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arXiv 2102.13432cond-mat.supr-concond-mat.str-el
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hydrostatic pressure下Hg基铜氧化物超导体的拉曼光谱研究

Exploration of the Hg-based cuprate superconductors by Raman spectroscopy under hydrostatic pressure

N. Auvray, B. Loret, S. Chibani, R. Grasset, Y. Guarnelli, P. Parisiades, A. Forget, D. Colson, M. Cazayous, Y. Gallais, Alain Sacuto

摘要:

用Raman光谱研究了$\mathrm{HgBa}_2\mathrm{CuO}_{4+δ}$(Hg-1201)和$\mathrm{HgBa}_2\mathrm{Ca}_2\mathrm{Cu}_3\mathrm{O}_{8+δ}$(Hg-1223)铜酸盐的超导相。我们的分析表明,由于Hg-1223的$\mathrm{CuO}_2$层之间的电荷载流子浓度不平衡(由压力加剧),Hg-1223铜酸盐中$T_c$随压力的增加比Hg-1201慢。我们发现,在压力下的顶端氧模式的电荷载流子转移到$\mathrm{CuO}_2$层的能量变化,是相同的Hg-1223和Hg-1223铜酸盐,它是由层间压缩性控制。最后,我们证明了与$d-$波超导能隙的最大振幅有关的Cooper对的结合能不随压力的变化服从$T_c$.当$T_c$增加时,其减少。在Hg-1201的特定情况下,当压力增加到10 GPa时,结合能从10下降到2 $K_B T_c$。这些直接的光谱观测结合了这样一个事实,即在反节点处的库珀对的结合能并不遵循$T_c$,也没有掺杂,提出了它与赝能隙能量尺度的联系的问题,赝能隙能量尺度遵循掺杂的相同趋势。

英文摘要:

The superconducting phase of the $\mathrm{HgBa}_2\mathrm{CuO}_{4+δ}$ (Hg-1201) and $\mathrm{HgBa}_2\mathrm{Ca}_2\mathrm{Cu}_3\mathrm{O}_{8+δ}$ (Hg-1223) cuprates has been investigated by Raman spectroscopy under hydrostatic pressure. Our analysis reveals that the increase of $T_c$ with pressure is slower in Hg-1223 cuprate compared to the Hg-1201 due to a charge carrier concentration imbalance (accentuated by pressure) between the $\mathrm{CuO}_2$ layers of Hg-1223. We find that the energy variation under pressure of the apical oxygen mode from which the charge carriers are transferred to the $\mathrm{CuO}_2$ layers, is the same for both the Hg-1223 and Hg-1223 cuprates and it is controlled by the inter-layer compressibility. At last, we show that the binding energy of the Cooper pairs related to the maximum amplitude of the $d-$ wave superconducting gap at the anti-nodes, does not follow $T_c$ with pressure. It decreases while $T_c$ increases. In the particular case of Hg-1201, the binding energy collapses from 10 to 2 $K_B T_c$ as the pressure increases up to 10 GPa. These direct spectroscopic observations joined to the fact that the binding energy of the Cooper pairs at the anti-nodes does not follow $T_c$ either with doping, raises the question of its link with the pseudogap energy scale which follows the same trend with doping.

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