We analyze the zero-temperature phases of an array of neutral atoms on the kagome lattice, interacting via laser excitation to atomic Rydberg states. Density-matrix renormalization group calculations reveal the presence of a wide variety of complex solid phases with broken lattice symmetries. In addition, we identify a novel regime with dense Rydberg excitations that has a large entanglement entropy and no local order parameter associated with lattice symmetries. From a mapping to the triangular lattice quantum dimer model, and theories of quantum phase transitions out of the proximate solid phases, we argue that this regime could contain one or more phases with topological order. Our results provide the foundation for theoretical and experimental explorations of crystalline and liquid states using programmable quantum simulators based on Rydberg atom arrays.
The exploration of quantum spin liquids (QSLs) has been guided by different approaches including the resonating valence bond (RVB) picture, deconfined lattice gauge theories and the Kitaev model. More recently, a spin liquid ground state was numerically established on the ruby lattice, inspired by the Rydberg blockade mechanism. Here we unify these varied approaches in a single parent Hamiltonian, in which local fluctuations of anyons stabilize deconfinement. The parent Hamiltonian is defined on kagomé triangles -- each hosting four RVB-like states -- and includes only Ising interactions and s…
Two-dimensional Rydberg atoms are modeled at low temperatures by means of the classical Monte Carlo method. The Coulomb repulsion of charged ions competing with the repulsive van der Waals long-range tail is modeled by a number of interaction potentials. We find that under specific conditions the usual triangular crystal becomes unstable with respect to more exotic lattices such as Kagomé, flower, molecular crystal and rectangular chain packings. Ground-state configurations are obtained by means of the annealing procedure and their stability is additionally studied by the normal modes analysis…
Recurrent neural network wave functions for Rydberg atom arrays on kagome lattice
Department of Applied Mathematics, University of Waterloo（应用数学系，滑铁卢大学）；Perimeter Institute for Theoretical Physics（理论物理研究所）；Department of Physics and Astronomy, University of Waterloo（物理与天文学系，滑铁卢大学）；Vector Institute（向量研究所）；AWS Center for Quantum Computing（AWS量子计算中心）；Institute for Theoretical Physics, ETH Zürich（理论物理研究所，苏黎世联邦理工学院）
Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary Rydberg excitation becomes unlikely leading to the Rydberg blockade effect. In a related effect, off-resonant coupling of light to Rydberg states of atoms contributes to the Rydberg anti-blockade effect where the Rydberg interaction creates a resonant condition that promotes a secondary excitation in a Rydberg atomic gas. Here, we study the light-matter interact…
We propose a scheme to implement an optical Kagome lattice for ultra-cold atoms with controllable s-wave interactions between nearest neighbor sites and a gauge potential. The atoms occupy three different internal atomic levels with electromagnetically-induced coupling between the levels. We show that by appropriately shifting the triangular lattice potentials, experienced by atoms in different levels, the Kagome lattice can be realized using only two standing waves, generating a highly frustrated quantum system for the atoms.
Hybrid quantum systems involving cold atoms and microwave resonators can enable cavity-mediated infinite-range interactions between atomic spin systems and realize atomic quantum memories and transducers for microwave to optical conversion. To achieve strong coupling of atoms to on-chip microwave resonators, it was suggested to use atomic Rydberg states with strong electric dipole transitions. Here we report on the realization of coherent coupling of a Rydberg transition of ultracold atoms trapped on an integrated superconducting atom chip to the microwave field of an on-chip coplanar waveguid…
We propose a scheme to simulate lattice spin models based on strong and long-range interacting Rydberg atoms stored in a large-spacing array of magnetic microtraps. Each spin is encoded in a collective spin state involving a single $nP$ Rydberg atom excited from an ensemble of ground-state alkali atoms prepared via Rydberg blockade. After the excitation laser is switched off the Rydberg spin states on neighbouring lattice sites interact via general isotropic or anisotropic spin-spin interactions. To read out the collective spin states we propose a single Rydberg atom triggered avalanche scheme…
Results of numerical Monte Carlo simulations for the Stark-tuned Förster resonance and dipole blockade between two to five cold rubidium Rydberg atoms in various spatial configurations are presented. The effects of the atoms' spatial uncertainties on the resonance amplitude and spectra are investigated. The feasibility of observing coherent Rabi-like population oscillations at a Förster resonance between two cold Rydberg atoms is analyzed. Spectra and the fidelity of the Rydberg dipole blockade are calculated for various experimental conditions, including nonzero detuning from the Förster reso…
Non-destructive optical read-out and manipulation of circular Rydberg atoms
Laboratoire Kastler Brossel, Collège de France, CNRS, ENS-Université PSL, Sorbonne Université（卡斯特尔-布罗塞尔实验室，法兰西公学院，法国国家科学研究中心，巴黎高等师范学院-巴黎文理研究大学，索邦大学）；Institut Universitaire de France（法兰西学院）
The dipole blockade effect at laser excitation of mesoscopic ensembles of Rydberg atoms lies in the fact that the excitation of one atom to a Rydberg state blocks the excitation of other atoms due to the shift in the collective energy levels of interacting Rydberg atoms. It is used to obtain the entangled qubit states based on single neutral atoms in optical traps. In this paper, we present our experimental results on the observation of the dipole blockade for mesoscopic ensembles of 1-5 atoms when they are detected by the selective field ionization method. We investigated the spectra of the t…
Due to the intrinsic strong blockaded interaction shifting the energy level of Rydberg state, the steady Rydberg probability may be substantially restrained to a low level, especially for atoms suffering from weak drivings. We report an exotic excitation facilitation using strong blockaded energy shifting the double excitation state, leading to the weakly-driven atom deterministically excited by a significantly improved fraction even at far off-resonant regimes. This phenomenon is attributed to the effective induction of a reduced detuning to the weakly-driven atom by optimizing parameters of …
Three-body Förster resonances at long-range interactions of Rydberg atoms were first predicted and observed in Cs Rydberg atoms by R.Faoro et al., Nature Comm. 6, 8173 (2015). In these resonances, one of the atoms carries away an energy excess preventing the two-body resonance, leading thus to a Borromean type of Förster energy transfer. But they were in fact observed as the average signal for the large number of atoms $N\gg1$. In this Letter we report on the first experimental observation of the three-body Förster resonances ${\rm 3}\times nP_{3/2} (|{\rm M}|)\to nS_{1/2} +(n+1)S_{1/2} +nP_{3…
Recent experiments with Bose-Einstein condensates have entered a regime in which thousands of ground-state condensate atoms fill the Rydberg-electron orbit. After the excitation of a single atom into a highly excited Rydberg state, scattering off the Rydberg electron sets ground-state atoms into motion, such that one can study the quantum-many-body dynamics of atoms moving within the Rydberg atom. Here we study this many-body dynamics using Gross-Pitaevskii and truncated Wigner theory. Our simulations focus in particular on the scenario of multiple sequential Rydberg excitations on the same Ru…
We demonstrate three-dimensional trapping of individual Rydberg atoms in holographic optical bottle beam traps. Starting with cold, ground-state $^{87}$Rb atoms held in standard optical tweezers, we excite them to $nS_{1/2}$, $nP_{1/2}$, or $nD_{3/2}$ Rydberg states and transfer them to a hollow trap at 850 nm. For principal quantum numbers $60 \leqslant n \leqslant 90$, the measured trapping time coincides with the Rydberg state lifetime in a 300~K environment. We show that these traps are compatible with quantum information and simulation tasks by performing single qubit microwave Rabi flopp…
We propose an approach to detect individual Rydberg molecules with each molecule consisting of two atoms in different Rydberg states. The scheme exploits the movement of atoms in the presence of an external force that exerts only on atoms in one Rydberg state. Since the movement of atoms in the other Rydberg state depends on whether they are bound with atoms directly driven by the applied force, bound atoms can be distinguished from unbound atoms. By utilizing electromagnetically induced transparency, it is possible to non-destructively image the positions of molecules. The scheme is sensitive…
Quantum information processing based on Rydberg atoms emerged as a promising direction two decades ago. Recent experimental and theoretical progresses have shined exciting light on this avenue. In this concise review, we will briefly introduce the basics of Rydberg atoms and their recent applications in associated areas of neutral atom quantum computation and simulation. We shall also include related discussions on quantum optics with Rydberg atomic ensembles, which are increasingly used to explore quantum computation and quantum simulation with photons.
We investigate the collective excitation effect in a scheme where three identical Rydberg atoms are arranged in an equilateral triangular lattice. By using a static electric field polarizing the atomic dipoles, the dipole-dipole interactions between two Rydberg atoms are essentially anisotropic and can even disappear in the several special resonance cases. For that fact, we observe collectively enhanced excitation probability of single Rydberg atom in resonant areas in the case of strong blockade, and that of double or triple Rydberg atoms in the case of partial blockade. To give more evidence…
We report on the realization of high resolution electron microscopy of Rydberg-excited ultracold atomic samples. The implementation of an ultraviolet laser system allows us to excite the atom, with a single-photon transition, to Rydberg states. By using the electron microscopy technique during the Rydberg excitation of the atoms, we observe a giant enhancement in the production of ions. This is due to $l$-changing collisions, which broaden the Rydberg level and therefore increase the excitation rate of Rydberg atoms. Our results pave the way for the high resolution spatial detection of Rydberg…
An array of single Rydberg atoms driven by a frequency modulated light field is studied. The periodic modulation effectively modifies the Rabi coupling, leading to unprecedented dynamics in the presence of Rydberg-Rydberg interactions. They include state dependent population trapping, the Rydberg blockade for small and anti-blockades at large interaction strengths. Interestingly, the Schrieffer-wolf transformation reveals a fundamental process in Rydberg gases, correlated Rabi oscillations, arising from the long-range interactions, provides an alternative depiction for Rydberg blockade and it …
We experimentally realize Rydberg excitations in Bose-Einstein condensates of rubidium atoms loaded into quasi one-dimensional traps and in optical lattices. Our results for condensates expanded to different sizes in the one-dimensional trap agree well with the intuitive picture of a chain of Rydberg excitations. We also find that the Rydberg excitations in the optical lattice do not destroy the phase coherence of the condensate, and our results in that system agree with the picture of localized collective Rydberg excitations including nearest-neighbour blockade.
We propose to track position and velocity of mobile Rydberg excited impurity atoms through the elastic interactions of the Rydberg electron with a host condensate. Tracks first occur in the condensate phase, but are then naturally converted to features in the condensate density or momentum distribution. The condensate thus acts analogous to the cloud or bubble chambers in the early days of elementary particle physics. The technique will be useful for exploring Rydberg-Rydberg scattering, rare inelastic processes involving the Rydberg impurities, coherence in Rydberg motion and forces exerted b…
We numerically analyze the impact of a single Rydberg electron onto a Bose-Einstein condensate. Both $S-$ and $D-$ Rydberg states are studied. The radial size of $S-$ and $D-$states are comparable, hence the only difference is due to the angular dependence of the wavefunctions. We find the atom losses in the condensate after the excitation of a sequence of Rydberg atoms. Additionally, we investigate the mechanical effect in which the Rydberg atoms force the condensate to oscillate. Our numerical analysis is based on the classical fields approximation. Finally, we compare numerical results to e…
Rydberg blockade sphere persists an intriguing picture by which a number of collective many-body effects caused by the strong Rydberg-Rydberg interactions can be clearly understood and profoundly investigated. In the present work, we develop a new definition for the effective two-atom blockade radius and show that the original spherically shaped blockade surface would be deformed when the real number of atoms increases from two to three. This deformation of blockade sphere reveals spatially anisotropic and shrunken properties which strongly depend on the interatomic distance. In addition, we a…
We study a driven-dissipative system of atoms in the presence of laser excitation to a Rydberg state and spontaneous emission. The atoms interact via the blockade effect, whereby an atom in the Rydberg state shifts the Rydberg level of neighboring atoms. We use mean-field theory to study how the Rydberg population varies in space. As the laser frequency changes, there is a continuous transition between the uniform and antiferromagnetic phases. The nonequilibrium nature also leads to a novel oscillatory phase and bistability between the uniform and antiferromagnetic phases.
We study an open quantum system of atoms with long-range Rydberg interaction, laser driving, and spontaneous emission. Over time, the system occasionally jumps between a state of low Rydberg population and a state of high Rydberg population. The jumps are inherently collective and in fact exist only for a large number of atoms. We explain how entanglement and quantum measurement enable the jumps, which are otherwise classically forbidden.
We present a novel binding mechanism where a neutral Rydberg atom and an atomic ion form a molecular bound state at large internuclear distance. The binding mechanism is based on Stark shifts and level crossings which are induced in the Rydberg atom due to the electric field of the ion. At particular internuclear distances between Rydberg atom and ion, potential wells occur which can hold atom-ion molecular bound states. Apart from the binding mechanism we describe important properties of the long-range atom-ion Rydberg molecule, such as its lifetime and decay paths, its vibrational and rotati…
We consider a system consisting of Rydberg dressed atoms interacting with BEC condensate of diatomic molecules. Using random phase approximation (RPA) we calculate the effective interactions between Rydberg atoms accounting for their Wan der Waals repulsion and exchange of virtual excitations of the condensate and demonstrate that total interaction can become attractive and BCS state of Rydberg dressed atoms can be formed. Using the example of 6Li atoms we demonstrate that the strength of the interactions can be controlled optically, and BCS regime is achievable at realistic experimental condi…
