The one-dimensional Ising model with its connections to several physical concepts plays a vital role in comprehension of several principles, phenomena and numerical methods. The Hamiltonian of a coupled one-dimensional dissipative spin system in the presence of magnetic field can be obtained from the Ising model. We simulate the above Hamiltonian by designing a quantum circuit with precise gate measurement and execute with the IBMQ experience platform through different $N$ states with controlled energy separation where we can check quantum synchronization in a dissipative lattice system. Our result shows the relation between various entangled states, the relation between the different energy separation ($ω$) with the spin-spin coupling ($λ$) in the lattice, along with fidelity calculations for several iterations of the model used. We also estimate the ground and first excited energy states of Ising-Hamiltonian using VQE algorithm and investigate the lowest energy values varying the number of layers of ansatz.
Synchronization phenomena have been recently reported in the quantum realm at atomic level due to collective dissipation. In this work we propose a dimer lattice of trapped atoms realizing a dissipative spin model where quantum synchronization occurs instead in presence of local dissipation. Atoms synchronization is enabled by the inhomogeneity of staggered local losses in the lattice and is favored by an increase of spins detuning. A comprehensive approach to quantum synchronization based on different measures considered in the literature allows to identify the main features of different sync…
We show that the temperature of a cavity field can be drastically varied by its interaction with suitably-entangled atom pairs (dimers) traversing the cavity under realistic atomic decoherence. To this end we resort to the hitherto untapped resource of naturally entangled dimers whose state can be simply controlled via molecular dissociation, collisions forming the dimer, or unstable dimers such as positronium. Depending on the chosen state of the dimer, the cavity-field mode can be driven to a steady-state temperature that is either much lower or much higher than the ambient temperature, desp…
We predict the existence of high frequency modes in the interference pattern of two condensates made of fermionic-atom dimers. These modes, which result from fermion exchanges between condensates, constitute a striking signature of the dimer composite nature. From the 2-coboson spatial correlation function, that we derive analytically, and the Shiva diagrams that visualize many-body effects specific to composite bosons, we identify the physical origin of these high frequency modes and determine the conditions to see them experimentally by using bound fermionic-atom pairs trapped on optical lat…
Understanding the mechanism through which an open quantum system exchanges information with an environment is central to the creation and stabilization of quantum states. This theme has been explored recently, with attention mostly focused on system control or environment engineering. Here, we bring these ideas together to describe the many-body dynamics of an extended atomic array coupled to a squeezed vacuum. We show that fluctuations can drive the array into a pure dark state decoupled from the environment. The dark state is obtained for an even number of atoms and consists of maximally ent…
A powerful method to interface quantum light with matter is to propagate the light through an ensemble of atoms. Recently, a number of such interfaces have emerged, most prominently Rydberg ensembles, that enable strong nonlinear interactions between propagating photons. A largely open problem is whether these systems produce exotic many-body states of light and developing new tools to study propagation in the large photon number limit is highly desirable. Here, we provide a method based on a "spin model" that maps quasi one-dimensional (1D) light propagation to the dynamics of an open 1D inte…
The shifted Tietz-Wei (sTW) oscillator is as good as traditional Morse potential in simulating the atomic interaction in diatomic molecules. By using the Pekeris-type approximation to deal with the centrifugal term, we obtain the bound-state solutions of the radial Schrödinger equation with this typical molecular model via the exact quantization rule (EQR). The energy spectrum for a set of diatomic molecules ($NO \left(a^4Π_i\right)$, $NO \left(B^2Π_r\right)$, $NO \left(L'^2ϕ\right)$, $NO \left(b^4Σ^{-}\right)$, $ICl\left(X^1Σ_g^{+}\right)$, $ICl\left(A^3Π_1\right)$ and $ICl\left(A'^3Π_2\right…
Diborane (B$_2$H$_6$) is a promising molecular precursor for atomic precision p-type doping of silicon that has recently been experimentally demonstrated [T. {Š}kere{ň}, \textit{et al.,} Nature Electronics (2020)]. We use density functional theory (DFT) calculations to determine the reaction pathway for diborane dissociating into a species that will incorporate as electrically active substitutional boron after adsorbing onto the Si(100)-2$\times$1 surface. Our calculations indicate that diborane must overcome an energy barrier to adsorb, explaining the experimentally observed low sticking coef…
We consider three-body recombination into deep dimers in a mass-imbalanced two-component atomic gas. We use an optical model where a phenomenological imaginary potential is added to the lowest adiabatic hyper-spherical potential. The consequent imaginary part of the energy eigenvalue corresponds to the decay rate or recombination probability of the three-body system. The method is formulated in details and the relevant qualitative features are discussed as functions of scattering lengths and masses. We use zero-range model in analyses of recent recombination data. The dominating scattering len…
We consider the non-equilibrium dynamics of a driven dissipative spin chain with chiral coupling to a 1D bosonic bath, and its atomic implementation with a two-species mixture of cold quantum gases. The reservoir is represented by a spin-orbit coupled 1D quasi-condensate of atoms in a magnetized phase, while the spins are identified with motional states of a separate species of atoms in an optical lattice. The chirality of reservoir excitations allows the spins to couple differently to left and right moving modes, which in our atomic setup can be tuned from bidirectional to purely unidirection…
Conical intersections are common in molecular physics and photochemistry, and are often invoked to explain observed reaction products. A conical intersection can occur when an excited electronic potential energy surface intersects with the ground electronic potential energy surface in the coordinate space of the nuclear positions. Theory predicts that the conical intersection will result in a geometric phase for a wavepacket on the ground potential energy surface. Although conical intersections have been observed experimentally, the geometric phase has not been observed in a molecular system. …
We propose a scheme involving cold atoms trapped in optical lattices to observe different phenomena traditionally linked to quantum-optical systems. The basic idea consists of connecting the trapped atomic state to a non-trapped state through a Raman scheme. The coupling between these two types of atoms (trapped and free) turns out to be similar to that describing light-matter interaction within the rotating-wave approximation, the role of matter and photons being played by the trapped and free atoms, respectively. We explain in particular how to observe phenomena arising from the collective s…
The Efimov effect, with its ladder of weakly bound three-atomic molecules, poses intriguing questions in the theoretically controversial and experimentally demanding regime of merging of the first excited Efimov energy level with the atom-dimer continuum. Using an original experimental technique, where a coherent superposition state of diatomic and triatomic molecules is utilized, we investigate this regime and reveal a striking behavior: Instead of merging with the atom-dimer continuum the trimer energy level rebounds from it and becomes a deeper bound state again. In addition, instead of a t…
Proposals for systems embodying condensed matter spin qubits cover a very wide range of length scales, from atomic defects in semiconductors all the way to micron-sized lithographically-defined structures. Intermediate scale molecular components exhibit advantages of both limits: like atomic defects, large numbers of identical components can be fabricated; as for lithographically defined structures, each component can be tailored to optimize properties such as quantum coherence. Here, we demonstrate what is perhaps the most potent advantage of molecular spin qubits, the scalability of quantum …
Simulating chemical systems on quantum computers has been limited to a few electrons in a minimal basis. We demonstrate experimentally that the virtual quantum subspace expansion [Phys. Rev. X 10, 011004 (2020)] can achieve full basis accuracy for hydrogen and lithium dimers, comparable to simulations requiring twenty or more qubits. We developed an approach to minimize the impact of experimental noise on the stability of the generalized eigenvalue problem, a crucial component of the quantum algorithm. In addition, we were able to obtain an accurate potential energy curve for the nitrogen dime…
Elucidating similarities and differences between quantum-optics biphoton interference phenomena and the quantum physics of quasi-one-dimensional double-well optically-trapped ultracold neutral bosonic or fermionic atoms, we show that the analog of the optical biphoton joint-coincidence spectral correlations, studied with massless non-interacting biphotons emanating from EPR-Bell-Bohm single-occupancy sources, corresponds to a distinct contribution in the total second-order momentum correlations of the massive, interacting, and time-evolving ultracold atoms. This single-occupancy contribution c…
We propose a scheme to simulate lattice spin models based on strong and long-range interacting Rydberg atoms stored in a large-spacing array of magnetic microtraps. Each spin is encoded in a collective spin state involving a single $nP$ Rydberg atom excited from an ensemble of ground-state alkali atoms prepared via Rydberg blockade. After the excitation laser is switched off the Rydberg spin states on neighbouring lattice sites interact via general isotropic or anisotropic spin-spin interactions. To read out the collective spin states we propose a single Rydberg atom triggered avalanche scheme…
We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects. Depending on the considered species, the atomic spin-orbit may be comparable to the atom-molecule electrostatic energy and to the dimer rotational structure. Here we extend our general description in the framework of the second-order degenerate perturbation theory [M. Lepers and O. D…
Single-molecule nuclear magnetic resonance (NMR) is a crown-jewel challenge in the field of magnetic resonance spectroscopy and has important applications in chemical analysis and in quantum computing. Recently, it becomes possible to tackle this grand challenge thanks to experimental advances in preserving quantum coherence of nitrogen-vacancy (NV) center spins in diamond as a sensitive probe and theoretical proposals on atomic-scale magnetometry via dynamical decoupling control. Through decoherence measurement of NV centers under dynamical decoupling control, sensing of single $^{13}\textbf{…
Quantum spin ice represents a paradigmatic example on how the physics of frustrated magnets is related to gauge theories. In the present work we address the problem of approximately realizing quantum spin ice in two dimensions with cold atoms in optical lattices. The relevant interactions are obtained by weakly admixing van der Waals interactions between laser admixed Rydberg states to the atomic ground state atoms, exploiting the strong angular dependence of interactions between Rydberg p-states together with the possibility of designing step-like potentials. This allows us to implement Abeli…
Ultracold atomic lattice systems for simulating topological phases: A review
School of Physics and Institute for Quantum Science and Engineering, Huazhong University of Science and Technology（华中科技大学物理学院与量子科学与工程研究院）；Hefei National Research Center for Physical Sciences at the Microscale and School of Physical Sciences, University of Science and Technology of China（中国科学技术大学微尺度物质科学国家研究中心与物理科学学院）；Shanghai Research Center for Quantum Sciences and CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China（中国科学技术大学上海量子科学研究中心与中科院量子信息重点实验室）；Hefei National Laboratory（合肥国家实验室）
We consider inter-atomic forces due to resonant dipole-dipole interactions within a dimer of highly excited Rydberg atoms, embedded in an ultra-cold gas. These forces rely on a coherent superposition of two-atom electronic states, which is destroyed by continuous monitoring of the dimer state through a detection scheme utilizing controllable interactions with the background gas atoms. We show that this intrinsic decoherence of the molecular energy surface can gradually deteriorate a repulsive dimer state, causing a mixing of attractive and repulsive character. For sufficiently strong decoheren…
