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arXiv 2407.20501cond-mat.str-el
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超越自旋波理论的铜氧化物磁子谱

Magnon Spectra of Cuprates beyond Spin Wave Theory

Jiahui Bao, Matthias Gohlke, Jeffrey G. Rau, Nic Shannon

AI总结:

本文利用矩阵乘积态(MPS)计算超越自旋波理论的铜氧化物磁子谱,发现低阶自旋波理论会系统性高估交换参数,修正后标准模型能较好解释La$_2$CuO$_4$的磁子色散与线型,但无法完全捕捉高能连续谱。

摘要:

理解La$_2$CuO$_4$等铜氧化物反铁磁体中磁子的通常出发点是包含循环交换的自旋模型,该模型源自单带Hubbard模型,其参数取自基于非相互作用自旋波理论的拟合。在此,我们探讨这是否能可靠地描述实验,使用矩阵乘积态(MPS)计算超越自旋波理论的磁子谱。我们发现,基于低阶自旋波理论的分析会导致交换参数的系统性高估,并伴随Hubbard $t/U$估计的相应误差。修正这些问题后,该“标准”模型能很好地解释La$_2$CuO$_4$中的磁子色散与线型,但无法完全捕捉高能区观测到的连续谱。本文还讨论了该分析向CaCuO$_2$和Sr$_2$IrO$_4$的扩展。

英文摘要:

The usual starting point for understanding magnons in cuprate antiferromagnets such as La$_2$CuO$_4$ is a spin model incorporating cyclic exchange, which descends from a one-band Hubbard model, and has parameters taken from fits based on non-interacting spin wave theory. Here we explore whether this provides a reliable description of experiment, using matrix product states (MPS) to calculate magnon spectra beyond spin wave theory. We find that analysis based on low orders of spin wave theory leads to systematic overestimates of exchange parameters, with corresponding errors in estimates of Hubbard $t/U$. Once these are corrected, the ''standard'' model provides a good account of magnon dispersion and lineshape in La$_2$CuO$_4$, but fails to fully capture the continuum observed at high energies. The extension of this analysis to CaCuO$_2$ and Sr$_2$IrO$_4$ is also discussed.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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