We report the results of two-photon-excited fluorescence (TPEF) measurements of the $5\mathrm{S}_{1/2} \rightarrow 5\mathrm{D}_{5/2}$ transition of $^{85}$Rb and $^{87}$Rb cooled in a magneto-optical trap (MOT). We observe TPEF at excitation powers as low as 1 $μ$W or fluxes as low as $2.98_{-0.94}^{+1.37} \times 10^{18}\ \text{photons}\,\text{cm}^{-2}\,\text{s}^{-1}$ ($^{85}$Rb) and $3.31_{-1.33}^{+2.21} \times 10^{18}\ \text{photons}\,\text{cm}^{-2}\,\text{s}^{-1}$ ($^{87}$Rb). Our results demonstrate that optically cooled Rb is a promising platform for observing sensitive two-photon spectral signatures at low photon fluxes.
In this paper we present a method to measure transient fluorescent dynamics with single trapped ions in a Paul trap. We use $^{40}$Ca$^+$ ions which exhibit a $Λ$-type three-level system and measure the characteristic optical pumping times between the ground $S_{1/2}$ and the meta-stable $D_{3/2}$ levels. We prepare one of these states, then pump it to the opposite via the excited $P_{1/2}$ state. By measuring the scattered photons of the ion, we retrieve transient curves of the atomic fluorescence. These curves provide fundamental information about the atomic system, such as branching fractio…
We experimentally investigate trap-loss spectra of the cesium 6S1/2(F=4)-71P3/2 Rydberg state by combining the cesium atomic magneto-optical trap with the narrow-linewidth, continuously-tunable 318.6 nm ultraviolet laser. That is, the atoms in the magneto-optical trap are excited to the Rydberg state due to the ultraviolet laser single-step Rydberg excitation, which leads to the reduction of atomic fluorescence. Based on the trap-loss spectroscopy technology, the Autler-Townes splitting due to strong cooling laser is observed, and the parameter dependence of the AT splitting interval of trap-l…
We report on magneto-optical resonances observed in sodium fluorescence from D2 manifold with an intensity modulated light. Fluorescence resonances are measured in the perpendicular and backward directions to the light propagation, in laboratory experiments using a sodium cell containing neon buffer gas. Properties of these resonances are studied by varying the magnetic field at fixed light modulation frequency, and vice-versa. Modulation with low-duty cycle shows higher-harmonic resonances of the modulation frequency and sub-harmonic resonances of the Larmor frequency. A dark resonance with m…
Light-induced polarization effects in atoms with partially resolved hyperfine structure and applications to absorption, fluorescence, and nonlinear magneto-optical rotation
It is known from ensemble measurements that rubidium atoms trapped in solid parahydrogen have favorable properties for quantum sensing of magnetic fields. To use a single rubidium atom as a quantum sensor requires a technique capable of efficiently measuring the internal state of a single atom, such as laser-induced fluorescence. In this work we search for laser-induced fluorescence from ensembles of rubidium atoms trapped in solid parahydrogen and, separately, in solid neon. In parahydrogen we find no evidence of fluorescence over the range explored, and place upper limits on the radiative br…
We report a new technique for generating magnetic resonance with synchronous modulation of two-photon resonant light fields. Magnetic resonances in fluorescence from a sodium cell are measured to demonstrate suitability of this technique for remote magnetometry. A strong magnetic resonance with its dip corresponding to the Larmor frequency is produced in the presence of a transverse magnetic field. An additional resonance at 3\{Omega_L} is observed, which can be used to determine the magnetic field orientation. We have developed a theoretical model based on the density matrix equations to veri…
We demonstrate an optical method for detecting the mechanical oscillations of an atom with single-phonon sensitivity. The measurement signal results from the interference between the light scattered by a single trapped atomic ion and that of its mirror image. The motion of the atom modulates the interference path length and hence the photon detection rate. We detect the oscillations of the atom in the Doppler cooling limit and reconstruct average trajectories in phase space. We demonstrate single-phonon sensitivity near the ground state of motion after EIT cooling. These results could be appli…
Metastable (1s)(2s) $^3{\rm S}_1$ helium atoms produced in a supersonic beam were excited to Rydberg-Stark states (with $n$ in the $27-30$ range) in a cryogenic environment and subsequently decelerated by, and trapped above, a surface-electrode decelerator. In the trapping experiments, the Rydberg atoms were brought to rest in 75~$μ$s and over a distance of 33~mm and kept stationary for times $t_{\mathrm{trap}}$ in the $0-525$~$μ$s range, before being re-accelerated for detection by pulsed field ionization. The use of a home-built valve producing short gas pulses with a duration of about 20~$μ…
We report high-fidelity state readout of a trapped ion qubit using a trap-integrated photon detector. We determine the hyperfine qubit state of a single $^9$Be$^+$ ion held in a surface-electrode rf ion trap by counting state-dependent ion fluorescence photons with a superconducting nanowire single-photon detector (SNSPD) fabricated into the trap structure. The average readout fidelity is 0.9991(1), with a mean readout duration of 46 $μ$s, and is limited by the polarization impurity of the readout laser beam and by off-resonant optical pumping. Because there are no intervening optical elements…
We have developed a compact setup which enables loading a magneto-optical trap (MOT) in ultra-high vacuum (UHV) environment. Nearly $1 \times 10^{8}$ atoms of $^{87}Rb$ are trapped in the MOT at $\sim 2 \times 10^{-10}$ Torr base pressure in the chamber. After the MOT loading, we have successfully demonstrated working of quadrupole magnetic trap in this chamber with a lifetime of $\sim 8 $ s
We realize a scanning probe microscope using single trapped $^{87}$Rb atoms to measure optical fields with subwavelength spatial resolution. Our microscope operates by detecting fluorescence from a single atom driven by near-resonant light and determining the ac Stark shift of an atomic transition from other local optical fields via the change in the fluorescence rate. We benchmark the microscope by measuring two standing-wave Gaussian modes of a Fabry-Pérot resonator with optical wavelengths of 1560 nm and 781 nm. We attain a spatial resolution of 300 nm, which is superresolving compared to t…
We present a realization of a magneto-optical trap of mercury atoms on the intercombination line. We report on trapping of all stable mercury isotopes. We characterize the effect of laser detuning, laser intensity, and gradient field on the trapping performance of our system. The atom number for the most abundant isotope Hg-202 is 50 million atoms. Moreover, we study the difference in cooling processes for bosonic and fermionic isotopes. We observe agreement with the Doppler cooling theory for the bosonic species and show sub-Doppler cooling for the fermionic species. We reach a phase space de…
We present a novel, single-ion trap with integrated optical fibers directly embedded within the trap structure to deliver laser light as well as collect the ion's fluorescence. This eliminates the need for optical windows. We characterise the system's performance and measure signal-to-background ratios in the ion's fluorescence on the order of 50, which allows us to perform state readout with a fidelity over 99% in 600 $μ$s. We test the system's resilience to thermal variations in the range between 22°C and 53°C, and the system's vibration resilience at 34 Hz and 300 Hz and find no effect on i…
We demonstrate the use of spatial emission patterns to measure the magnetic fields used in a magneto-optical trap. The directional aspect of the Hanle effect gives a direct, visual presentation of the magnetic fields, in which brighter fluorescence indicates larger fields. It can be used to determine the direction as well as the magnitude of the field. It is particularly well suited for characterizing and aligning magneto-optical traps, requiring little additional equipment or setup beyond what is ordinarily used in a magneto-optical trap, and being most sensitive to fields of the size typical…
We perform balanced homodyne detection of the electromagnetic field in a single-mode tapered optical nanofiber surrounded by rubidium atoms in a magneto-optical trap. Resonant fluorescence of atoms into the nanofiber mode manifests itself as increased quantum noise of the field quadratures. The autocorrelation function of the homodyne detector's output photocurrent exhibits exponential fall-off with a decay time constant of $26.3\pm 0.6$ ns, which is consistent with the theoretical expectation under our experimental conditions. To our knowledge, this is the first experiment in which fluorescen…
We report on the design, implementation, and performance of a compact two-dimensional magneto-optical trap (2D MOT) for cesium. In a small-volume vacuum chamber, the setup uses cesium dispensers in close proximity to the trapping region of the 2D MOT and operates at low vapor pressures in the $10^{-9}$ torr range. We achieve a cold atom flux of $4 \times 10^8$ atoms/s that is comparable to the performance of more complex atomic sources. The setup is simple to construct and can be adapted to a broad range of atomic species.
Large clouds of cold atoms prepared in a magneto-optical trap can develop spatio-temporal instabilities when the frequency of the trapping lasers is brought close to the atomic resonance. This system bears close similarities with trapped plasmas, whereby effective Coulomb interactions are induced by the exchange of scattered photons and lead to collective nonlinear dynamics of the trapped atoms. We report in this paper a detailed experimental study of the instability threshold, and comparisons with three-dimensional simulations of the interacting, laser-driven cloud.
A single atom emitting resonance fluorescence into a coherent beam, and its use for non-destructive atom thermometry
ICFO - Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology（光子科学研究所，巴塞罗那科学技术学院）；ICREA - Institució Catalana de Recerca i Estudis Avançats（加泰罗尼亚高级研究学院）
We propose and demonstrate a novel technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient fluorophores with discrete absorption and emission profiles that are readily separated for sensitive fluorescence detection in high background light environments. Using a molecular beam of our test species, SrF, we realize up to an average of $\approx20$ spontaneously emitted photons per molecule, limited by the interaction time, while using a bandpass filter to suppr…
