Bidirectional nanoantennas are of key relevance for advanced functionalities to be implemented at the nanoscale, and in particular for color routing in an ultracompact flat-optics configuration. Here we demonstrate a novel approach avoiding complex collective geometries and/or restrictive morphological parameters, based on cross-polarized detuned plasmonic nanoantennas in a uniaxial (quasi-1D) bimetallic configuration. The nanofabrication of such a flat-optics system is controlled over a large-area (cm^2) by a novel self-organized technique exploiting ion-induced nanoscale wrinkling instability on glass templates to engineer tilted bimetallic nanostrip dimers. These nanoantennas feature broadband color routing with superior light scattering directivity figures, which are well described by numerical simulations and turn out to be competitive with the response of lithographic nanoantennas. These results demonstrate that our large-area self-organized metasurfaces can be implemented in real world applications of flat optics color routing from telecom photonics to optical nanosensing.
Optical metasurfaces have emerged as a new generation of building blocks for multi-functional optics. Design and realization of metasurface elements place ever-increasing demands on accurate assessment of phase alterations introduced by complex nanoantenna arrays, a process referred to as quantitative phase imaging. Despite considerable effort, the widefield (non-scanning) phase imaging that would approach resolution limits of optical microscopy and indicate the response of a single nanoantenna still remains a challenge. Here, we report on a new strategy in incoherent holographic imaging of me…
We report on a chiral nanostructure, which we term a "butterfly nanoantenna," that, when used in a metasurface, allows the direct conversion of a linearly polarized beam into a nonlinear optical far-field of arbitrary complexity. The butterfly nanoantenna exhibits field enhancement in its gap for every incident linear polarization, which can be exploited to drive nonlinear optical emitters within the gap, for the structuring of light within a frequency range not accessible by linear plasmonics. As the polarization, phase and amplitude of the field in the gap are highly controlled, nonlinear em…
We report on the fabrication of metasurface phase plates consisting of gold nanoantenna arrays that generate Laguerre-Gaussian modes from a circularly polarized Gaussian input beam. The corresponding helical phase profiles with radial discontinuities are encoded in the metasurfaces by the orientation of the nanoantennas. A common-path interferometer is used to determine the orbital angular momentum of the generated beams. Additionally, we employ digital holography to record detailed phase profiles of the Laguerre-Gaussian modes. Experiments with different laser sources demonstrate the broadban…
We show that a broadband Fabry-Perot microcavity can assist an emitter coupled to an off-resonant plasmonic nanoantenna to inhibit the nonradiative channels that affect the quenching of fluorescence. We identify the interference mechanism that creates the necessary enhanced couplings and bandwidth narrowing of the hybrid resonance and show that it can assist entering into the strong coupling regime. Our results provide new possibilities for improving the efficiency of solid-state emitters and accessing diverse realms of photophysics with hybrid structures that can be fabricated using existing …
Metasurfaces are ultrathin nanostructured surfaces that can allow arbitrary manipulation of light. Implementing dynamic tunability into their design could allow the optical functions of metasurfaces to be rapidly modified at will. The most pronounced and robust tunability of optical properties is provided by phase-change materials such as vanadium dioxide (VO2) and germanium antimony telluride (GST), but their implementations have been limited only to near-infrared wavelengths. Here, we demonstrate that VO2 nanoantennas with widely tunable Mie resonances can be utilized for designing tunable m…
In nanoscale photonic devices, the demand for multifunctionality from metasurface 2D optics increases rapidly. To explore fine-tuning in the design metric, we reinvestigated the trapezoid shape copper metasurface with Finite-Difference Time-Domain simulation for efficiently using linearly polarized light for two different functionalities. From the plasmonic band structure, we see how the degree of asymmetry in geometry affects the efficient resonance coupling of the traveling plasmonic modes, along with different types of mode hybridization profiles related to the nanoantenna's geometric shape…
Freed from phase-matching constraints, plasmonic metasurfaces have contributed significantly to the control of the optical nonlinearity and enhancing the nonlinear generation efficiency by engineering subwavelength meta-atoms. However, the high dissipative losses and the inevitable thermal heating limit their applicability in nonlinear nanophotonics. All-dielectric metasurfaces, supporting both electric and magnetic Mie-type resonances in their nanostructures, have appeared as a promising alternative to nonlinear plasmonics. High-index dielectric nanostructures, allowing additional magnetic re…
We present the experimental realization of ordered arrays of hyper-doped silicon nanodisks, which exhibit a localized surface plasmon resonance. The plasmon is widely tunable in a spectral window between 2 and 5 $μ$m by adjusting the free carrier concentration between 10$^{20}$ and 10$^{21}$ cm$^{-3}$. We show that strong infrared light absorption can be achieved with all-silicon plasmonic metasurfaces employing nano-structures with dimensions as low as 100\,nm in diameter and 23 nm in height. Our numerical simulations show an excellent agreement with the experimental data and provide physical…
The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with $1L-WS_2$ by transferring it onto a plasmonic nanoantenna array, a hybrid metasurface is realized impacting the polarization dependency of its SHG. Here, we investigate how plasmonic dipole resonances affect the process of SHG in plasmonic-TMD hybrid metasurfaces by nonlinear spectroscopy. We show, that the polarization dependency is affected by the lattice str…
Nanostructures of conventional metals offer manipulation of light at the nanoscale but are limited to static behavior due to their fixed material properties. To develop the next frontier of dynamic nanooptics and metasurfaces, we utilize the redox-tunable optical properties of conducting polymers, which were recently shown to be capable of sustaining plasmons in their most conducting oxidized state. Using nanodisks of poly(3,4-ethylenedioxythiophene:sulfate) (PEDOT:Sulf) as a model system, we present the first electrically tunable conducting polymer nanooptical antennas. In addition to repeate…
The concept of optical phase discontinuities is applied to the design and demonstration of aberration-free planar lenses and axicons, comprising a phased array of ultrathin subwavelength spaced optical antennas. The lenses and axicons consist of radial distributions of V-shaped nanoantennas that generate respectively spherical wavefronts and non-diffracting Bessel beams at telecom wavelengths. Simulations are also presented to show that our aberration-free designs are applicable to high numerical aperture lenses such as flat microscope objectives.
Advances in understanding chemical and physical driving forces in self-assembly allow the fabrication of unique nanoarchitectures with subwavelength building blocks as the basis for plasmonic and metamaterial devices. Chemical crosslinking of colloidal nanospheres has produced among the smallest gap spacings, necessary to obtain regions of greatly enhanced electric field, hotspots, which are critical to tailor light-matter interactions. However, obtaining uniform electromagnetic response of dense nanoantennas over large area for use in devices remains challenging. In this work, electrohydrodyn…
Metasurfaces have achieved fruitful results in tailoring complexing light fields in free space. However, a systematic investigation on applying the concept of meta-optics to completely control waveguide modes is still elusive. Here we present a comprehensive catalog capable of selectively and exclusively excite almost arbitrary high-order waveguide modes of interest, leveraging silicon metasurface-patterned silicon nitride waveguides. By simultaneously engineering the phase-matched gradient of the metasurface and the vectorial spatial modal overlap between the nanoantenna near-field and target…
Controlling the phase and amplitude of light emitted by the elements (i.e., pixels) of an optical phased array is of paramount importance to realizing dynamic beam steering for LIDAR applications. In this paper, we propose a plasmonic pixel composed of a metallic nanoantenna covered by a thin oxide layer, and a conductive oxide, e.g., ITO, for use in a reflectarray metasurface. By considering voltage biasing of the nanoantenna via metallic connectors, and exploiting the carrier refraction effect in the metal-oxide-semiconductor capacitor in the accumulation and depletion regions, our simulatio…
Printing technology based on plasmonic structures has many advantages over pigment based color printing such as high resolution, ultra-compact size and low power consumption. However, due to high losses and broad resonance behavior of metals in the visible spectrum, it becomes challenging to produce well-defined colors. Here, we investigate cross-shaped dielectric nanoresonators which enable high quality resonance in the visible spectral regime and, hence, high quality colors. We numerically predict and experimentally demonstrate that the proposed all-dielectric nanostructures exhibit high qua…
Thermonanophotonics, i.e. the study of photothermal effects in optical nanoantennas, has recently attracted growing interest. While thermoplasmonic structures enable a broad range of applications, from imaging and optofluidics devices to medical and photochemical systems, dielectric nanoantennas open new opportunities for thermo-optical modulation and reconfigurable metasurfaces. However, computing both photo-thermal and thermo-optical effects in large arrays of nanoantennas remains a challenge. In this work, we implement a fast numerical method to compute the temperature increase of multi-dim…
A plasmonic nanoantenna probed by a plane-polarized optical field in a medium with no gain materials can show zero absorption or even amplification, while exhibiting maximal polarizability. This occurs through coupling to an adjacent nanoantenna in a specially designed metamolecule, which is pumped by an orthogonal optical field with phase shift. The introduced scheme is a classical counterpart of an effect known in quantum optics as enhancement of the index of refraction (EIR). In contrary to electromagnetically induced transparency (EIT), where the medium is rendered highly dispersive at the…
We discuss the recent advances in meta-optics and nanophotonics associated with the physics of bound states in the continuum (BICs). Such resonant states appear due to a strong coupling between leaky modes in optical guiding structures being supported by subwavelength high-index dielectric Mie-resonant nanoantennas or all-dielectric metasurfaces. First, we review briefly very recent developments in the BIC physics in application to isolated subwavelength particles. We pay a special attention to novel opportunities for nonlinear nanophotonics due to the large field enhancement inside the partic…
All-dielectric resonant nanophotonics lies at the heart of modern optics and nanotechnology due to the unique possibilities to control scattering of light from high-index dielectric nanoparticles and metasurfaces. One of the important concepts of dielectric Mie-resonant nanophotonics is associated with the Kerker effect that drives the unidirectional scattering of light from nanoantennas and Huygens' metasurfaces. Here we suggest and demonstrate experimentally a novel effect manifested in the nearly complete simultaneous suppression of both forward and backward scattered fields. This effect is…
Efficient hybrid plasmonic-photonic metasurfaces that simultaneously take advantage of the potential of both pure metallic and all-dielectric nanoantennas are identified as an emerging technology in flat optics. Nevertheless, post-fabrication tunable hybrid metasurfaces are still elusive. Here, we present a reconfigurable hybrid metasurface platform by incorporating the phase-change material Ge$_{2}$Sb$_{2}$Te$_{5}$ (GST) into metal-dielectric meta-atoms for active and non-volatile tuning of properties of light. We systematically design a reduced-dimension meta-atom, which selectively controls…
Intermixed light-matter quasiparticles - polaritons - possess unique optical properties owned to their compositional nature. These intriguing hybrid states have been extensively studied over the past decades in a wide range of realizations aiming at both basic science and emerging applications. However, recently it has been demonstrated that not only optical, but also material-related properties, such as chemical reactivity and charge transport, may be significantly altered in the strong coupling regime of light-matter interactions. Here, we show that a nanoscale system, comprised of a plasmon…
We propose a novel numerical approach for the optimal design of wide-area heterogeneous electromagnetic metasurfaces beyond the conventionally used unit-cell approximation. The proposed method exploits the combination of Rigorous Coupled Wave Analysis (RCWA) and global optimization techniques (two evolutionary algorithms namely the Genetic Algorithm (GA) and a modified form of the Artificial Bee Colony (ABC with memetic search phase method) are considered). As a specific example, we consider the design of beam deflectors using all-dielectric nanoantennae for operation in the visible wavelength…
Meta-optics based on optically resonant all-dielectric structures is a rapidly developing research area driven by its potential applications for low-loss efficient metadevices. Active, light-emitting subwavelengh nanostructures and metasurfaces are of a particular interest for meta-optics, as they offer unique opportunities for novel types of compact light sources and nanolasers. Recently, the study of halide perovskites has attracted an enormous attention due to their exceptional optical and electrical properties. As a result, this family of materials can provide a prospective platform for mo…
Plasmonic color generation utilizing ultra-thin metasurfaces as well as metallic nanoparticles hold a great promise for a wide range of applications, including color displays, data storage, and information encryption due to its high spatial resolution and mechanical/chemical stability. Most of the recently demonstrated systems generate static colors; however, more advanced applications such as data storage require fast and flexible means to tune the plasmonic colors, while keeping them vibrant and stable. Here, a surface-relief aluminum metasurface that reflects polarization-tunable plasmonic …
Room-temperature strong coupling between plasmonic nanocavities and monolayer semiconductors is a prominent path towards efficient, integrated light-matter interactions. However, designing such systems is challenging due to the nontrivial dependence of the strong coupling on various properties of the cavity and emitter, as well as the subwavelength scale of the interaction. In this work, we develop a methodology for obtaining hybrid nanostructures consisting of plasmonic metasurfaces coupled to atomically thin WS2 layers, exhibiting extreme values of Rabi splitting, by inverse design of the ne…
