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arXiv 2402.18359cond-mat.str-elcond-mat.mtrl-sci
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揭示Sr$_2$RuO$_4$表面的非传统磁性

Unveiling unconventional magnetism at the surface of Sr$_2$RuO$_4$

Rosalba Fittipaldi, Roman Hartmann, Maria Teresa Mercaldo, Sachio Komori, Anders Bjørlig, Wonshik Kyung, Yuuki Yasui, Takuto Miyoshi, Linde Olde-Olthof, Carla P… 展开作者

Rosalba Fittipaldi, Roman Hartmann, Maria Teresa Mercaldo, Sachio Komori, Anders Bjørlig, Wonshik Kyung, Yuuki Yasui, Takuto Miyoshi, Linde Olde-Olthof, Carla Palomares-Garcia, Veronica Granata, Itai Keren, Wataru Higemoto, Andreas Suter, Thomas Prokscha, Alfonso Romano, Canio Noce, Changyoung Kim, Yoshiteru Maeno, Elke Scheer, Beena Kalisky, Jason W. A. Robinson, Mario Cuoco, Zaher Salman, Antonio Vecchione, Angelo Di Bernardo

AI总结:

本研究利用低能μ子自旋谱发现Sr$_2$RuO$_4$正常态表面在50 K以上存在弱静态磁性,并将其归因于重构表面的轨道环流电流电子有序。

摘要:

具有强关联电子的材料表现出通常难以预测的物理性质,因为这些性质源于大量电子的相互作用与多种量子自由度的结合。层状氧化物钙钛矿Sr$_2$RuO$_4$是一种强关联电子材料,自发现以来因其不同寻常的物理性质而得到深入研究。尽管近期实验重新引发了关于Sr$_2$RuO$_4$超导态确切对称性的争论,但更深入理解Sr$_2$RuO$_4$的正常态似乎至关重要,因为这是电子配对发生的背景。本文中,通过使用低能μ子自旋谱,我们发现Sr$_2$RuO$_4$在正常态下其表面存在磁性。我们检测到静态弱偶极场,但这些场在高于50 K的相对较高起始温度以下显现,这揭示了所观测磁性的非传统本质。我们将这种破坏时间反演对称性的相的起源,与重构的Sr$_2$RuO$_4$表面产生的轨道环流电流形式的电子有序联系起来。我们的观测为在其他材料中发现相同磁相确立了参照,并揭示了一种电子有序机制;在观测到的磁相与超导共存的那些材料中,该机制能够影响伴随时间反演对称性破缺的非传统电子配对。

英文摘要:

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered oxide perovskite Sr$_2$RuO$_4$ is a strongly correlated electron material that has been intensively investigated since its discovery due to its unusual physical properties. Whilst recent experiments have reopened the debate on the exact symmetry of the superconducting state in Sr$_2$RuO$_4$, a deeper understanding of the Sr$_2$RuO$_4$ normal state appears crucial as this is the background in which electron pairing occurs. Here, by using low-energy muon spin spectroscopy we discover the existence of magnetism at the surface of Sr$_2$RuO$_4$ in its normal state. We detect static weak dipolar fields yet manifesting below a relatively high onset temperature larger than 50 K, which reveals the unconventional nature of the observed magnetism. We relate the origin of this phase breaking time reversal symmetry to electronic ordering in the form of orbital loop currents that originate at the reconstructed Sr$_2$RuO$_4$ surface. Our observations set a reference for the discovery of the same magnetic phase in other materials and unveil an electronic ordering mechanism that can influence unconventional electron pairing with broken time reversal symmetry in those materials where the observed magnetic phase coexists with superconductivity.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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