We theoretically analyze recent experiments [G. Semeghini et al., Science 374, 1242 (2021)] demonstrating the onset of a topological spin liquid using a programmable quantum simulator based on Rydberg atom arrays. In the experiment, robust signatures of topological order emerge in out-of-equilibrium states that are prepared using a quasi-adiabatic state preparation protocol. We show theoretically that the state preparation protocol can be optimized to target the fixed point of the topological phase -- the resonating valence bond (RVB) state of hard dimers -- in a time that scales linearly with the number of atoms. Moreover, we provide a two-parameter variational manifold of tensor network (TN) states that accurately describe the many-body dynamics of the preparation process. Using this approach we analyze the nature of the non-equilibrium state, establishing the emergence of topological order.
We propose and analyze an approach for preparation of high fidelity entanglement and antiferromagnetic states using Rydberg mediated interactions with dissipation. Using asymmetric Rydberg interactions the two-atom Bell singlet is a dark state of the Rydberg pumping process. Master equation simulations demonstrate Bell singlet preparation fidelity $\mcF=0.998$. Antiferromagnetic states are generated on a four spin plaquette in agreement with results found from diagonalization of the transverse field Ising Hamiltonian.
We describe the dynamical preparation of anisotropic crystalline phases obtained by laser-exciting ultracold Alkali atoms to Rydberg p-states where they interact via anisotropic van der Waals interactions. We develop a time- dependent variational mean field ansatz to model large, but finite two-dimensional systems in experimentally accessible parameter regimes, and we present numerical simulations to illustrate the dynamical formation of anisotropic Rydberg crystals.
Motivated by recent progress in the experimental manipulation of cold atoms in optical lattices, we study three different protocols for non-adiabatic quantum state preparation and state transport in chains of Rydberg atoms. The protocols we discuss are based on the blockade mechanism between atoms which, when excited to a Rydberg state, interact through a van der Waals potential, and rely on single-site addressing. Specifically, we discuss protocols for efficient creation of an antiferromagnetic GHZ state, a class of matrix product states including a so-called Rydberg crystal and for the state…
We examine the adiabatic preparation of crystalline phases of Rydberg excitations in a one-dimensional lattice gas by frequency sweep of the excitation laser, as proposed by Pohl et al. [Phys. Rev. Lett. 104, 043002 (2010)] and recently realized experimentally by Schauß et al. [Science 347, 1455 (2015)]. We find that the preparation of crystals of a few Rydberg excitations in a unitary system of several tens of atoms requires exceedingly long times for the adiabatic following of the ground state of the system Hamiltonian. Using quantum stochastic (Monte-Carlo) wavefunction simulations, we show…
Alkaline earth Rydberg atoms are very promising tools for quantum technologies. Their highly excited outer electron provides them with the remarkable properties of Rydberg atoms and, notably, with a huge coupling to external fields or to other Rydberg atoms while the ionic core retains an optically active electron. However, low angular-momentum Rydberg states suffer almost immediate autoionization when the core is excited. Here, we demonstrate that strontium circular Rydberg atoms with a core excited in a $4D$ metastable level are impervious to autoionization over more than a few millisecond t…
We propose a technique for engineering momentum-dependent dissipation in Bose-Einstein condensates with non-local interactions. The scheme relies on the use of momentum-dependent dark-states in close analogy to velocity-selective coherent population trapping. During the short-time dissipative dynamics, the system is driven into a particular finite-momentum phonon mode, which in real space corresponds to an ordered structure with non-local density-density correlations. Dissipation-induced ordering can be observed and studied in present-day experiments using cold atoms with dipole-dipole or off-…
We investigate a one-dimensional atomic lattice laser-driven to a Rydberg state, in which engineered dissipation channels lead to entanglement in the many-body system. In particular, we demonstrate the efficient generation of ground states of a frustration-free Hamiltonian, as well as $W$ states. We discuss the realization of the required coherent and dissipative terms, and we perform extensive numerical simulations characterizing the fidelity of the state preparation procedure. We identify the optimum parameters for high fidelity entanglement preparation and investigate the scaling with the s…
We present a driven dissipative protocol for creating an optical analog of the Laughlin state in a system of Rydberg polaritons in a twisted optical cavity. We envision resonantly driving the system into a 4-polariton state by injecting photons in carefully selected modes. The dissipative nature of the polariton-polariton interactions leads to a decay into a two-polariton analog of the Laughlin state. Generalizations of this technique could be used to explore fractional statistics and anyon based quantum information processing. We also model recent experiments that attempt to coherently drive …
We use coherent excitation of 3-16 atom ensembles to demonstrate collective Rabi flopping mediated by Rydberg blockade. Using calibrated atom number measurements, we quantitatively confirm the expected $\sqrt{N}$ Rabi frequency enhancement to within 4%. The resulting atom number distributions are consistent with essentially perfect blockade. We then use collective Rabi $π$ pulses to produce ${\cal N}=1,2$ atom number Fock states with fidelities of 62% and 48% respectively. The ${\cal N}=2$ Fock state shows the collective Rabi frequency enhancement without corruption from atom number fluctuatio…
We examine the adiabatic preparation of spatially-ordered Rydberg excitations of atoms in finite one-dimensional lattices by frequency-chirped laser pulses, as realized in a number of recent experiments simulating quantum Ising model. Our aims are to unravel the microscopic mechanism of the phase transition from the unexcited state of atoms to the antiferromagnetic-like state of Rydberg excitations by traversing an extended gapless phase, and to estimate the preparation fidelity of the target state in a moderately sized system amenable to detailed numerical analysis. We find that, in the basis…
A proposal for the generation of singlet states of three $Λ$-type Rydberg atoms is presented. The singlet state is prepared through the combination of a Rydberg state and an EPR pair, and the scheme relies on the Rydberg blockade effect which prevents the simultaneous excitation of the two atoms to a Rydberg state. In addition, some frequency detuning between lasers and atomic transitions is set to eliminate the degenerate of the two ground states. And finally, a series of numerical simulations are made to show the feasibility of the scheme.
We demonstrate a new approach for fast preparation, manipulation, and collective readout of an atomic Rydberg-state qubit. By making use of Rydberg blockade inside a small atomic ensemble, we prepare a single qubit within 3~$μ$s with a success probability of $F_p=0.93 \pm 0.02$, rotate it, and read out its state in $6$ $μs$ with a single-shot fidelity of $F_d=0.92 \pm 0.04$. The ensemble-assisted detection is $10^3$ times faster than imaging of a single atom with the same optical resolution, and enables fast repeated non-destructive measurement. We observe qubit coherence times of 15~$μ$s, muc…
Preparation of entangled steady states via dissipation and pumping in Rydberg atoms has been recently found to be useful for quantum information processing. The driven-dissipative dynamics is closely related to the natural linewidth of the Rydberg states and can be usually modulated by engineering the thermal reservior. Instead of modifying the effectively radiative decay, we propose an alternatively optimized scheme, which combines the resonant Rydberg antiblockade excitation and the Lyapunov control of the ground states to speed up the prepration of the singlet state for two interacting Rydb…
Arrays of Rydberg atoms constitute a highly tunable, strongly interacting venue for the pursuit of exotic states of matter. We develop a new strategy for accessing a family of fractionalized phases known as quantum spin liquids in two-dimensional Rydberg arrays. We specifically use effective field theory methods to study arrays assembled from Rydberg chains tuned to an Ising phase transition that famously hosts emergent fermions propagating within each chain. This highly entangled starting point allows us to naturally access spin liquids familiar from Kitaev's honeycomb model, albeit from an e…
Inspired by recent work [A. W. Carr and M. Saffman, Phys. Rev. Lett. 111, 033607 (2013)], we propose a simplified scheme to prepare the two-atom maximally entangled states via dissipative Rydberg pumping. Compared with the former scheme, the simplified one involves less classical laser fields and Rydberg interactions, and the asymmetric Rydberg interactions are avoided. Master equation simulations demonstrate that the fidelity and the Clauser-Horne-Shimony-Holt correlation of the maximally entangled state could reach up to 0.999 and 2.821, respectively, under certain conditions. Furthermore, w…
Inspired by a recent work [Reiter, Reeb, and Sørensen, Phys. Rev. Lett. {\bf117}, 040501 (2016)], we present a simplified proposal for dissipatively preparing a Greenberger-Horne-Zeilinger (GHZ) state of three Rydberg atoms in a cavity. The $Z$ pumping is implemented under the action of the spontaneous emission of $Λ$-type atoms and the quantum Zeno dynamics induced by strong continuous coupling. In the meantime, a dissipative Rydberg pumping breaks up the stability of the state $|{\rm GHZ}_+\rangle$ in the process of $Z$ pumping, making $|{\rm GHZ}_-\rangle$ be the unique steady state of syst…
Dirac Spin Liquid Candidate in a Rydberg Quantum Simulator
Université Paris-Saclay, Institut d’Optique Graduate School, CNRS, Laboratoire Charles Fabry（巴黎萨克雷大学、高等光学学院、法国国家科学研究中心、夏尔·法布里实验室）；Princeton University（普林斯顿大学）；Harvard University（哈佛大学）；Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所）；Max-Born-Institut（马克斯·玻恩研究所）；Nanomaterials and Nanotechnology Research Center (CINN-CSIC), Universidad de Oviedo (UO)（纳米材料与纳米技术研究中心（CINN-CSIC）、阿斯图里亚斯大学）；Carnegie Mellon University（卡内基梅隆大学）
Recently the Rydberg blockade effect has been utilized to realize quantum spin liquid on the kagome lattice. Evidence of quantum spin liquid has been obtained experimentally by directly measuring non-local string order. In this letter, we report a BCS-type variational wave function study of the spin liquid state in this model. This wave function is motivated by mapping the Rydberg blockade model to a lattice gauge theory, where the local gauge conservations replace the role of constraints from the Rydberg blockade. We determine the variational parameter from the experimental measurement of the…
Quantum spin liquids are exotic phases of matter that are prevented from being frozen even at zero temperature, and appear disordered by local probes that monitor the subsystems. Driven by quantum fluctuations, topological spin liquids are manifested by their long-range entanglement, and are characterized by quasiparticles with fractional statistics. Here, we make contact of a 2D Rydberg ice to a QED vacuum of an ultra-high-finesse optical cavity, and dynamically promote the frustrated background field of the spin ice to a $\mathbb{Z}_2$ spin liquid. We characterize the deconfined nature of th…
We investigate the zero-temperature phases of bosonic and fermionic gases confined to one dimension and interacting via a class of finite-range soft-shoulder potentials (i.e. soft-core potentials with an additional hard-core onsite interaction). Using a combination of analytical and numerical methods, we demonstrate the stabilization of critical quantum liquids with qualitatively new features with respect to the Tomonaga-Luttinger liquid paradigm. These features result from frustration and cluster formation in the corresponding classical ground-state. Characteristic signatures of these liquids…
The emergent phases of strongly correlated spin-1/2 Fermi gases of Rydberg dressed atoms in a one dimensional optical lattice are theoretically investigated. At weak coupling a bosonization description is used to demonstrate the ability to drive alternating quantum phase transitions between distinct Luttinger liquids. At strong coupling the ground state develops non-trivial phase separation exhibiting Luttinger liquid ''puddles'' separated by magnetic domain walls due to the interplay of the incommensurate filling and the Rydberg core length scale. These phases can be detected in ultracold gas…
Preparation of a so-called circular state in a Rydberg atom where the projection of the electron angular momentum takes its maximum value is challenging due to the required amount of angular momentum transfer. Currently available protocols for circular state preparation are either accurate but slow or fast but error-prone. Here, we show how to use quantum optimal control theory to derive pulse shapes that realize fast and accurate circularization of a Rydberg atom. In particular, we present a theoretical proposal for optimized radio-frequency pulses that achieve high fidelity in the shortest p…
Recent atomic physics experiments and numerical works have reported complementary signatures of the emergence of a topological quantum spin liquid in models with blockade interactions. However, the specific mechanism stabilizing such a phase remains unclear. Here, we introduce an exact relation between an Ising-Higgs lattice gauge theory on the kagome lattice and blockaded models on Ruby lattices. This relation elucidates the origin of previously observed topological spin liquids by directly linking the latter to a deconfined phase of a solvable gauge theory. By means of exact diagonalization …
The exploration of quantum spin liquids (QSLs) has been guided by different approaches including the resonating valence bond (RVB) picture, deconfined lattice gauge theories and the Kitaev model. More recently, a spin liquid ground state was numerically established on the ruby lattice, inspired by the Rydberg blockade mechanism. Here we unify these varied approaches in a single parent Hamiltonian, in which local fluctuations of anyons stabilize deconfinement. The parent Hamiltonian is defined on kagomé triangles -- each hosting four RVB-like states -- and includes only Ising interactions and s…
Fast and robust cat state preparation utilizing higher order nonlinearities in Rydberg ensembles
Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院）；Freie Universität Berlin（柏林自由大学）；CESQ/ISIS (UMR 7006), CNRS and University of Strasbourg（CNRS与斯特拉斯堡大学 CESQ/ISIS (UMR 7006)）；Nordita, KTH Royal Institute of Technology and Stockholm University（诺尔迪塔，皇家理工学院与斯德哥尔摩大学）；Department of Physics, Stockholm University（斯德哥尔摩大学物理系）；Institute for Theory of Condensed Matter, Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院凝聚态理论研究所）
We study two-photon excitation of Rydberg states of atoms under stimulated adiabatic passage with delayed laser pulses. We find that the combination of strong interaction between the atoms in Rydberg state and the spontaneous decay of the intermediate exited atomic state leads to the Rydberg excitation of precisely one atom within the atomic ensemble. The quantum Zeno effect offers a lucid interpretation of this result: the Rydberg blocked atoms repetitively scattering photons effectively monitor a randomly excited atom which therefore remains in the Rydberg state. This system can be used for …
Strongly interacting arrays of Rydberg atoms provide versatile platforms for exploring exotic many-body phases and dynamics of correlated quantum systems. Motivated by recent experimental advances, we show that the combination of Rydberg interactions and appropriate lattice geometries naturally leads to emergent $\mathbb{Z}_2$ gauge theories endowed with matter fields. Based on this mapping, we describe how Rydberg platforms could realize two distinct classes of topological $\mathbb{Z}_2$ quantum spin liquids, which differ in their patterns of translational symmetry fractionalization. We also …
The ability to prepare non-classical states in a robust manner is essential for quantum sensors beyond the standard quantum limit. We demonstrate that Bayesian optimal control is capable of finding control pulses that drive trapped Rydberg atoms into highly entangled GHZ states. The control sequences have a physically intuitive functionality based on the quasi-integrability of the Ising dynamics. They can be constructed in laboratory experiments resulting in preparation times that scale very favourably with the system size.
We study the quantum melting of quasi-one-dimensional lattice models in which the dominant energy scale is given by a repulsive dipolar interaction. By constructing an effective low-energy theory, we show that the melting of crystalline phases can occur into two distinct liquid phases, having the same algebraic decay of density-density correlations, but showing a different non-local correlation function expressing string order. We present possible experimental realizations using ultracold atoms and molecules, introducing an implementation based on resonantly driven Rydberg atoms that offers ad…
Arrays of optically trapped atoms excited to Rydberg states have recently emerged as a competitive physical platform for quantum simulation and computing, where high-fidelity state preparation and readout, quantum logic gates and controlled quantum dynamics of more than 100 qubits have all been demonstrated. These systems are now approaching the point where reliable quantum computations with hundreds of qubits and realistically thousands of multiqubit gates with low error rates should be within reach for the first time. In this article we give an overview of the Rydberg quantum toolbox, emphas…
We present optimal control protocols to prepare different many-body quantum states of Rydberg atoms in optical lattices. Specifically, we show how to prepare highly ordered many-body ground states, GHZ states as well as some superposition of symmetric excitation number Fock states, that inherit the translational symmetry from the Hamiltonian, within sufficiently short excitation times minimizing detrimental decoherence effects. For the GHZ states, we propose a two-step detection protocol to experimentally verify the optimal preparation of the target state based only on standard measurement tec…
We devise a cold-atom approach to realizing a broad range of bi-linear quantum magnets. Our scheme is based on off-resonant single-photon excitation of Rydberg $P$-states (Rydberg-dressing), whose strong interactions are shown to yield controllable XYZ-interactions between effective spins, represented by different atomic ground states. The distinctive features of Förster-resonant Rydberg atom interactions are exploited to enhance the effectiveness of Rydberg-dressing and, thereby, yield large spin-interactions that greatly exceed corresponding decoherence rates. We illustrate the concept on a …
The exquisite properties of Rydberg levels make them particularly appealing for emerging quantum technologies. The lifetime of low-angular-momentum laser-accessible levels is however limited to a few $100\,μ\mathrm{s}$ by optical transitions and microwave blackbody radiation (BBR) induced transfers at room temperature. A considerable improvement would be obtained with the few $10\,\mathrm{ms}$ lifetime of circular Rydberg levels in a cryogenic environment reducing the BBR temperature. We demonstrate the preparation of long-lived circular Rydberg levels of laser-cooled Rubidium atoms in a cryos…
We study the Landau-Zener (LZ) dynamics in a setup of two Rydberg atoms with time-dependent detuning, both linear and periodic, using both the exact numerical calculations as well as the method of adiabatic impulse approximation (AIA). By varying the Rydberg-Rydberg interaction strengths, the system can emulate different three-level LZ models, for instance, bow-tie and triangular LZ models. The LZ dynamics exhibits non-trivial dependence on the initial state, the quench rate, and the interaction strengths. For large interaction strengths, the dynamics is well captured by AIA. In the end, we an…
We analyze the zero-temperature phases of an array of neutral atoms on the kagome lattice, interacting via laser excitation to atomic Rydberg states. Density-matrix renormalization group calculations reveal the presence of a wide variety of complex solid phases with broken lattice symmetries. In addition, we identify a novel regime with dense Rydberg excitations that has a large entanglement entropy and no local order parameter associated with lattice symmetries. From a mapping to the triangular lattice quantum dimer model, and theories of quantum phase transitions out of the proximate solid p…
Removing exactly one photon from an arbitrary input pulse is an elementary operation in quantum optics and enables applications in quantum information processing and quantum simulation. Here we demonstrate a deterministic single-photon absorber based on the saturation of an optically thick free-space medium by a single photon due to Rydberg blockade. Single-photon subtraction adds a new component to the Rydberg quantum optics toolbox, which already contains photonic logic building-blocks such as single-photon sources, switches, transistors, and conditional $π$-phase shifts. Our approach is sca…
