Quantum transport is often characterized not just by mean observables like the particle or energy current, but by their fluctuations and higher moments, which can act as detailed probes of the physical mechanisms at play. However, relatively few theoretical methods are able to access the full counting statistics (FCS) of transport processes through electronic junctions in strongly correlated regimes. While most experiments are concerned with the steady state properties, most accurate theoretical methods rely on computationally expensive propagation from a tractable initial state. Here, we propose a simple approach for computing the FCS through a junction directly at the steady state, utilizing the propagator noncrossing approximation (NCA). Compared to time propagation, our method offers reduced computational cost at the same level of approximation; but the idea can also be used within other approximations or as a basis for numerically exact techniques. We demonstrate the method's capabilities by investigating the impact of lead dimensionality on electronic transport in the nonequilibrium Anderson impurity model at the onset of Kondo physics. Our results reveal a distinct signature of one dimensional leads in the noise and Fano factor not present for other dimensionalities, showing the potential of FCS measurements as a probe of the environment surrounding a quantum dot.
We present a method for calculating the full counting statistics of a nonequilibrium quantum system based on the propagator noncrossing approximation (NCA). This numerically inexpensive method can provide higher order cumulants for extended parameter regimes, rendering it attractive for a wide variety of purposes. We compare NCA results to Born-Markov quantum master equations (QME) results to show that they can access different physics, and to numerically exact inchworm quantum Monte-Carlo data to assess their validity. As a demonstration of its power, the NCA method is employed to study the i…
Using the Schwinger-Keldysh approach and the drone (Majorana) fermion representation, we evaluate current distribution in a single-electron transistor in a regime where a total tunnel resistance is small. Nonequilibrium quantum fluctuations of charge induce a lifetime broadening of charge-state level, as well as renormalization of system parameters. We find that the lifetime broadening effect may suppress the probability of relatively large current.
The time dependent full counting statistics of charge transport through an interacting quantum junction is evaluated from its generating function, controllably computed with the inchworm Monte Carlo method. Exact noninteracting results are reproduced; then, we continue to explore the effect of electron--electron interactions on the time-dependent charge cumulants, first-passage time distributions and $n$-electron transfer distributions. We observe a crossover in the noise from Coulomb blockade- to Kondo-dominated physics as the temperature is decreased. In addition, we uncover long-tailed spin…
We study theoretically the current-voltage characteristics, shot noise, and full counting statistics of a quantum wire double barrier structure. We model each wire segment by a spinless Luttinger liquid. Within the sequential tunneling approach, we describe the system's dynamics using a master equation. We show that at finite bias the non-equilibrium distribution of plasmons in the central wire segment leads to increased average current, enhanced shot noise, and full counting statistics corresponding to a super-Poissonian process. These effects are particularly pronounced in the strong interac…
To study the full counting statistics of quantum heat transfer in a driven nonequilibrium spin-boson model, we develop a generalized nonequilibrium polaron-transformed Redfield equation with an auxiliary counting field. This enables us to study the impact of qubit-bath coupling ranging from weak to strong regimes. Without external modulations, we observe maximal values of both steady state heat flux and noise power at moderate coupling regimes, below which we find those two transport quantities are enhanced by the finite qubit energy bias. With external modulations, the geometric-phase-induced…
We evaluate the current distribution for a single-electron transistor with intermediate strength tunnel conductance. Using the Schwinger-Keldysh approach and the drone (Majorana) fermion representation we account for the renormalization of system parameters. Nonequilibrium effects induce a lifetime broadening of the charge-state levels, which suppress large current fluctuations.
We investigate the rectification and negative differential effects of full-counting statistics of conjugate thermal spin transport in a spin Seebeck engine. The engine is made by an electron/magnon interface diode driven by a temperature bias, of which the scaled cumulant generating function is formulated in the framework of nonequilibrium Green's function. The strongly fluctuating interfacial electron density of states induced by quantum dot is responsible for these intriguing properties. This work is relevant for designing efficient spin caloritronic engine and can broaden our view in nonequ…
The coupling of the charge carriers passing through a molecule bridging two bulky conductors with local vibrational modes of the molecule, gives rise to distinct features in the electronic transport properties on one hand, and to nonequilibrium features in the vibrations' properties, e.g., their population, on the other. Here we explore theoretically a generic model for a molecular junction biased by an arbitrary dc voltage in the weak-coupling regime. We analyze the signature of the electron-vibration interaction on the full-counting statistics of the current fluctuations (i.e., the cumulant …
Time-dependent driving influences the quantum and thermodynamic fluctuations of a system, changing the familiar physical picture of electronic noise which is an important source of information the about microscopic mechanism of quantum transport. Giving access to all cumulants of the current, the full counting statistics (FCS) is the powerful theoretical method to study fluctuations in nonequilibrium quantum systems. In this paper, we propose the application of FCS to consider periodic driven junctions. The combination of Floquet theory for time dynamics and nonequilibrium counting-field Green…
We develop and test a computational framework to study heat exchange in interacting, nonequilibrium open quantum systems. Our iterative full counting statistics path integral (iFCSPI) approach extends a previously well-established influence functional path integral method, by going beyond reduced system dynamics to provide the cumulant generating function of heat exchange. The method is straightforward; we implement it for the nonequilibrium spin boson model to calculate transient and long-time observables, focusing on the steady-state heat current flowing through the system under a temperatur…
We report the investigation of full-counting statistics (FCS) of transferred charge and spin in the transient regime where the connection between central scattering region (quantum dot) and leads are turned on at $t=0$. A general theoretical formulation for the generating function (GF) is presented using a nonequilibrium Green's function approach for the quantum dot system. In particular, we give a detailed derivation on how to use the method of path integral together with nonequilibrium Green's function technique to obtain the GF of FCS in electron transport systems based on the two-time quan…
We study the full counting statistics (FCS) of electron tunneling through a multi-terminal quantum dot in the Kondo regime within the slave-boson mean field theory. By employing the A.O. Gogolin and A. Komnik's method of calculating the FCS generating function based on the nonequilibrium Green's function [Phys. Rev. B {\bf 73}, 195301 (2006)], we obtain the counting field $λ$-dependent self-consistent equations for the mean values of the slave-boson fields and the explicit expression for the derivative of the adiabatic potential of the system with respect to the counting fields. Performing per…
We develop a general approach to nonequilibrium nanostructures formed by one-dimensional channels coupled by tunnel junctions and/or by impurity scattering. The formalism is based on nonequilibrium version of functional bosonization. A central role in this approach is played by the Keldysh action that has a form reminiscent of the theory of full counting statistics. To proceed with evaluation of physical observables, we assume the weak-tunneling regime and develop a real-time instanton method. A detailed exposition of the formalism is supplemented by two important applications: (i) tunneling i…
We present a theory of modified reduced dynamics in the presence of counting fields. Reduced dynamics techniques are useful for describing open quantum systems at long emergent timescales when the memory timescales are short. However, they can be difficult to formulate for observables spanning the system and its environment, such as those characterizing transport properties. A large variety of mixed system--environment observables, as well as their statistical properties, can be evaluated by considering counting fields. Given a numerical method able to simulate the field-modified dynamics over…
We present a hierarchical quantum master equation (HQME) approach, which allows the numerically exact evaluation of higher-order current cumulants in the framework of full counting statistics for nonequilibrium charge transport in nanosystems. The novel methodology is exemplarily applied to a model of vibrationally coupled electron transport in a molecular nanojunction. We investigate the influence of cotunneling on avalanche-like transport, in particular in the nonresonant transport regime, where we find that inelastic cotunneling acts as trigger process for resonant avalanches. In this regim…
We analyze the nonequilibrium transport properties of a parallel double quantum dot in terms of its full counting statistics (FCS). The parameters of the setup are assumed to be such that both subsystems are driven into the Kondo regime. After a series of transformations the Hamiltonian is then mapped onto a Majorana resonant level model, which effectively describes the Toulouse point of the respective double impurity two-terminal Kondo model. Its FCS is then obtained at arbitrary constellation of voltage, temperature, and local magnetic fields. We identify two different transport processes co…
We investigate nonequilibrium energy transfer in a single-site Bose-Hubbard model coupled to two thermal baths. By including a quantum kinetic equation combined with full counting statistics, we investigate the steady state energy flux and noise power. The influence of the nonlinear Bose-Hubbard interaction on the transfer behaviors is analyzed, and the nonmonotonic features are clearly exhibited. Particularly, in the strong on-site repulsion limit, the results become identical with the nonequilibrium spin-boson model. We also extend the quantum kinetic equation to study the geometric-phase-in…
We investigate the quantum thermal transistor effect in nonequilibrium three-level systems by applying the polaron transformed Redfield equation combined with full counting statistics. The steady state heat currents are obtained via this unified approach over a wide region of system-bath coupling, and can be analytically reduced to the Redfield and nonequilibrium noninteracting blip approximation results in the weak and strong coupling limits, respectively. A giant heat amplification phenomenon emerges in the strong system-bath coupling limit, where transitions mediated by the middle thermal b…
Nonequilibrium Green's functions provide a powerful tool for computing the dynamical response and particle exchange statistics of coupled quantum systems. We formulate the theory in terms of the density matrix in Liouville space and introduce superoperator algebra that greatly simplifies the derivation and the physical interpretation of all quantities. Expressions for various observables are derived directly in real time in terms of superoperator nonequilibrium Green's functions (SNGF), rather than the artificial time-loop required in Schwinger's Hilbert-space formulation. Applications for com…
We investigate theoretically and experimentally the full counting statistics of bidirectional single-electron tunneling through a double quantum dot in a GaAs/GaAlAs heterostructure and compare with predictions of the fluctuation theorem (FT) for Markovian stochastic processes. We observe that the quantum point contact electrometer used to study the transport induces nonequilibrium shot noise and dot-level fluctuations and strongly modifies the tunneling statistics. As a result, the FT appears to be violated. We show that it is satisfied if the back-action of the electrometer is taken into acc…
We apply a recently developed 1/(N-1) expansion to the full counting statistics for the N-fold degenerate Anderson impurity model in the Kondo regime. This approach is based on the perturbation theory in the Coulomb interaction U and is different from the conventional large N theories, such as the usual 1/N expansion and non-crossing approximation. We have confirmed that the calculations carried out up to order 1/(N-1)^2 agree closely with those of the numerical renormalization group at N=4, where the degeneracy is still not so large. This ensures the applicability of our approach for N>4. We …
We investigate the full counting statistics of a single quantum dot strongly coupled to a local phonon and weakly tunnel-connected to two metallic electrodes. By employing the generalized nonequilibrium Green function method and the Lang-Firsov transformation, we derive an explicit analytical formula for the cumulant generating function, which makes one to be able to identify distinctly the elastic and inelastic contributions to the current and zero-frequency shot noise. We find that at zero temperature, the inelastic effect causes upward steps in the current and downward jumps in the noise at…
We analyze the effects of a distortion of the nuclear potential of a molecular quantum dot (QD), as well as a shift of its equilibrium position, on nonequilibrium-vibration-assisted tunneling through the QD with a single level ($ε_d$) coupled to the vibrational mode. For this purpose, we derive an explicit analytical expression for the Franck-Condon (FC) factor for a displaced-distorted oscillator surface of the molecule and establish rate equations in the joint electron-phonon representation to examine the current-voltage characteristics and zero-frequency shot noise, and skewness as well. Ou…
We review connections between the cumulant generating function of full counting statistics of particle number and the Rényi entanglement entropy. We calculate these quantities based on the fermionic and bosonic path-integral defined on multiple Keldysh contours. We relate the Rényi entropy with the information generating function, from which the probability distribution function of self-information is obtained in the nonequilibrium steady state. By exploiting the distribution, we analyze the information content carried by a single bosonic particle through a narrow-band quantum communication ch…
Full counting statistics of electron transport is a powerful diagnostic tool for probing the nature of quantum transport beyond what is obtainable from the average current or conductance measurement alone. In particular, the non-Markovian dynamics of quantum dot molecule plays an important role in the nonequilibrium electron tunneling processes. It is thus necessary to understand the non-Markovian full counting statistics in a quantum dot molecule. Here we study the non-Markovian full counting statistics in two typical quantum dot molecules, namely, serially coupled and side-coupled double qua…
Phase transitions occur in a wide range of physical systems and are characterized by the abrupt change of a physical observable in response to the variation of an external control parameter. Phase transitions are not restricted to equilibrium situations but can also be found in nonequilibrium settings, both for classical and quantum mechanical systems. Here, we investigate a nonequilibrium phase transition in a single-electron micromaser consisting of a microwave cavity that is driven by the electron transport in a double quantum dot. For weak electron-photon couplings, only a tiny fraction of…
This review deals with the nonequilibrium Green's function (NEGF) method applied to the problems of energy transport due to atomic vibrations (phonons), primarily for small junction systems. We present a pedagogical introduction to the subject, deriving some of the well-known results such as the Laudauer-like formula for heat current in ballistic systems. The main aim of the review is to build the machinery of the method so that it can be applied to other situations, which are not directly treated here. In addition to the above, we consider a number of applications of NEGF, not in routine mode…
We study the full-counting statistics of charges transmitted through a single-level quantum dot weakly coupled to a local Einstein phonon which causes fluctuations in the dot energy. An analytic expression for the cumulant generating function, accurate up to second order in the electron-phonon coupling and valid for finite voltages and temperatures, is obtained in the extended wide-band limit. The result accounts for nonequilibrium phonon distributions induced by the source-drain bias voltage, and concomitantly satisfies the fluctuation theorem. Extending the counting field to the complex plan…
We present a method, based on characterizing efficiency fluctuations, to asses the performance of nanoscale thermoelectric junctions. This method accounts for effects typically arising in small junctions, namely, stochasticity in the junction's performance, quantum effects, and nonequilibrium features preventing a linear response analysis. It is based on a nonequilibrium Green's function (NEGF) approach, which we use to derive the full counting statistics (FCS) for heat and work, and which in turn allows us to calculate the statistical properties of efficiency fluctuations. We simulate the lat…
We present a theoretical investigation for the full counting statistics of the Andreev tunneling through a quantum dot (QD) embedded between superconducting (SC) and normal leads in the presence of a strong on-site electron-phonon interaction using nonequilibrium Green function method. For this purpose, we generalize the dressed tunneling approximation (DTA) recently developed in dealing with inelastic tunneling in a normal QD system to the Andreev transport issue, which takes account of vibrational effect in evaluation of electronic tunneling self energy in comparison with other simple approa…
We investigate the full-counting statistics (FCS) of energy transport carried by electrons in molecular junctions for the Anderson-Holstein model in the polaronic regime. Using two-time quantum measurement scheme, generating function (GF) for the energy transport is derived and expressed as a Fredholm determinant in terms of Keldysh nonequilibrium Green's function in the time domain. Dressed tunneling approximation is used in decoupling the phonon cloud operator in the polaronic regime. This formalism enables us to analyze the time evolution of energy transport dynamics after a sudden switch-o…
We present a nonperturbative and formally exact approach for the charge transport in interacting nanojunctions based on a real time path integral formulation of the reduced system dynamics. An expansion of the influence functional in terms of the number of tunneling transitions, and integration of the Grassmann variables between the tunneling times, allows us to obtain a still exact generalized master equation (GME) for the populations of the reduced density matrix (RDM) in the occupation number representation, as well as a formally exact expression for the current. By borrowing the nomenclatu…
We propose to investigate the full counting statistics of nonequilibrium spin transport with an ultracold atomic quantum gas. The setup makes use of the spin control available in atomic systems to generate spin transport induced by an impurity atom immersed in a spin-imbalanced two-component Fermi gas. In contrast to solid-state realizations, in ultracold atoms spin relaxation and the decoherence from external sources is largely suppressed. As a consequence, once the spin current is turned off by manipulating the internal spin degrees of freedom of the Fermi system, the nonequilibrium spin pop…
We analyze the nonequilibrium transport properties of a quantum dot with a harmonic degree of freedom (Holstein phonon) coupled to metallic leads, and derive its full counting statistics (FCS). Using the Lang-Firsov (polaron) transformation, we construct a diagrammatic scheme to calculate the cumulant generating function. The electron-phonon interaction is taken into account exactly, and the employed approximation represents a summation of a diagram subset with respect to the tunneling amplitude. By comparison to Monte Carlo data the formalism is shown to capture the basic properties of the st…
Entanglement plays a prominent role in the study of condensed matter many-body systems: Entanglement measures not only quantify the possible use of these systems in quantum information protocols, but also shed light on their physics. However, exact analytical results remain scarce, especially for systems out of equilibrium. In this work we examine a paradigmatic one-dimensional fermionic system that consists of a uniform tight-binding chain with an arbitrary scattering region near its center, which is subject to a DC bias voltage at zero temperature. The system is thus held in a current-carryi…
For open systems described by the quantum master equation (QME), we investigate the excess entropy production under quasistatic operations between nonequilibrium steady states. The average entropy production is composed of the time integral of the instantaneous steady entropy production rate and the excess entropy production. We propose to define average entropy production rate using the average energy and particle currents, which are calculated by using the full counting statistics with QME. The excess entropy production is given by a line integral in the control parameter space and its integ…
In this thesis, we considered quantum systems coupled to several baths. We supposed that the system state is governed by the quantum master equation (QME). We investigated the quantum pump and the excess entropy production. In the first half of the thesis, we investigated the quantum pump using the full counting statistics with quantum master equation (FCS-QME) approach. In the latter part of the thesis, we investigated the excess entropy production. The average entropy production is composed of the time integral of the instantaneous steady entropy production rate and the excess entropy produc…
A theoretical study is reported of electron transport at finite temperature in a double quantum dot (DQD) capacitively coupled to a quantum point contact (QPC). Starting from a Hamiltonian model, a master equation is obtained for the stochastic process taking place in the DQD while the QPC is at or away from equilibrium, allowing us to study the backaction of the QPC onto the DQD. The QPC is treated non-perturbatively in our analysis. Effective fluctuation theorems are established for the full counting statistics of the DQD current under different limiting conditions. These fluctuation theorem…
A full quantum theory beyond the mean-field regime is developed for an exciton polariton condensate, to gain a complete understanding of quantum fluctuations. We find analytical solution for the polariton density matrix, showing the polariton nonlinearity causing fast relaxation correlated with the pump so as to yield the condensation at threshold. Increasing the pump intensity, a nonequilibrium phase transition towards the condensation of lower polaritons emerges, with a statistics transiting from a thermal, through a super-Poissonian and to a nonclassical distribution beyond the understandin…
We study the statistical properties of currents in two particular systems of capacitively coupled parallel transport channels. In the first system, each transport channel contains a single quantum dot in contact with two electron reservoirs. The second system we study is constituted of a double quantum dot coupled to two electrodes and probed by a quantum point contact detector. Thermodynamic forces are applied to each transport channel that generate fluctuating stationary currents. The full counting statistics of the currents is obtained starting from a microscopic Hamiltonian describing the …
The notion of fractional charges was up until now reserved for quasiparticle excitations emerging in strongly correlated quantum systems, such as Laughlin states in the fractional quantum Hall effect, Luttinger quasiparticles, or parafermions. Here, we consider topological transitions in the full counting statistics of standard sequential electron tunneling, and find that they lead to the same type of charge fractionalization - strikingly without requiring exotic quantum correlations. This conclusion relies on the realization that fundamental integer charge quantization fixes the global proper…
