Complexity of quantum phases of matter is often understood by the underlying gauge structures, as was recognized by the $\mathbb{Z}_2$ and U(1) gauge theory description of spin liquid in frustrated magnets. Anomalous Hall effect of conducting electrons can intrisically arise from U(1) gauges expressing the spatial modulation of ferromagnetic moments or from SU(2) gauges representing the spin-orbit coupling effect. Similarly, in insulating ferro and antiferromagnets, the magnon excitations can contribute to anomalous transports by feeling the U(1) and SU(2) gauges arising from the features of ordered moments or interactions. In this work, we report the emergent higher rank SU(3) gauge structure in the magnon transport based on the thermal conductivity measurements of MnSc$_2$S$_4$ in an applied field up to 14\,T. The thermal Hall coefficient takes a substantial value when the material enters a three-sublattice antiferromagnetic skyrmion phase, which is confirmed by the large-scale spin wave theory. The excited magnons are dressed with SU(3) gauge field, which is a mixture of three species of U(1) gauge fields originating from the slowly varying magnetic moments on these sublattices.
Chiral magnets support topological skyrmion textures due to the Dzyaloshinskii-Moriya spin-orbit interaction. In the presence of a sufficiently large applied magnetic field, such skyrmions are large amplitude excitations of the field-polarized magnetic state. We investigate analytically the interaction between such a skyrmion excitation and its small amplitude fluctuations, i.e., the magnons in a clean two-dimensional chiral magnet. The magnon spectrum is found to include two magnon-skyrmion bound states corresponding to a breathing mode and, for intermediate fields, a quadrupolar mode, which …
We discuss the scattering of high-energy magnons off a single magnetic skyrmion within the field-polarized ground state of a two-dimensional chiral magnet. For wavevectors larger than the inverse skyrmion radius, $k r_s \gg 1$, the magnon scattering is dominated by an emerging magnetic field whose flux density is essentially determined by the topological charge density of the skyrmion texture. This leads to skew and rainbow scattering characterized by an asymmetric and oscillating differential cross section. We demonstrate that the transversal momentum transfer to the skyrmion is universal due…
The stability of a single Belavin-Polyakov (BP) skyrmion in isotropic Heisenberg ferromagnet is studied. Such skyrmion is higher in energy than the uniform ferromagnetic state and is thus metastable. Starting from the lattice model in two spatial dimensions and using Maleyev-Dyson representation for spin operators, we examine the effects of magnon-magnon interaction for two quantities at $T=0$. First we discuss the self-energy corrections to magnon energy. Second we analyze the two-particle Green's function and possible bound states of two magnons. The simplicity of the model makes possible fu…
Topological transports of fermions are governed by the Chern numbers of the energy bands lying below the Fermi energy. For bosons, e.g. phonons and magnons in a crystal, topological transport is dominated by the Chern number of the lowest energy band when the band gap is comparable to the thermal energy. Here, we demonstrate the presence of topological transport by bosonic magnons in a lattice of magnetic skyrmions - topological defects formed by a vortex-like texture of spins. We find a distinct thermal Hall signal in the magnetic skyrmion phase of an insulating polar magnet GaV4Se8, identifi…
We study the low-energy magnon spectrum of the skyrmion crystal (SkX) ground state, appearing in two-dimensional ferromagnet with Dzyaloshinskii-Moriya interaction and magnetic field. We approximate SkX hexagonal superlattice by a set of overlapping disks, and find the lattice period by minimizing the classical energy density. The determined spectrum of magnons on the disc of optimal radius is stable and only two lowest energy levels can be considered as localized. The subsequent hybridization of these levels in the SkX lattice leads to tight-binding spectrum. The localized character of the lo…
We study theoretically the dynamics of magnons in the presence of a single skyrmion in chiral magnets featuring Dzyaloshinskii-Moriya interaction. We show by micromagnetic simulations that the scattering process of magnons by a skyrmion can be clearly defined although both originate in the common spins. We find that (i) the magnons are deflected by a skyrmion, with the angle strongly dependent on the magnon wavenumber due to the effective magnetic field of the topological texture, and (ii) the skyrmion motion is driven by magnon scattering through exchange of the momenta between the magnons an…
Using semiclassical method combined with stereographic projection approach, we investigate the magnetic dynamics of the skyrmion crystal (SkX), formed in planar ferromagnet with both Dzyaloshinskii-Moriya interaction and uniform magnetic field. The topologically non-trivial ground state of SkX is described in stereographic projection by the complex valued function with simple poles at skyrmions' positions. We use the earlier proposed ansatz for this ground state function in the form of the sum of individual skyrmions. The dynamics follows from the second variation of the classical action. Nume…
Magnonics is now an attractive field which focuses on the dynamic characteristics of magnons, a kind of quasiparticles in magnetic media, and attempt to apply magnons for functional devices. In order to construct magnon based devices, it is necessary to fabricate materials with specific and tunable magnon bands and band gaps. Skyrmion based magnonic crystals is one of the most suitable materials which possess periodical skyrmion structure and show applicative magnon bands and band gaps. In this review, we provide an overview over recent theoretical and experimental research on skyrmion based m…
We present a theory of magnetoelectric magnon-photon coupling in cavities hosting noncentrosymmetric magnets. Analogously to nonreciprocal phenomena in multiferroics, the magnetoelectric coupling is time-reversal and inversion asymmetric. This asymmetry establishes a means for exceptional tunability of magnon-photon coupling, which can be switched on and off by reversing the magnetization direction. Taking the multiferroic skyrmion-host Cu$_2$OSeO$_3$ with ultralow magnetic damping as an example, we reveal the electrical activity of skyrmion eigenmodes and propose it for magnon-photon splittin…
We construct Holstein-Primakoff Hamiltonian for magnons in arbitrary slowly varying spin background, for a microscopic spin Hamiltonian consisting of ferromagnetic spin exchange,Dzyaloshinskii-Moriya exchange, and the Zeeman term. The Gross-Pitaevskii-type equation for magnon dynamics contains several background gauge fields pertaining to local spin chirality, inhomogeneous potential, and anomalous scattering that violates the boson number conservation. Non-trivial corrections to previous formulas derived in the literature are given. Subsequent mapping to hydrodynamic fields yields the continu…
Magnetic skyrmions have been receiving growing attention as potential information storage and magnetic logic devices since an increasing number of materials have been identified that support skyrmion phases. Explorations of artificial frustrated systems have led to new insights into controlling and engineering new emergent frustration phenomena in frustrated and disordered systems. Here, we propose a skyrmion spin ice, giving a unifying framework for the study of geometric frustration of skyrmion crystals in a non-frustrated artificial geometrical lattice as a consequence of the structural con…
Inspired by the recent achievements of the strong magnons- and spin textures-photons coupling via dipolar interaction, the coupling between magnons and the local resonances of spin textures through direct exchange interaction is expected but not realized yet. In this work, we demonstrated the coherent coupling between propagating magnons and local skyrmion resonances. Besides the Rabbi coupling gap (RCG) in the frequency field dispersion, a magnonic analog of polariton gap, polaragnonic band gap (PBG), is also observed in the frequency-wavenumber dispersion. The realization of coupling require…
The analysis of the spin wave excitations in two-dimensional isotropic Heisenberg ferromagnet is performed with a single skyrmion in the ground state. We employ the ideas of semiclassical quantization method, duly modified for the use of the lattice model and Maleyev-Dyson boson representation of spin operators. The resulting Schrödinger equation for magnons describes the dispersion and wave functions of spin-wave excitations with strictly non-negative spectrum. In contrast to usual ferromagnet, we demonstrate the existence of three zero modes, corresponding to conformal symmetries spontaneous…
Achieving control over magnon spin currents in insulating magnets - where dissipation due to Joule heating is highly suppressed - is an active area of research that could lead to energy-efficient spintronics applications. However, magnon spin currents supported by conventional systems with uniform magnetic order have proven hard to control. An alternative approach that relies on topologically protected magnonic edge states of spatially periodic magnetic textures has recently emerged. A prime example of such textures is the ferromagnetic skyrmion crystal which hosts chiral edge states providing…
The motion of a spin excitation across topologically non-trivial magnetic order exhibits a deflection that is analogous to the effect of the Lorentz force on an electrically charged particle in an orbital magnetic field. We used polarized inelastic neutron scattering to investigate the propagation of magnons (i.e., bosonic collective spin excitations) in a lattice of skyrmion tubes in manganese silicide. For wave vectors perpendicular to the skyrmion tubes, the magnon spectra are consistent with the formation of finely spaced emergent Landau levels that are characteristic of the fictitious mag…
Properties of magnon modes localized on a ferromagnetic skyrmion are studied. Three types of possible asymptotic behavior of the modes eigenfrequencies are found for the case of large skyrmion radius $R_s$, namely $ω_0\sim R_s^{-2}$ for the breathing mode, $ω_{-|μ|}\sim R_s^{-1}$ and $ω_{|μ|}\sim R_s^{-3}$ for modes with negative and positive azimuthal quantum numbers, respectively. A number of properties of the magnon eigenfunctions are determined. This enables us to demonstrate that the skyrmion dynamics based on the traveling wave model is described by the massless Thiele equation.
Magnetic materials hosting correlated electrons play an important role for information technology and signal processing. The currently used ferro-, ferri- and antiferromagnetic materials provide microscopic moments (spins) that are mainly collinear. Recently more complex spin structures such as spin helices and cycloids have regained a lot of interest. The interest has been initiated by the discovery of the skyrmion lattice phase in non-centrosymmetric helical magnets. In this review we address how spin helices and skyrmion lattices enrich the microwave characteristics of magnetic materials. W…
We report studies of thermal conductivity as functions of magnetic field and temperature in the helimagnetic insulator Cu$_2$OSeO$_3$ that reveal novel features of the spin-phase transitions as probed by magnon heat conduction. The tilted conical spiral and low-temperature skyrmion phases, recently identified in small-angle neutron scattering studies, are clearly identified by sharp signatures in the magnon thermal conductivity. Magnon scattering associated with the presence of domain boundaries in the tilted conical phase and regions of skyrmion and conical-phase coexistence are identified.
Inhomogeneous strain applied to lattice systems can induce artificial gauge fields for particles moving on this lattice. Here we demonstrate how to engineer a novel state of matter, namely an antiferromagnet with a Landau-level excitation spectrum of magnons. We consider a honeycomb-lattice Heisenberg model and show that triaxial strain leads to equally spaced pseudo-Landau levels at the upper end of the magnon spectrum, with degeneracies characteristic of emergent supersymmetry. We also present a particular strain protocol which induces perfectly quantized magnon Landau levels over the whole …
Recent advances in the physics of current-driven antiferromagnetic skyrmions have observed the absence of a Magnus force. We outline the symmetry reasons for this phenomenon, and show that this cancellation will fail in the case of spin polarized currents. Pairing micromagnetic simulations with semiclassical spin wave transport theory, we demonstrate that skyrmions produce a spin-polarized transverse magnon current, and that spin-polarized magnon currents can in turn produce transverse motion of antiferromagnetic skyrmions. We examine qualitative differences in the frequency dependence of the …
A domain wall in a magnet with easy-axis anisotropy is shown to harbor spin superfluid associated with its spontaneous breaking of the U(1) spin-rotational symmetry. The spin superfluid is shown to have several topological properties, which are absent in conventional superfluids. First, the associated phase slips create and destroy skyrmions to obey the conservation of the total skyrmion charge, which allows us to use a domain wall as a generator and detector of skyrmions. Secondly, the domain wall engenders the emergent magnetic flux for magnons along its length, which are proportional to the…
In this work, we present a comprehensive study of the low energy optical magnetic response of the skyrmionic Mott insulator Cu$_2$OSeO$_3$ via high resolution time-domain THz spectroscopy. In zero field, a new magnetic excitation not predicted by spin-wave theory with frequency $f$ = 2.03 THz is observed and shown, with accompanying time-of-flight neutron scattering experiments, to be a zone folded magnon from the $\mathrm{R}$ to $\mathrmΓ$ points of the Brillouin zone. Highly sensitive polarimetry experiments performed in weak magnetic fields, $μ_0$H $<$ 200 mT, observe Faraday and Kerr rotat…
Spontaneously emergent chirality is an issue of fundamental importance across the natural sciences. It has been argued that a unidirectional (chiral) rotation of a mechanical ratchet is forbidden in thermal equilibrium, but becomes possible in systems out of equilibrium. Here we report our finding that a topologically nontrivial spin texture known as a skyrmion - a particle-like object in which spins point in all directions to wrap a sphere - constitutes such a ratchet. By means of Lorentz transmission electron microscopy we show that micron-sized crystals of skyrmions in thin films of Cu2OSeO…
Experimental and theoretical aspects of Hall-type transport of spins in magnetic insulators are reviewed, with emphasis on their spin chirality origin. A general formalism for linear response theory of thermal Hall transport in the spin model is developed, which can be applied to both the magnon and the paramagnetic, spin-liquid regimes. Recent experiments on magnon-mediated thermal Hall transport in the two-dimensional kagome, and three-dimensional pyrochlore ferromagnetic insulators are reviewed in light of the multi-band magnon theory of Hall transport, and compared to the more mysterious t…
When an electron moves in a smoothly varying non-collinear magnetic structure, its spin-orientation adapts constantly, thereby inducing forces that act on both the magnetic structure and the electron. These forces may be described by electric and magnetic fields of an emergent electrodynamics. The topologically quantized winding number of so-called skyrmions, i.e., certain magnetic whirls, discovered recently in chiral magnets are theoretically predicted to induce exactly one quantum of emergent magnetic flux per skyrmion. A moving skyrmion is therefore expected to induce an emergent electric …
Scalar spin chirality is expected to induce a finite contribution to the Hall response at low temperatures. We study this spin-chirality-driven Hall effect, known as the topological Hall effect, at the manganite side of the interface between La$_{1-x}$Sr$_{x}$MnO$_{3}$ and SrIrO$_3$. The ferromagnetic double-exchange hopping at the manganite layer, in conjunction with the Dzyaloshinskii-Moriya (DM) interaction which arises at the interface due to broken inversion symmetry and strong spin-orbit coupling from the iridate layer, could produce a skyrmion-crystal (SkX) phase in the presence of an e…
Partially filled Landau levels host competing orders, with electron solids prevailing close to integer fillings before giving way to fractional quantum Hall liquids as the Landau level fills. Here, we report the observation of an electron solid with noncolinear spin texture in monolayer graphene, consistent with solidification of skyrmions---topological spin textures characterized by quantized electrical charge. In electrical transport, electron solids reveal themselves through a rapid metal-insulator transition in the bulk electrical conductivity as the temperature is lowered, accompanied by …
A skyrmion crystal (SkX) expressed as a multiple number of spiral modulations manifests itself not only in its peculiar magnetic texture but also in nontrivial transport properties originating from an emergent magnetic field. We here report our numerical results for multiple SkXs in a centrosymmetric tetragonal crystal system. By performing simulated annealing for an effective spin model for itinerant magnets, we find that three types of the SkXs with the skyrmion numbers of one and two, which are characterized by different superpositions of helices, are stabilized in the ground state, and are…
Topological spin textures, such as a skyrmion crystal, are a source of unusual physical phenomena owing to the interplay between magnetism and topology. Since physical phenomena depend on the topological property and the symmetry of underlying spin structures, the search for new topological spin textures and emergent phenomena is one of the challenges in condensed matter physics. In this letter, we theoretically explore new topological spin textures arising from the synergy between spin, charge, and sublattice degrees of freedom in an itinerant magnet. By performing simulated annealing for an …
Topological order is important in many aspects of condensed matter physics, and has been extended to bosonic systems. In this Letter we report on the nontrivial topology of the magnon bands in two distinct quantum skyrmion crystals appearing in zero external magnetic field. This is revealed by nonzero Chern numbers for some of the bands. As a bosonic analog of the quantum anomalous Hall effect, we show that topological magnons can appear in skyrmion crystals without explicitly breaking time-reversal symmetry with an external magnetic field. By tuning the value of the easy-axis anisotropy at ze…
Uniquely in Cu2OSeO3, the Skyrmions, which are topologically protected magnetic spin vortex-like objects, display a magnetoelectric coupling and can be manipulated by externally applied electric (E) fields. Here, we explore the E-field coupling to the magnetoelectric Skyrmion lattice phase, and study the response using neutron scattering. Giant E-field induced rotations of the Skyrmion lattice are achieved that span a range of $\sim$25$^{\circ}$. Supporting calculations show that an E-field-induced Skyrmion distortion lies behind the lattice rotation. Overall, we present a new approach to Skyr…
Tunable Emergent Gauge Fields from Skyrmions in a Quasicrystalline Lattice
Department of Physics and Astronomy, The University of Tennessee（田纳西大学物理与天文学系）；Instituto de Física de Líquidos y Sistemas Biológicos, CONICET, Facultad de Ciencias Exactas, Universidad Nacional de La Plata（拉普拉塔国立大学精确科学学院液体与生物系统物理研究所，阿根廷国家科学研究委员会）；Departamento de Ciencias Básicas, Facultad de Ingeniería, UNLP（拉普拉塔国立大学工程学院基础科学系）；Neutron Scattering Division and Shull-Wollan Center, Oak Ridge National Laboratory（橡树岭国家实验室中子散射处和舒尔-沃兰中心）；Centro Atómico Bariloche and Instituto Balseiro, CNEA（巴里洛切原子中心巴尔塞罗研究所，阿根廷核能委员会）；Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET)（阿根廷国家科学研究委员会）；Instituto de Nanociencia y Nanotecnología CNEA-CONICET（CNEA-CONICET纳米科学与技术研究所）
Using the low-energy effective field theory for hole-doped antiferromagnets on the honeycomb lattice, we study the localization of holes on Skyrmions, as a potential mechanism for the preformation of Cooper pairs. In contrast to the square lattice case, for the standard radial profile of the Skyrmion on the honeycomb lattice, only holes residing in one of the two hole pockets can get localized. This differs qualitatively from hole pairs bound by magnon exchange, which is most attractive between holes residing in different momentum space pockets. On the honeycomb lattice, magnon exchange unambi…
The hallmark of a skyrmion crystal (SkX) is the topological Hall effect (THE). In this Article, we predict and explain an unconventional behavior of the topological Hall conductivity in SkXs. In simple terms, the spin texture of the skyrmions causes an inhomogeneous emergent magnetic field whose associated Lorentz force acts on the electrons. By making the emergent field homogeneous, the THE is mapped onto the quantum Hall effect (QHE). Consequently, each electronic band of the SkX is assigned to a Landau level. This correspondence of THE and QHE allows to explain the unconventional behavior o…
We study both analytically and numerically the edge of two-dimensional ferromagnets with Dzyaloshinskii-Moriya (DM) interactions, considering both chiral magnets and magnets with interface-induced DM interactions. We show that in the field-polarized ferromagnetic phase magnon states exist which are bound to the edge, and we calculate their spectra within a continuum field theory. Upon lowering an external magnetic field, these bound magnons condense at a finite momentum and the edge becomes locally unstable. Micromagnetic simulations demonstrate that this edge instability triggers the creation…
Symmetry-broken electronic phases support neutral collective excitations. For example, monolayer graphene in the quantum Hall regime hosts a nearly ideal ferromagnetic phase at filling factor $ν=1$ that spontaneously breaks spin rotation symmetry. This ferromagnet has been shown to support spin-wave excitations known as magnons which can be generated and detected electrically. While long-distance magnon propagation has been demonstrated via transport measurements, important thermodynamic properties of such magnon populations--including the magnon chemical potential and density--have thus far p…
Multi-orbital optical lattices have been attracting rapidly growing research interests in the last several years, providing fascinating opportunities for orbital-based quantum simulations. Here, we consider bosonic atoms loaded in the degenerate $p$-orbital bands of a two-dimensional triangular optical lattice. This system is described by a multi-orbital Bose-Hubbard model. We find the confined atoms in this system develop spontaneous orbital polarization, which forms a chiral Skyrmion lattice pattern in a large regime of the phase diagram. This is in contrast to its spin analogue which largel…
The formation and destruction of topologically quantized magnetic whirls, so-called skyrmions, in chiral magnets is driven by the creation and motion of singular hedgehog defects. These can be identified with emergent magnetic monopoles and antimonopoles. We investigate how the energetics of and forces between monopoles and antimonopoles influence their creation rate and dynamics. We study a single skyrmion line defect in the helical phase using both micromagnetic simulations and a Ginzburg-Landau analysis. Monopole-antimonople pairs are created in a thermally activated process, largely contro…
Magnetic field effects on spin-split band and magnon transport in altermagnets and emergent compensated ferrimagnets
Graduate School of Advanced Science and Engineering, Hiroshima University（广岛大学先进理工学研究科）；Center for Life Photonic Innovation, Kobe University（神户大学生命光子创新中心）
A superposition of spin helices can yield topological spin textures, such as skyrmion and hedgehog lattices. Based on the analogy with the moiré in optics, we study the magnetic and topological properties of such superpositions in a comprehensive way by modulating the interference pattern continuously. We find that the control of the angles between the superposed helices and the net magnetization yields successive topological transitions associated with pair annihilation of hedgehogs and antihedgehogs. Accordingly, emergent electromagnetic fields, magnetic monopoles and antimonopoles, and Dira…
Berry phases occur when a system adiabatically evolves along a closed curve in parameter space. This tutorial-like article focuses on Berry phases accumulated in real space. In particular, we consider the situation where an electron traverses a smooth magnetic structure, while its magnetic moment adjusts to the local magnetization direction. Mapping the adiabatic physics to an effective problem in terms of emergent fields reveals that certain magnetic textures - skyrmions - are tailormade to study these Berry phase effects.
Quintuplet condensation in the skyrmionic insulator Cu2OSeO3 at ultrahigh magnetic fields
Shizuoka University（静冈大学）；Loughborough University（拉夫堡大学）；Leibniz Institute for Solid State and Materials Research Dresden（德累斯顿莱布尼茨固体与材料研究所）；University of Tokyo（东京大学）
We investigate the skyrmion formation process in nano-structured FeGe Hall-bar devices by measurements of topological Hall effect, which extracts the winding number of a spin texture as an emergent magnetic field. Step-wise profiles of topological Hall resistivity are observed in the course of varying the applied magnetic field, which arise from instantaneous changes in the magnetic nano-structure such as creation, annihilation, and jittering motion of skyrmions. The discrete changes in topological Hall resistivity demonstrate the quantized nature of emergent magnetic flux inherent in each sky…
Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the sample. Study of this skyrmion tube (SkT) state is highly relevant for investigating skyrmion metastability and for implementation in recently proposed magnonic computing. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we de…
We demonstrate that an electric field could activate the three low-energy eigenmodes of the Neel-type skyrmion lattice via the electrically induced Dzyaloshinskii-Moriya interaction. In particular, we predict that the relative intensity of the clockwise rotation mode against the counter-clockwise rotation mode is significantly enhanced for the electrical activation in comparison with the magnetic activation. We also discover that the electrically and magnetically active modes obey unique selection rules. These findings promise a fresh pathway towards energy-efficient electrical manipulation of…
We show that classical Heisenberg antiferromagnets on the breathing kagome lattice can be a platform to realize a zero-field topological order of the scalar spin chirality which can be viewed as a miniature skyrmion crystal (SkX) of discrete form with a small number of spins in its magnetic unit cell. In the model, a third nearest-neighbor (NN) antiferromagnetic interaction along the bond direction $J_3$ and the breathing bond-alternation characterized by the ratio of the NN interaction for large triangles to that for small ones, $J_1'/J_1$, are essential. It is found by means of Monte Carlo s…
The elementary excitations of skyrmion crystals experience both emergent magnetic fields and anharmonic interactions brought about by the topologically nontrivial noncollinear texture. The resulting flat bands cause strong spontaneous quasiparticle decay, dressing the eigenmodes of skyrmion crystals with a finite zero-temperature quantum lifetime. Sweeping the flat bands through the spectrum by changing the magnetic field leads to an externally controllable energy-selective magnon breakdown. In particular, we uncover that the three fundamental modes, i.e., the anticlockwise, breathing, and clo…
