平面成像清晰地揭示了预期的极化依赖发射行为,其中x-极化(y-极化)发射显示出磁偶极/电偶极发射强度比的降低(增强),其中磁偶极发射通过纳米结构的磁场增强而增强。所展示的极化依赖交互表明,设计的纳米结构与三价稀土离子的电和磁偶极跃迁之间的相互作用,为将不同多极阶次的发射路由到不同极化通道开辟了新途径。

英文摘要:

We investigate the polarization properties of emission associated with the magnetic dipole and electric dipole transitions of europium(III) coupled to an anisotropic dielectric metasurface with polarization-engineered electric and magnetic photonic local density of states. The metasurface consists of a square array of Mie-resonant elliptical a-Si:H dimers situated on an SiO$_2$ substrate and embedded in a PMMA film containing Eu(TTA)$_3$. Based on reciprocity principle, it was designed to achieve maximum electric (magnetic) field enhancement in the dimer gap at 610 nm (590 nm) for $x$-polarized ($y$-polarized) normally incident light in order to selectively enhance the electric dipole (magnetic dipole) emission into the $x$-polarized ($y$-polarized) emission channel, respectively. Momentum-resolved spectroscopy and back-focal plane imaging of emission of the fabricated light-emitting metasurface clearly reveal the intended polarization-dependent emission behaviour, with the $x$-polarized ($y$-polarized) emission showing a reduced (enhanced) ratio of the magnetic-/electric dipole emission intensity, correspondingly where the magnetic dipole emission is enhanced with a magnetic field enhancement from the nanostructures. The demonstrated polarization-dependent interaction of a designed nanostructure with the electric- and magnetic dipolar transitions of trivalent lanthanide ions opens an avenue towards routing of emission of different multipolar orders into different polarization channels.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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