We prove the STP=BQP conjecture of Freedman, Hastings and Shokrian-Zini [1], namely that the two-qubit singlet/triplet measurement is quantum computationally universal given only an initial ensemble of maximally mixed single qubits. This provides a method for quantum computing that is fully rotationally symmetric (i.e. reference frame independent), using primitives that are both physically very-accessible and provably the simplest possible.
Coupled pairs of nuclear spins-1/2 support one singlet state and three triplet states. Transitions between the singlet state and one of the triplet states may be driven by an oscillating low-frequency magnetic field, in the presence of couplings to a third nuclear spin, and a weak bias magnetic field.This phenomenon allows the generation of strong nuclear hyperpolarization of ${}^{13}\mathrm{C}$ nuclei, starting from the nuclear singlet polarization of a ${}^{1}\mathrm{H}$ spin pair, associated with the enriched para spin isomer of hydrogen gas. Hyperpolarization is demonstrated for two molecu…
Coupled pairs of spin-1/2 nuclei support one singlet state and three triplet states. In many circumstances the nuclear singlet order, defined as the difference between the singlet population and the mean of the triplet populations, is a long-lived state which persists for a relatively long time in solution. Various methods have been proposed for generating singlet order, starting from nuclear magnetization. This requires the stimulation of singlet-to-triplet transitions by modulated radiofrequency fields. We show that a recently described pulse sequence, known as PulsePol (Schwartz $\textit{et…
Geometric gates that use the global property of the geometric phase is believed to be a powerful tool to realize fault-tolerant quantum computation. However, for singlet-triplet qubits in semiconductor quantum dot, the low Rabi frequency of the microwave control leads to overly long gating time, and thus the constructing geometric gate suffers more from the decoherence effect. Here we investigate the key issue of whether the fast geometric gate can be realized for singlet-triplet qubits without introducing an extra microwave-driven pulse, while maintaining the high-fidelity gate operation at t…
Open quantum system description of singlet-triplet qubits in quantum dots
我们建立了一个理论模型来描述GaAs量子点中单重态-三重态量子比特的耗散动力学。利用实验获得的共点[M. D. Shulman等人，Science 336，202（2012）]作为指导，我们发现每个逻辑量子比特在模拟$1/f^α$噪声的随机电报噪声（RTN）的作用下波动。我们还研究了作为RTN的振幅，RTN的相关时间，状态的准备时间，和两个量子比特耦合的函数的并发的动力学。此外，我们还发现两个量子比特的耦合以及制备时间对纠缠耗散动力学有很大的影响，这两个物理量都可以用来增强单重态-三重态量子比特之间的纠缠.
The search of a sweet spot, locus in qubit parameters where quantum control is first-order insensitive to noises, is key to achieve high-fidelity quantum gates. Efforts to search for such a sweet spot in conventional double-quantum-dot singlet-triplet qubits where each dot hosts one electron ("two-electron singlet-triplet qubit"), especially for two-qubit operations, have been unsuccessful. Here we consider singlet-triplet qubits allowing each dot to host more than one electron, with a total of four electrons in the double quantum dots ("four-electron singlet-triplet qubit"). We theoretically …
Charge noise is the main hurdle preventing high-fidelity operation, in particular that of two-qubit gates, of semiconductor-quantum-dot-based spin qubits. While certain sweet spots where charge noise is substantially suppressed have been demonstrated in several types of spin qubits, the existence of one for coupled singlet-triplet qubits is unclear. We theoretically demonstrate, using full configuration-interaction calculations, that a range of nearly sweet spots appear in the coupled singlet-triplet qubit system when a strong enough magnetic field is applied externally. We further demonstrate…
The exchange interaction in a singlet-triplet qubit defined by two-electron states in the double-quantum-dot system ("two-electron singlet-triplet qubit") typically varies monotonically with the exchange interaction and thus carries no sweet spot. Here we study a singlet-triplet qubit defined by four-electron states in the double-quantum-dot system ("four-electron singlet-triplet qubit"). We demonstrate, using configuration-interaction calculations, that in the four-electron singlet-triplet qubit the exchange energy as a function of detuning can be non-monotonic, suggesting existence of sweet …
Probing extended polyene systems with energy in excess of the bright state ($1^1B_u^+$/$S_2$) band edge generates triplets via singlet fission. This process is not thought to involve the $2^1A_g^-$/$S_1$ state, suggesting that other states play a role. Using density matrix renormalisation group (DMRG) calculations of the Pariser-Parr-Pople-Peierls Hamiltonian, we investigate candidate states that could be involved in singlet fission. We find that the relaxed $1^1B_u^-$, and $3^1A_g^-$ singlet states and $1^5A_g^-$ quintet state lie below the $S_2$ state. The $1^1B_u^-$, $3^1A_g^-$ and $1^5A_g^…
