In this work, we report numerical results on the flow instability and bifurcation of a viscoelastic fluid in the upstream region of a confined cylinder in a narrow channel. Two-dimensional direct numerical simulations based on the FENE-P model (the finite-extensible nonlinear elastic model with the Peterlin closure) are conducted with numerical stabilization techniques. Our results show that the macroscopic viscoelastic constitutive relation can capture the viscoelastic upstream instability reported in previous experiments for low-Reynolds-number flows. The numerical simulations reveal that the non-dimensional recirculation length ($L_D$) is affected by the cylinder blocking rate ($BR$), the Weissenberg number ($Wi$), the viscosity ratio ($β$), and the maximum polymer extension ($L$). Close to the onset of upstream recirculation, depending on the values of $L$ and $β$, the bifurcation can be supercritical or subcritical. $β$ has a nonlinear influence on the upstream recirculation length. This work contributes to our theoretical understanding of this new instability mechanism in viscoelastic wake flows.
The interaction of flexible structures with viscoelastic flows can result in very rich dynamics. In this paper, we present the results of the interactions between the flow of a viscoelastic polymer solution and a cantilevered beam in a confined microfluidic geometry. Cantilevered beams with varying length and flexibility were studied. With increasing flow rate and Weissenberg number, the flow transitioned from a fore-aft symmetric flow to a stable detached vortex upstream of the beam, to a time-dependent unstable vortex shedding. The shedding of the unstable vortex upstream of the beam imposed…
In this paper I analyze the onset of Rayleigh-Taylor instability between two linear viscoelastic fluids assuming that the perturbations at the interface are small. In the first half, the paper analyzes a stratified viscoelastic fluid in which I prove that the perturbations rise or fall exponentially without oscillating. The second half of the paper examines the effect of electric and magnetic fields on viscoelastic fluids. I show that it is possible to choose electric or magnetic field gradient such that the effective acceleration due to gravity is zero. If a heavy Newtonian fluid rests on top…
Interior stagnation point flows of viscoelastic liquids arise in a wide variety of applications including extensional viscometry, polymer processing and microfluidics. Experimentally, these flows have long been known to exhibit instabilities, but the mechanisms underlying them have not previously been elucidated. We computationally demonstrate the existence of a supercritical oscillatory instability of low-Reynolds number viscoelastic flow in a two-dimensional cross-slot geometry. The fluctuations are closely associated with the "birefringent strand" of highly stretched polymer chains associat…
We report experimental results on elastic instability in a viscoelastic channel shear flow due to only a natural non-smoothed inlet and small holes along the channel for pressure measurements. We show that non-normal mode instability results in elastic waves and chaotic flow self-organized into periodically cycled stream-wise streaks synchronized by elastic wave frequency. The chaotic flow persists above the transition with increasing $Wi$ further into elastic turbulence and drag reduction regimes. Thus, we resolve the recent puzzle whether strong prearranged perturbations are necessary to get…
A modal stability analysis shows that pressure-driven pipe flow of an Oldroyd-B fluid is linearly unstable to axisymmetric perturbations, in stark contrast to its Newtonian counterpart which is linearly stable at all Reynolds numbers. The dimensionless groups that govern stability are the Reynolds number, the elasticity number, and the ratio of solvent to solution viscosity. The unstable mode has a phase speed close to the base-state maximum over the entire unstable region in the relevant parameter space, implying that the unstable mode belongs to a class of viscoelastic center modes. Unlike t…
Viscoelastic flow through an abrupt planar contraction geometry above a certain Weissenberg number (Wi) is well known to become unstable upstream of the contraction plane via a central jet separating from the walls and forming vortices in the salient corners. Here, for the first time we consider three-dimensional (3D) viscoelastic contraction flows in a microfabricated glass square-square contraction geometry. We employ state-of-the-art microtomographic particle image velocimetry to produce time-resolved and volumetric quantification of the 3D viscoelastic instabilities arising in a dilute pol…
The effects of polymer additives on Rayleigh--Taylor (RT) instability of immiscible fluids is investigated using the Oldroyd-B viscoelastic model. Analytic results obtained exploiting the phase-field approach show that in polymer solution the growth rate of the instability speeds up with elasticity (but remains slower than in the pure solvent case). Numerical simulations of the viscoelastic binary fluid model confirm this picture.
The recently-discovered centre-mode instability of rectilinear viscoelastic shear flow (Garg et al. Phy. Rev. Lett. 121, 024502, 2018) has offered an explanation for the origin of elasto-inertial turbulence (EIT) which occurs at lower Weissenberg ($Wi$) numbers. In support of this, we show using weakly nonlinear analysis that the subcriticality found in Page et al. (Phys. Rev. Lett. 125, 154501, 2020) is generic across the neutral curve with the instability only becoming supercritical at low Reynolds ($Re$) numbers and high $Wi$. We demonstrate that the instability can be viewed as purely elas…
We review three different types of viscoelastic surface instabilities: The Rayleigh -- Plateau, the Saffman -- Taylor and the Faraday instability. These instabilities are classical examples of hydrodynamic surface instabilities. The addition of a small amount of polymers to pure water can alter its flow behavior drastically and the type of instability may change not only quantitatively but also qualitatively. We will show that some of the observed new phenomena can be explained by the use of simple rheological models that contain most of the underlying physical mechanisms leading to the instab…
We study the Marangoni instability in a thin polymeric liquid film heated from the free surface. Polymeric solutions are usually the binary mixture of a Newtonian solvent with polymeric solute and exhibit viscoelastic behaviour. In the presence of a temperature gradient, stratification of these polymeric solutes can take place via the Soret effect, which may give rise to the solutocapillary effect at the free surface. Considering the Soret effect and incorporating the effects of gravity, here we analyse the stability characteristics of this polymeric thin film bounded between its deformable fr…
The viscoelastic fluids are usually the blends of a polymeric solute and a Newtonian solvent. In the presence of a temperature gradient, stratification of these solutes can take place via the Soret effect. Here, we investigate the classical Marangoni instability problem for a thin viscoelastic film considering this binary aspect of the fluid. The film, bounded above by a deformable free surface, is subjected to heating from below by a solid substrate. Linear stability analysis performed numerically for perturbations of finite wavelength (short-wave perturbations) reveals that both monotonic an…
When two fluids of different electrical conductivities are transported side by side in a microfluidic device under the influence of an electric field, an electrokinetic instability (EKI) is often generated after some critical values of the applied electric field strength and conductivity ratio. Many prior experimental and numerical studies show that this phenomenon results in a chaotic flow field inside a microdevice, thereby facilitating the mixing of two fluids if they are Newtonian in behaviour. However, the present numerical study shows that this chaotic convection arising due to the elect…
In this fluid dynamics video prepared for the APS-DFD Gallery of Fluid Motion we study the Kelvin-Helmholtz instability for both Newtonian and viscoelastic jets. The nonlinear dynamics of the jet motion are slowed down by orders of magnitude using a synchronized strobe effect coupled with precise timing control of perturbation frequencies. Our results show that at high wave-numbers the imposed perturbations initially grow linearly with time and the jet axis remains straight while the Kelvin-Helmholtz wave amplitude grows and rolls up into bags that encapsulate the central jet within themselves…
I shortly describe the main results on elastically driven instabilities and elastic turbulence in viscoelastic inertia-less flows with curved streamlines. Then I describe a theory of elastic turbulence and prediction of elastic waves at Re<<1 and Wi>>1, which speed depends on the elastic stress similarly to the Alfven waves in magneto-hydrodynamics and in in a contrast to all other fluid flows with wave speed depending on medium elasticity. Since the established and testified mechanism of elastic instability of viscoelastic flows with curvilinear streamlines becomes ineffective at zero curvatu…
We revisit the problem of the two-dimensional spatiotemporal linear stability of viscoelastic slender jets obeying linear Phan-Thien-Tanner (PTT) stress constitutive equation, and investigate the role of finite stresses on the elasto-capilliary stability of the Beads-on-a-String (BOAS) structure (structures which include the formation of very thin filament between drops) and identify the regions of topological transition of the advancing jet interface, in the limit of low to moderate Ohnesorge number ($Oh$) and high values of Weissenberg number ($We$). The Briggs idea of analytic continuation …
A modal stability analysis shows that plane Poiseuille flow of an Oldroyd-B fluid becomes unstable to a `center mode' with phase speed close to the maximum base-flow velocity, $U_{max}$. The governing dimensionless groups are the Reynolds number $Re = ρU_{max} H/η$, the elasticity number $E = λη/(H^2ρ)$, and the ratio of solvent to solution viscosity $η_s/η$; here, $λ$ is the polymer relaxation time, $H$ is the channel half-width, and $ρ$ is the fluid density. For experimentally relevant values (e.g., $E \sim 0.1$ and $β\sim 0.9$), the predicted critical Reynolds number, $Re_c$, for the center…
In the finite element analysis with fast decoupled time integration scheme for viscoelastic fluid (the Leonov model) flow, we investigate strong nonlinear behavior in 2D creeping contraction flow. The algorithm is applicable in the whole range of the retardation parameter. In the analysis of steady solutions, there exists upper convergence limit of available numerical solutions in this contraction flow that is free from the frustrating mesh dependence when we incorporate the tensor-logarithmic formulation [Fattal and Kupferman, JNNFM, 2004]. With adjustment of a nonlinear parameter, 2 kinds of…
We report quantitative evidence of mixing-layer elastic instability in a viscoelastic fluid flow between two widely spaced obstacles hindering a channel flow at $Re\ll1$ and $Wi\gg1$. Two mixing layers with nonuniform shear velocity profiles are formed in the region between the obstacles. The mixing-layer instability arises in the vicinity of an inflection point on the shear velocity profile with a steep variation in the elastic stress. The instability results in an intermittent appearance of small vortices in the mixing layers and an amplification of spatio-temporal averaged vorticity in the …
When a dilute polymer solution experiences capillary thinning, it forms an almost uniformly cylindrical thread, which we study experimentally. In the last stages of thinning, when polymers have become fully stretched, the filament becomes prone to instabilities, of which we describe two: A novel "breathing" instability, originating from the edge of the filament, and a sinusoidal instability in the interior, which ultimately gives rise to a "blistering" pattern of beads on the filament. We describe the linear instability with a spatial resolution of 80 nm in the disturbance amplitude. For suffi…
The rimming flow of a viscoelastic thin film inside a rotating horizontal cylinder is studied theoretically. Attention is given to the onset of non-Newtonian free-surface instability in creeping flow. This non-inertial instability has been observed in experiments, but current theoretical models of Newtonian fluids can neither describe its origin nor explain its onset. This study examines two models of non Newtonian fluids to see if the experimentally observed instability can be predicted analytically. The non-Newtonian viscosity and elastic properties of the fluid are described by the Generali…
Interactions between microorganisms and their complex flowing environments are essential in many biological systems. We develop a model for microswimmer dynamics in non-Newtonian Poiseuille flows. We predict that swimmers in shear-thickening (-thinning) fluids migrate upstream more (less) quickly than in Newtonian fluids and demonstrate that viscoelastic normal stress differences reorient swimmers causing them to migrate upstream at the centreline, in contrast to well-known boundary accumulation in quiescent Newtonian fluids. Based on these observations, we suggest a sorting mechanism to selec…
In this paper, we discuss whether the instability of viscoelastic flow around a circular cylinder is subcritical or supercritical by numerical simulation. The Oldroyd-B model is selected to describe the viscoelastic constitutive relationship. The Log-conformation reformulation is employed to stabilize numerical simulation. The parameter ranges investigated are the Reynolds numbers ($Re$) spanning from 5 to 100 and the Weissenberg number ($Wi$) spanning from 0 to 10, with a fixed viscosity ratio of $β= 0.9$. Simulations are performed under two paths, i.e., 1) increasing $Re$ (or $Wi$) and 2) de…
Newtonian pipe flow is known to be linearly stable at all Reynolds numbers. We report, for the first time, a linear instability of pressure driven pipe flow of a viscoelastic fluid, obeying the Oldroyd-B constitutive equation commonly used to model dilute polymer solutions. The instability is shown to exist at Reynolds numbers significantly lower than those at which transition to turbulence is typically observed for Newtonian pipe flow. Our results qualitatively explain experimental observations of transition to turbulence in pipe flow of dilute polymer solutions at flow rates where Newtonian …
We show that viscoelastic plane Poiseuille flow becomes linearly unstable in the absence of inertia, in the limit of high elasticities, for ultra-dilute polymer solutions. While inertialess elastic instabilities have been predicted for curvilinear shear flows, this is the first ever report of a purely elastic linear instability in a rectilinear shear flow. The novel instability continues upto a Reynolds number ($Re$) of $O(1000)$, corresponding to the recently identified elasto-inertial turbulent state believed to underlie the maximum-drag-reduced regime. Thus, for highly elastic ultra-dilute …
Attempts to achieve "top kill" of actively flowing oil wells by insertion of dense drilling "muds", i.e., slurries of dense minerals, from above will fail if the Kelvin-Helmholtz instability in the gravity-driven counterflow produces turbulence that breaks up the denser fluid into small droplets. Here we estimate the droplet size to be sub-mm for fast flows and suggest the addition of a shear-thickening polymer to suppress turbulence. Laboratory experiments show a progression from droplet formation to complete turbulence suppression at the relevant high velocities, illustrating rich new physic…
We examine the response of an inertia-less viscoelastic channel flow to localized perturbations. A simplified model shows that the non-linear interaction between the velocity and elastic stress fields can split an initial pulsed disturbance into two separate pulses if the initial disturbance and the base elastic stress are sufficiently high. In accordance, we demonstrate that a transition to a pulse-splitting regime can be achieved experimentally. These results suggest a possible new direction for studying the elastic instability of viscoelastic channel flows at high elasticity through the gro…
Here we report some interesting new features of the spatio-temporal instability of the incompressible plane Couette-Poiseuille flow (CPF). First of all, this flow represents the first instance of a "non-inflectional" absolute instability, within constant-viscosity formulation, which is triggered when one of the plates moves opposite to the bulk motion. More strikingly, with further increase in the negative plate motion, the absolute instability ($\textrm{AI}$) transitions to an "upstream" convective instability ($\textrm{CI}^-$), wherein an unstable wave packet moves opposite to the direction …
In this work, we study the role of viscoelastic instability in the mechanical dispersion of fluid flow through porous media at high Peclet numbers. Using microfluidic experiments and numerical simulations, we show that viscoelastic instability in flow through a hexagonally ordered (staggered) medium strongly enhances dispersion transverse to the mean flow direction with increasing Weissenberg number (Wi). In contrast, preferential flow paths can quench the elastic instability in disordered media, which has two important consequences for transport: First, the lack of chaotic velocity fluctuatio…
We report a technique based on Fresnel diffraction with white illumination that permits the resolution of capillary surface patterns of less than 100 nanometers. We investigate Rayleigh Plateaux like instability on a viscoelastic capillary bridge and show that we can overcome the resolution limit of optical microscopy. The viscoelastic filaments are approximately 20 microns thick at the end of the thinning process when the instability sets in. The wavy distortions grow exponentially in time and the pattern is resolved by an image treatment that is based on an approximation of the measured risi…
Elasto-inertial turbulence (EIT) is a new, two-dimensional chaotic flow state observed in polymer solutions with possible connections to inertialess elastic turbulence and drag-reduced Newtonian turbulence. In this Letter, we argue that the origins of EIT are fundamentally different from Newtonian turbulence by finding a dynamical connection between EIT and an elasto-inertial linear instability recently found at high Weissenberg numbers (Garg et al. Phys. Rev. Lett. 121, 024502, 2018). This link is established by isolating the first known exact coherent structures in viscoelastic parallel flow…
Using branch continuation in the FENE-P model, we show that finite-amplitude travelling waves borne out of the recently-discovered linear instability of viscoelastic channel flow (Khalid et al. {\em J. Fluid Mech.} {\bf 915}, A43, 2021) are substantially subcritical reaching much lower Weissenberg ($Wi$) numbers than on the neutral curve at a given Reynolds ($Re$) number over $Re \in [0,3000]$. The travelling waves on the lower branch are surprisingly weak indicating that viscolastic channel flow is susceptible to (nonlinear) instability triggered by small finite amplitude disturbances for $Wi…
Inertial cavitation in soft matter is an important phenomenon featured in a wide array of biological and engineering processes. Recent advances in experimental, theoretical, and numerical techniques have provided access into a world full of nonlinear physics, yet most of our quantitative understanding to date has been centered on a spherically symmetric description of the cavitation process. However, cavitation bubble growth and collapse rarely occur in a perfectly symmetrical fashion, particularly in soft materials. Predicting the onset of dynamically arising, non-spherical instabilities has …
For decades, transition to turbulence in viscoelastic parallel shear flows was believed to require nonlinear instabilities. We provide numerical evidences for a new wall-mode linear instability that directly triggers the transition to elastoinertial turbulence in channel flow. The instability is 2D but 3D features become important as nonlinear effects grow. With larger disturbances, direct transition to nonlinear instabilities, leading to turbulent states of both inertial and elastoinertial natures, are observed.
We explore the interfacial instability that results when a Newtonian fluid (a glycerol-water mixture, inner fluid) displaces a viscoelastic fluid (a dense cornstarch suspension, outer fluid) in a radial Hele-Shaw cell. As the ratio of viscosities of the inner and outer fluids is increased, side branched interfacial patterns are replaced by more stable interfaces that display proportionate growth and finger coalescence. We correlate the average finger spacing with the most dominant wavelength of interfacial instability, computed using a mathematical model that accounts for viscous fingering in …
Viscoelastic flows are pervasive in a host of natural and industrial processes, where the emergence of nonlinear and time-dependent dynamics regulate flow resistance, energy consumption, and particulate dispersal. Polymeric stress induced by the advection and stretching of suspended polymers feeds back on the underlying fluid flow, which ultimately dictates the dynamics, instability, and transport properties of viscoelastic fluids. However, direct experimental quantification of the stress field is challenging, and a fundamental understanding of how Lagrangian flow structure regulates the distr…
This work explains a scaling law of the first Landau coefficient of the derived Ginzburg-Landau equation (GLE) in the weakly nonlinear analysis of axisymmetric viscoelastic pipe flows in the large-Weissenberg-number ($Wi$) limit, recently reported in Wan et al. J. Fluid Mech. (2021), vol. 929, A16. Using an asymptotic method, we derive a reduced system, which captures the characteristics of the linear centre-mode instability near the critical condition in the large-$Wi$ limit. Based on the reduced system we then conduct a weakly nonlinear analysis using a multiple-scale expansion method, which…
Polymer additives can substantially reduce the drag of turbulent flows and the upper limit, the so called "maximum drag reduction" (MDR) asymptote is universal, i.e. independent of the type of polymer and solvent used. Until recently, the consensus was that, in this limit, flows are in a marginal state where only a minimal level of turbulence activity persists. Observations in direct numerical simulations using minimal sized channels appeared to support this view and reported long "hibernation" periods where turbulence is marginalized. In simulations of pipe flow we find that, indeed, with inc…
We report the temporal and spatio-temporal stability analyses of anti-symmetric, free shear, viscoelastic flows obeying the Oldroyd-B constitutive equation in the limit of low to moderate Reynolds number and Weissenberg number. The resulting fourth order Orr-Sommerfeld equation is reduced to a set of six auxiliary equations which are numerically integrated starting from the rescaled far-field conditions, i.~e., via the Compound Matrix Method. Numerical results indicate that with increasing Weissenberg number: (a) the peak of the maximal growth rate (i. e., the maximum value of the imaginary co…
In this study, the OpenFOAM platform, based on the finite volume method, is applied to investigate the two-dimensional viscoelastic flow past a circular cylinder. The FENE-P model, which considers the bounded elongation of polymer molecules, is chosen to describe the elastic constitutive relationship of the polymer solution. The maximum molecular chain lengths of L = 10, 50, 100, and 200 are considered, which describe the molecular conformation characteristics of the polymer solution. To improve the numerical instability of the viscoelastic flow simulation, three different methods, i.e., the t…
We present experimental evidence of global viscoelastic flow transitions in 2:1, 8:1 and 32:1 planar contractions under inertia-less conditions. Light sheet visualization and laser Doppler velocimetry techniques are used to probe spatial structure and time scales associated with the onset of these instabilities. The results are reported in terms of critical Weissenberg numbers characterizing the fluid flow rates. For a given contraction ratio and polymer fluid, a two-dimensional, steady flow with converging streamlines transitions to a two-dimensional pattern with diverging streamlines beyond …
The flow of viscoelastic fluids in porous media is encountered in many practical applications, such as in the enhanced oil recovery process or in the groundwater remediation. Once the flow rate exceeds a critical value in such flows, an elastic instability with fluctuating flow field is observed, which ultimately transits to a more chaotic and turbulence-like flow structure as the flow rate further increases. In a recent study, it has been experimentally shown that this chaotic flow behaviour of viscoelastic fluids can be suppressed by increasing the geometric disorder in a model porous media …
An analytic, asymptotic approximation of the nonlinear steady-state equations for viscoelastic creeping flow, modeled by the Oldroyd-B equations with polymer stress diffusion, is derived. Near the extensional stagnation point the flow stretches and aligns polymers along the outgoing streamlines of the stagnation point resulting in a stress-island, or birefringent strand. The polymer stress diffusion coefficient is used, both, as an asymptotic parameter and a regularization parameter. The structure of the singular part of polymer stress tensor is a Gaussian aligned with the incoming streamline …
