We develop a theory for cavity cooling of the center-of-mass motion of a levitated nanoparticle through coherent scattering into an optical cavity. We analytically determine the full coupled Hamiltonian for the nanoparticle, cavity, and free electromagnetic field. By tracing out the latter, we obtain a Master Equation for the cavity and the center of mass motion, where the decoherence rates ascribed to recoil heating, gas pressure, and trap displacement noise are calculated explicitly. Then, we benchmark our model by reproducing published experimental results for three-dimensional cooling. Finally, we use our model to demonstrate the possibility of ground-state cooling along each of the three motional axes. Our work illustrates the potential of cavity-assisted coherent scattering to reach the quantum regime of levitated nanomechanics.
Imaging-based detection of the motion of the levitated nanoparticles complements a widely-used interferometric detection method, providing a precise and robust way to estimate the position of the particle. Here, we show the camera-based feedback cooling of a charged nanoparticle levitated in a linear Paul trap. A charged nanoparticle levitated in a vacuum was observed by CMOS camera systems. The nanoparticle images were processed in realtime with a microcontroller integrated with a CMOS image sensor. The phase-delayed position signal was fed-back to one of the trap electrodes resulting in the …
Cooling the center-of-mass motion of levitated nanoparticles provides a route to quantum experiments at mesoscopic scales. Here we demonstrate three-dimensional sympathetic cooling and detection of the center-of-mass motion of a levitated silica nanoparticle. The nanoparticle is electrostatically coupled to a feedback-cooled particle while both particles are trapped in the same Paul trap. We identify two regimes, based on the strength of the cooling: in the first regime, the sympathetically cooled particle thermalizes with the directly cooled one, while in the second regime, the sympatheticall…
We experimentally study the interference of dipole scattered light from two optically levitated nanoparticles in vacuum, which present an environment free of particle-substrate interactions. We illuminate the two trapped nanoparticles with a linearly polarized probe beam orthogonal to the propagation of the trapping laser beams. The scattered light from the nanoparticles are collected by a high numerical aperture (NA) objective lens and imaged. The interference fringes from the scattered vector light for the different dipole orientations in image and Fourier space are observed. Especially, the…
Coherent scattering of photons is a novel mechanism of optomechanical coupling for optically levitated nanoparticles promising strong, versatile interactions with light and between nanoparticles. We show that it allows efficient deterministic generation of Gaussian entanglement between two particles in separate tweezers. A combination of red- and blue-detuned tweezers brings a mechanical Bogoliubov mode to its ground state. An additional, dispersively coupled cavity mode can reduce noise in the orthogonal mode, resulting in strong entanglement as quantified by the logarithmic negativity and ve…
Quantum measurements of mechanical systems can produce optical squeezing via ponderomotive forces. Its observation requires high environmental isolation and efficient detection, typically achieved by using optical cavities and cryogenic cooling. Here we realize these conditions by measuring the position of an optically levitated nanoparticle at room temperature and without the overhead of an optical cavity. We use a fast heterodyne detection to reconstruct simultaneously orthogonal optical quadratures, and observe a noise reduction of $9\%\pm0.5\%$ below shot noise. Our experiment offers a nov…
The field of levitodynamics has made significant progress towards controlling and studying the motion of a levitated nanoparticle. Motional control relies on either autonomous feedback via a cavity or measurement-based feedback via external forces. Recent demonstrations of measurement-based ground-state cooling of a single nanoparticle employ linear velocity feedback, also called cold damping, and require the use of electrostatic forces on charged particles via external electrodes. Here we introduce a novel all-optical cold damping scheme based on spatial modulation of the trap position that i…
We propose and theoretically analyze an experiment where displacement sensing of an optically levitated nanoparticle in front of a surface can be used to measure the induced dipole-dipole interaction between the nanoparticle and its thermal image. This is achieved by using a surface that is transparent to the trapping light but reflective to infrared radiation, with a reflectivity that can be time modulated. This dipole-dipole interaction relies on the thermal radiation emitted by a silica nanoparticle having sufficient temporal coherence to correlate the reflected radiation with the thermal f…
Inert shell coating for enhanced laser refrigeration of nanoparticles: application in levitated optomechanics
Sydney Quantum Academy（悉尼量子学院）；School of Mathematical and Physical Sciences, Macquarie University（麦考瑞大学数理科学学院）；ARC Centre of Excellence for Engineered Quantum Systems, Macquarie University（麦考瑞大学工程量子系统卓越研究中心）；School of Engineering, Macquarie University（麦考瑞大学工程学院）；ARC Centre for Nanoscale BioPhotonics, Macquarie University（麦考瑞大学纳米生物光子学中心）
All three motional modes of a charged dielectric nanoparticle in a Paul trap are cooled by direct feedback to temperatures of a few mK. We test two methods, one based on electrical forces and the other on optical forces; for both methods, we find similar cooling efficiencies. Cooling is characterized for both feedback forces as a function of feedback parameters, background pressure, and the particle's position.
Three-Dimensional and Selective Displacement Sensing of a Levitated Nanoparticle via Spatial Mode Decomposition
School of Mathematical and Physical Sciences, Macquarie University（麦考瑞大学数学与物理科学学院）；ARC Centre for Engineered Quantum Systems (EQUS), Macquarie University（麦考瑞大学ARC工程量子系统中心）；Sydney Quantum Academy（悉尼量子学院）；School of Physics, The University of Sydney（悉尼大学物理学院）
We experimentally observe the dipole scattering of a nanoparticle using a high numerical aperture (NA) imaging system. The optically levitated nanoparticle provides an environment free of particle-substrate interaction. We illuminate the silica nanoparticle in vacuum with a 532 nm laser beam orthogonally to the propagation direction of the 1064 nm trapping laser beam strongly focused by the same high NA objective used to collect the scattering, which results in a dark background and high signal-noise ratio. The dipole orientations of the nanoparticle induced by the linear polarization of the i…
We report an experimental observation of a record-breaking ultra-high rotation frequency about 6 GHz in an optically levitated nanoparticle system. We optically trap a nanoparticle in the gravity direction with a high numerical aperture (NA) objective lens, which shows significant advantages in compensating the influences of the scattering force and the photophoretic force on the trap, especially at intermediate pressure (about 100 Pa). This allows us to trap a nanoparticle from atmospheric to low pressure ($10^{-3}$ Pa) without using feedback cooling. We measure a highest rotation frequency a…
This chapter is intended as a pedagogical introduction to the dynamics of optically levitated nanoparticles with a focus on the study of single particle thermodynamics. Much of the work studying thermodynamics with nano- and micro-particles has taken place in liquid, and this chapter will avoid reviewing this impressive body of work, focussing instead on studies of thermodynamics with nanoparticles levitated in a gas. For a recent literature review we refer the reader to Gieseler & Millen Entropy 20, 326 (2018). The authors will discuss extensions into the quantum regime where relevant through…
Nanoparticles trapped in optical tweezers emerged as an interesting platform for investigating fundamental effects in quantum physics. The ability to shape the optical trapping potential using spatial light modulation and quantum control of their motion using coherent scattering to an optical cavity mode predispose them for emulating a range of physical systems and studying quantum phenomena with massive objects. To extend these capabilities of levitated nanoparticles to quantum many-body systems, it is crucial to develop feasible strategies to couple and entangle multiple particles either dir…
Interferometric methods for detecting the motion of a levitated nanoparticle provide a route to the quantum ground state, but such methods are currently limited by mode mismatch between the reference beam and the dipolar field scattered by the particle. Here we demonstrate a self-interference method to detect the particle's motion that solves this problem. A Paul trap confines a charged dielectric nanoparticle in high vacuum, and a mirror retro-reflects the scattered light. We measure the particle's motion with a sensitivity of $1.7\times 10^{-12} \text{m}/\sqrt{\text{Hz}}$, corresponding to a…
Preparing and observing quantum states of nanoscale particles is a challenging task with great relevance for quantum technologies and tests of fundamental physics. In contrast to atomic systems with discrete transitions, nanoparticles exhibit a practically continuous absorption spectrum and thus their quantum dynamics cannot be easily manipulated. Here, we demonstrate that charged nanoscale dielectrics can be artificially endowed with a discrete level structure by coherently interfacing their rotational and translational motion with a superconducting qubit. We propose a pulsed scheme for the g…
Feedback cooling of a levitated nanoparticle in a radially polarized vector beam trap
University College London（伦敦大学学院）；David Potter Institute for Quantum Information and Spacetime, University College London（伦敦大学学院戴维·波特量子信息与时空研究所）；Department of Physics and Astronomy, University College London（伦敦大学学院物理与天文学系）
Realizing a large-scale fully controllable quantum system is a challenging task in current physical research and has broad applications. Ultracold atom and molecule arrays in optical tweezers in vacuum have been used for quantum simulation, quantum metrology and quantum computing. Recently, quantum ground state cooling of the center-of-mass motion of a single optically levitated nanoparticle in vacuum was demonstrated, providing unprecedented opportunities for studying macroscopic quantum mechanics and precision measurements. In this work, we create a reconfigurable optically-levitated nanopar…
We propose to optimally control the harmonic potential of a levitated nanoparticle to quantum delocalize its center-of-mass motional state to a length scale orders of magnitude larger than the quantum zero-point motion. Using a bang-bang control of the harmonic potential, including the possibility to invert it, the initial ground-state-cooled levitated nanoparticle coherently expands to large scales and then contracts to the initial state in a time-optimal way. We show that this fast loop protocol can be used to enhance force sensing as well as to dramatically boost the entangling rate of two …
Time crystal is defined as a phase of matter spontaneously exhibiting a periodicity in time. Previous studies focused on discrete quantum time crystals under periodic drive. Here, we propose a time crystal model based on a levitated charged nanoparticle in a static magnetic field without drive. Both the classical time crystal in thermal equilibrium and the quantum time crystal in the ground state can emerge in the spin rotational mode, under the strong magnetic field or the large charge-to-mass ratio limit. Besides, for the first time, the \emph{time polycrystal} is defined and naturally appea…
A mechanically compliant element can be set into motion by the interaction with light. In turn, this light-driven motion can give rise to ponderomotive correlations in the electromagnetic field. In optomechanical systems, cavities are often employed to enhance these correlations up to the point where they generate quantum squeezing of light. In free-space scenarios, where no cavity is used, observation of squeezing remains possible but challenging due to the weakness of the interaction, and has not been reported so far. Here, we measure the ponderomotively squeezed state of light scattered by …
We report on measurements of photon induced heating of silica nanospheres levitated in vacuum by a thermal light source formed by a superluminescent diode. Heating of the nanospheres motion along the three trap axes was measured as a function of gas pressure and for two particle sizes. Heating rates were also compared with the much lower reheating of the same sphere when levitated by a laser. We find the measured trap heating rates are dominated by the much larger heating rates expected from the recoil of thermal photons.
