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arXiv 2505.03250cond-mat.mtrl-scicond-mat.other
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从晶格动力学与穆斯堡尔谱学看RuO$_2$的磁性与关联约束

Constraints on magnetism and correlations in RuO$_2$ from lattice dynamics and Mössbauer spectroscopy

Oak Ridge National Laboratory(橡树岭国家实验室);The Hamburg Centre for Ultrafast Imaging CUI(汉堡超快成像中心);Argonne National Laboratory(阿贡国家实验室);George Mason University(乔治梅森大学);University of Tennessee, Knoxville(田纳西大学诺克斯维尔分校);Brigham Young University(杨百翰大学)
George Yumnam, Parul R. Raghuvanshi, John D. Budai, Dipanshu Bansal, Lars Bocklage, Douglas Abernathy, Yongqiang Cheng, Ayman Said, Igor I. Mazin, Haidong Zhou,… 展开作者

George Yumnam, Parul R. Raghuvanshi, John D. Budai, Dipanshu Bansal, Lars Bocklage, Douglas Abernathy, Yongqiang Cheng, Ayman Said, Igor I. Mazin, Haidong Zhou, Benjamin A. Frandsen, David S. Parker, Lucas R. Lindsay, Valentino R. Cooper, Michael E. Manley, Raphaël P. Hermann

AI总结:

本研究结合多种谱学散射实验与密度泛函理论计算,证实候选反铁磁体块体RuO₂无磁矩,且电子关联对其晶格动力学起关键作用,为理解该材料的磁性与电子关联特性提供了实验依据。

摘要:

我们通过结合穆斯堡尔谱学、核前向散射、非弹性X射线与中子散射以及密度泛函理论计算,为候选反铁磁体块体RuO$_2$中不存在磁矩提供了实验证据。利用互补的穆斯堡尔谱与核前向散射,我们测定$^{99}$Ru的磁超精细分裂可忽略不计。将非弹性X射线与中子散射得到的RuO$_2$晶格动力学,与不同类型的密度泛函理论计算结果进行了对比。理论与实验的比较表明,电子关联而非磁有序是描述晶格动力学的关键。

英文摘要:

We provide experimental evidence for the absence of a magnetic moment in bulk RuO$_2$, a candidate altermagnetic material, by using a combination of Mössbauer spectroscopy, nuclear forward scattering, inelastic X-ray and neutron scattering, and density functional theory calculations. Using complementary Mössbauer and nuclear forward scattering we determine the $^{99}$Ru magnetic hyperfine splitting to be negligible. Inelastic X-ray and neutron scattering derived lattice dynamics of RuO$_2$ are compared to density functional theory calculations of varying flavors. Comparisons among theory with experiments indicate that electronic correlations, rather than magnetic order, are key in describing the lattice dynamics.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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