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arXiv 2402.06541cond-mat.str-el
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关联电子系统中的电荷集体模式:超越随机相近似的等离激元

Charge Collective Modes in Correlated Electron Systems: Plasmons Beyond the Random Phase Approximation

Loïc Philoxene, Vu Hung Dao, Raymond Frésard

AI总结:

本文采用新开发的径向 Kotliar-Ruckenstein 从属玻色子表示分析扩展 Hubbard 模型的电荷激发谱,发现超越弱耦合区域后其结果与标准 RPA 存在显著定量和定性差异,深化了对关联系统电荷集体模式的理解。

摘要:

阐明强电子相互作用对金属系统集体激发的影响一直备受关注,这主要由于随机相近似(RPA)在强关联区域存在不足。在此,我们采用新开发的径向 Kotliar 和 Ruckenstein 从属玻色子表示,来分析扩展了长程相互作用的 Hubbard 模型的电荷激发谱。在面心立方晶格上,处于半填充状态,并在从非关联到金属-绝缘体相变的不同耦合区域中,我们将结果与作为基准的常规 RPA 进行了比较。我们重点关注局域和长程耦合对粒子-空穴激发连续谱,以及等离激元和上 Hubbard 带集体模式的影响。在弱耦合区域之外,我们发现我们的方法与标准 RPA 之间存在大量定量乃至定性的差异。因此,我们的工作加深了对关联系统中电荷集体模式的理解,并为未来广泛系列材料的研究奠定了基础。

英文摘要:

Elucidating the impact of strong electronic interactions on the collective excitations of metallic systems has been of longstanding interest, mainly due to the inadequacy of the random phase approximation (RPA) in the strongly correlated regime. Here, we adopt our newly developed radial Kotliar and Ruckenstein slave boson representation to analyze the charge excitation spectrum of a Hubbard model, extended with long range interactions. Working on the face centered cubic lattice, at half filling, and in different coupling regimes ranging from uncorrelated to the metal-to-insulator transition, we compare our results to conventional RPA as a benchmark. We focus on the influence of the local and long range couplings on the particle-hole excitation continuum and the plasmon and upper Hubbard band collective modes. Beyond the weak coupling regime, we find numerous quantitative and even qualitative discrepancies between our method and standard RPA. Our work thus deepens the understanding of charge collective modes in correlated systems, and lays the foundations for future studies of a broad series of materials.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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