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arXiv 2409.14520nucl-ex
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在激发能E$^{\star}$≈31.8–45.4 MeV下研究$^{12}$C + $^{208}$Pb系统中的类裂变碎片

Investigating the fission-like fragments in the $^{12}$C + $^{208}$Pb system at E$^{\star}$ $\approx$ 31.8--45.4 MeV

Rupinderjeet Kaur, Amanjot, Priyanka, Malika Kaushik, Subham Kumar, Arshiya Sood, Yashraj Jangid, R. Kumar, Manoj Kumar Sharma, Pushpendra P. Singh

AI总结:

本研究测量了$^{12}$C+$^{208}$Pb反应在两个入射能量下的类裂变碎片截面,分析了产额分布与弥散参数,验证了复合核裂变机制,并发现两种医用同位素的潜在生成路径。

摘要:

本研究采用活化技术结合离线γ射线能谱法,测量了$^{12}$C+$^{208}$Pb反应在实验室入射能量E$_{\rm lab}$=81.9 MeV和75.8 MeV条件下,质量范围76≤A≤141的25种类裂变碎片的截面;这些碎片预期由完全和/或非完全熔合产生的中等激发复合核发生裂变而生成。研究分析了不同类裂变碎片的产额,生成了同位素产额分布和同量异位素产额分布。结果显示,锑(Sb)同位素在激发能E$^{\star}$=45.4 MeV和39.6 MeV时的质量弥散参数$σ^2_A$分别为2.93和2.65,铟(In)同位素在E$^{\star}$=45.4 MeV时的$σ^2_A$为1.24。Sb的电荷弥散参数$σ_Z$在E$^{\star}$=45.4 MeV和39.6 MeV时分别估计为0.769和0.714;In同位素在E$^{\star}$=45.4 MeV时的$σ_Z$估计为0.430。Sb和In同位素的质量、电荷弥散参数值与文献中类似系统的报道值吻合良好。类裂变碎片的质量分布除少数数据点外均符合高斯函数,表明这些碎片通过复合核裂变产生。此外,质量方差($σ^2_M$)随激发能升高呈线性增长。该系统中生成了两种重要医用同位素$^{99m}$Tc和$^{111}$In,提示了一种潜在的制备途径。

英文摘要:

In this work, the cross-sections of 25 fission-like fragments within the mass range 76$\leq$A$\leq$141, expected to be populated via fission of moderately excited compound nucleus produced as a result of complete and/or incomplete fusion in $^{12}$C+$^{208}$Pb reaction at E$_{\rm lab}$ = 81.9 and 75.8 MeV, have been measured using activation technique followed by offline $γ$-ray spectroscopy. The yields of different fission-like fragments have been analyzed to generate isotopic and isobaric yield distributions. The value of the mass dispersion parameter, $σ^2_A$, is found to be 2.93 and 2.65 for Antimony (Sb) isotope at excitation energy E$^{\star}$ = 45.4 and 39.6 MeV, and 1.24 for Indium (In) isotope at E$^{\star}$ = 45.4 MeV. The charge dispersion parameter $σ_Z$ for Sb is estimated to be 0.769 and 0.714 at E$^{\star}$ = 45.4 and 39.6 MeV, respectively. For In isotopes, the value of $σ_Z$ is estimated to be 0.430 at E$^{\star}$ = 45.4 MeV. The value of mass and charge dispersion parameters for Sb and In isotopes have been found to be in good agreement with the values reported in the literature for similar systems. The mass distribution of fission-like fragments is found to be fitted with a Gaussian function, except for a few data points, indicating their population via compound nucleus fission. Further, the mass variance ($σ^2_M$) displays linear increment with an increase in excitation energy. Two medically important isotopes, $^{99m}$Tc and $^{111}$In, are populated in this system, suggesting a potential formation route.

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