Luttinger semimetals represent materials with strong spin-orbit coupling, harbouring doubly-degenerate quadratic band touchings at the Brillouin zone center. In the presence of Coulomb interactions, such a system exhibits a non-Fermi liquid phase [dubbed as the Luttinger-Abrikosov-Beneslavskii (LAB) phase], at low temperatures and zero doping. However, a clear experimental evidence of this emergent state remains elusive to this date. Hence, we focus on extracting the Raman response as a complementary experimental signature. At frequencies much larger than the temperature, the Raman response exhibits a power-law behavior, which can be verified experimentally. On the other hand, at lower frequencies, the Raman response displays a quasi-elastic peak. We also compute the ratio of the shear viscosity and the entropy density, and the value obtained is a consequence of the hyperscaling violation that emerges in the LAB phase.
We study both noncentrosymmetric and time-reversal breaking Weyl semimetal systems under a strong magnetic field with the Coulomb interaction. The three-dimensional bulk system is reduced to many mutually interacting quasi-one-dimensional wires. Each strongly correlated wire can be approached within the Tomonaga-Luttinger liquid formalism. Including impurity scatterings, we inspect the localization effect and the temperature dependence of the electrical resistivity. The effect of a large number of Weyl points in real materials is also discussed.
We show that hybrid Dirac and Weyl semimetals can be realized in a three-dimensional Luttinger semimetal with quadratic band touching (QBT). We illustrate this using periodic kicking scheme. In particular, we focus on a momentum-dependent drivings (nonuniform driving) and demonstrate the realization of various hybrid Dirac and Weyl semimetals. We identify a unique hybrid dispersion Dirac semimetal with two nodes, where one of the nodes is linear while the other is dispersed quadraticlly. Next, we show that by tilting QBT via periodic driving and in the presence of an external magnetic field, o…
Due to strong spin-orbit coupling, charge carriers in three-dimensional quadratic band touching Luttinger semimetals have non-trivial wavefunctions characterized by a pseudospin of 3/2. We compute the dielectric permittivity of such semimetals at finite doping, within the random phase approximation. Because of interband coupling, the dielectric screening shows a reduced plasma frequency and an increased spectral weight at small wavevectors, compared to a regular quadratic band. This weakens the effective Coulomb potential, modifying the single-particle self-energy for which we present both ana…
We study the interaction between elliptically polarized light and a three-dimensional Luttinger semimetal with quadratic band touching using Floquet theory. In the absence of light, the touching bands can have the same or the opposite signs of the curvature; in each case, we show that simply tuning the light parameters allows us to create a zoo of Weyl semimetallic phases. In particular, we find that double and single Weyl points can coexist at different energies, and they can be tuned to be type I or type II. We also find an unusual phase transition, in which a pair of Weyl nodes form at fini…
Luttinger semimetals have quadratic band crossings at the Brillouin zone-center in three spatial dimensions. Coulomb interactions in a model that describes these systems stabilize a non-trivial fixed point associated with a non-Fermi liquid state, also known as the Luttinger-Abrikosov-Beneslavskii phase. We calculate the optical conductivity $σ(ω) $ and the dc conductivity $σ_{dc} (T) $ of this phase, by means of the Kubo formula and the Mori-Zwanzig memory matrix method, respectively. Interestingly, we find that $σ(ω) $, as a function of the frequency $ω$ of an applied ac electric field, is c…
Luttinger semimetals include materials like gray tin ($α$-Sn) and mercury telluride, which are three-dimensional gapless semiconductors having a quadratic band crossing point (QBCP). Due to a growing interest in QBCPs and new experimental efforts, it is essential to study the finite-temperature properties of such systems. In this paper, we investigate the emergence of plasmons in the presence of Coulomb interactions in isotropic Luttinger semimetals, for zero as well as generic nonzero temperatures. When the Fermi level lies right at the QBCP, which is the point where twofold degenerate conduc…
Luttinger semimetals are three-dimensional electron systems with a parabolic band touching and an effective total spin $J=3/2$. In this paper, we present an analytical theory of dielectric screening of inversion-symmetric Luttinger semimetals with an arbitrary carrier density and conduction-valence effective mass asymmetry. Assuming a spherical approximation for the single-particle Luttinger Hamiltonian, we determine analytically the dielectric screening function in the random phase approximation for arbitrary values of the wave vector and frequency, the latter in the complex plane. We use thi…
We study a simple model of three-dimensional fermions close to a quadratic band touching point, built from the celebrated Luttinger single-particle Hamiltonian and an attractive contact interaction between the particles. Such a system displays a novel quantum critical point between the semimetallic and an s-wave superconducting phase at which the low-energy "Luttinger fermions" are inextricably coupled to the order parameter fluctuations. The quantum critical point is perturbatively accessible near four spatial dimensions, where it features nontrivial scaling with dynamical exponent 1<z<2 and …
The differential cross section for resonant Raman scattering from the collective modes in a one dimensional system of interacting electrons is calculated non-perturbatively using the bosonization method. The results indicate that resonant Raman spectroscopy is a powerful tool for studying Tomonaga-Luttinger liquid behaviour in quasi-one dimensional electron systems.
The surface of a Weyl semimetal famously hosts an exotic topological metal that contains open Fermi arcs rather than closed Fermi surfaces. In this work, we show that the surface is also endowed with a feature normally associated with strongly interacting systems, namely, Luttinger arcs, defined as zeros of the electron Green's function. The Luttinger arcs connect surface projections of Weyl nodes of opposite chirality and form closed loops with the Fermi arcs when the Weyl nodes are undoped. Upon doping, the ends of the Fermi and Luttinger arcs separate and the intervening regions get filled …
We compute the effects of electronic interactions on gapless spin-3/2 excitations that in a noninteracting system emerge at a bi-quadratic touching of Kramers degenerate valence and conduction bands, known as Luttinger semimetal. This model can describe the low-energy physics of HgTe, gray-Sn, 227 pyrochlore iridates and half-Heuslers. For the sake of concreteness we only consider the short-range components of the Coulomb interaction. By combining mean-field analysis with a renormalization group (RG) calculation, we construct multiple cuts of the global phase diagram of interacting spin-3/2 fe…
We study superconductivity driven by screened Coulomb repulsion in three-dimensional Luttinger semimetals with a quadratic band touching and strong spin-orbit coupling. In these semimetals, the Cooper pairs are formed by spin-3/2 fermions with non-trivial wavefunctions. We numerically solve the linear Eliashberg equation to obtain the critical temperature of a singlet s-wave gap function as a function of doping, with account of spin-orbit and self-energy corrections. In order to understand the underlying mechanism of superconductivity, we compute the sensitivity of the critical temperature to …
Dirac and Weyl semimetals with linearly crossing bands are the focus of much recent interest in condensed matter physics. Although they host fascinating phenomena, their physics can be understood in terms of weakly interacting electrons. In contrast, more than 40 years ago, Abrikosov pointed out that quadratic band touchings are generically strongly interacting. We have performed terahertz spectroscopy on films of the conducting pyrochlore Pr$_2$Ir$_2$O$_7$, which has been shown to host a quadratic band touching. A dielectric constant as large as $\tilde{\varepsilon }/ε_0 \sim 180 $ is observe…
Superconducting instability can occur in three-dimensional quadratic band crossing semimetals only at a finite coupling strength, due to the vanishing of density of states at the quadratic band touching point. Since realistic materials are always disordered to some extent, we study the effect of short-ranged correlated disorder on this superconducting quantum critical point, using a controlled loop-expansion applying dimensional regularization. The renormalization group (RG) scheme allows us to determine the RG flows of the various interaction strengths, and shows that disorder destroys the su…
We investigate the superconductivity of 3D Luttinger semimetals, such as YPtBi, where Cooper pairs are constituted of spin-3/2 quasiparticles. Various pairing mechanisms have already been considered for these semimetals, such as from polar phonons modes, and in this work we explore pairing from the screened electron-electron Coulomb repulsion. In these materials, the small Fermi energy and the spin-orbit coupling strongly influence how charge fluctuations can mediate pairing. We find the superconducting critical temperature as a function of doping for an s-wave order parameter, and determine i…
Luttinger's theorem is a fundamental result in the theory of interacting Fermi systems: it states that the volume inside the Fermi surface is left invariant by interactions, if the number of particles is held fixed. Although this is traditionally justified using perturbation theory, it can be viewed as arising from a momentum balance argument that examines the response of the ground state to the insertion of a single flux quantum [M. Oshikawa, Phys. Rev. Lett. 84, 3370 (2000)]. This reveals that the Fermi sea volume is a topologically protected quantity. Extending this approach, I show that sp…
Topological superconductivity in multiband systems has received much attention due to a variety of possible exotic superconducting order parameters as well as non-trivial bulk and surface states. While the impact of coexisting magnetic order on superconductivity has been studied for many years, such as ferromagnetic superconductors, the implication of coexisting multipolar order has not been explored much despite the possibility of multipolar hidden order in a number of $f$-electron materials. In this work, we investigate topological properties of multipolar superconductors that may arise when…
Luttinger's theorem connects a basic microscopic property of a given metallic crystalline material, the number of electrons per unit cell, to the volume, enclosed by its Fermi surface, which defines its low-energy observable properties. Such statements are valuable since, in general, deducing a low-energy description from microscopics, which may perhaps be regarded as the main problem of condensed matter theory, is far from easy. In this paper we present a unified framework, which allows one to discuss Luttinger theorems for ordinary metals, as well as closely analogous exact statements for to…
We illuminate the intriguing role played by spatial anisotropy in three-dimensional Luttinger semimetals featuring quadratic band touching and long-range Coulomb interactions. We observe the anisotropy to be subject to an exceptionally slow renormalization group (RG) evolution so that it can be considered approximately constant when computing the impact of quantum fluctuations on the remaining couplings of the system. Using perturbative RG we then study the competition of all local short-range interactions that are generated from the long-range interactions for fixed anisotropy. Two main effec…
We study the band structure topology and engineering from the interplay between local moments and itinerant electrons in the context of pyrochlore iridates. For the metallic iridate Pr$_2$Ir$_2$O$_7$, the Ir $5d$ conduction electrons interact with the Pr $4f$ local moments via the $f$-$d$ exchange. While the Ir electrons form a Luttinger semimetal, the Pr moments can be tuned into an ordered spin ice with a finite ordering wavevector, dubbed "Melko-Hertog-Gingras" state, by varying Ir and O contents. We point out that the ordered spin ice of the Pr local moments generates an internal magnetic …
We consider the three-dimensional spin-orbit-coupled Luttinger semimetal of "spin" $3/2$ particles in presence of weak attractive interaction in the $l=1$ (p-wave) channel, and determine the low-temperature phase diagram for both particle- and hole-dopings. The phase diagram depends crucially on the sign of the chemical potential, with two different states (with total angular momentum $j=0$ and $j=3$) competing on the hole-doped side, and three (one $j=1$ and two different $j=2$) states on the particle-doped side. The ground state condensates of Cooper pairs with the total angular momentum $j=…
We investigate the optical response properties of three-dimensional Luttinger semimetals with the Fermi energy close to a quadratic band touching point. In particular, in order to address recent experiments on the spectroscopy of Pyrochlore Iridates and half-Heusler superconductors, we derive expressions for the optical conductivity in both the normal and general superconducting states in the linear response regime within the random phase approximation. The response functions can be decomposed into contributions from intraband and interband transitions, the latter comprising a genuine signatur…
We investigate topological Cooper pairing, including gapless Weyl and fully gapped class DIII superconductivity, in a three-dimensional doped Luttinger semimetal. The latter describes effective spin-3/2 carriers near a quadratic band touching and captures the normal-state properties of the 227 pyrochlore iridates and half-Heusler alloys. Electron-electron interactions may favor non-$s$-wave pairing in such systems, including even-parity $d$-wave pairing. We argue that the lowest energy $d$-wave pairings are always of complex (e.g., $d + i d$) type, with nodal Weyl quasiparticles. This implies …
In this paper, we review recent development in the theory of resonant inelastic light (Raman) scattering in one-dimensional electron systems. The particular systems we have in mind are electron doped GaAs based semiconductor quantum wire nanostructures, although the theory can be easily modified to apply to other one-dimensional systems. We compare the traditional conduction-band-based non-resonant theories with the full resonant theories including the effects of interband transitions. We find that resonance is essential in explaining the experimental data in which the single particle excitati…
We report a polarized Raman study of Weyl semimetal TaAs. We observe all the optical phonons, with energies and symmetries consistent with our first-principles calculations. We detect additional excitations assigned to multiple-phonon excitations. These excitations are accompanied by broad peaks separated by 140~cm$^{-1}$ that are also most likely associated with multiple-phonon excitations. We also noticed a sizable B$_1$ component for the spectral background, for which the origin remains unclear.
We investigate unconventional superconductivity in three-dimensional electronic systems with the chemical potential close to a quadratic band touching point in the band dispersion. Short-range interactions can lead to d-wave superconductivity, described by a complex tensor order parameter. We elucidate the general structure of the corresponding Ginzburg--Landau free energy and apply these concepts to the case of an isotropic band touching point. For vanishing chemical potential, the ground state of the system is given by the superconductor analogue of the uniaxial nematic state, which features…
This chapter describes topological (Dirac and Weyl) semimetals from the viewpoint of their observable electromagnetic response. We argue that this response may be represented by topological terms with unquantized (non-integer) coefficients and make a connection with the Luttinger's theorem, which relates the size of the Fermi surface of an ordinary metal to the number of electrons per unit cell. We discuss observable transport phenomena, associated with this topological response.
A theory of resonant Raman scattering spectroscopy of one dimensional electronic systems is developed on the assumptions that (i) the excitations of the one dimensional electronic system are described by the Luttinger Liquid model, (ii) Raman processes involve virtual excitations from a filled valence band to an empty state of the one dimensional electronic system and (iii) excitonic interactions between the valence and conduction bands may be neglected. Closed form analytic expressions are obtained for the Raman scattering cross sections, and are evaluated analytically and numerically for sca…
We present the theoretical basis for analyzing resonant Raman scattering experiments in one-dimensional systems described by the Luttinger liquid fixed point. We make experimentally testable predictions for distinguishing Luttinger liquids from Fermi liquid and argue that presently available quantum wire systems are \textit{not} in the regime where Luttinger liquid effects are important.
We study finite temperature transport in the Luttinger-Abrikosov-Beneslavskii phase -- an interacting, scale invariant, non-Fermi liquid phase found in quadratic semimetals. We develop a kinetic equation formalism to describe the d.c. transport properties, which are dominated by collisions, and compute the shear viscosity $η$. The ratio of shear viscosity to entropy density $η/s$ is a measure of the strength of interaction between the excitations of a quantum fluid. As a consequence of the quantum critical nature of the system, $η/ s$ is a universal number and we find it to be consistent with …
We used Raman light scattering to study the current-stabilized nonequilibrium semimetallic and metallic phases in Ca$_2$RuO$_4$. By determining the local temperature through careful analysis of the Stokes and anti-Stokes intensities, we find that Joule heating can be completely avoided by supplying sufficient cooling power in a helium-flow cryostat, and that the current induces the semimetallic state without inducing any significant heating. We further investigate the current-induced semimetallic state as a function of temperature and current. We confirm the absence of long-range antiferromagn…
Topological semimetals are a new class of metallic materials, which exist at band fillings that ordinarily correspond to insulators or compensated accidental semimetals with zero Luttinger volume. Their metallicity is a result of nontrivial topology in momentum space and crystal symmetry, wherein topological charges may be assigned to point band-touching nodes, preventing gap opening, unless protecting crystal symmetries are violated. These topological charges, however, are defined from noninteracting band eigenstates, which raises the possibility that the physics of topological semimetals may…
We analyze a model of two-leg Hubbard ladders weakly coupled by interladder tunneling. At half filling a semimetallic state with small Fermi pockets is induced beyond a threshold tunneling strength. The sign changes in the single electron Green's function relevant for the Luttinger Sum Rule now take place at surfaces with both zeroes and infinities with important consequences for the interpretation of ARPES experiments. Residual interactions between electron and hole-like quasi-particles cause a transition to long range order at low temperatures. The theory can be extended to small doping lead…
We determine the shear viscosity and the dc electrical conductivity of interacting three-dimensional Luttinger semimetals, which have a quadratic band touching point in the energy spectrum, in the hydrodynamic regime. It is well-known that when the chemical potential is right at the band touching point the long-range Coulomb interaction induces the Luttinger-Abrikosov-Beneslavskii (LAB) phase at T = 0, which is an interacting, scale-invariant, non-Fermi-liquid state of electrons. Upon combining the renormalization-group (RG) analysis near the upper critical spatial dimension of four with the B…
The interplay of electronic correlations, multi-orbital excitations, and strong spin-orbit coupling is a fertile ground for new states of matter in quantum materials. Here, we report on a confocal Raman scattering study of momentum-resolved charge dynamics from a thin film of semimetallic perovskite $\mathbf{SrIrO_3}$. We demonstrate that the charge dynamics, characterized by a broad continuum, is well described in terms of the marginal Fermi liquid phenomenology. In addition, over a wide temperature regime, the inverse scattering time is for all momenta close to the Planckian limit $\mathbf{τ…
Recently, the notion of topological phases of matter has been extended to higher-order incarnations, supporting gapless modes on even lower dimensional boundaries, such as corners and hinges. We here identify a collection of cubic spin-3/2 fermions with biquadratic touching of Kramers degenerate valence and conduction bands as a platform to strain-engineer higher-order topological (HOT) phases: external uniaxial strain gives birth to a HOT Dirac semimetal or an insulator, depending on its sign, featuring topological \emph{hinge} modes in the strain direction. The insulator in fact exhibits \em…
We study the competition between Kondo screening and frustrated magnetism on the non-symmorphic Shastry-Sutherland Kondo lattice at a filling of two conduction electrons per unit cell. A previous analysis of this model identified a set of gapless partially Kondo screened phases intermediate between the Kondo-destroyed paramagnet and the heavy Fermi liquid. Based on crystal symmetries, we argue that (i)~both the paramagnet and the heavy Fermi liquid are {\it semimetals} protected by a glide symmetry; and (ii)~partial Kondo screening breaks the symmetry, removing this protection and allowing the…
We present a review of theoretical investigations into the Kohn-Luttinger nonphonon superconductivity mechanism in various 3D and 2D repulsive electron systems described by the Fermi-gas, Hubbard, and Shubin-Vonsovsky models. Phase diagrams of the superconducting state are considered, including regions of anomalous $s$-, $p$-, and $d$-wave pairing. The possibility of a strong increase in the superconducting transition temperature $T_c$ even for a low electron density is demonstrated by analyzing the spin-polarized case or the two-band situation. The Kohn-Luttinger theory explains or predicts s…
Topological semimetals have revealed a wide array of novel transport phenomena, including electron hydrodynamics, quantum field theoretic anomalies, and extreme magnetoresistances and mobilities. However, the scattering mechanisms central to these behaviors remain largely unexplored. Here we reveal signatures of significant phonon-electron scattering in the type-II Weyl semimetal WP$_{2}$ via temperature-dependent Raman spectroscopy. Over a large temperature range, we find that the decay rates of the lowest energy $A_{1}$ modes are dominated by phonon-electron rather than phonon-phonon scatter…
Layered van der Waals semimetallic $T_\mathrm{d}$-WTe$_{2}$, exhibiting intriguing properties which include non-saturating extreme positive magnetoresistance (MR) and tunable chiral anomaly, has emerged as model topological type-II Weyl semimetal system. Here, $\sim$45 nm thick mechanically exfoliated flakes of $T_\mathrm{d}$-WTe$_{2}$ are studied $via$ atomic force microscopy, Raman spectroscopy, low-$T$/high-$μ_{0}H$ magnetotransport measurements and optical reflectivity. The contribution of anisotropy of the Fermi liquid state to the origin of the large positive transverse $\mathrm{MR}_\per…
In spin-1/2 Mott insulators, non-magnetic quantum liquid phases are often argued to arise when the system shows no magnetic ordering, but identifying positive signatures of these phases or related spinon quasiparticles can be elusive. Here we use Raman scattering to provide three signatures for spinons in a possible spin-orbit quantum liquid material Ba${}_4$Ir${}_3$O${}_{10}$: (1) A broad hump, which we show can arise from Luttinger Liquid spinons in Raman with parallel photon polarizations normal to 1D chains; (2) Strong phonon damping from phonon-spin coupling via the spin-orbit interaction…
We propose a scheme to dynamically generate optical flux lattices with nontrivial band topology using amplitude-modulated Raman lasers and radio-frequency (rf) magnetic fields. By tuning the strength of Raman and rf fields, three distinct phases are realized at unit filling for a unit cell. Respectively, these three phases correspond to normal insulator, topological Chern insulator, and semimetal. Nearly nondispersive bands are found to appear in the topological phase, which promises opportunities for investigating strongly correlated quantum states within a simple cold-atom setup. The validit…
We present experimental evidence of an intriguing phase transition between distinct topological states in the type-II Weyl semimetal MoTe2. We observe anomalies in the Raman phonon frequencies and linewidths as well as electronic quasielastic peaks around 70 K, which, together with structural, thermodynamic measurements, and electron-phonon coupling calculations, demonstrate a temperature-induced transition between two topological phases previously identified by contrasting spectroscopic measurements. An analysis of experimental data suggests electron-phonon coupling as the main driving mechan…
TaAs as one of the experimentally discovered topological Weyl semimetal has attracted intense interests recently. The ambient TaAs has two types of Weyl nodes which are not on the same energy level. As an effective way to tune lattice parameters and electronic interactions, high pressure is becoming a significant tool to explore new materials as well as their exotic states. Therefore, it is highly interesting to investigate the behaviors of topological Weyl fermions and possible structural phase transitions in TaAs under pressure. Here, with a combination of ab initio calculations and crystal …
We compare two crystallographic phases of the low-dimensional WP$_2$ to better understand features of electron-electron and electron-phonon interactions in topological systems. The topological $β$-phase, a Weyl semimetal with a giant magneto-resistance, shows a larger intensity of electronic Raman scattering compared to the topologically trivial $α$-phase. This intensity sharply drops for $T < T^* = 20$ K which evidences a crossover in the topological phase from marginal quasiparticles to a coherent low temperature regime. In contrast, the non-topological $α$-phase shows more pronounced signat…
New plasmon-like mode in PdTe$_{2}$: Raman scattering and memory function study
Physical Research Laboratory（物理研究实验室）；Indian Institute of Technology, Gandhinagar（印度理工学院甘地纳加尔分校）；School of Physical Sciences, Indian Institute of Technology Mandi（印度理工学院曼迪校物理科学学院）
We present inelastic light scattering measurements of EuO and Eu$_{1-x}$La$_{x}$B$_6$ ($x$=0, 0.005, 0.01, 0.03, and 0.05) as functions of doping, B isotope, magnetic field, and temperature. Our results reveal a variety of distinct regimes as a function of decreasing T: (a) a paramagnetic semimetal regime, which is characterized by a collision-dominated electronic scattering response whose scattering rate $Γ$ decreases with decreasing temperature; (b) a spin-disorder scattering regime, which is characterized by a collision-dominated electronic scattering response whose scattering rate $Γ$ scal…
A grand challenge underlies the entire field of topology-enabled quantum logic and information science: how to establish topological control principles driven by quantum coherence and understand the time-dependence of such periodic driving? Here we demonstrate a THz pulse-induced phase transition in Dirac materials that is periodically driven by vibrational coherence due to excitation of the lowest Raman-active mode. Above a critical field threshold, there emerges a long-lived metastable phase with unique Raman coherent phonon-assisted switching dynamics, absent for optical pumping. The switch…
