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arXiv 2602.21603cond-mat.mes-hall
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厚度驱动控制室温铁磁Skyrmion及其拓扑Hall特征在GdFe单层中

Thickness-Driven Control of Room Temperature Ferrimagnetic Skyrmions and their Topological Hall signature in GdFe Single Layers

Indian Institute of Technology Hyderabad(印度理工学院海德拉巴分校);National Institute for Materials Science(国立材料研究所);Tata Institute of Fundamental Research(塔塔基础研究所)

Saroj Kumar Mishra, Y. K. Takahashi, C. Malavika, Karthik V. Raman, Jyoti Ranjan Mohanty

AI总结:

通过控制GdFe单层薄膜厚度,实现室温下铁磁Skyrmion的尺寸和密度调控,并观察到拓扑Hall特征的增强。

摘要:

磁性Skyrmion是纳米级、拓扑保护的自旋纹理,具有极高的密度数据存储和节能计算潜力。在各种Skyrmion宿主系统中,稀土过渡金属铁磁体提供了一个有前景的平台,由于其可调磁性特性和内在低净磁化率。尽管如此,单层薄膜中铁磁Skyrmion的基本控制仍处于未探索状态。在这里,我们展示了一种通过精确控制薄膜厚度(60至80纳米)来在GdFe单层中工程室温Skyrmion的可行途径。厚度变化能够系统地调节关键磁性参数,包括垂直磁各向异性及饱和磁化率,从而允许对Skyrmion尺寸和密度进行精确控制。磁力显微镜(MFM)揭示了厚度依赖的孤立Skyrmion特征演变,其中Skyrmion尺寸随着GdFe薄膜厚度的增加而减小,而Skyrmion密度增加,与微磁模拟结果一致。同时,磁输运测量显示拓扑Hall电阻率随厚度系统性增强,进一步证实了MFM中观察到的Skyrmion密度增加。扫描透射电子显微镜揭示了薄膜厚度方向上的组分梯度,表明了结构不对称性和可能的反演对称性破坏,促成体态Dzyaloshinskii-Moriya相互作用的出现。值得注意的是,亚60纳米的高面积密度Skyrmion在室温下被稳定。这项工作提供了一种调节单层GdFe薄膜中铁磁Skyrmion性质的可行途径,为高密度铁磁Skyrmionic器件的发展铺平了道路。

英文摘要:

Magnetic skyrmions are nanoscale, topologically protected spin textures with exceptional potential for high density data storage and energy efficient computing. Among various skyrmion hosting systems, rare earth transition metal ferrimagnets offer a promising platform due to their tunable magnetic properties and intrinsically low net magnetization. Despite this, the fundamental control of ferrimagnetic skyrmions in single layer films remains unexplored. Here, we demonstrate a viable route for engineering room temperature skyrmions in GdFe single layers through precise control of film thickness (60 to 80 nm). Thickness variation enables the systematic tuning of key magnetic parameters, including perpendicular magnetic anisotropy and saturation magnetization, thereby allowing precise control over skyrmion size and density. Magnetic force microscopy (MFM) reveals a clear thickness dependent evolution of isolated skyrmion characteristics, where skyrmion size decreases while skyrmion density increases with increasing GdFe film thickness, in agreement with micromagnetic simulations. At the same time, magnetotransport measurements show a systematic enhancement in the topological Hall resistivity with thickness, further corroborating the increased skyrmion density observed in MFM. Scanning transmission electron microscopy reveals a compositional gradient across the film thickness, indicative of structural asymmetry and potential inversion symmetry breaking, contributing to the emergence of a bulk Dzyaloshinskii Moriya interaction. Notably, sub 60nm skyrmions with high areal density are stabilized at room temperature. This work provides a viable route to tailor the properties of ferrimagnetic skyrmions in single-layer GdFe films, paving the way for the development of high-density ferrimagnetic skyrmionic devices.

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