We study the three-body recombination of identical fermionic atoms. Using a zero-range model for the $p$-wave interaction, we show that the rate constant of three-body recombination into weakly bound $p$-wave dimers can be written as $α_{\rm rec} \propto v^{5/2}R^{1/2} k_T^4 (1+ C k_T^2 l_{\rm d}^2)$ for large and positive scattering volume $v$. Here $R$ is the $p$-wave effective range, $k_T^2$ gives the average thermal kinetic energy of the colliding atoms, and $l_{\rm d}$ is the size of the $p$-wave dimer. The leading term is different from the usually stated $v^{8/3}$-scaling law, but is consistent with an earlier two-channel calculation. For the subleading term, we compute the constant $C$ by solving the relevant three-body problem perturbatively when the parameter $γ\equiv R/v^{1/3}$ is small. The additional $C k_T^2 l_{\rm d}^2$ term provides important corrections for the temperature and interaction dependence of $α_{\rm rec}$, especially close to resonance when $k_T l_{\rm d}$ is relatively large.
We report on measurements of three-body recombination rates in an ultracold gas of $^7$Li atoms in the extremely nonuniversal regime where the two-body scattering length vanishes. We show that the rate is well defined and can be described by two-body parameters only: the scattering length $a$ and the effective range $R_e$. We find the rate to be energy independent, and, by connecting our results with previously reported measurements in the universal limit, we cover the behavior of the three-body recombination in the whole range from weak to strong two-body interactions. We identify a nontrivia…
We investigate three-body recombination rates into deep dimers in cold atomic gases with large scattering length within hyper-spherical adiabatic zero-range approach. We derive closed analytic expressions for the rates for one- and two-species gases. Although the deep dimers are beyond the zero-range theory the latter can still describe the recombination into deep dimers by use of one additional short-range absorption parameter. The recombination rate, as function of the scattering length, retains the known universal behavior --- the fourth power trend with characteristic log-periodic peaks --…
We study three-body recombination in two dimensions for systems interacting via short-range two-body interactions in the regime of large scattering lengths. Using the adiabatic hyperspherical representation, we derive semi-analytical formulas for three-body recombination in both weakly and deeply bound diatom states. Our results demonstrate the importance of long-range corrections to the three-body potentials by showing how they alter the low-energy and scattering length dependence of the recombination rate for both bosonic and fermionic systems, which exhibit suppressed recombination if compa…
We consider three-body recombination into deep dimers in a mass-imbalanced two-component atomic gas. We use an optical model where a phenomenological imaginary potential is added to the lowest adiabatic hyper-spherical potential. The consequent imaginary part of the energy eigenvalue corresponds to the decay rate or recombination probability of the three-body system. The method is formulated in details and the relevant qualitative features are discussed as functions of scattering lengths and masses. We use zero-range model in analyses of recent recombination data. The dominating scattering len…
The simplest model for itinerant ferromagnetism, the Stoner model, has so far eluded experimental observation in repulsive ultracold fermions due to rapid three-body recombination at large scattering lengths. Here we show that a ferromagnetic phase can be stabilised by imposing a moderate optical lattice. The reduced kinetic energy drop upon formation of a polarized phase in an optical lattice extends the ferromagnetic phase to smaller scattering lengths where three-body recombination is small enough to permit experimental detection of the phase. We also show, using time dependent density func…
A general method to study classical scattering in $n$-dimension is developed. Through classical trajectory calculations, the three-body recombination is computed as a function of the collision energy for helium atoms, as an example. Quantum calculations are also performed for the $J^Π$ = $0^{+}$ symmetry of the three-body recombination rate in order to compare with the classical results, yielding good agreement for $E\gtrsim$ 1 K. The classical threshold law is derived and numerically confirmed for the Newtonian three-body recombination rate. Finally, a relationship is found between the quantu…
We study theoretically several aspects of the dynamics of coherent atom-molecule conversion in spin-1 Bose-Einstein condensates. Specifically, we discuss how for a suitable dark-state condition the interplay of spin-exchange collisions and photoassociation leads to the stable creation of an atom- molecule pairs from three initial spin-zero atoms. This process involves two two-body interactions and can be intuitively viewed as an effective three-body recombination. We investigate the relative roles of photoassociation and of the initial magnetization in the \resonant" case where the dark state …
In the systems of spin $\frac12$ fermions with resonant $S$-wave interactions supporting only weakly bound dimers the antisymmetry forbids recombination of three (or more) fermions at zero energy. However, the fermion-fermion-dimer recombination is only partially suppressed. It is studied in the framework of momentum-space integral equations for the four-particle transition operators. In the vicinity of the unitary limit the fermion-fermion-dimer recombination rate, rescaled to build dimensionless quantity, is found to be linear in the effective range parameter, enabling a simple and accurate …
Three-body recombination is a prime example of the fundamental interaction between three particles. Due to the complexity of this process it has resisted a comprehensive description. Experimental investigations have mainly focussed on the observation of corresponding loss rates without revealing information on the reaction products. Here, we provide the first general experimental study on the population distribution of molecular quantum states after three-body recombination in a non-resonant regime. We have developed a highly sensitive detection scheme which combines photoionization of the mol…
Three-body recombination in quantum gases is traditionally associated with heating, but it was recently found that it can also cool the gas. We show that in a partially condensed three-dimensional homogeneous Bose gas three-body loss could even purify the sample, that is, reduce the entropy per particle and increase the condensed fraction $η$. We predict that the evolution of $η$ under continuous three-body loss can, depending on small changes in the initial conditions, exhibit two qualitatively different behaviours - if it is initially above a certain critical value, $η$ increases further, wh…
We investigate three-boson recombination of equal mass systems as function of (negative) scattering length, mass, finite energy, and finite temperature. An optical model with an imaginary potential at short distance reproduces experimental recombination data and allows us to provide a simple parametrization of the recombination rate as function of scattering length and energy. Using the two-body van der Waals length as unit we find that the imaginary potential range and also the potential depth agree to within thirty percent for Lithium and Cesium atoms. As opposed to recent studies suggesting…
We discuss the impact of a finite effective range on three-body systems interacting through a large two-body scattering length. By employing a perturbative analysis in an effective field theory well suited to this scale hierarchy we find that an additional three-body parameter is required for consistent renormalization once range corrections are considered. This allows us to extend previously discussed universal relations between different observables in the recombination of cold atoms to account for the presence of a finite effective range. We show that such range corrections allow us to simu…
Three-body recombination is a phenomenon common in atomic and molecular collisions, producing heating in the system. However, we find the cooling effect of the three-body recombination of a 6Li Fermi gas near its s-wave narrow Feshbach resonance. Such counter-intuitive behavior is explained as follows, the threshold energy of the quasi-bounded Feshbach molecule acts as the knife of cooling, expelling the scattering atoms with selected kinetic energy from the trap. When the threshold energy happens to be larger than 3/2kBT, each lost atom in the three-body recombination process has more than 3k…
We combine theory and experiment to investigate five-body recombination in an ultracold gas of atomic cesium at negative scattering length. A refined theoretical model, in combination with extensive laboratory tunability of the interatomic interactions, enables the five-body resonant recombination rate to be calculated and measured. The position of the new observed recombination feature agrees with a recent theoretical prediction and supports the prediction of a family of universal cluster states at negative $a$ that are tied to an Efimov trimer.
Systems of three particles show a surprising feature in their bound state spectrum: a series of geometrically scaled states, known as Efimov states. These states have not yet been observed directly, but many recent experiments show indirect evidence of their existence via the so-called recombination process. The theories that predict the Efimov states also predicts either resonant enhancement of the recombination process or suppression by destructive interference, depending on the sign of the interaction between the particles. The theories predict universal features for the Efimov states, for …
We have studied the three-body recombination rates on both sides of the interspecies d-wave Feshbach resonance in the $^{85}$Rb\,-$^{87}$Rb-$^{87}$Rb system using the $R$-matrix propagation method in the hyperspherical coordinate frame. Two different mechanisms of recombination rate enhancement for positive and negative $^{85}$Rb\,-$^{87}$Rb d-wave scattering lengths are analyzed. On the positive scattering length side, the recombination rate enhancement occurs due to the existence of three-body shape resonance, while on the negative scattering length side, the coupling between the lowest entr…
The mass-imbalanced three-body recombination process that forms a shallow dimer is shown to possess a rich Efimov-Stückelberg landscape, with corresponding spectra that differ fundamentally from the homonuclear case. A semi-analytical treatment of the three-body recombination predicts an unusual spectra with intertwined resonance peaks and minima, and yields in-depth insight into the behavior of the corresponding Efimov spectra. In particular, the patterns of the Efimov-Stückelberg landscape are shown to depend inherently on the degree of diabaticity of the three-body collisions, which strongl…
First-order phase transition in atom-molecule quantum degenerate mixtures with coherent three-body recombination
Missouri University of Science and Technology（密苏里科技大学）；Ben-Gurion University of the Negev（内盖夫本古里安大学）；Harvard & Smithsonian（哈佛大学与史密森尼学会）；University of Chicago（芝加哥大学）
A very recently method for classical trajectory calculations for three-body collision [J. Pérez-Ríos, S. Ragole, J. Wang and C. H. Greene, J. Chem. Phys. {\bf 140}, 044307 (2014)] has been applied to describe ion-neutral-neutral ternary processes for low energy collisions: 0.1 mK - 10 mK. As a result, a threshold law for the three-body recombination cross section is obtained and corroborated both, experimentally and numerically. The derived threshold law predicts the formation of weakly bound dimers, with binding energies comparable to the collision energy of the collisional partners. In this …
We report the creation and the study of the stability of a repulsive quasi-homogeneous spin-$1/2$ Fermi gas with contact interactions. For the range of scattering lengths $a$ explored, the dominant mechanism of decay is a universal three-body recombination towards a Feshbach bound state. We observe that the recombination coefficient $K_3\propto ε_\text{kin} a^6$, where the first factor, the average kinetic energy per particle $ε_\text{kin}$, arises from a three-body threshold law, and the second one from the universality of recombination. Both scaling laws are consequences of Pauli blocking ef…
We experimentally measure, and theoretically analyze the three-atom recombination rate, $L_3$, around a narrow $s$ wave magnetic Feshbach resonance of $^6$Li-$^6$Li at 543.3 Gauss. By examining both the magnetic field dependence and especially the temperature dependence of $L_3$ over a wide range of temperatures from a few $μ$K to above 200 $μ$K, we show that three-atom recombination through a narrow resonance follows a universal behavior determined by the long-range van der Waals potential, and can be described by a set of rate equations in which three-body recombination proceeds via successi…
We study Efimov resonances via three-body loss in an ultracold two-component gas of fermionic $^6$Li and bosonic $^{133}$Cs atoms close to a Feshbach resonance at 843~G, extending results reported previously [Pires \textit{et al.}, Phys. Rev. Lett. 112, 250404 (2014)] to temperatures around 120~nK. The experimental scheme for reaching lower temperatures is based upon compensating the gravity-induced spatial separation of the mass-imbalanced gases with bichromatic optical dipole traps. We observe the first and second excited Li-Cs-Cs Efimov resonance in the magnetic field dependence of the thre…
Within the universal zero-range theory, we compute the three-body recombination rate to deep molecular states for two identical bosons resonantly interacting with each other and with a third atom of another species, in the absence of weakly bound dimers. The results allow for a quantitative understanding of loss resonances at finite temperature and, combined with experimental data, can be used for testing the Efimov universality and extracting the corresponding three-body parameters in a given system. Curiously, we find that the loss rate can be dramatically enhanced by the resonant heavy-heav…
We investigate local three-body correlations for bosonic particles in three and one dimensions as a function of the interaction strength. The three-body correlation function g(3) is determined by measuring the three-body recombination rate in an ultracold gas of Cs atoms. In three dimensions, we measure the dependence of g(3) on the gas parameter in a BEC, finding good agreement with the theoretical prediction accounting for beyond-mean-field effects. In one dimension, we observe a reduction of g(3) by several orders of magnitude upon increasing interactions from the weakly interacting BEC to …
We investigate universal behavior in the recombination rate of three bosons close to threshold. Using the He-He system as a reference, we solve the three-body Schrödinger equation above the dimer threshold for different potentials having large values of the two-body scattering length $a$. To this aim we use the hyperspherical adiabatic expansion and we extract the $S$-matrix through the integral relations recently derived. The results are compared to the universal form, $α\approx 67.1\sin^2[s_0\ln(κ_*a)+γ]$, for different values of $a$ and selected values of the three-body parameter $κ_*$. A g…
We reveal a significant spin-exchange pathway in the three-body recombination process for ultracold lithium-7 atoms near a zero-crossing of the two-body scattering length. This newly discovered recombination pathway involves the exchange of spin between all three atoms, which is not included in many theoretical approaches with restricted spin structure. Taking it into account, our calculation is in excellent agreement with experimental observations. To contrast our findings, we predict the recombination rate around a different zero-crossing without strong spin-exchange effects to be two orders…
We report on three-body recombination of a single trapped Rb^+ ion and two neutral Rb atoms in an ultracold atom cloud. We observe that the corresponding rate coefficient K_3 depends on collision energy and is about a factor of 1000 larger than for three colliding neutral Rb atoms. In the three-body recombination process large energies up to several 0.1eV are released leading to an ejection of the ion from the atom cloud. It is sympathetically recooled back into the cloud via elastic binary collisions with cold atoms. Further, we find that the final ionic product of the three-body processes is…
We study entropy generation in a one-dimensional (1D) model of bosons in an optical lattice experiencing two-particle losses. Such heating is a major impediment to observing exotic low temperature states, and "simulating" condensed matter systems. Developing intuition through numerical simulations, we present a simple empirical model for the entropy produced in this 1D setting. We also explore the time evolution of one and two particle correlation functions, showing that they are robust against two-particle loss. Because of this robustness, induced two-body losses can be used as a probe of sho…
We study three-body recombination of fully spin-polarized ${}^6$Li atoms that are interacting resonantly in relative p-waves. Motivated by a recent experiment, we focus on negative scattering volumes where three atoms recombine into a deep dimer and another atom. We calculate the three-body recombination rate using a Faddeev equation derived from effective field theory. In particular, we study the magnetic field and temperature dependences of the loss rate and use the recombination data to determine the effective range of the p-wave atom-atom interaction. We also predict the existence of a sha…
We develop a full multichannel spin model in momentum space to investigate three-body recombination of identical alkali-metal atoms colliding in a magnetic field. The model combines the exact three-atom spin structure and realistic pairwise atom-atom interactions. By neglecting the interaction between two particles when the spectating particle is not in its initial spin state we arrive at an approximate model. With this approximate model we achieve excellent agreement with the recent precise measurement of the ground Efimov resonance position in potassium-39 close to 33.58 G [Chapurin $et$ $al…
We investigate three-body recombination loss across a Feshbach resonance in a gas of ultracold 7Li atoms prepared in the absolute ground state and perform a comparison with previously reported results of a different nuclear-spin state [N. Gross et.al., Phys. Rev. Lett. 103 163202, (2009)]. We extend the previously reported universality in three-body recombination loss across a Feshbach resonance to the absolute ground state. We show that the positions and widths of recombination minima and Efimov resonances are identical for both states which indicates that the short-range physics is nuclear-s…
Correlation properties in ultracold Fermi gas with negative scattering length and its impact on the three-body recombination is analyzed. We find that Cooper pairing enhances the recombination rate in contrast to the decrease of this rate accompanying Bose-Einstein condensation in a Bose gas. This trend is characteristic for all interval of temperatures T<Tc.
We study the recombination process of three atoms scattering into an atom and diatomic molecule in heteronuclear mixtures of ultracold atomic gases with large and positive interspecies scattering length at finite temperature. We calculate the temperature dependence of the three-body recombination rates by extracting universal scaling functions that parametrize the energy dependence of the scattering matrix. We compare our results to experimental data for the 40K-87Rb mixture and make a prediction for 6Li-87Rb. We find that contributions from higher partial wave channels significantly impact th…
We study three-body recombination in an ultracold Bose-Fermi mixture. We first show theoretically that, for weak inter-species coupling, the loss rate is proportional to Tan's contact. Second, using a 7 Li/ 6 Li mixture we probe the recombination rate in both the thermal and dual superfluid regimes. We find excellent agreement with our model in the BEC-BCS crossover. At unitarity where the fermion-fermion scattering length diverges, we show that the loss rate is proportional the 4/3 power of the fermionic density. Our results demonstrate that impurity-induced losses can be used as a quantitati…
Motivated by recent experimental progresses, we investigate few-body properties of interacting spinless bosons nearby a d-wave resonance. Using the Skorniakov-Ter-Martirosion (STM) equations, we calculate the scattering length between an atom and a d-wave dimer, and we find that the atom-dimer scattering length is positive and is much smaller the result from the mean-field approximation. We also reveal unique properties of the three-body recombination rate for a degenerate Bose condensate nearby the d-wave resonance. We find that the total recombination rate is nearly a constant at the quasi-b…
We report on the observation of triatomic Efimov resonances in an ultracold gas of cesium atoms. Exploiting the wide tunability of interactions resulting from three broad Feshbach resonances in the same spin channel, we measure magnetic-field dependent three-body recombination loss. The positions of the loss resonances yield corresponding values for the three-body parameter, which in universal few-body physics is required to describe three-body phenomena and in particular to fix the spectrum of Efimov states. Our observations show a robust universal behavior with a three-body parameter that st…
We describe the three-body loss coefficient of identical fermions with $p$-wave interactions using a set of rate equations in which three-body recombination happens via an indirect process. Our theoretical treatment explains experimental results just above the universal scaling law regime of weak interactions. Furthermore, we theoretically extend and experimentally verify the rate equation model for the case of atoms trapped in two dimensions. Moreover, we find that the three-body loss coefficient in a two-dimensional trap is proportional to $A_{p}^{3}$ in the weakly interacting regime, where …
A new narrow 3-atom loss resonance associated with an Efimov trimer crossing the 3-atom threshold has recently been discovered in a many-body system of ultracold 6Li atoms in the three lowest hyperfine spin states at a magnetic field near 895 G. O'Hara and coworkers have used measurements of the 3-body recombination rate in this region to determine the complex 3-body parameter associated with Efimov physics. Using this parameter as the input, we calculate the universal predictions for the spectrum of Efimov states and for the 3-body recombination rate in the universal region above 600 G where …
We determine the three-body bound states of an atom in a Fermi mixture. Compared to the Efimov spectrum of three atoms in vacuum, we show that the Fermi seas deform the Efimov spectrum systematically. We demonstrate that this effect is more pronounced near unitarity, for which we give an analytical estimate. We show that in the presence of Fermi seas, the three-body bound states obey a generalized discrete scaling law. For an experimental confirmation of our prediction, we propose three signatures of three-body bound states of an ultracold Fermi mixture of Yb isotopes, and provide an estimate …
The low-energy scattering of three bosons or distinguishable particles with short-range interactions is characterized by a fundamental parameter, the three-body scattering hypervolume. Its imaginary part is directly related to the three-body recombination rate in a quantum gas consisting of such particles. We derive an analytical formula of it for weak interactions, and perform its first numerical calculations for bosons with a variable nonzero-range potential. For attractive interactions, we identify several three-body resonances at which the three-body scattering hypervolume becomes divergen…
Ultracold atomic gases have recently become a driving force in few-body physics due to the observation of the Efimov effect. While initially observed in equal mass systems, one expects even richer few-body physics in the heteronuclear case. In previous experiments with ultracold mixtures of potassium and rubidium, an unexpected non-universal behavior of Efimov resonances was observed. In contrast, we measure the scattering length dependent three-body recombination coefficient in ultracold heteronuclear mixtures of $^{39}\mathrm{K}$-\87Rb and $^{41}\mathrm{K}$-\87Rb and do not observe any signa…
We report on high-resolution Feshbach spectroscopy on a degenerate, spin-polarized Fermi gas of $^{161}$Dy atoms, measuring three-body recombination losses at low magnetic field. For field strength up to 1\,G, we identify as much as 44 resonance features and observe plateaus of very low losses. For four selected typical resonances, we study the dependence of the three-body recombination rate coefficient on the magnetic resonance detuning and on the temperature. We observe a strong suppression of losses with decreasing temperature already for small detunings from resonance. The characterization…
We investigate the three-body properties of two identical "up" fermions and one distinguishable "down" atom interacting in a strongly confined two-dimensional geometry. We compute exactly the atom-dimer scattering properties and the three-body recombination rate as a function of collision energy and mass ratio m_up/m_down. We find that the recombination rate for fermions is strongly energy dependent, with significant contributions from higher partial waves at low energies. For m_up < m_down, the s-wave atom-dimer scattering below threshold is completely described by the scattering length. Furt…
We report on the measurement of four-body recombination rate coefficients in an atomic gas. Our results obtained with an ultracold sample of cesium atoms at negative scattering lengths show a resonant enhancement of losses and provide strong evidence for the existence of a pair of four-body states, which is strictly connected to Efimov trimers via universal relations. Our findings confirm recent theoretical predictions and demonstrate the enrichment of the Efimov scenario when a fourth particle is added to the generic three-body problem.
We point out at the possible relationship between the two many-body phenomena: Friedel oscillations and Mahan exciton/Fermi edge singularity in a recombination process of a localized valence band hole with a degenerate electron system. It is qualitatively described that the oscillating electron density around the screened potential of a neutral acceptor can modify the wavefunction of the valence band hole and thus promote its recombination with electrons near Fermi-surface. The role of a finite hole mass for the net balance of the two hole energies: the kinetic energy and Coulomb attraction to…
The low temperature unitary Bose gas is a fundamental paradigm in few-body and many-body physics, attracting wide theoretical and experimental interest. Here we first present a theoretical model that describes the dynamic competition between two-body evaporation and three-body re-combination in a harmonically trapped unitary atomic gas above the condensation temperature. We identify a universal magic trap depth where, within some parameter range, evaporative cooling is balanced by recombination heating and the gas temperature stays constant. Our model is developed for the usual three-dimension…
We use the zero-range approximation to study a system of two identical bosons interacting resonantly with a third particle. The method is derived from effective field theory. It reduces the three-body problem to an integral equation which we then solve numerically. We also develop an alternative approach which gives analytic solutions of the integral equation in coordinate representation in the limit of vanishing total energy. The atom-dimer scattering length, the rates of atom-dimer relaxation and three-body recombination to shallow and to deep molecular states are calculated either analytica…
We have measured the interaction energy and three-body recombination rate for a two-component Fermi gas near a narrow Feshbach resonance and found both to be strongly energy dependent. Even for deBroglie wavelengths greatly exceeding the van der Waals length scale, the behavior of the interaction energy as a function of temperature cannot be described by atoms interacting via a contact potential. Rather, energy-dependent corrections beyond the scattering length approximation are required, indicating a resonance with an anomalously large effective range. For fields where the molecular state is …
We study three-body loss in an ultracold mixture of a thermal Bose gas and a degenerate Fermi gas. We find that at unitarity, where the interspecies scattering length diverges, the usual inverse-square temperature scaling of the three-body loss found in non-degenerate systems is strongly modified and reduced with the increasing degeneracy of the Fermi gas. While the reduction of loss is qualitatively explained within the few-body scattering framework, a remaining suppression provides evidence for the long-range RKKY interactions mediated by fermions between bosons. Our model based on RKKY inte…
A recent rejuvenation of experimental and theoretical interest in the physics of few- body systems has provided deep, fundamental insights into a broad range of problems. Few-body physics is a cross-cutting discipline not restricted to conventional subject ar- eas such as nuclear physics or atomic or molecular physics. To a large degree, the recent explosion of interest in this subject has been sparked by dramatic enhancements of experimental capabilities in ultracold atomic systems over the past decade, which now permit atoms and molecules to be explored deep in the quantum mechanical limit w…
The experimental realization of quantum degenerate cold Fermi gases with large hyperfine spins opens up a new opportunity for exotic many-body physics.
We discuss the three-body properties of identical bosons exhibiting large scattering length in two spatial dimensions. Within an effective field theory for resonant interactions, we calculate the leading non-universal corrections from the two-body effective range to bound-state and scattering observables. In particular, we compute the three-body binding energies, the boson-dimer scattering properties, and the three-body recombination rate for finite energies. We find significant effective range effects in the vicinity of the unitary limit. The implications of this result for future experiments…
In one spatial dimension, quantum systems with an attractive three-body contact interaction exhibit a scale anomaly. In this work, we examine the few-body sector for up to six particles. We study those systems with a self-consistent, non-perturbative, iterative method, in the subspace of zero total momentum. Exploiting the structure of the contact interaction, the method reduces the complexity of obtaining the wavefunction by three powers of the dimension of the Hilbert space. We present results on the energy, and momentum and spatial structure, as well as Tan's contact. We find a Fermi-Fermi …
