We use state-of-the-art molecular dynamics simulations to study the effects of annealed disorder on the phase separating kinetics and aging phenomena of a segregating binary fluid mixture. In the presence of disorder, we observe a dramatic slowing down in the phase separation dynamics. The domain growth follows the power-law with a disorder-dependent exponent. Due to the energetically favorable positions, the domain boundary roughens which modifies the correlation function and structure factor to a non-Porod behavior. The correlation function and structure factor provide clear evidence that the superuniversality does not hold in our system. The role of annealed disorder on the non-equilibrium aging dynamics is studied qualitatively by computing the two-time order parameter autocorrelation function. The decay of the correlation function slows down significantly with the disorder. This quantity exhibits scaling laws with respect to the ratio of the domain length at the observation time and the age of the system. We find the scaling laws hold good for the disordered system and therefore, robust and generic to such segregating fluid mixtures.
Theory of associating polymers with annealed and quenched sticker disorder: Mean-field solution and phase behavior
Scuola Internazionale Superiore di Studi Avanzati (SISSA)(高等师范研究所);Università Ca’ Foscari Venezia(威尼斯大学);European Centre for Living Technology (ECLT)(生命技术欧洲中心);University of Padova(帕多瓦大学);INFN, Sezione di Padova(意大利国家核物理研究所帕多瓦分部)
NANOG assembles into self-limiting aging micelles that drive a sol-gel transition and modulate DNA dynamics
Centre for Regenerative Medicine, Institute for Regeneration and Repair(再生医学中心,再生与修复研究所);School of Physics and Astronomy, University of Edinburgh(爱丁堡大学物理与天文学院);School of Molecular Biosciences, University of Glasgow(格拉斯哥大学生物分子科学学院);Institute for Stem Cell Research, School of Biological Sciences, University of Edinburgh(爱丁堡大学生物科学学院干细胞研究所)