arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2201.10719cond-mat.supr-concond-mat.mtrl-sci
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具有低反铁磁transition temperatures的准一维超导母体化合物NaMn $_6$ Bi $_5$

A new quasi-one-dimensional superconductor parent compound NaMn$_6$Bi$_5$ with lower antiferromagnetic transition temperatures

Ying Zhou, Long Chen, Gang Wang, Yuxin Wang, Zhichuan Wang, Congcong Chai, Zhongnan Guo3, Jiangping Hu, Xiaolong Chen

摘要:

Mn基超导体是一种罕见的超导体,最近报道了在高压下的准一维KMn $_6$ Bi $_5$与[Mn $_6$ Bi $_5$ ]柱。本文报道了新发现的准一维NaMn $_6$ Bi $_5$单晶的合成、磁性、电阻率和比热容。与其它AMn $_6$ Bi $_5$(A = K,Rb,Cs)相比,NaMn $_6$ Bi $_5$具有更大的Bi-Bi键长,这可能导致了47.3 K和52.3 K的两个退耦反铁磁跃迁.相对较低的反铁磁转变温度使NaMn $_6$ Bi $_5$成为探索Mn基超导体的更合适平台。在低温下观察到各向异性电阻率和非费米液体行为。热容测量表明,NaMn $_6$ Bi $_5$具有与AMn $_6$ Bi $_5$(A = K和Rb)相似的德拜温度,而索末菲系数却异常大。利用第一性原理计算,与AMn $_6$ Bi $_5$(A = K,Rb,and Cs)化合物相比,NaMn $_6$ Bi $_5$具有非常不同的态密度,并在费米能级附近有不寻常的增强.

英文摘要:

Mn-based superconductor is rare and recently reported in quasi-one-dimensional KMn$_6$Bi$_5$ with [Mn$_6$Bi$_5$]-columns under high pressure. Here we report the synthesis, magnetic properties, electrical resistivity, and specific heat capacity of the newly-discovered quasi-one-dimensional NaMn$_6$Bi$_5$ single crystal. Compared with other AMn$_6$Bi$_5$ (A = K, Rb, and Cs), NaMn$_6$Bi$_5$ has larger intra-column Bi-Bi bond length, which may result in the two decoupled antiferromagnetic transitions at 47.3 K and 52.3 K. The relatively lower antiferromagnetic transition temperatures make NaMn$_6$Bi$_5$ a more suitable platform to explore Mn-based superconductors. Anisotropic resistivity and non-Fermi liquid behavior at low temperature are observed. Heat capacity measurement reveals that NaMn$_6$Bi$_5$ has similar Debye temperature with those of AMn$_6$Bi$_5$ (A = K and Rb), whereas the Sommerfeld coefficient is unusually large. Using first-principles calculations, the quite different density of states and an unusual enhancement near the Fermi level are observed for NaMn$_6$Bi$_5$, when compared with those of other AMn$_6$Bi$_5$ (A = K, Rb, and Cs) compounds.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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