Thin, viscous liquid films subjected to impact events can deform. Here we investigate free surface oil film deformations that arise due to the air pressure buildup under the impacting and rebouncing water drops. Using Digital Holographic Microscopy, we measure the 3D surface topography of the deformed film immediately after the drop rebound, with a resolution down to 20 nm. We first discuss how the film is initially deformed during impact, as a function of film thickness, film viscosity, and drop impact speed. Subsequently, we describe the slow relaxation process of the deformed film after the rebound. Scaling laws for the broadening of the width and the decay of the amplitude of the perturbations are obtained experimentally and found to be in excellent agreement with the results from a lubrication analysis. We finally arrive at a detailed spatio-temporal description of the oil film deformations that arise during the impact and rebouncing of water drops.
The off-center collision of binary bouncing droplets of equal size was studied numerically by a volume-of-fluid (VOF) method with two marker functions, which has been validated by comparing with available experimental results. A non-monotonic kinetic energy recovery with varying impact parameters was found based on the energy budget analysis. This can be explained by the prolonged entanglement time and the enhanced internal-flow-induced viscous dissipation for bouncing droplets at intermediate impact parameters, compared with those at smaller or larger impact parameters. The universality of th…
Soft surfaces impacted by liquid droplets trap more air underneath than their rigid counterpart. The extended lifetime of the air film not only facilitates bouncing behaviours of the impacting droplets but also increases the possibility of an interaction between the air film itself and the air cavity formed inside the droplets by capillary waves. Such interaction may cause rupture of the trapped air film by a so-called dimple inversion phenomenon and suppress bouncing. In this work, we systematically investigate the relation between air cavity collapse and air film rupture for water droplets i…
The impact of droplets is a ubiquitous phenomenon, and reducing the residence time of the impact process is important for many potential applications. In this study of the impact dynamics on heated surfaces, we identify a mode of droplet bouncing (bouncing-with-spray mode) that can reduce the residence time significantly compared with the traditional retraction-bouncing mode. Comparing with other strategies to reduce the residence time, this approach induced by heat is simple and reliable. The reduction in the residence time is due to the burst of vapor bubbles in the liquid film, which result…
When a liquid drop falls on a solid substrate, the air layer in between them delays the occurrence of liquid--solid contact. For impacts on smooth substrates, the air film can even prevent wetting, allowing the drop to bounce off with dynamics identical to that observed for impacts on superamphiphobic materials. In this article, we investigate similar bouncing phenomena, occurring on viscous liquid films, that mimic atomically smooth substrates, with the goal to probe their effective repellency. We elucidate the mechanisms associated to the bouncing to non-bouncing (floating) transition using …
Non-wetting substrates allow impacting liquid drops to spread, recoil, and takeoff, provided they are not too heavy (Biance et al. 2006) or too viscous (Jha et al. 2020). In this article, using direct numerical simulations with the volume of fluid method, we investigate how viscous stresses and gravity conspire against capillarity to inhibit drop rebound. Close to the bouncing to non-bouncing transition, we evidence that the initial spreading stage can be decoupled from the later retraction and takeoff, allowing to understand the rebound as a process converting the surface energy of the spread…
Modelling wetting-bouncing transitions of droplet impact on random rough surfaces
State Key Laboratory of Mesoscience and Engineering, Institute of Process Engineering, Chinese Academy of Sciences（中国科学院过程工程研究所介科学工程国家重点实验室）；School of Civil Engineering, University of Sydney（悉尼大学土木工程学院）；School of Chemical Engineering, University of Chinese Academy of Sciences（中国科学院大学化学工程学院）
Droplets can self-propel when immersed in another liquid in which a concentration gradient is present. Here we report the experimental and numerical study of a self-propelling oil droplet in a vertically stratified ethanol/water mixture: At first, the droplet sinks slowly due to gravity, but then, before having reached its density matched position, jumps up suddenly. More remarkably, the droplet bounces repeatedly with an ever increasing jumping distance, until all of a sudden it stops after about 30 min. We identify the Marangoni stress at the droplet/liquid interface as responsible for the j…
It is generally accepted that the Worthington jet occurs when a droplet impacts onto a liquid pool. However, in this experimental study of the impact of viscous droplets onto a less-viscous liquid pool, we identify another jet besides the Worthington jet, forming a two-jet phenomenon. The two jets, a surface-climbing jet and the Worthington jet, may appear successively during one impact event. By carefully tuning the impact condition, we find that the two-jet phenomenon is jointly controlled by the droplet-pool viscosity ratio, the droplet Weber number, and the droplet-pool miscibility. The me…
The physico-chemistry of surfactants (amphiphilic surface active agents) is often used to control the dynamics of viscous drops and bubbles. Surfactant sorption kinetics has been shown to play a critical role in the deformation of drops in extensional and shear flows, yet to the best of our knowledge these kinetics effects on a viscous drop in an electric fieldhave not been accounted for. In this paper we numerically investigate the effects of sorption kinetics on a surfactant-covered viscous drop in an electric field. Over a range of electric conductivity and permittivity ratios between the i…
We present convincing evidence of a direct connection between the pressure drop, viscous dissipation, and the turbulent energy spectrum. We use this finding to explain Nikuradse's experimental results of pressure drop for turbulent flows in rough pipes, in terms of a modified Kolmogorov length scale that varies with the surface roughness. Furthermore, we use Laufer's measurements of turbulent energy spectra in pipe flow to calculate -- to a good approximation -- the turbulent component of the pressure drop directly from an averaged turbulent energy spectrum. We also show that the incompressibi…
We study drop impacts on immiscible viscous liquid pool and investigate the formation of droplet surface craters using experimental and theoretical analysis. We attribute the formation of air craters to the rapid deceleration of the droplet due to viscous drag force. The droplet response to the external impulsive decelerating force induces oscillatory modes on the surface exposed to the air forming capillary waves that superimpose to form air craters of various shapes and sizes. We introduce a non-dimensional parameter ($Γ$), that is, the ratio of drag force to the capillary force acting on th…
In a companion paper [Pitrou, Phys. Rev. E 97, 043115 (2018)], a formalism allowing to describe viscous fibers as one-dimensional objects was developed. We apply it to the special case of a viscous fluid torus. This allows to highlight the differences with the basic viscous string model and with its viscous rod model extension. In particular, an elliptic deformation of the torus section appears because of surface tension effects, and this cannot be described by viscous string nor viscous rod models. Furthermore, we study the Rayleigh-Plateau instability for periodic deformations around the per…
The behaviour of a viscous drop squeezed between two horizontal planes is treated by both theory and experiment. When the squeezing force F is constant and surface tension is neglected, the theory predicts ultimate growth of the radius a~ t^{1/8}, in excellent agreement with our experiment. Surface tension at the drop boundary is included in the analysis, although negligibly small in the squeezing experiments. The circular evolution is found to be stable under small perturbations. If the force is reversed (F < 0), so that the plates are pulled or levered apart, the boundary of the drop is subj…
The experimental observation of D. Duft, T. Achtzehn, R. Muller, B. A. Huber, and T. Leisner, Nature 421, 128 (2003) on the sequential progression of the instability of a charged liquid drop points at the formation of a jet followed by the emission of progeny droplets as a crucial pathway of the Rayleigh fission process. In spite of considerable theoretical progress, a quantitative understanding of this breakup pathway through mathematical models has largely remained inconclusive. This limitation has mainly been due to the fact that the generally applied electrostatic boundary condition of the…
The aim of this study is to derive accurate models for quantities characterizing the dynamics of droplets of non-vanishing viscosity in capillaries. In particular, we propose models for the uniform-film thickness separating the droplet from the tube walls, for the droplet front and rear curvatures and pressure jumps, and for the droplet velocity in a range of capillary numbers, $Ca$, from $10^{-4}$ to $1$ and inner-to-outer viscosity ratios, $λ$, from $0$, i.e. a bubble, to high viscosity droplets. Theoretical asymptotic results obtained in the limit of small capillary number are combined with…
From the Navier-Stokes-Korteweg (NSK) equations, the exact relations between the fundamental surface physical quantities for two-phase viscous flow with diffuse interface are derived, including density gradient, shear stress, vorticity, pressure, enstrophy flux and surface curvature. These theoretical results provide a solid foundation of the boundary/interfacial vorticity dynamics and a new tool for analysis of complex interfacial phenomena in two-phase viscous flows. To demonstrate the application of the developed results, simulation of a droplet impacting and spreading on a solid wall is co…
