Electromagnetic resonators, which are based on optical cavities or electronic circuits, are key elements to enhance and control light-matter interaction. In the THz range, current optical cavities exhibit very high-quality factors with $(λ/2)^3$ mode volumes limited by diffraction, whereas resonant electronic circuits show low quality factor but provide strong subwavelength effective volume ($10^{-6} λ^3$). To overcome the limitations of each type of resonator, great efforts are being devoted to improving the performances of current methods or to the emergence of original approaches. Here, we report on an optical resonator based on Tamm modes newly applied to the THz range, comprising a metallic layer on a distributed Bragg reflector and demonstrating a high-quality factor of 230 at $\sim$1 THz. We further experimentally and theoretically show a fine-tuning of the Tamm mode frequency (over a 250 GHz range) and polarization sensitivity by subwavelength structuration of the metallic layer. Electromagnetic simulations also reveal that THz Tamm modes are confined over a $λ$/2 length within the distributed Bragg reflector and can be ideally coupled to both bulk materials and 2D materials. These THz Tamm cavities are therefore attractive as basic building blocks of lasers, for the development of advanced THz optoelectronic devices such as sensitive detectors, high-contrast modulators, narrow filters, and polarizers, as well as for THz cavity quantum electrodynamics in nanostructures.
We propose a composite multilayer structure consist of graphene Tamm plasmon and Bragg reflector with defect layer to realize the low threshold and tunable optical bistability (OB) at the terahertz frequencies. This low-threshold OB originates from the couple of the Tamm plasmon (TP) and the defect mode (DM). We discuss the influence of graphene and the DM on the hysteretic response of the TM-polarized reflected light. It is found that the switch-up and switch-down threshold required to observe the optical bistable behavior are lowered markedly due to the excitation of the TP and DM. Besides, …
We consider a periodic chain of oscillating dipoles, interacting via long-range dipole-dipole interactions, embedded inside a cuboid cavity waveguide. We show that the mixing between the dipolar excitations and cavity photons into polaritons can lead to the appearance of new states localized at the ends of the dipolar chain, which are reminiscent of Tamm surface states found in electronic systems. A crucial requirement for the formation of polaritonic Tamm states is that the cavity cross-section is above a critical size. Above this threshold, the degree of localization of the Tamm states is hi…
The enhanced photonic spin hall effect (PSHE) plays a positive role in the flexible manipulation of photons. Here, by combining Dirac semimetals with Bragg reflector constructed by one-dimensional photonic crystal, we theoretically design a simple multilayer structure to enhance and manipulate the PSHE. Through the detailed and optimal design of the conductivity characteristics of Dirac semimetals and the structural parameters of the whole model, we realize the excitation of Optical Tamm states (OTSs) in the multilayer structure, so that the PSHE can be enhanced and controllable. The theoretic…
We report for the first time the bandgap engineering of Tamm plasmon photonic crystals - Tamm plasmon structures of which the metalic layer is periodically patterned into lattice of subwavelength period. By adopting a double period design, we evidenced experimentally a complete photonic bandgap up to $150\,nm$ in the telecom range. Moreover, such design offers a great flexibility to tailor on-demand, and independently, the band-gap size from $30\,nm$ to $150\,nm$ and its spectral position within $50\,nm$. Finally, by implementing a defect cavity within the Tamm plasmon photonic crystal, an ult…
It was widely accepted that embedding of metallic layers into optoelectronic structures is detrimental to lasing due absorption in metal. However, recently macroscopic optical coherence and lasing was observed in microcavities with intra-cavity single metallic layer. Here we propose the design of the of microcavity-type structure with two intra-cavity metallic layers which could serve as contacts for electrical pumping. The design of optical modes based on utilizing peculiarities of Tamm plasmon provides vanishing absorption due to fixing of the node of electric field of optical mode to metall…
Photonic crystals and metamaterials have emerged as two classes of tailorable materials that enable precise control of light. Plasmonic crystals, which can be thought of as photonic crystals fabricated from plasmonic materials, Bragg scatter incident electromagnetic waves from a repeated unit cell. However, plasmonic crystals, like metamaterials, are composed of subwavelength unit cells. Here, we study terahertz plasmonic crystals of several periods in a two dimensional electron gas. This plasmonic medium is both extremely subwavelength ($\approx λ/100$) and reconfigurable through the applicat…
This paper reports on design, measurement and optimisation of a Tamm plasmon metal-DBR cavity for use in the green part of the visible spectrum. It uses an optimised silver layer thickness and a porous DBR created using a novel electro-chemical etching technique. This device has applications in low cost lasers, photodetectors and photoconductive switches for the visible wavelength range.
Rabi-like splitting and self-referenced refractive index sensing in hybrid plasmonic-1D photonic crystal structures have been theoretically demonstrated. The coupling between Tamm plasmon and cavity photon modes are tuned by incorporating a low refractive index spacer layer adjacent to the metallic layer to form their hybrid modes. Anticrossing of the modes observed at different values of spacer layer thickness validates the strong coupling between the two modes and causes Rabi-like splitting with different splitting energy. Rabi-like splitting energy decreases with increasing number of period…
It is shown that cavities formed between a multilayer quarter-wave Bragg reflector and a metal mirror which support Tamm plasmons can be modelled by using a hard-mirror approximation including appropriate penetration depths into the mirrors. Results from this model are in excellent agreement with those found by numerical methods. In addition Tamm modes that are laterally confined by the presence of a metallic disc deposited on the Bragg reflector can be described by the effective index model that is commonly used for vertical-cavity surface-emitting lasers (VCSELs). This enables the lateral mo…
We report on the development, testing, and performance analysis of a bow-tie resonant cavity for terahertz (THz) radiation, injected with a continuous-wave 2.55 THz quantum cascade laser. The bow-tie cavity employs a wire-grid polarizer as input/output coupler and a pair of copper spherical mirrors coated with an unprotected 500 nm thick gold layer. The improvements with respect to previous setups have led to a measured finesse value F=123, and a quality factor Q = 5.1x10^5. The resonator performances and the relevant parameters are theoretically predicted and discussed, and a comparison among…
We systematically study the pump-wavelength dependence of terahertz pulse generation in thin-film spintronic THz emitters composed of a ferromagnetic Fe layer between adjacent nonmagnetic W and Pt layers. We find that the efficiency of THz generation is essentially at for excitation by 150 fs pulses with center wavelengths ranging from 900 to 1500 nm, demonstrating that the spin current does not depend strongly on the pump photon energy. We show that the inclusion of dielectric overlayers of TiO2 and SiO2, designed for a particular excitation wavelength, can enhance the terahertz emission by a…
Ultrafast atomic vibrations mediate heat transport, serve as fingerprints for chemical bonds and drive phase transitions in condensed matter systems. Light pulses shorter than the atomic oscillation period can not only probe, but even stimulate and control collective excitations. In general, such interactions are performed with free-propagating pulses. Here, we demonstrate intra-cavity excitation and time-domain sampling of coherent optical phonons inside an active laser oscillator. Employing real-time spectral interferometry, we reveal that Terahertz beats of Raman-active optical phonons can …
We consider a periodically gated two-dimensional electron system, with a central gate finger biased independently creating a tunable plasmonic cavity in a planar plasmonic crystal. We demonstrate that the plasmons resonantly excited in the periodic plasmonic lattice by incident terahertz radiation can strongly pump the cavity plasmon modes leading to a deep sub-wavelength concentration of terahertz energy with giant electric field enhancement factor up to 10000.
Vertical cavity surface emitting terahertz lasers can be realized in conventional semiconductor microcavities with embedded quantum wells in the strong coupling regime. The cavity is to be pumped optically at half the frequency of the 2p exciton state. Once a threshold population of 2p excitons is achieved, a stimulated terahertz transition populates the lower exciton-polariton branch, and the cavity starts emitting laser light both in the optical and terahertz ranges. The lasing threshold is sensitive to the statistics of photons of the pumping light.
We propose a scheme for efficient cavity-enhanced nonlinear THz generation via difference-frequency generation (DFG) processes using a triply resonant system based on photonic crystal cavities. We show that high nonlinear overlap can be achieved by coupling a THz cavity to a doubly-resonant, dual-polarization near-infrared (e.g. telecom band) photonic-crystal nanobeam cavity, allowing the mixing of three mutually orthogonal fundamental cavity modes through a chi(2) nonlinearity. We demonstrate through coupled-mode theory that complete depletion of the pump frequency - i.e., quantum-limited con…
A one-dimensional photonic-crystal (PC) cavity with nanoholes is proposed for extremely enhancing the THz electric fields by utilizing the electromagnetic (EM) boundary conditions, where both slot effect (for the perpendicular component of the electric displacement field) and anti-slot effect (for the parallel component of the electric field) contribute to the considerable field enhancement. The EM energy density can be enhanced in the high refractive index material by a factor of (εh/εl)^2, where εh and εl are the permittivities of the high and low refractive index materials, respectively. Co…
We report a new scheme of realizing terahertz fingerprint detection with ultrahigh sensitivity. Instead of using the direct absorption of terahertz through a bare sample in the regular transmission scheme, a cavity mode resonating at the characteristic frequency of the sample is used and due to the high dependence of the cavity mode transmission on the material loss, an amplified transmission decaying is observed when the sample is loaded into the cavity. Furthermore, this scheme retains the feature of substance identification. A one-dimensional photonic crystal cavity is used as the example f…
Tunable low-phase-noise terahertz synthesis using a fiber-interferometer-referenced optical frequency comb and an EDFA-integrated Vernier cavity
Graduate School of Sciences and Technology for Innovation, Tokushima University（德岛大学科学技术创新研究生院）；Department of Physics, Toho University（东海大学物理系）；Institute of Post-LED Photonics (pLED), Tokushima University（德岛大学后LED光子学研究所）；Institute of Photonics and Human Health Frontier (IPHF), Tokushima University（德岛大学光子学与人类健康前沿研究所）；Sevensix Inc.（Sevensix公司）
Presented here is the development and demonstration of a tunable cavity-enhanced terahertz frequency-domain optical Hall effect technique. The cavity consists of at least one fixed and one tunable Fabry-Pérot resonator. The approach is suitable for enhancement of the optical signatures produced by the optical Hall effect in semi-transparent conductive layer structures with plane parallel interfaces. The physical principle is the constructive interference of electric field components that undergo multiple optical Hall effect induced polarization rotations upon multiple light passages through th…
Dual-comb generation from a single laser cavity provides a simple and high-performance solution to time sampling applications. We demonstrate a compact single-cavity dual-comb laser operating at gigahertz repetition rates and high repetition rate differences up to more than 100 kHz with sub-100 fs pulse duration. The single cavity approach leads to passive common noise suppression resulting in ultra-low relative timing jitter and fully resolvable comb lines in free-running operation. We showcase the laser performance with two application demonstrations: (a) time-domain spectroscopy of acetylen…
The effect of a tunable, externally coupled Fabry-Pérot cavity to resonantly enhance the optical Hall effect signatures at terahertz frequencies produced by a traditional Drude-like two-dimensional electron gas is shown and discussed in this communication. As a result, the detection of optical Hall effect signatures at conveniently obtainable magnetic fields, for example by neodymium permanent magnets, is demonstrated. An AlInN/GaN-based high electron mobility transistor structure grown on a sapphire substrate is used for the experiment. The optical Hall effect signatures and their dispersions…
It is believed that passive mode locking is virtually impossible in quantum cascade lasers (QCLs) because of too fast carrier relaxation time. Here, we revisit this possibility and theoretically show that stable mode locking and pulse durations in the few cycle regime at terahertz (THz) frequencies are possible in suitably engineered bound-to-continuum QCLs. We achieve this by utilizing a multi-section cavity geometry with alternating gain and absorber sections. The critical ingredients are the very strong coupling of the absorber to both field and environment as well as a fast absorber carrie…
Deep-Subwavelength Plasmon Polariton Atomic Cavity Detector for Frequency- and Polarization-Sensitive Terahertz Detection and Imaging
State Key Laboratory of Optoelectronic Materials and Technologies（光电信息材料与技术国家重点实验室）；Guangdong Province Key Laboratory of Display Material and Technology（广东省显示材料与技术重点实验室）；School of Electronics and Information Technology（电子与信息学院）；Sun Yat-sen University（中山大学）
A new tuning mechanism is demonstrated for single-mode metal-clad plasmonic lasers, in which refractive-index of the laser's surrounding medium affects the resonant-cavity mode in the same vein as refractive-index of gain medium inside the cavity. Reversible, continuous, and mode-hop-free tuning of ~57GHz is realized for single-mode narrow-beam terahertz plasmonic quantum-cascade lasers (QCLs), which is demonstrated at much more practical temperature of 78K. The tuning is based on post-process deposition/etching of a dielectric (Silicon-dioxide) on a QCL chip that has already been soldered and…
The achievable instrument sensitivity is a critical parameter for the continued development of THz applications. Techniques such as Cavity-Enhanced Techniques and Cavity Ring Down Spectroscopy have not yet been employed at THz frequency due to the difficulties to construct a high finesse Fabry-Pérot cavity. Here, we describe such a THz resonator based on a low-loss oversized corrugated waveguide with highly reflective photonic mirrors obtaining a finesse above 3000 around 620 GHz. These components enable a Fabry-Perot THz Absorption Spectrometer with an equivalent interaction length of one kil…
Mode-resolved dual-comb spectroscopy (DCS) is an emerging spectroscopic tool with the potential to simultaneously achieve a broad spectral coverage and ultrahigh spectral resolution in terahertz (THz) spectroscopy. However, the need for two independently stabilized ultrafast lasers significantly hampers the potential application of DCS techniques. In this article, we demonstrate mode-resolved DCS in the THz region based on a free-running single-cavity dual-comb fiber laser with adaptive sampling. Low-pressure spectroscopy of acetonitrile gas with absorption features approaching the Doppler lim…
Nonperturbative coupling of light with condensed matter in an optical cavity is expected to reveal a host of coherent many-body phenomena and states. In addition, strong coherent light-matter interaction in a solid-state environment is of great interest to emerging quantum-based technologies. However, creating a system that combines a long electronic coherence time, a large dipole moment, and a high cavity quality ($Q$) factor has been a challenging goal. Here, we report collective ultrastrong light-matter coupling in an ultrahigh-mobility two-dimensional electron gas in a high-$Q$ terahertz p…
Giant enhancement of terahertz high-harmonic generation by cavity engineering of a three-dimensional Dirac semimetal
TU Dortmund University（多特蒙德工业大学）；CNR-Istituto Nanoscienze（国家研究委员会纳米科学研究所）；Scuola Normale Superiore（比萨高等师范学院）；University of Basel（巴塞尔大学）；Fudan University（复旦大学）；Shanghai Research Center for Quantum Sciences（上海量子科学研究中心）；Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）
Terahertz quantum cascade laser sources based on intra-cavity difference frequency generation from mid-IR devices are an important asset for applications in rotational molecular spectroscopy and sensing, beingthe only electrically pumped device able to operate in the 0.6-6 THz range without the need of bulky andexpensive liquid helium cooling. Here we present comb operation obtained by intra-cavity mixing of adistributed feedback laser at λ = 6.5 μm and a Fabry-Pérot device at around λ = 6.9 μm. The resultingultra-broadband THz emission extends from 1.8 to 3.3 THz, with a total output power of…
Dipolaritons are mixed light-matter quasiparticles formed in double quantum wells embedded in microcavities. Due to resonant coupling between direct and indirect excitons via electronic tunnelling, dipolaritons possess large dipole moments. Resonant excitation of the cavity mode by a short pulse of light induces oscillations of the indirect exciton density with a characteristic frequency of Rabi flopping. This results in oscillations of classical Hertz dipoles array which generate supperradiant emission on a terahertz (THz) frequency. Resulting THz signal may be enhanced using the supplementar…
High spectral purity frequency agile room temperature sources in the terahertz spectrum are foundational elements for imaging, sensing, metrology, and communications. Here we present a chip scale optical parametric oscillator based on an integrated nonlinear microresonator that provides broadly tunable single frequency and multi frequency oscillators in the terahertz regime. Through optical to terahertz down conversion using a plasmonic nanoantenna array, coherent terahertz radiation spanning 2.8 octaves is achieved from 330 GHz to 2.3 THz, with 20 GHz cavity mode limited frequency tuning step…
Solid state cavity quantum electrodynamics is a rapidly advancing field which explores the frontiers of light-matter coupling. Plasmonic approaches are of particular interest in this field, since they carry the potential to squeeze optical modes to spaces significantly below the diffraction limit1,2, enhancing light-matter coupling. They further serve as an architecture to design ultra-fast, non-linear integrated circuits with smallest footprints3. Transition metal dichalcogenides are ideally suited as the active material in such circuits as they interact strongly with light at the ultimate mo…
We have performed ultrafast pump-probe experiments on a GaAs-AlAs microcavity with a resonance near 1300 nm in the "original" telecom band. We exploit the virtually instantaneous electronic Kerr effect to repeatedly and reproducibly switch a GaAs-AlAs planar microcavity. We achieve repetition times as fast as 300 fs, thereby breaking the THz modulation barrier. The rate of the switching in our experiments is only determined by optics and not by material related relaxation. Our results offer novel opportunities for fundamental studies of cavity-QED and optical information processing in sub-pico…
We present quasi-analytical solutions (QANS) of hybrid platform (HP) comprising metallic grating (MG) and stacked-dielectric layers for terahertz (THz) radiation. The QANS are validated by finite difference time domain simulation. It is found that the Wood anomalies induce the high-order spoof surface plasmon resonances in the HP. The QANS are applied to optimize new perfect absorber for THz sensing of large-area thin film with ultrahigh figure of merit reaching fifth order of magnitude for the film thickness 0.0001p (p: MG period). The first-order Wood's anomaly of the insulator layer and the…
We suggest an indirect method of detection of photons with zero projection of spin mediated by emission of terahertz photons. This terahertz source is based on a system of microcavity exciton polaritons in the regime of polariton BEC formation when the cavity photons acquire an effective mass being localised in the cavity and therefore receive the third spin degree of freedom (corresponding to the longitudinal polarization with chirality l = 0). The optical transitions can occur between two polariton ground states based on the light-hole and heavy-hole excitons, respectively, accompanied by th…
The vast majority of resonant systems show a red-shift for the resonance frequency when a perturbation, e.g. losses, are introduced to the system. In contrast, here we report for the first time the experimental demonstration of both red- and anomalous blue-shifting of whispering-gallery modes (WGMs) using dielectric and metallic substrates. The maximum blue-shift is more than three times as large as the expected red-shift, proving that the anomalous blue-shift is more than a peculiar curiosity. The experiments are performed in the terahertz (THz) frequency range with coherent continuous-wave s…
We report on an attempt to generate highly stable continuous terahertz (THz) wave by using optical frequency comb (OFC). About 10-nm wide OFC has been generated through a deep phase modulation of a 852 nm laser line in lithium niobate crystal cavity. The multiple optical modes (side bands) of the OFC, which are equally separated from each other by the modulation frequency (=6 GHz) are taken as the frequency reference. When another semiconductor laser is frequency locked, the stability of the difference frequency between the master laser and the second laser is improved on the same order of the…
The ability to engineer quantum-cascade-lasers (QCLs) with ultrabroad gain spectra and with a full compensation of the group velocity dispersion, at Terahertz (THz) frequencies, is a fundamental need for devising monolithic and miniaturized optical frequency-comb-synthesizers (FCS) in the far-infrared. In a THz QCL four-wave mixing, driven by the intrinsic third-order susceptibility of the intersubband gain medium, self-lock the optical modes in phase, allowing stable comb operation, albeit over a restricted dynamic range (~ 20% of the laser operational range). Here, we engineer miniaturized T…
The majority of sources of coherent optical radiation rely on laser oscillators driven by population inversion. Despite their technological importance in communications, medicine, industry, and other fields, it remains a challenge to access the spectral range of 0.1-10 THz (the "terahertz gap"), a frequency band for applications ranging from spectroscopy to security and high-speed wireless communications. Here, we propose a way to produce coherent radiation spanning the THz gap by efficient second-harmonic generation (SHG) in low-loss dielectric structures, starting from technologically mature…
We present an electrically switchable graphene terahertz (THz) modulator with a tunable-by-design optical bandwidth and we exploit it to compensate the cavity dispersion of a quantum cascade laser (QCL). Electrostatic gating is achieved by a metal-grating used as a gate electrode, with an HfO2/AlOx gate dielectric on top. This is patterned on a polyimide layer, which acts as a quarter wave resonance cavity, coupled with an Au reflector underneath. We get 90% modulation depth of the intensity, combined with a 20 kHz electrical bandwidth in the 1.9 _ 2.7 THz range. We then integrate our modulato…
The device applications of plasmonic systems such as graphene and two dimensional electron gases (2DEGs) in III-V heterostructures include terahertz detectors, mixers, oscillators and modulators. These two dimensional (2D) plasmonic systems are not only well-suited for device integration, but also enable the broad tunability of underdamped plasma excitations via an applied electric field. We present demonstrations of the coherent coupling of multiple voltage tuned GaAs/AlGaAs 2D plasmonic resonators under terahertz irradiation. By utilizing a plasmonic homodyne mixing mechanism to downconvert …
Dual THz comb spectroscopy has the potential to be used as universal THz spectroscopy with high spectral resolution, high spectral accuracy, and broad spectral coverage; however, the requirement for dual stabilized femtosecond lasers hampers its versatility due to the bulky size, high complexity, and high cost. We here report the first demonstration of dual THz comb spectroscopy using a single free-running fibre laser. By tuning the cavity-loss-dependent gain profile with an intracavity Lyot filter together with precise management of the cavity length and dispersion, dual-wavelength pulsed lig…
On the basis of an energy-recovery linac, a terahertz (THz) source with kilowatts average power is proposed in Shanghai, which will serve as an effective tool in material and biological sciences. In this paper, the physical design of two free electron laser (FEL) oscillators, in the frequency range of 2~10THz and 0.5~2THz respectively, are presented. By using three dimensional, time-dependent numerical modeling of GENESIS in combination with paraxial optical propagation code (OPC), the THz oscillator performances, the detuning effects, and the tolerance requirements on the electron beam, the u…
The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the equidistant lines from a laser frequency comb are simultaneously injected into the cavity over a large spectral range, multiple trace-gases may be identified within a few milliseconds. Analyzing efficiently the light transmitted through the cavity however still remains challenging. Here, a novel approach, cavity-enhanced frequency comb Fourier transform spectroscopy,…
Quantum cascade lasers (QCLs) represent a fascinating accomplishment of quantum engineering and enable the direct generation of terahertz (THz) frequency radiation from an electrically-biased semiconductor heterostructure. Their large spectral bandwidth, high output powers and quantum-limited linewidths have facilitated the realization of THz pulses by active mode-locking and passive generation of optical frequency combs (FCs) through intracavity four-wave-mixing, albeit over a restricted operational regime. Here, we conceive an integrated architecture for the generation of high power (10 mW) …
