Recent experiments have shown that the reduced multilayer rare-earth (RE) nickel oxides of form RE$_{p+1}$Ni$_p$O$_{2p+2}$ may belong to the novel family of superconducting lanthanide nickelates. Here, the correlated electronic structure of Pr$_{4}$Ni$_3$O$_{8}$ and Nd$_{6}$Ni$_5$O$_{12}$ is studied by means of an advanced realistic many-body framework. It is revealed that the low-energy physics of both systems is dominated by an interplay of Ni-$d_{x^2-y^2}$ and Ni-$d_{z^2}$ degrees of freedom. Whilst the Ni-$d_{x^2-y^2}$ orbitals are always highly correlated near an (orbital-selective) Mott-insulating regime, the Ni-$d_{z^2}$ orbitals give rise to intriguing non-dispersive features. At low temperature, the Pr compound still displays QP-like Ni-$d_{x^2-y^2}$-derived states at the Fermi level, but the interacting fermiology of the Nd compound is outshined by an emergent Ni-$d_{z^2}$-controlling flat band. These findings translate well to the previous characterization of doped infinite-layer nickelates, and hence further make the case for a mechanism of unconventional superconductivity which is distinct from the one in high-$T_{\rm c}$ cuprates.
The prediction of high $T_c$ superconductivity in layers of LaNiO$_3$ through orbital engineering has led to extensive research efforts over the last fifteen years. During this period, a plethora of thin films and heterostructures based rare-earth nickelate family with perovskite structure has been synthesized and explored. In this short perspective, we briefly review the complexity of bulk $RE$NiO$_3$, spotlighting several recent findings of emergent phenomena in heterostructures containing the interface between $RE$NiO$_3$ and another transition metal oxide. Finally, we outline potentially i…
Itinerant Nature of Spin-Density-Wave Order in Ruddlesden-Popper Nickelates
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院)
Magnetic configurations and excitations in high-$T_{c}$ multilayer nickelates
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所,凝聚态物理北京国家实验室);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院);Institute of Theoretical Physics, Chinese Academy of Sciences(中国科学院理论物理研究所);New Cornerstone Science Laboratory, Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所,新基石科学实验室)
Emergent quantum phenomena via phase-coherence engineering in infinite-layer nickelate superconductors
Peking University(北京大学);University of Electronic Science and Technology of China(电子科技大学);Renmin University of China(中国人民大学);ShanghaiTech University(上海科技大学);Tsinghua University(清华大学);Institute of Physics Chinese Academy of Sciences(中国科学院物理研究所);University of Chinese Academy of Sciences(中国科学院大学);Songshan Lake Materials Laboratory(松山湖材料实验室);Beijing Normal University(北京师范大学);Fudan University(复旦大学);Hefei National Laboratory(合肥国家实验室)
Hierarchical structure of primary and hybridization-induced superconducting correlations in bilayer nickelates
College of Industrial Technology, Nihon University(日本大学工业技术学部);Research Organization of Science and Technology, Ritsumeikan University(立命馆大学科学技术研究院);Faculty of Engineering, Tottori University(鸟取大学工学部);Department of Physics, The University of Osaka(大阪大学物理学系)
Perfect dc conductance of a finite width Mott insulator sandwiched between metallic leads at zero temperature: a quantum emergent phenomenon in strongly correlated multilayers
Emergent $s+id$ Superconductivity from the Interplay between Electronic Correlations and Electron-Phonon Coupling in $\mathrm{R}_{1-x}\mathrm{Sr}_x\mathrm{NiO}_2$
Northeastern University(东北大学);Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院);CAS Key Laboratory of Theoretical Physics, Institute of Theoretical Physics, Chinese Academy of Sciences(中国科学院理论物理研究所)
Microscopic mechanism of high-temperature superconductivity revealed by ab initio studies on hole-doped multilayer cuprates HgBa$_2$Ca$_2$Cu$_3$O$_8$ under pressure
Sophia University(上智大学);The University of Tokyo(东京大学)
We consider a hitherto unexplored setting of stacked multilayer ($\mathcal{N}$) Lieb lattice which undergoes an unusual topological transition in the presence of intra-layer spin-orbit coupling (SOC). The specific stacking configuration induces an effective non-symmorphic 2D lattice structure, even though the constituent monolayer Lieb lattice is characterized by a symmorphic space group. This emergent non-symmorphicity leads to multiple doubly-degenerate bands extending over the edge of the Brillouin zone (i.e. Quadratic Band Crossing Lines). In the presence of intra-layer SOC, these doubly-d…
Electronic structure and magnetic tendencies of trilayer La$_4$Ni$_3$O$_{10}$ under pressure: structural transition, molecular orbitals, and layer differentiation
Competing Orders Driven by Wigner Crystal Phase in Rhombohedral Graphene
Institute of Physics, Ecole Polytechnique Fédérale de Lausanne(洛桑联邦理工学院物理研究所);SPEC, CEA, CNRS, Université Paris-Saclay(法国原子能和替代能源委员会、国家科学研究中心、萨克雷大学SPEC实验室);Department of Physics, Florida State University(佛罗里达州立大学物理系);National High Magnetic Field Laboratory(国家高磁场实验室);FSU Quantum Initiative, Florida State University(佛罗里达州立大学FSU量子倡议项目);Research Center for Functional Materials, National Institute for Materials Science(日本物质材料研究机构功能材料研究中心)
Topological phases of matter have established a new paradigm in physics, bringing quantum phenomena to the macroscopic scale and hosting exotic emergent quasiparticles. In this thesis, I theoretically and experimentally demonstrate with my collaborators the first Weyl semimetal, TaAs, using angle-resolved photoemission spectroscopy (ARPES), directly observing its emergent Weyl fermions and topological Fermi arc surface states [Science 349, 6248 (2015); Nat. Commun. 6, 7373 (2015); PRL 116, 066802 (2016)]. Next, I discover high-degeneracy topological chiral fermions in the chiral crystals RhSi …