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arXiv 2311.07697cond-mat.supr-con
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Ba(Fe1-xMx)2As2 (M = Co, Ni) 单晶中选择性轨道配对导致的向列超导电性

Nematic superconductivity from selective orbital pairing in Ba(Fe1-xMx)2As2 (M = Co, Ni) single crystals

Mason Klemm, Shirin Mozaffari, Rui Zhang, Brian W. Casas, Alexei E. Koshelev, Ming Yi, Luis Balicas, Pengcheng Dai

AI总结:

本研究通过输运测量揭示欠掺杂铁基超导体中上临界场的面内各向异性,结合中子散射和光电子能谱,证明超导电性源于dyz轨道选择性配对,并与自旋激发紧密关联。

摘要:

我们利用输运测量确定了去孪晶超导 Ba(Fe1-xMx)2As2 (M = Co, Ni) 单晶中上临界场 Hc2 的面内各向异性。在先前对孪晶单晶的测量中,发现沿层间(c轴)和面内方向磁场的上临界场各向异性随载流子掺杂浓度 (x) 的变化在过掺杂区域增加。对于欠掺杂样品,其在四方到正交结构转变温度 Ts 以下表现出自旋向列相,我们发现沿 a 轴的 Hc2 明显低于沿 b 轴的 Hc2。当体系变为四方结构时,上临界场各向异性在过掺杂区域消失。通过将这些结果与非弹性中子散射研究自旋激发以及角分辨光电子能谱相结合,我们得出结论:欠掺杂铁基砷化物中的超导电性是轨道选择性的——其中具有 dyz 轨道特征的电子贡献占主导,并且与自旋激发密切相关。

英文摘要:

We use transport measurements to determine the in-plane anisotropy of the upper critical field Hc2 in detwinned superconducting Ba(Fe1-xMx)2As2 (M = Co, Ni) single crystals. In previous measurements on twinned single crystals, the charge carrier doping dependence (x) of the upper critical field anisotropy for fields along the inter-planar (c-axis) and in-plane field directions was found to increase in the overdoped regime. For underdoped samples, which exhibit a spin nematic phase below the tetragonal to orthorhombic structural transition temperature Ts , we find that Hc2 along the a-axis is considerably lower than that along the b-axis. The upper critical field anisotropy disappears in the over-doped regime when the system becomes tetragonal. By combining these results with inelastic neutron scattering studies of spin excitations, and angle-resolved photoemission spectroscopy, we conclude that superconductivity in under-doped iron pnictides is orbital selective - with a dominant contribution from electrons with the dyz orbital character and being intimately associated with spin excitations.

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