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arXiv 2111.15313quant-phphysics.comp-ph
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分子自旋量子点的最优控制

Optimal control of molecular spin qudits

Alberto Castro, Adrian Garcia Carrizo, David Zueco, Fernando Luis

摘要:

我们证明,数值,操纵分子纳米磁体的自旋状态与形状的微波脉冲量子最优控制理论技术设计的可能性。可以以这种方式在比使用简单的单色共振脉冲更短的时间内执行状态到状态或全门变换。因此,这种操作速率的提高可以减轻退相干的影响。的优化协议和它们的潜力,为实际的实施所示的一个简单的分子团簇托管一个单一的Gd $^{3+}$离子的模拟。它的八个可访问级别(对应于总自旋$S=7/2$)允许对$8$级别的量子比特或三个耦合量子比特的系统进行编码。通用操作所需的所有必要的门可以使用本征耦合在这个系统中存在的最佳脉冲。最优控制技术的应用可以促进基于分子自旋量子点的量子技术的实现。

英文摘要:

We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can be performed in this way in shorter times than using simple monochromatic resonant pulses. This enhancement in the operation rates can therefore mitigate the effect of decoherence. The optimization protocols and their potential for practical implementations are illustrated by simulations performed for a simple molecular cluster hosting a single Gd$^{3+}$ ion. Its eight accessible levels (corresponding to a total spin $S=7/2$) allow encoding an $8$-level qudit or a system of three coupled qubits. All necessary gates required for universal operation can be obtained with optimal pulses using the intrinsic couplings present in this system. The application of optimal control techniques can facilitate the implementation of quantum technologies based on molecular spin qudits.

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