Quantum mechanics predicts that massive particles exhibit wave-like behavior. Matterwave interferometry has been able to validate such predictions through ground-breaking experiments involving microscopic systems like atoms and molecules. The wavefunction of such systems coherently extends over a distance much larger than their size, an achievement that is incredibly challenging for massive and more complex objects. Yet, reaching similar level of coherent diffusion will enable tests of fundamental physics at the genuinely macroscopic scale, as well as the development of quantum sensing apparata of great sensitivity. We report on experimentally achieving an unprecedented degree of position diffusion in a massive levitated optomechanical system through frequency modulation of the trapping potential. By starting with a pre-cooled state of motion and employing a train of sudden pulses yet of mild modulation depth, we surpass previously attained values of position diffusion in this class of systems to reach diffusion lengths that exceed the physical dimensions of the trapped nanoparticle.
We report on measurements of photon induced heating of silica nanospheres levitated in vacuum by a thermal light source formed by a superluminescent diode. Heating of the nanospheres motion along the three trap axes was measured as a function of gas pressure and for two particle sizes. Heating rates were also compared with the much lower reheating of the same sphere when levitated by a laser. We find the measured trap heating rates are dominated by the much larger heating rates expected from the recoil of thermal photons.
We report quantum ground state cooling of a levitated nanoparticle in a room temperature environment. Using coherent scattering into an optical cavity we cool the center of mass motion of a $143$ nm diameter silica particle by more than $7$ orders of magnitude to $n_x=0.43\pm0.03$ phonons along the cavity axis, corresponding to a temperature of $12~μ$K. We infer a heating rate of $Γ_x/2π= 21\pm 3$ kHz, which results in a coherence time of $7.6~μ$s -- or $15$ coherent oscillations -- while the particle is optically trapped at a pressure of $10^{-6}$ mbar. The inferred optomechanical coupling ra…
A nanoscale object evidenced in a non-classical state of its centre of mass will hugely extend the boundaries of quantum mechanics. To obtain a practical scheme for the same, we exploit a hitherto unexplored coupled system: an atom and a nanoparticle coupled by an optical field. We show how to control the center-of-mass of a large $\sim500$nm nanoparticle using the internal state of the atom so as to create, as well as detect, nonclassical motional states of the nanoparticle. Specifically, we consider a setup based on a silica nanoparticle coupled to a Cesium atom and discuss a protocol for pr…
The beam splitter and phase shifter, which are the key elements in the experiments of light interference, are realized in the motion of trapped ions. Some applications, such as the creation of quantum motional states and the realization of Mach-Zehnder interferometer, are illustrated. Several detection methods of motional states used in the interferometer are also discussed.
A theoretical scheme for the realization of the sphere-coherent motional states in an optomechanical cavity in the presence of a two-level atom is proposed. To this end, the analogy between an atom-assisted optomechanical cavity and a laser-driven trapped-ion system is used. This analogy provides us with a theoretical tool to show how sphere-coherent states can be generated for the motional degree of freedom of the macroscopic mechanical oscillator from atom-field-mirror interactions in a multi-mode optomechanical cavity. Some nonclassical properties of the generated state of the mechanical os…
Entangling gates in trapped-ion quantum computing have primarily targeted stationary ions with initial motional distributions that are thermal and close to the ground state. However, future systems will likely incur significant non-thermal excitation due to, e.g., ion transport, longer operational times, and increased spatial extent of the trap array. In this paper, we analyze the impact of such coherent motional excitation on entangling-gate error by performing simulations of Molmer-Sorenson (MS) gates on a pair of trapped-ion qubits with both thermal and coherent excitation present in a shar…
We propose a theoretical scheme to show the possibility of generating motional nonlinear coherent states and their superposition for an undamped vibrating micromechanical membrane inside an optical cavity. The scheme is based on an intensity-dependent coupling of the membrane to the radiation pressure field. We show that if the cavity field is initially prepared in a Fock state, the motional state of the membrane may evolve from vacuum state to a special type of nonlinear coherent states. By examining the nonclassical properties of the generated state of the membrane, including the quadrature …
Preparing and observing quantum states of nanoscale particles is a challenging task with great relevance for quantum technologies and tests of fundamental physics. In contrast to atomic systems with discrete transitions, nanoparticles exhibit a practically continuous absorption spectrum and thus their quantum dynamics cannot be easily manipulated. Here, we demonstrate that charged nanoscale dielectrics can be artificially endowed with a discrete level structure by coherently interfacing their rotational and translational motion with a superconducting qubit. We propose a pulsed scheme for the g…
Quantum coherence is one of the clearest departures from classical physics, exhibited when a system is in a superposition of different basis states. Here the coherent superposition of three motional Fock states of a single trapped ion is experimentally certified, with a procedure provably robust against imperfect operation. As the motional state cannot be directly interrogated, our scheme uses an interference pattern generated by projective measurement of the coupled qubit state. The minimum number of coherently superposed states is inferred from a series of threshold values based on analysis …
All three motional modes of a charged dielectric nanoparticle in a Paul trap are cooled by direct feedback to temperatures of a few mK. We test two methods, one based on electrical forces and the other on optical forces; for both methods, we find similar cooling efficiencies. Cooling is characterized for both feedback forces as a function of feedback parameters, background pressure, and the particle's position.
We present a method for measuring the polarizability of Rydberg ions confined in the harmonic potential of a Paul trap. For a highly excited electronic state, the coupling between the electronic wave function and the trapping field modifies the excitation probability depending on the motional state of the ion. This interaction strongly depends on the polarizability of the excited state and manifests itself in the state-dependent secular frequencies of the ion. We initialize a single trapped $^{40}$Ca$^+$ ion from the motional ground state into coherent states with $|α|$ up to 12 using electric…
We study the potential for controlled transfer of population to the biexciton state of a semiconductor quantum dot coupled with a metal nanoparticle, under the influence of an electromagnetic pulse with hyperbolic secant shape, and derive analytical solutions of the density matrix equations, for both zero and nonzero biexciton energy shift. These solutions lead to efficient transfer to the biexciton state, for various interparticle distances, including relatively small values. In certain cases, when the distance between the two particles is small, the transfer of population is strongly modifie…
We present an efficient scheme to generate two-mode SU(2) macroscopic quantum superposition (Schrödinger cat) states, entangled number states and entangled coherent states for the vibrational motion of an ion trapped in a two-dimensional harmonic potential well. We also show that the same scheme can be used to realize a Fredkin gate operation.
Superconducting circuits with Josephson junctions are promising candidates for developing future quantum technologies. Of particular interest is to use these circuits to study effects that typically occur in complex condensed-matter systems. Here, we employ a superconducting quantum bit (qubit),a transmon, to carry out an analog simulation of motional averaging, a phenomenon initially observed in nuclear magnetic resonance (NMR) spectroscopy. To realize this effect, the flux bias of the transmon is modulated by a controllable pseudo-random telegraph noise, resulting in stochastic jumping of th…
The scattering of a single photon with sufficiently high energy can cause a recoil of a motional scatterer. We study its backaction on the photon's coherent transport in one dimension by modeling the motional scatterer as a two-level system, which is trapped in a harmonic potential. While the reflection spectrum is of a single peak in the Lamb-Dicke limit, multi-peaks due to phonon excitations can be observed in the reflection spectrum as the trap becomes looser or the mass of the two-level system becomes smaller.
We present theoretical and experimental progress towards a new approach for the precision spectroscopy, coherent manipulation and state-to-state chemistry of single isolated molecular ions in the gas phase. Our method consists of a molecular beam for creating packets of rotationally cold neutrals from which a single molecule is state-selectively ionized and trapped inside a radiofrequency ion trap. In addition to the molecular ion, a single co-trapped atomic ion is used to cool the molecular external degrees of freedom to the ground state of the trap and to detect the molecular state using sta…
We report phase-coherent Doppler detection of optical dipole forces using large ion crystals in a Penning trap. The technique is based on laser Doppler velocimetry using a cycling transition in $^{9}$Be$^{+}$ near 313 nm and the center-of-mass (COM) ion motional mode. The optical dipole force is tuned to excite the COM mode, and measurements of photon arrival times synchronized with the excitation potential show oscillations with a period commensurate with the COM motional frequency. Experimental results compare well with a quantitative model for a driven harmonic oscillator. This technique pe…
We propose to optimally control the harmonic potential of a levitated nanoparticle to quantum delocalize its center-of-mass motional state to a length scale orders of magnitude larger than the quantum zero-point motion. Using a bang-bang control of the harmonic potential, including the possibility to invert it, the initial ground-state-cooled levitated nanoparticle coherently expands to large scales and then contracts to the initial state in a time-optimal way. We show that this fast loop protocol can be used to enhance force sensing as well as to dramatically boost the entangling rate of two …
The reduced dynamics of an atomic qubit coupled both to its own quantized center of mass motion through the spatial mode functions of the electromagnetic field, as well as the vacuum modes, is calculated in the influence functional formalism. The formalism chosen can describe the entangled non-Markovian evolution of the system with a full account of the coherent back-action of the environment on the qubit. We find a slight increase in the decoherence due to the quantized center of mass motion and give a condition on the mass and qubit resonant frequency for which the effect is important. In op…
Non-Gaussian states represent a powerful resource for quantum information protocols in the continuous variables regime. Cat states, in particular, have been produced in the motional degree of freedom of trapped ions by controlled displacements dependent on the ionic internal state. An alternative method harnesses the Kerr nonlinearity naturally existent in this kind of system. We present detailed calculations confirming its feasibility for typical experimental conditions. Additionally, this method permits the generation of complex non-Gaussian states with negative Wigner functions. Especially,…
Nanoparticles trapped in optical tweezers emerged as an interesting platform for investigating fundamental effects in quantum physics. The ability to shape the optical trapping potential using spatial light modulation and quantum control of their motion using coherent scattering to an optical cavity mode predispose them for emulating a range of physical systems and studying quantum phenomena with massive objects. To extend these capabilities of levitated nanoparticles to quantum many-body systems, it is crucial to develop feasible strategies to couple and entangle multiple particles either dir…
We develop a theory for cavity cooling of the center-of-mass motion of a levitated nanoparticle through coherent scattering into an optical cavity. We analytically determine the full coupled Hamiltonian for the nanoparticle, cavity, and free electromagnetic field. By tracing out the latter, we obtain a Master Equation for the cavity and the center of mass motion, where the decoherence rates ascribed to recoil heating, gas pressure, and trap displacement noise are calculated explicitly. Then, we benchmark our model by reproducing published experimental results for three-dimensional cooling. Fin…
We show how entanglement between two optically levitated nanoparticles can be generated and detected by coherent scattering of tweezer photons into a single cavity mode. Triggered by the detection of a Stokes photon, the tweezer detuning is switched from the blue to the red; entanglement is then verified by the conditioned anti-Stokes photon flux, which oscillates with the mechanical beat frequency. The proposed setup is realizable with near-future technology and opens the door to the first experimental observation of non-classical center-of-mass correlations between two or more levitated nano…
We demonstrate the preparation and coherent control of the angular momentum state of a two-ion crystal. The ions are prepared with an average angular momentum of $7780\hbar$ freely rotating at 100~kHz in a circularly symmetric potential, allowing us to address rotational sidebands. By coherently exciting these motional sidebands, we create superpositions of states separated by up to four angular momentum quanta. Ramsey experiments show the expected dephasing of the superposition which is dependent on the number of quanta separating the states. These results demonstrate coherent control of a co…
Coherent scattering of an elliptically polarised tweezer into a cavity mode provides a promising platform for cooling levitated nanoparticles into their combined rotational and translational quantum regime [Phys. Rev. Lett. 126, 163603 (2021)]. This article presents the theory of how aspherical nanoparticles are affected by elliptically polarised laser beams, how two orthogonal cavity modes enable rotational and translational cooling, and how the resulting power spectra contain signatures of rotational non-linearities. We provide analytic expressions for the resulting trapping frequencies, opt…
Quantum memories for light are essential components in quantum technologies like long-distance quantum communication and distributed quantum computing. Recent studies have shown that long optical and spin coherence lifetimes can be observed in rare earth doped nanoparticles, opening exciting possibilities over bulk materials e.g. for enhancing coupling to light and other quantum systems, and material design. Here, we report on coherent light storage in Eu$^{3+}$:Y$_2$O$_3$ nanoparticles using the Stark Echo Modulation Memory (SEMM) quantum protocol. We first measure a nearly constant Stark coe…
A procedure is discussed for creating coherent superpositions of motional states of ion strings. The motional states are across the structural transition linear-zigzag, and their coherent superposition is achieved by means of spin-dependent forces, such that a coherent superposition of the electronic states of one ion evolves into an entangled state between the chain's internal and external degrees of freedom. It is shown that the creation of such an entangled state can be revealed by performing Ramsey interferometry with one ion of the chain.
Quantum interfaces between photons and ensembles of atoms have emerged as powerful tools for quantum technologies. A major objective for such interfaces is high fidelity storage and retrieval of a photon in a collective quantum state of many atoms. This requires long-lived collective superposition states, which is typically achieved with immobilized atoms. Thermal atomic vapors, which present a simple and scalable resource, have, so far, only been used for continuous variable processing or for discrete variable processing on short time scales where atomic motion is negligible. We develop a the…
We show that the motion of a cold trapped ion can be squeezed by modulating the intensity of a phase-stable optical lattice placed inside the trap. As this method is reversible and state selective it effectively implements a controlled-squeeze gate. We show how to use this resource, that can be useful for quantum information processing with continuous variables, in order to prepare coherent superpositions of states which are squeezed along complementary quadratures. We show that these states, which we denote as "${\mathcal X}$-states", exhibit high sensitivity to small displacements along two …
We present a theoretical study of the resonance fluorescence spectra of an optically driven quantum dot placed near a single metal nanoparticle. The metallic reservoir coupling is calculated for an 8-nm metal nanoparticle using a time-convolutionless master equation approach where the exact photon reservoir function is included using Green function theory. By exciting the system coherently near the nanoparticle dipole mode, we show that the driven Mollow spectrum becomes highly asymmetric due to internal coupling effects with higher-order plasmons. We also highlight regimes of resonance squeez…
Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence. Quantum control of mechanical motion has been achieved by engineering the radiation-pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for …
Coherently displaced harmonic oscillator number states of a harmonically bound ion can be coupled to two internal states of the ion by a laser-induced motional sideband interaction. The internal states can subsequently be read out in a projective measurement via state-dependent fluorescence, with near-unit fidelity. This leads to a rich set of line shapes when recording the internal-state excitation probability after a sideband excitation, as a function of the frequency detuning of the displacement drive with respect to the ion's motional frequency. We precisely characterize the coherent displ…
We experimentally realize cavity cooling of all three translational degrees of motion of a levitated nanoparticle in vacuum. The particle is trapped by a cavity-independent optical tweezer and coherently scatters tweezer light into the blue detuned cavity mode. For vacuum pressures around $10^{-5}\,{\rm mbar}$, minimal temperatures along the cavity axis in the mK regime are observed. Simultaneously, the center-of-mass (COM) motion along the other two spatial directions is cooled to minimal temperatures of a few hundred $\rm mK$. Measuring temperatures and damping rates as the pressure is varie…
Characterization and cancellation of power-line-induced motional-mode frequency noise in a trapped-ion system
Seoul National University（首尔大学）；Department of Computer Science and Engineering, Seoul National University（首尔大学计算机科学与工程系）；Automation and Systems Research Institute, Seoul National University（首尔大学自动化与系统研究所）；NextQuantum, Seoul National University（首尔大学NextQuantum）
Ground state cooling and coherent manipulation of ions in an rf-(Paul) trap is the prerequisite for quantum information experiments with trapped ions. With resolved sideband cooling on the optical S1/2 - D5/2 quadrupole transition we have cooled one and two 40Ca+ ions to the ground state of vibration with up to 99.9% probability. With a novel cooling scheme utilizing electromagnetically induced transparency on the S1/2 - P1/2 manifold we have achieved simultaneous ground state cooling of two motional sidebands 1.7 MHz apart. Starting from the motional ground state we have demonstrated coherent…
We investigate the motional dynamics of single and multiple ions during transport between and separation into spatially distinct locations in a multi-zone linear Paul trap. A single 9Be+ ion in a 2 MHz harmonic well located in one zone was laser-cooled to near its ground state of motion and transported 370 micrometers by moving the well to another zone. This was accomplished in 8 microseconds, corresponding to 16 periods of oscillation. Starting from a state with n=0.1 quanta, during transport the ion was excited to a displaced coherent state with n=1.6 quanta but on completion was returned cl…
Two close parallel mirrors attract due to a small force (Casimir effect) originating from the electromagnetic quantum vacuum uctuations of the electromagnetic field. These vacuum uctuations can also induce motional forces exerted upon one mirror when the other one moves. Here we consider an optomechanical system consisting of two vibrating mirrors coupled to an optical resonator. We find that motional forces can determine noticeable coupling rates between the two spatially separated vibrating mirrors. We show that, by tuning the two mechanical oscillators into resonance, energy is exchanged be…
Laser cooling has given a boost to atomic physics throughout the last thirty years since it allows one to prepare atoms in motional states which can only be described by quantum mechanics. Most methods, such as Doppler cooling, polarization gradient cooling or sub-recoil laser cooling rely, however, on a near-resonant and cyclic coupling between laser light and well-defined internal states. Although this feat has recently even been achieved for diatomic molecules, it is very hard for mesoscopic particles. It has been proposed that an external cavity may compensate for the lack of internal cycl…
We investigate how superpositions of motional coherent states naturally arise in the dynamics of a two-level trapped ion coupled to the quantized field inside a cavity. We extend our considerations including a more realistic set up where the cavity is not ideal and photons may leak through its mirrors. We found that a detection of a photon outside the cavity would leave the ion in a pure state. The statistics of the ionic state still keeps some interference effects that might be observed in the weak coupling regime.
