Direct observation of terahertz frequency comb generationin difference-frequency quantum cascade lasers
Luigi Consolino, Malik Nafa, Michele De Regis, Francesco Cappelli, Saverio Bartalini, Akio Ito, Masahiro Hitaka, Tatsuo Dougakiuchi, Tadataka Edamura, Paolo De … 展开作者
Luigi Consolino, Malik Nafa, Michele De Regis, Francesco Cappelli, Saverio Bartalini, Akio Ito, Masahiro Hitaka, Tatsuo Dougakiuchi, Tadataka Edamura, Paolo De Natale, Kazuue Fujita
Terahertz quantum cascade laser sources based on intra-cavity difference frequency generation from mid-IR devices are an important asset for applications in rotational molecular spectroscopy and sensing, beingthe only electrically pumped device able to operate in the 0.6-6 THz range without the need of bulky andexpensive liquid helium cooling. Here we present comb operation obtained by intra-cavity mixing of adistributed feedback laser at λ = 6.5 μm and a Fabry-Pérot device at around λ = 6.9 μm. The resultingultra-broadband THz emission extends from 1.8 to 3.3 THz, with a total output power of 8 μW at 78K.The THz emission has been characterized by multi-heterodyne detection with a primary frequencystandard referenced THz comb, obtained by optical rectification of near infrared pulses. The down-converted beatnotes, simultaneously acquired, confirm an equally spaced THz emission down to 1 MHzaccuracy. In the next future this setup can be used for Fourier transform based evaluation of the phaserelation among the emitted THz modes, paving the way to room-temperature, compact and field-deployable metrological grade THz frequency combs.
We demonstrate a terahertz (THz) frequency comb that is flexible in terms of its frequency range and the number and spacing of comb lines. We use a combination of near-infrared laser diodes, phase modulation and opto-electronic frequency conversion. The THz comb lines are characterized to be < 10 MHz by resolving the pressure dependent collisional broadening of an ammonia molecule rotational mode.
In the terahertz frequency range, the quantum cascade laser (QCL) is a suitable platform for the frequency comb and dual-comb operation. Improved comb performances have been always much in demand. In this work, by employing a symmetric thermal dissipation scheme, we report an improved frequency comb and dual-comb operation of terahertz QCLs. Two configurations of cold fingers, i.e., type A and B with asymmetric and symmetric thermal dissipation schemes, respectively, are investigated here. A finite-element thermal analysis is carried out to study the parametric effects on the thermal managemen…
Real-time measurement of the absolute frequency of continuous-wave terahertz (CW-THz) waves is required for characterization and frequency calibration of practical CW-THz sources. We proposed a method for real-time monitoring of the absolute frequency of CW-THz waves involving temporally parallel, i.e., simultaneous, measurement of two pairs of beat frequencies and laser repetition frequencies based on dual THz combs of photocarriers (PC-THz combs) with different frequency spacings. To demonstrate the method, THz-comb-referenced spectrum analyzers were constructed with a dual configuration bas…
We present a monolithic solution to extract efficiently light from terahertz quantum cascade lasers with metal-metal waveguides suitable for broadband frequency comb applications. The design is optimized for a bandwidth of 500 GHz around a center frequency of 2.6 THz. A five-fold increase in total output power is observed compared to standard metal-metal waveguides. The extractor features a single-lobed far-field pattern and increases the frequency comb dynamical range to cover more than 50 % of the laser dynamic range. Frequency comb operation up to a spectral bandwidth of 670 GHz is achieved…
We demonstrated combination of gapless terahertz (THz) comb with dual-comb spectroscopy, namely gapless dual-THz-comb spectroscopy, to achieve the spectral resolution equal to width of the THz comb tooth. The gapless THz comb was realized by interpolating frequency gaps between the comb teeth with sweeping of a laser mode-locked frequency. The demonstration of low-pressure gas spectroscopy with gapless dual-THz-comb spectroscopy clearly indicated that the spectral resolution was decreased down to 2.5-MHz width of the comb tooth and the spectral accuracy was enhanced to 10-6 within the spectral…
Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multi-heterodyne spectroscopy using two terahertz quantum cascade laser combs. With just 100 $μ$s of integration time, we achieve peak signal-to-noise ratios exceeding 60 dB and a spectral coverage greater than 250 GHz centered at 2.8 THz. Even with room-temperature detectors we are able to achieve peak signal-to-noise ratios of 50 dB, and as a proof-of-principle we use these…
Dual terahertz (THz) comb spectroscopy is a promising methods for high accuracy, high resolution, and broadband THz spectroscopy because the mode-resolved THz comb spectrum possesses both characteristics of broadband THz radiation and narrow-linewidth continuous-wave THz radiation and all frequency mode of THz comb can be phase-locked to a microwave frequency standard. However, requirement of stabilized dual femtosecond lasers has often hindered wide use of this method. In this article, we demonstrated the adaptive sampling, dual THz comb spectroscopy, enabling use of free-running dual femtose…
We report on an attempt to generate highly stable continuous terahertz (THz) wave by using optical frequency comb (OFC). About 10-nm wide OFC has been generated through a deep phase modulation of a 852 nm laser line in lithium niobate crystal cavity. The multiple optical modes (side bands) of the OFC, which are equally separated from each other by the modulation frequency (=6 GHz) are taken as the frequency reference. When another semiconductor laser is frequency locked, the stability of the difference frequency between the master laser and the second laser is improved on the same order of the…
Hyperspectral imaging is a technique that allows for the creation of multi-color images. At terahertz wavelengths, it has emerged as a prominent tool for a number of applications, ranging from non-ionizing cancer diagnosis and pharmaceutical characterization to non-destructive artifact testing. Contemporary terahertz imaging systems typically rely on non-linear optical down-conversion of a fiber-based near-infrared femtosecond laser, requiring complex optical systems. Here, we demonstrate hyperspectral imaging with chip-scale frequency combs based on terahertz quantum cascade lasers. The dual …
Using an affordable ytterbium laser with sub-mJ of energy combined with a novel pulse compression technique, we demonstrate an extremely competitive state-of-the-art terahertz (THz) source with 53 mW of average power and 310 kV/cm at focus from the tilted-pulse front pumping scheme in lithium niobate at room temperature. Key points of this demonstration include the use of a pump pulse duration of 280 fs in combination with an echelon mirror. Our results present unmatched combined characteristics and are highly competitive with the existing THz sources pumped at the mJ range. This demonstration…
Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of molecules are located, multiheterodyne spectroscopy that employs the dual-comb technique shows an advantage in real-time spectral detection over the traditional Fourier transform infrared or time domain spectroscopies. Here, we demonstrate compact terahertz dual-comb spectroscopy based on quantum cascade lasers (QCLs). In our experiment, two free-running QCLs …
Broadband dual-comb spectroscopy has attracted increasing interests due to its unique advantages in high spectral resolution, fast detection, and so on. Although the dual-comb technique is relatively mature in the infrared wavelengths, it is, currently, not commercially capable of practical applications in the terahertz regime due to the lack of high performance broadband terahertz dual-comb sources. In the terahertz frequency range, the electrically pumped quantum cascade laser (QCL) is a suitable candidate for the dual-comb operation. However, free running terahertz QCL dual-comb sources nor…
By using two mutually phase-locked optical frequency combs with slightly different repetition rates, we demonstrate asynchronous optical-sampling terahertz time-domain spectroscopy (ASOPS THz-TDS) without using any trigger signals or optical delay lines. Due to a tight stabilization of the repetition frequencies, it was possible to accumulate the data over 48 minutes in a triggerless manner without signal degradation. The fractional frequency stability of the measured terahertz signal is evaluated to be $\sim$8.0$\times$10$^{- 17}$ after 730 s. The frequency accuracy of the obtained terahertz …
We present an antipodal Vivaldi antenna for broadband double metal waveguide terahertz quantum cascade lasers and frequency combs. Its exponentially curved flare profile results in an adiabatic in-plane mode expansion, producing an improved far-field with a single-lobed beam of (23°x19°) full width half maximum with an octave-spanning bandwidth. The antenna also acts as a wave retarder, rotating the polarization from vertical toward horizontal polarization by a frequency-dependent angle. The laser's emission spectrum and current-voltage characteristics are not affected, as well as frequency co…
Topological Insulator-based devices can transport electrons/photons at the surfaces of materials without any back reflections, even in the presence of obstacles. Topological properties have recently been studied using non-reciprocal materials such as gyromagnetics or using bianisotropy. However, these effects usually saturate at optical frequencies and limit our ability to scale down devices. In order to implement topological devices that we introduce in this paper for the terahertz range, we show that semiconductors can be utilized via their cyclotron resonance in combination with small magne…
The recent demonstration of a terahertz (THz) molecular gas laser pumped by a mid-infrared quantum cascade laser (QCL) has opened up new perspectives for this family of sources, traditionally relying on CO2-laser pumping. A so far open question concerning QCL-pumped THz molecular lasers (MLs) is related to their spectral purity. Indeed, assessing their frequency/phase noise is crucial for a number of applications potentially exploiting these sources as local oscillators. Here this question is addressed by reporting the measurement of the frequency noise power spectral density (PSD) of a THz ML…
We report a homogeneous quantum cascade laser (QCL) emitting at Terahertz (THz) frequencies, with a total spectral emission of about 0.6 THz centered around 3.3 THz, a current density dynamic range of Jdr=1.53, and a continuous wave output power of 7 mW. The analysis of the intermode beatnote unveils that the devised laser operates as optical frequency comb (FC) synthesizer over the whole laser operational regime, with up to 36 optically active laser modes delivering ~ 200 uW of optical power per comb tooth, a power level unreached so far in any THz QCL FC. A stable and narrow single beatnote,…
Carrier conversion from terahertz wave to dual-wavelength near-infrared light injection-locking to optical comb using asynchronous nonpolarimetric electro-optic downconversion with electro-optic polymer modulator
Quantum cascade lasers (QCLs) represent a fascinating accomplishment of quantum engineering and enable the direct generation of terahertz (THz) frequency radiation from an electrically-biased semiconductor heterostructure. Their large spectral bandwidth, high output powers and quantum-limited linewidths have facilitated the realization of THz pulses by active mode-locking and passive generation of optical frequency combs (FCs) through intracavity four-wave-mixing, albeit over a restricted operational regime. Here, we conceive an integrated architecture for the generation of high power (10 mW) …
We present a combined theoretical and experimental study of spatio-temporal propagation effects in terahertz (THz) generation in gases using two-color ionizing laser pulses. The observed strong broadening of the THz spectra with increasing gas pressure reveals the prominent role of spatio-temporal reshaping and of a plasma-induced blue-shift of the pump pulses in the generation process. Results obtained from (3+1)-dimensional simulations are in good agreement with experimental findings and clarify the mechanisms responsible for THz emission.
We report on the first direct measurement of the emission character of quantum cascade laser based frequency combs, using intensity autocorrelation. The correlation technique is based on fast electro-optic sampling, with a bandwidth optimized to match the emission spectra of the comb laser, centered around 2.5~THz. We find the output light to be amplitude and frequency modulated at the same time, with intensity modulation depth as high as 90\%, occuring on timescales as short as few picoseconds. We compare these findings with intensity autocorrelation measurements of pulsed Terahertz light ori…
Mode-resolved dual-comb spectroscopy (DCS) is an emerging spectroscopic tool with the potential to simultaneously achieve a broad spectral coverage and ultrahigh spectral resolution in terahertz (THz) spectroscopy. However, the need for two independently stabilized ultrafast lasers significantly hampers the potential application of DCS techniques. In this article, we demonstrate mode-resolved DCS in the THz region based on a free-running single-cavity dual-comb fiber laser with adaptive sampling. Low-pressure spectroscopy of acetonitrile gas with absorption features approaching the Doppler lim…
We demonstrate a convenient and fast method to measure the spectrally resolved far-fields of multimode terahertz quantum cascade lasers by combining a microbolometer focal plane array with an FTIR spectrometer. Far-fields of fundamental TM0 and higher lateral order TM1 modes of multimode Fabry-Pérot type lasers have been distinguished, which very well fit to the results obtained by a 3D finite-element simulation. Furthermore, multimode random laser cavities have been investigated, analyzing the contribution of each single laser mode to the total far-field. The presented method is thus an impor…
Arising from modulation instability, Turing rolls in optical Kerr microresonators have been used in the generation of optical frequency combs and the synthesis of microwave and terahertz frequencies. In this work, by applying electro-optic modulation on terahertz-frequency Turing rolls, we implement electro-optic frequency division with a microcomb to synthesize variable low-noise microwave signals. We also actively stabilize the terahertz oscillations to a microwave reference via intracavity power modulation, obtaining fractional frequency instabilities that are better than those of the free-…
Dual terahertz frequency combs for photonic RF readout of refractive index sensing with frequency multiplication and active-dummy temperature compensation
Graduate School of Sciences and Technology for Innovation, Tokushima University（德岛大学创新科学与技术研究生院）；Department of Physics, Toho University（东邦大学物理系）；School of System Engineering, Kochi University of Technology（高知工科大学系统工程学部）；Institute of Post-LED Photonics (pLED), Tokushima University（德岛大学后LED光子学研究所（pLED））；Institute of Photonics and Human Health Frontier (IPHF), Tokushima University（德岛大学光子学与人类健康前沿研究所（IPHF））；Graduate School of Engineering Science, The University of Osaka（大阪大学工程科学研究生院）
Dual-comb sources with equally spaced and low phase noise frequency lines are of great importance for high resolution spectroscopy and metrology. In the terahertz frequency range, electrically pumped semiconductor quantum cascade lasers (QCLs) are suitable candidates for frequency comb and dual-comb operation. For a single laser frequency comb, the repetition rate can be locked using a microwave injection locking and the carrier frequency can be locked to a highly stable source. However, for the locking of two laser combs, four frequencies (two repetition rates and two carrier offset frequenci…
Broadband terahertz comb with sub-Hz comb linewidth
Jinan Institute of Quantum Technology（济南量子技术研究院）；Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences（中国科学院上海微系统与信息研究所）
Excitation of antiferromagnetic spin waves in HoFeO$_{3}$ crystal combined with a split ring resonator (SRR) is studied using terahertz (THz) electromagnetic pulses. The magnetic field in the vicinity of the SRR induced by the incident THz electric field component excites and the Faraday rotation of the polarization of a near-infrared probe pulse directly measures oscillations that correspond to the antiferromagnetic spin resonance mode. The good agreement of the temperature-dependent magnetization dynamics with the calculation using the two-lattice Landau-Lifshitz-Gilbert equation confirms th…
We demonstrate a coherent imaging system based on a terahertz (THz) frequency quantum cascade laser (QCL) phase-locked to a near-infrared fs-laser comb. The phase locking enables coherent electro-optic sampling of the continuous-wave radiation emitted by the QCL through the generation of a heterodyne beat-note signal. We use this beat-note signal to demonstrate raster scan coherent imaging using a QCL emitting at 2.5 THz. At this frequency the detection noise floor of our system is of 3 pW/Hz and the long-term phase stability is <3 degrees/h, limited by the mechanical stability of the apparatu…
In this work we report two designs of subwavelength fibers packaged for practical terahertz wave guiding. We describe fabrication, modeling and characterization of microstructured polymer fibers featuring a subwavelength-size core suspended in the middle of a large porous outer cladding. This design allows convenient handling of the subwavelength fibers without distorting their modal profile. Additionally, the air-tight porous cladding serves as a natural enclosure for the fiber core, thus avoiding the need for a bulky external enclosure for humidity-purged atmosphere. Fibers of 5 mm and 3 mm …
Tunable low-phase-noise terahertz synthesis using a fiber-interferometer-referenced optical frequency comb and an EDFA-integrated Vernier cavity
Graduate School of Sciences and Technology for Innovation, Tokushima University（德岛大学科学技术创新研究生院）；Department of Physics, Toho University（东海大学物理系）；Institute of Post-LED Photonics (pLED), Tokushima University（德岛大学后LED光子学研究所）；Institute of Photonics and Human Health Frontier (IPHF), Tokushima University（德岛大学光子学与人类健康前沿研究所）；Sevensix Inc.（Sevensix公司）
Dual-comb generation from a single laser cavity provides a simple and high-performance solution to time sampling applications. We demonstrate a compact single-cavity dual-comb laser operating at gigahertz repetition rates and high repetition rate differences up to more than 100 kHz with sub-100 fs pulse duration. The single cavity approach leads to passive common noise suppression resulting in ultra-low relative timing jitter and fully resolvable comb lines in free-running operation. We showcase the laser performance with two application demonstrations: (a) time-domain spectroscopy of acetylen…
We report the coherent generation and detection of terahertz (THz) pulses covering the bandwidth of 0.1-9 THz in a high repetition rate, low pulse energy laser system. In this work we demonstrate the application and evaluation of solid-state biased coherent detection in combination with a spintronic emitter. This combination was used to generate and detect THz pulses in a time-domain spectroscopy (TDS) setup and tested on bulk nonlinear crystals. These results establish a new promising candidate to extend the possibilities for compact, broadband THz TDS systems driven by high repetition rate l…
To achieve high efficiency and good performance of spintronic terahertz sources, we propose and corroborate a remnant magnetization method to radiate continuously and stably terahertz pulses from W/CoFeB/Pt magnetic nanofilms without carrying magnets on the transmitters driven by femtosecond laser pulses. We systematically investigate the influences of the pumping central wavelength and find out the optimal wavelength for a fixed sample thickness. We also optimize the incidence angle of the pumping laser and find the emission efficiency is enhanced under oblique incidence. Combing the aforemen…
We experimentally investigate the limits to 800 nm-to-terahertz (THz) energy conversion in lithium niobate at room temperature driven by amplified Ti:Sapphire laser pulses with tilted-pulse-front. The influence of the pump central wavelength, pulse duration, and fluence on THz generation is studied. We achieved a high peak efficiency of 0.12% using transform limited 150 fs pulses and observed saturation of the optical to THz conversion efficiency at a fluence of 15 mJ/cm2. We experimentally identify two main limitations for the scaling of optical-to-THz conversion efficiencies: (i) the large s…
We report on a waveguide engineering technique that enables the generation of a bandwidth up to 1 THz and record ultra-short pulse length of 2.5 ps in injection seeded terahertz quantum cascade lasers. The reported technique is able to control and fully suppress higher order lateral modes in broadband terahertz quantum cascade lasers by introducing side-absorbers to metal-metal waveguides. The side-absorbers consist of a top metalization set-back with respect to the laser ridge and an additional lossy metal layer. In continuous wave operation the side-absorbers lead to octave spanning laser em…
The Terahertz or millimeter wave frequency band (300 GHz - 3 THz) is spectrally located between microwaves and infrared light and has attracted significant interest for applications in broadband wireless communications, space-borne radiometers for Earth remote sensing, astrophysics, and imaging. In particular optically generated THz waves are of high interest for low-noise signal generation. In particular optically generated THz waves are of high interest for low-noise signal generation. Here, we propose and demonstrate stabilized terahertz wave generation using a microresonator-based frequenc…
Detailed simulations for Terahertz quantum cascade lasers based on two-well designs are presented. We reproduce the maximal operation temperatures observed and attribute the degradation with temperature to the occupation of parasitic levels and thermal backfilling. Furthermore, we demonstrate that the current injection can be conveniently studied by using EZ states, which combine energy selectivity and spatial localisation. Improving the injection allows to achieve higher maximal operation temperatures around 265 Kelvin.
Amplified bursts of laser pulses are sought for various machining, deposition, spectroscopic and strong-field applications. Standard frequency- and time-domain techniques for pulse division become inadequate when intraburst repetition rates reach the terahertz (THz) range as a consequence of inaccessible spectral resolution, requirement for interferometric stability, and collapse of the chirped pulse amplification (CPA) concept due to the loss of usable bandwidth needed for safe temporal stretching. Avoiding the burst amplification challenge and resorting to a lossy post-division of an isolate…
We report on the first experimental demonstration of terahertz (THz) whispering-gallery modes (WGMs) with an ultra high quality (Q) factor of $1.5 \times {10}^{4}$ at 0.62THz. The WGMs are observed in a high resistivity float zone silicon (HRFZ-Si) spherical resonator coupled to a sub-wavelength silica waveguide. A detailed analysis of the coherent continuous wave (CW) THz spectroscopy measurements combined with a numerical model based on Mie-Debye-Aden-Kerker (MDAK) theory allows to unambiguously identify the observed higher order radial THz WGMs.
The majority of sources of coherent optical radiation rely on laser oscillators driven by population inversion. Despite their technological importance in communications, medicine, industry, and other fields, it remains a challenge to access the spectral range of 0.1-10 THz (the "terahertz gap"), a frequency band for applications ranging from spectroscopy to security and high-speed wireless communications. Here, we propose a way to produce coherent radiation spanning the THz gap by efficient second-harmonic generation (SHG) in low-loss dielectric structures, starting from technologically mature…
