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arXiv 2406.04474cond-mat.mtrl-scicond-mat.other
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交错磁候选材料MnTe中由化学计量比诱导的铁磁性

Stoichiometry-induced ferromagnetism in altermagnetic candidate MnTe

Michael Chilcote, Alessandro R. Mazza, Qiangsheng Lu, Isaiah Gray, Qi Tian, Qinwen Deng, Duncan Moseley, An-Hsi Chen, Jason Lapano, Jason S. Gardner, Gyula Eres… 展开作者

Michael Chilcote, Alessandro R. Mazza, Qiangsheng Lu, Isaiah Gray, Qi Tian, Qinwen Deng, Duncan Moseley, An-Hsi Chen, Jason Lapano, Jason S. Gardner, Gyula Eres, T. Zac Ward, Erxi Feng, Huibo Cao, Valeria Lauter, Michael A. McGuire, Raphael Hermann, David Parker, Myung-Geun Han, Asghar Kayani, Gaurab Rimal, Liang Wu, Timothy R. Charlton, Robert G. Moore, Matthew Brahlek

AI总结:

本文研究了MBE生长的MnTe/InP(111)薄膜,发现其本征富Mn化学计量比诱导弱铁磁性,并显著影响电子响应,为调控交错磁有序提供了新机制。

摘要:

由于新的理论预测和众多可能的应用,自旋电子学领域对交错磁性产生了浓厚的兴趣。MnTe是一种领先的交错磁候选材料,因其层状反铁磁结构、高奈尔温度(TN ~ 310 K)和半导体特性而在自旋电子学领域受到广泛关注。我们展示了分子束外延(MBE)生长的MnTe/InP(111)薄膜的研究结果。研究发现,MnTe的电子和磁学性质由其本征化学计量比所决定。电子输运测量和原位角分辨光电子能谱表明,这些薄膜天然呈金属性,费米能级位于价带中,且能带结构与交错磁自旋劈裂的第一性原理计算结果高度吻合。中子衍射证实该薄膜具有平面各向异性的反铁磁性,极化中子反射测量则表明存在弱铁磁性,这与MBE生长样品中固有的轻微富Mn成分有关。结合反常霍尔效应的测量结果,本工作表明电子响应受到铁磁矩的强烈影响。总而言之,这项工作揭示了在多种自旋电子学应用中调控交错磁有序的潜在机制。

英文摘要:

The field of spintronics has seen a surge of interest in altermagnetism due to novel predictions and many possible applications. MnTe is a leading altermagnetic candidate that is of significant interest across spintronics due to its layered antiferromagnetic structure, high Neel temperature (TN ~ 310 K) and semiconducting properties. We present results on molecular beam epitaxy (MBE) grown MnTe/InP(111) films. Here, it is found that the electronic and magnetic properties are driven by the natural stoichiometry of MnTe. Electronic transport and in situ angle-resolved photoemission spectroscopy show the films are natively metallic with the Fermi level in the valence band and the band structure is in good agreement with first principles calculations for altermagnetic spin-splitting. Neutron diffraction confirms that the film is antiferromagnetic with planar anisotropy and polarized neutron reflectometry indicates weak ferromagnetism, which is linked to a slight Mn-richness that is intrinsic to the MBE grown samples. When combined with the anomalous Hall effect, this work shows that the electronic response is strongly affected by the ferromagnetic moment. Altogether, this highlights potential mechanisms for controlling altermagnetic ordering for diverse spintronic applications.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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