Optically levitated nonspherical particles in vacuum are excellent candidates for torque sensing, rotational quantum mechanics, high-frequency gravitational wave detection, and multiple other applications. Many potential applications, such as detecting the Casimir torque near a birefringent surface, require simultaneous cooling of both the center-of-mass motion and the torsional vibration (or rotation) of a nonspherical nanoparticle. Here we report the first 5D cooling of a levitated nanoparticle. We cool the 3 center-of-mass motion modes and 2 torsional vibration modes of a levitated nanodumbbell in a linearly-polarized laser simultaneously. The only uncooled rigid-body degree of freedom is the rotation of the nanodumbbell around its long axis. This free rotation mode does not couple to the optical tweezers directly. Surprisingly, we observe that it strongly affects the torsional vibrations of the nanodumbbell. This work deepens our understanding of the nonlinear dynamics and rotation coupling of a levitated nanoparticle and paves the way towards full quantum control of its motion.
Levitated optomechanics has great potentials in precision measurements, thermodynamics, macroscopic quantum mechanics and quantum sensing. Here we synthesize and optically levitate silica nanodumbbells in high vacuum. With a linearly polarized laser, we observe the torsional vibration of an optically levitated nanodumbbell in vacuum. The linearly-polarized optical tweezer provides a restoring torque to confine the orientation of the nanodumbbell, in analog to the torsion wire which provides restoring torque for suspended lead spheres in the Cavendish torsion balance. Our calculation shows its …
According to quantum theory, measurement and backaction are inextricably linked. In optical position measurements, this backaction is known as radiation pressure shot noise. In analogy, a measurement of the orientation of a mechanical rotor must disturb its angular momentum by radiation torque shot noise. In this work, we observe the shot-noise torque fluctuations arising in a measurement of the angular orientation of an optically levitated nanodumbbell. We feedback cool the dumbbell's rotational motion and investigate its reheating behavior when released from feedback. In high vacuum, the hea…
We theoretically investigate the rigid body dynamics of an optically levitated nanodumbbell under parametric feedback cooling and provide a simplified model for describing the motion. Differing from previous studies, the spin of the nanoparticle about its symmetry axis is considered non-negligible. Simulations reveal that standard parametric feedback cooling can extract energy from two of the five rotational degrees of freedom when the nanoparticle is levitated using a linearly polarized laser beam. The dynamics after feedback cooling are characterized by a normal mode describing precession ab…
Levitated optomechanics is showing potential for precise force measurements. Here, we report a case study, to show experimentally the capacity of such a force sensor. Using an electric field as a tool to detect a Coulomb force applied onto a levitated nanosphere. We experimentally observe the spatial displacement of up to 6.6 nm of the levitated nanosphere by imposing a DC field. We further apply an AC field and demonstrate resonant enhancement of force sensing when a driving frequency, $ω_{AC}$, and the frequency of the levitated mechanical oscillator, $ω_0$, converge. We directly measure a f…
The linear momentum and angular momentum of virtual photons of quantum vacuum fluctuations can induce the Casimir force and the Casimir torque, respectively. While the Casimir force has been measured extensively, the Casimir torque has not been observed experimentally though it was predicted over forty years ago. Here we propose to detect the Casimir torque with an optically levitated nanorod near a birefringent plate in vacuum. The axis of the nanorod tends to align with the polarization direction of the linearly polarized optical tweezer. When its axis is not parallel or perpendicular to the…
Optically levitated nanoparticles have recently emerged as versatile platforms for investigating macroscopic quantum mechanics and enabling ultrasensitive metrology. In this article we theoretically consider two damping regimes of an optically levitated nanoparticle cooled by cavityless parametric feedback. Our treatment is based on a generalized Fokker-Planck equation derived from the quantum master equation presented recently and shown to agree very well with experiment [1]. For low damping, we find that the resulting Wigner function yields the single-peaked oscillator position distribution …
We experimentally study the interference of dipole scattered light from two optically levitated nanoparticles in vacuum, which present an environment free of particle-substrate interactions. We illuminate the two trapped nanoparticles with a linearly polarized probe beam orthogonal to the propagation of the trapping laser beams. The scattered light from the nanoparticles are collected by a high numerical aperture (NA) objective lens and imaged. The interference fringes from the scattered vector light for the different dipole orientations in image and Fourier space are observed. Especially, the…
We present the first evidence of nitrogen vacancy (NV) photoluminescence from a nanodiamond suspended in a free-space optical dipole trap at atmospheric pressure. The photoluminescence rates are shown to decrease with increasing trap laser power, but are inconsistent with a thermal quenching process. For a continuous-wave trap, the neutral charge state (NV$^0$) appears to be suppressed. Chopping the trap laser yields higher total count rates and results in a mixture of both NV$^0$ and the negative charge state (NV$^-$).
Optically levitated rotors are prime candidates for torque sensors whose precision is limited by the fluctuationsof the rotation frequency. In this work we investigate an optically levitated rotor at its fundamental thermal limitof frequency stability, where rotation-frequency fluctuations arise solely due to coupling to the thermal bath.
We implement a cold damping scheme to cool one mode of the center-of-mass motion of an optically levitated nanoparticle in ultrahigh vacuum from room temperature to a record-low temperature of 100 micro-Kelvin. The measured temperature dependence on feedback gain and thermal decoherence rate is in excellent agreement with a parameter-free model. We determine the imprecision-backaction product for our system and provide a roadmap towards ground-state cooling of optically levitated nanoparticles.
Optically levitated nanoparticles in vacuum are a promising model system to test physics beyond our current understanding of quantum mechanics. Such experimental tests require extreme control over the dephasing of the levitated particle's motion. If the nanoparticle carries a finite net charge, it experiences a random Coulomb force due to fluctuating electric fields. This dephasing mechanism can be fully excluded by discharging the levitated particle. Here, we present a simple and reliable technique to control the charge on an optically levitated nanoparticle in vacuum. Our method is based on …
Electron spins of diamond nitrogen-vacancy (NV) centers are important quantum resources for nanoscale sensing and quantum information. Combining NV spins with levitated optomechanical resonators will provide a hybrid quantum system for novel applications. Here we optically levitate a nanodiamond and demonstrate electron spin control of its built-in NV centers in low vacuum. We observe that the strength of electron spin resonance (ESR) is enhanced when the air pressure is reduced. To better understand this system, we investigate the effects of trap power and measure the absolute internal temper…
We review recent works on optomechanics of optically trapped microspheres and nanoparticles in vacuum, which provide an ideal system for studying macroscopic quantum mechanics and ultrasensitive force detection. An optically trapped particle in vacuum has an ultrahigh mechanical quality factor as it is well-isolated from the thermal environment. Its oscillation frequency can be tuned in real time by changing the power of the trapping laser. Furthermore, an optically trapped particle in vacuum may rotate freely, a unique property that does not exist in clamped mechanical oscillators. In this re…
Optomechanical systems are suitable for elucidating quantum phenomena at the macroscopic scale in the sense of the mass scale. The systems should be well-isolated from the environment to avoid classical noises, which conceal quantum signals. Optical levitation is a promising way to isolate optomechanical systems from the environment. To realize optical levitation, all degrees of freedom need to be trapped. Until now, longitudinal trapping and rotational trapping of a mirror with optical radiation pressure have been studied in detail and validated with various experiments. However, less attenti…
The ability to trap and to manipulate individual atoms is at the heart of current implementations of quantum simulations, quantum computing, and long-distance quantum communication. Controlling the motion of larger particles opens up yet new avenues for quantum science, both for the study of fundamental quantum phenomena in the context of matter wave interference, and for new sensing and transduction applications in the context of quantum optomechanics. Specifically, it has been suggested that cavity cooling of a single nanoparticle in high vacuum allows for the generation of quantum states of…
We demonstrate that a Kalman filter applied to estimate the position of an optically levitated nanoparticle, and operated in real-time within a Field Programmable Gate Array (FPGA), is sufficient to perform closed-loop parametric feedback cooling of the centre of mass motion to sub-Kelvin temperatures. The translational centre of mass motion along the optical axis of the trapped nanoparticle has been cooled by three orders of magnitude, from a temperature of 300K to a temperature of 162 +/- 15mK.
We report an experimental observation of a record-breaking ultra-high rotation frequency about 6 GHz in an optically levitated nanoparticle system. We optically trap a nanoparticle in the gravity direction with a high numerical aperture (NA) objective lens, which shows significant advantages in compensating the influences of the scattering force and the photophoretic force on the trap, especially at intermediate pressure (about 100 Pa). This allows us to trap a nanoparticle from atmospheric to low pressure ($10^{-3}$ Pa) without using feedback cooling. We measure a highest rotation frequency a…
Torque sensors such as the torsion balance enabled the first determination of the gravitational constant by Cavendish and the discovery of Coulomb's law. Torque sensors are also widely used in studying small-scale magnetism, the Casimir effect, and other applications. Great effort has been made to improve the torque detection sensitivity by nanofabrication and cryogenic cooling. The most sensitive nanofabricated torque sensor has achieved a remarkable sensitivity of $10^{-24} \rm{Nm}/\sqrt{\rm{Hz}}$ at millikelvin temperatures in a dilution refrigerator. Here we dramatically improve the torque…
We propose and theoretically analyze an experiment where displacement sensing of an optically levitated nanoparticle in front of a surface can be used to measure the induced dipole-dipole interaction between the nanoparticle and its thermal image. This is achieved by using a surface that is transparent to the trapping light but reflective to infrared radiation, with a reflectivity that can be time modulated. This dipole-dipole interaction relies on the thermal radiation emitted by a silica nanoparticle having sufficient temporal coherence to correlate the reflected radiation with the thermal f…
A nitrogen-vacancy (NV$^-$) center in a nanodiamond, levitated in high vacuum, has recently been proposed as a probe for demonstrating mesoscopic center-of-mass superpositions \cite{Scala2013, Zhang2013} and for testing quantum gravity \cite{Albrecht2014}. Here, we study the behavior of optically levitated nanodiamonds containing NV$^-$ centers at sub-atmospheric pressures and show that while they burn in air, this can be prevented by replacing the air with nitrogen. However, in nitrogen the nanodiamonds graphitize below $\approx 10$ mB. Exploiting the Brownian motion of a levitated nanodiamon…
This paper demonstrates cooling of the center-of-mass motion of 10 $μ$m-diameter optically levitated silica spheres to an effective temperature of $50\pm22 μ$K, achieved by minimizing the technical pointing noise of the trapping laser. This low noise leads to an acceleration and force sensitivity of $95\pm41$ n$g/\sqrt{\mathrm{Hz}}$ ($g = 9.8$ m/s$^2$) and $0.95\pm0.11$ aN$/\sqrt{\mathrm{Hz}}$, respectively, at frequencies near 50 Hz. This force sensitivity is comparable to that demonstrated for optically levitated nanospheres that are $10^4$ times less massive, corresponding to an acceleratio…
We experimentally observe the dipole scattering of a nanoparticle using a high numerical aperture (NA) imaging system. The optically levitated nanoparticle provides an environment free of particle-substrate interaction. We illuminate the silica nanoparticle in vacuum with a 532 nm laser beam orthogonally to the propagation direction of the 1064 nm trapping laser beam strongly focused by the same high NA objective used to collect the scattering, which results in a dark background and high signal-noise ratio. The dipole orientations of the nanoparticle induced by the linear polarization of the i…
The center-of-mass motion of a single optically levitated nanoparticle resembles three uncoupled harmonic oscillators. We show how a suitable modulation of the optical trapping potential can give rise to a coupling between two of these oscillators, such that their dynamics are governed by a classical equation of motion that resembles the Schrödinger equation for a two-level system. Based on experimental data, we illustrate the dynamics of this parametrically coupled system both in the frequency and in the time domain. We discuss the limitations and differences of the mechanical analogue in com…
We describe a variety of searches for new physics beyond the Standard Model of particle physics which may be enabled in the coming years by the use of optically levitated masses in high vacuum. Such systems are expected to reach force and acceleration sensitivities approaching (and possibly eventually exceeding) the standard quantum limit over the next decade. For new forces or phenomena that couple to mass, high precision sensing using objects with masses in the fg-ng range have significant discovery potential for new physics. Such applications include tests of fundamental force laws, searche…
The hallmark of quantum physics is Planck's constant $h$, whose finite value entails the quantization that gave the theory its name. The finite value of $h$ gives rise to inevitable zero-point fluctuations even at vanishing temperature. The zero-point fluctuation of mechanical motion becomes smaller with growing mass of an object, making it challenging to observe at macroscopic scales. Here, we transition a dielectric particle with a diameter of 136 nm from the classical realm to the regime where its zero-point motion emerges as a sizeable contribution to its energy. To this end, we optically …
Quantum measurements of mechanical systems can produce optical squeezing via ponderomotive forces. Its observation requires high environmental isolation and efficient detection, typically achieved by using optical cavities and cryogenic cooling. Here we realize these conditions by measuring the position of an optically levitated nanoparticle at room temperature and without the overhead of an optical cavity. We use a fast heterodyne detection to reconstruct simultaneously orthogonal optical quadratures, and observe a noise reduction of $9\%\pm0.5\%$ below shot noise. Our experiment offers a nov…
Coherent scattering of photons is a novel mechanism of optomechanical coupling for optically levitated nanoparticles promising strong, versatile interactions with light and between nanoparticles. We show that it allows efficient deterministic generation of Gaussian entanglement between two particles in separate tweezers. A combination of red- and blue-detuned tweezers brings a mechanical Bogoliubov mode to its ground state. An additional, dispersively coupled cavity mode can reduce noise in the orthogonal mode, resulting in strong entanglement as quantified by the logarithmic negativity and ve…
We report results from a search for stable particles with charge > $10^{-5}$ e in bulk matter using levitated dielectric microspheres in high vacuum. No evidence for such particles was found in a total sample of 1.4 ng, providing an upper limit on the abundance per nucleon of 2.5 x $10^{-14}$ at the 95% confidence level for the material tested. These results provide the first direct search for single particles with charge < 0.1 e bound in macroscopic quantities of matter and demonstrate the ability to perform sensitive force measurements using optically levitated microspheres in vacuum.
Optically levitated nanoparticles offer enormous potential for precision sensing. However, as for any other metrology device, the absolute measurement performance of a levitated-particle sensor is limited by the accuracy of the calibration relating the measured signal to an absolute displacement of the particle. Here, we suggest and demonstrate calibration protocols for levitated-nanoparticle sensors. Our calibration procedures include the treatment of anharmonicities in the trapping potential, as well as a protocol using a harmonic driving force, which is applicable if the sensor is coupled t…
We explore, experimentally and theoretically, the emergence of coherent coupled oscillations and synchronization between a pair of non-Hermitian, stochastic, opto-mechanical oscillators, levitated in vacuum. Each oscillator consists of a polystyrene microsphere trapped in a circularly polarized, counter-propagating Gaussian laser beam. Non-conservative, azimuthal forces, deriving from inhomogeneous optical spin, push the micro-particles out of thermodynamic equilibrium. For modest optical powers each particle shows a tendency towards orbital circulation. Initially, their stochastic motion is w…
Quantum control of levitated dielectric particles is an emerging subject in quantum optomechanics. A major challenge is to efficiently measure and manipulate the particle's motion at the Heisenberg uncertainty limit. Here we present a nanophotonic interface suited to address this problem. By optically trapping a 150 nm silica particle and placing it in the near field of a photonic crystal cavity, we achieve tunable single-photon optomechanical coupling of up to $g_0/2π=9$ kHz, three orders of magnitude larger than previously reported for levitated cavity optomechanical systems. Efficient colle…
An optically levitated nanoparticle in vacuum is a paradigm optomechanical system for sensing and studying macroscopic quantum mechanics. While its center-of-mass motion has been investigated intensively, its torsional vibration has only been studied theoretically in limited cases. Here we report the first experimental observation of the torsional vibration of an optically levitated nonspherical nanoparticle in vacuum. We achieve this by utilizing the coupling between the spin angular momentum of photons and the torsional vibration of a nonspherical nanoparticle whose polarizability is a tenso…
We report on the electrically driven rotation of $2.4~μ$m-radius, optically levitated dielectric microspheres. Electric fields are used to apply torques to a microsphere's permanent electric dipole moment, while angular displacement is measured by detecting the change in polarization state of light transmitted through the microsphere (MS). This technique enables greater control than previously achieved with purely optical means because the direction and magnitude of the electric torque can be set arbitrarily. We measure the spin-down of a microsphere released from a rotating electric field, th…
Nano-mechanical resonators have gained an increasing importance in nanotechnology owing to their contributions to both fundamental and applied science. Yet, their small dimensions and mass raises some challenges as their dynamics gets dominated by nonlinearities that degrade their performance, for instance in sensing applications. Here, we report on the precise control of the nonlinear and stochastic bistable dynamics of a levitated nanoparticle in high vacuum. We demonstrate how it can lead to efficient signal amplification schemes, including stochastic resonance. This work paves the way for …
Position measurement of a levitated particle with vectorial light
Pontifical Catholic University of Rio de Janeiro（里约热内卢天主教大学）；Universidade Federal do Rio de Janeiro（里约热内卢联邦大学）；Tecnológico de Monterrey（蒙特雷理工学院）；University of Southampton（南安普顿大学）
Forces and torques exerted on dielectric disks trapped in a Gaussian standing wave are analyzed theoretically for disks of radius $2~μ\text{m}$ with index of refraction $n=1.45$ and $n=2.0$ as well as disks of radius 200 nm with $n=1.45$. Calculations of the forces and torques were conducted both analytically and numerically using a discrete-dipole approximation method. Besides harmonic terms, third order ro-translational coupling terms in the potential energy can be significant and a necessary consideration when describing the dynamics of disks outside of the Rayleigh limit. The coupling term…
We report on the injection locking of an optically levitated nanomechanical oscillator (a silica nanosphere) to resonant intensity modulations of an external optical signal. We explore the characteristic features of injection locking in this system, e.g. the phase pull-in effect and the injection-induced reduction of the oscillation linewidth. Our measurements are in good agreement with theoretical predictions and deepen the analogy of injection locking in levitated optomechanical systems to that in optical systems (lasers). By measuring the force noise of our feedback cooled free-running osci…
We report on the use of 4.7-$μ$m-diameter, optically levitated, charged microspheres to image the three-dimensional force field produced by charge distributions on an Au-coated, microfabricated Si beam in vacuum. An upward-propagating, single-beam optical trap, combined with an interferometric imaging technique, provides optimal access to the microspheres for microscopy. In this demonstration, the Au-coated surface of the Si beam can be brought as close as ${\sim}10~μ$m from the center of the microsphere while forces are simultaneously measured along all three orthogonal axes, fully mapping th…
Nanomechanical resonator based on levitated particle exhibits unique advantages in the development of ultrasensitive electric field detector. We demonstrate a three-dimensional, high-sensitivity electric field measurement technology using the optically levitated nanoparticle with a known net charge. By changing the relative position between nanoparticle and parallel electrodes, the three-dimensional electric field distribution is scanned. The measured noise equivalent electric intensity with charge amount of 100 reaches the order of {\rm{1μV/cm/H}}{\rm{z}^{\rm{1/2}}} at 1.4 \times {10^{ - 7}}m…
