Minute amount of long chain flexible polymer dissolved in a turbulent flow can drastically change flow properties, such as reducing the drag and enhancing mixing. One fundamental riddle is how these polymer additives interact with the eddies of different spatial scales existing in the turbulent flow and in turn alter the turbulence energy transfer. Here we show how turbulent kinetic energy is transferred through deferent scales in the presence of the polymer additives. In particular, we observed experimentally the emerging of a new scaling range, referred to as the elastic range, where increasing amount of energy is transferred by the elasticity of the polymers. In addition, the existence of the elastic range prescribes the scaling of high-order velocity statistics. Our findings have important implications to many turbulence systems such as turbulence in plasmas or superfluids where interaction between turbulent eddies and other nonlinear physical mechanisms are often involved.
We study the physics of turbulent/non-turbulent interface of an isolated turbulent region in dilute polymer solutions and Newtonian fluid. The performance of a FENE-P model with a localized homogeneous forcing is verified using the specially designed experimental setup of a turbulent patch growing in water/dilute polymer solution, without mean shear and far from the walls. The results of the small scale dynamics of vorticity and strain help to reveal the key mechanism of polymer action in turbulent flows without mean shear. Modified degrees of alignment between vorticity, the polymer conformat…
By tracking small particles in the bulk of an intensely turbulent flow, we show that even a very small concentration of long-chain polymers disrupts the usual turbulent energy cascade. The polymers affect scales much larger than their physical size, from the dissipation range to the inertial range. The effect depends strongly on the polymer concentration. While the dissipative-scale statistics change continuously as the polymer concentration is increased, the inertial-range energy transfer rate is only altered by the polymer additives when the concentration is above a threshold (approximately …
Measurements of heat transport, as expressed by the Nusselt number $Nu$, are reported for turbulent Rayleigh-Bénard convection of water containing up to 120 ppm by weight of poly-[ethylene oxide] with a molecular weight of $4\times10^6$ g/mole. Over the Rayleigh number range $ 5\times 10^9 \alt Ra \alt 7 \times 10^{10}$ $Nu$ is smaller than it is for pure water by up to 10%.
We present the most extensive direct numerical simulations, attempted so far, of statistically steady, homogeneous, isotropic turbulence in two-dimensional fluid films with air-drag-induced friction and with polymer additives. Our study reveals that the polymers (a) reduce the total fluid energy, enstrophy, and palinstrophy, (b) modify the fluid energy spectrum both in inverse- and forward-cascade regimes, (c) reduce small-scale intermittency, (d) suppress regions of large vorticity and strain rate, and (e) stretch in strain-dominated regions. We compare our results with earlier experimental s…
This letter confirms the existence of heat transfer enhancement (HTE) and reduction (HTR) in turbulent natural convection with polymer additives. HTE and HTR were numerically predicted by Benzi et al.(PRL, 104, 024502, 2010) in homogenous turbulent convection, but experiments by Ahlers & Nikolaenko(PRL, 104, 034503, 2010) in turbulent natural convection observed HTR only. Using direct numerical simulation of natural convection, the present study reconciles earlier numerical and experimental work on the basis of the dominant role of polymer length in the polymer dynamics in extensional flows.
The modification of dominant coherent structures that extend through the log-region of a drag reduced turbulent boundary layer is studied via examination of two-point correlations from time-resolved particle-image-velocimetry. Measurements were acquired in polymer oceans (uniform concentration) at drag reduction levels corresponding to the low drag reduction regime (< 40%), the high drag reduction (HDR) regime (>40%), and at an intermediate level (46%). The mean velocity profiles and two-point correlations were compared with that of water (Newtonian, DR = 0%). These results show that with incr…
We present an experimental investigation of turbulent drag reduction with flexible and rigid polymer solutions. The flexible polymer is partially hydrolyzed polyacrylamide (HPAM) and the rigid polymer is xanthan gum (XG). The experiments are carried out at low drag reduction ($\%DR < 40$), high drag reduction ($\%DR > 40$) and maximum drag reduction (where the velocity profile $U^+$ roughly matches Virk's asymptote). We compare velocity profiles, streamwise and wall-normal Reynolds stresses and power spectra of streamwise velocity fluctuations measured by Laser Doppler Anemometry (LDA). Our re…
We present direct numerical simulations of turbulent channel flow with passive Lagrangian polymers. To understand the polymer behavior we investigate the behavior of infinitesimal line elements and calculate the probability distribution function (PDF) of finite-time Lyapunov exponents and from them the corresponding Cramer's function for the channel flow. We study the statistics of polymer elongation for both the Oldroyd-B model (for Weissenberg number $\Wi <1$) and the FENE model. We use the location of the minima of the Cramer's function to define the Weissenberg number precisely such that w…
We report measurements of turbulent drag reduction of two different polyelectrolyte solutions: DNA and hydrolyzed Polyacrylamide. Changing the salt concentration in the solutions allows us to change the flexibility of the polymer chains. For both polymers the amount of drag reduction was found to increase with the flexibility. Rheological studies reveal that the elongational viscosity of the solutions increases simultaneously. Hence we conclude that the elongational viscosity is the pertinent macroscopic quantity to describe the ability of a polymer to cause turbulent drag reduction.
We have performed direct numerical simulation of the turbulent flow of a polymer solution in a square duct, with the FENE-P model used to simulate the presence of polymers. First, a simulation at a fixed moderate Reynolds number is performed and its results compared with those of a Newtonian fluid to understand the mechanism of drag reduction and how the secondary motion, typical of the turbulent flow in non-axisymmetric ducts, is affected by polymer additives. Our study shows that the Prandtl's secondary flow is modified by the polymers: the circulation of the streamwise main vortices increas…
Recent direct numerical simulations of the FENE-P model of non-Newtonian hydrodynamics revealed that the phenomenon of drag reduction by polymer additives exists (albeit in reduced form) also in homogeneous turbulence. We introduce here a simple shell model for homogeneous viscoelastic flows that recaptures the essential observations of the full simulations. The simplicity of the shell model allows us to offer a transparent explanation of the main observations. It is shown that the mechanism for drag reduction operates mainly on the large scales. Understanding the mechanism allows us to predic…
Polymer additives are commonly utilized to manipulate bubbly flows in various applications. Here, we investigate the effects of clean and contaminated bubbles driven upwards (upflow) in Newtonian and viscoelastic turbulent channel flows. Interface-resolved direct numerical simulations are performed to examine sole and combined effects of soluble surfactant and viscoelasticity using an efficient 3D finite-difference/front-tracking method. The incompressible flow equations are solved fully coupled with the FENE-P viscoelastic model and the equations governing interfacial and bulk surfactant conc…
We extend the analysis of the friction factor for turbulent pipe flow reported by G. Gioia, P. Chakraborty and N. Goldenfeld (GCG) (G. Gioia and P. Chakraborty, Phys. Rev. Lett. 96, 044502 (2006), N. Goldenfeld, Phys. Rev. Lett. 96, 044503 (2006)) to the case where drag is reduced by polymer additives.
We report experimental measurements of Lagrangian accelerations in the bulk of intense turbulent flows of dilute polymer solutions by following tracer particles with a high-speed optical tracking system. We observed a significant decrease in the acceleration variance in dilute polymer solutions. The shape of the normalized acceleration probability density functions, however, remain the same as in Newtonian water flows. We also observed an increase in the turbulent Lagrangian acceleration autocorrelation time in these dilute polymer solutions.
We address the "Additive Equivalence" discovered by Virk and coworkers: drag reduction affected by flexible and rigid rodlike polymers added to turbulent wall-bounded flows is limited from above by a very similar Maximum Drag Reduction (MDR) asymptote. Considering the equations of motion of rodlike polymers in wall-bounded turbulent ensembles, we show that although the microscopic mechanism of attaining the MDR is very different, the macroscopic theory is isomorphic, rationalizing the interesting experimental observations.
The interaction of polymers with small-scale velocity gradients can trigger a coil-stretch transition in the polymers. We analyze this transition within a direct numerical simulation of shear turbulence with an Oldroyd-B model for the polymer. In the coiled state the lengths of polymers are distributed algebraically with an exponent alpha=2 gamma-1/De, where gamma is a characteristic stretching rate of the flow and De the Deborah number. In the stretched state we demonstrate that the length distribution of the polymers is limited by the feedback to the flow.
This paper is focused on the fundamental mechanism(s) of viscoelastic turbulence that lead to polymer induced turbulent drag reduction phenomenon. A great challenge in this problem is the computation of viscoelastic turbulent flows, since the understanding of polymer physics is restricted to mechanical models. An effective state-of-the-art numerical method to solve the governing equation for polymers modelled as non-linear springs, without using any artificial assumptions as usual, was implemented here for the first time on a three-dimensional channel flow geometry. The capability of this algo…
Drag reduction by polymers in turbulent wall-bounded flows exhibits universal and non-universal aspects. The universal maximal mean velocity profile was explained in a recent theory. The saturation of this profile and the crossover back to the Newtonian plug are non-universal, depending on Reynolds number Re, concentration of polymer $c_p$ and the degree of polymerization $N_p$. We explain the mechanism of saturation stemming from the finiteness of extensibility of the polymers, predict its dependence on $c_p$ and $N$ in the limit of small $c_p$ and large Re, and present the excellent comparis…
The interaction of polymers with turbulent shear flows is examined. We focus on the structure of the elastic stress tensor, which is proportional to the polymer conformation tensor. We examine this object in turbulent flows of increasing complexity. First is isotropic turbulence, then anisotropic (but homogenous) shear turbulence and finally wall bounded turbulence. The main result of this paper is that for all these flows the polymer stress tensor attains a universal structure in the limit of large Deborah number $\De\gg 1$. We present analytic results for the suppression of the coil-stretch …
The statistics of polymers advected by a turbulent flow are investigated. To limit the polymer lengths above to coil-stretch transition, a FENE-P type relaxation law is used. The turbulence is modeled by a random strain, delta-correlated in time and with Gaussian statistics. The distribution of polymer lengths for both the coiled and stretched states are derived, from which are obtained analytical expressions for the moments of the distribution. The polymer stress on the fluid decreases linearly with the inverse of the Deborah number. The degradation (breaking) of the polymers is also discusse…
Polymers in a turbulent flow are subject to intense strain, which can cause their scission and thereby limit the experimental study and application of phenomena such as turbulent drag reduction and elastic turbulence. In this paper, we study polymer scission in homogeneous isotropic turbulence, through a combination of stochastic modelling, based on a Gaussian time-decorrelated random flow, and direct numerical simulations (DNSs) with both one-way (passive) and two-way (active) coupling of the polymers and the flow. For the first scission of passive polymers, the stochastic model yields analyt…
We carry out a direct numerical simulation (DNS) study that reveals the effects of polymers on statistically steady, forced, homogeneous, isotropic fluid turbulence. We find clear manifestations of dissipation-reduction phenomena: On the addition of polymers to the turbulent fluid, we obtain a reduction in the energy dissipation rate, a significant modification of the fluid energy spectrum, especially in the deep-dissipation range, a suppression of small-scale intermittency, and a decrease in small-scale vorticity filaments. We also compare our results with recent experiments and earlier DNS s…
The upper bound of polymer drag reduction is identified as a unique transitional state between laminar and turbulent flow corresponding to the onset of the nonlinear breakdown of flow instabilities.
We study the clustering properties of inertial particles in a turbulent viscoelastic fluid. The investigation is carried out by means of direct numerical simulations of turbulence in the Oldroyd-B model. The effects of polymers on the small scale properties of homogeneous turbulence are considered in relation with their consequences on clustering of particles, both lighter and heavier than the carrying fluid. We show that, depending on particle and flow parameters, polymers can either increase or decrease clustering.
Drag reduction, or, what is the same, mean velocity increase in a turbulent flow at a fixed pressure drop through the addition of tiny amounts (several parts per million) of high molecular weight polymers (Thoms effect), is known already for more than sixty years. Rather long ago it was understood that this effect is related to supramolecular structures formed in the flow. Recent experiments by S. Chu, E.S.G. Shaqfeh and their associates, where the motion of supramolecular structures was directly observed, made it possible to understand and quantify the dynamic interaction of the polymeric str…
The drag of turbulent flows can be drastically decreased by addition of small amounts of high molecular weight polymers. While drag reduction initially increases with polymer concentration, it eventually saturates to what is known as the maximum drag reduction (MDR) asymptote; this asymptote is generally attributed to the dynamics being reduced to a marginal yet persistent state of subdued turbulent motion. Contrary to this accepted view we will show in the following that for an appropriate choice of parameters polymers can reduce the drag beyond the suggested asymptotic limit, eliminating tur…
The existence of drag reduction by polymer additives, well established for wall-bounded turbulent flows, is controversial in homogeneous, isotropic turbulence. To settle this controversy we carry out a high-resolution direct numerical simulation (DNS) of decaying, homogeneous, isotropic turbulence with polymer additives. Our study reveals clear manifestations of drag-reduction-type phenomena: On the addition of polymers to the turbulent fluid we obtain a reduction in the energy dissipation rate, a significant modification of the fluid energy spectrum especially in the deep-dissipation range, a…
We study the impact of the Peterlin approximation on the statistics of the end-to-end separation of poly- mers in a turbulent flow. The FENE and FENE-P models are numerically integrated along a large number of Lagrangian trajectories resulting from a direct numerical simulation of three-dimensional homogeneous isotropic turbulence. Although the FENE-P model yields results in qualitative agreement with those of the FENE model, quantitative differences emerge. The steady-state probability of large extensions is overesti- mated by the FENE-P model. The alignment of polymers with the eigenvectors …
Electroconvection in rechargeable batteries enhances the growth of dendrites at the electrode surface. The addition of low molecular weight polymers to the electrolyte in batteries results in the formation of a thin layer of higher polymer concentration near the electrode. This is due to van der Waals forces of attraction between the metal electrode and the polymers dissolved in the electrolyte. The van der Waals forces act as a restoring body force on the electrolyte and oppose the growth of perturbations. Using linear stability analysis, we show that this force opposes electroconvective flow…
A small amount of polymer additives can cause substantial reduction in the energy dissipation and friction loss of turbulent flow. The problem of polymer-induced drag reduction has attracted continuous attention over the seven decades since its discovery. However, changes in research paradigm and perspectives have triggered a wave of new advancements in the past decade. This review attempts to bring researchers of all levels, from beginners to experts, to the forefront of this area. It starts with a comprehensive coverage of fundamental knowledge and classical findings and theories. It then hi…
We study properties of dilute polymer solutions which are known to depend strongly on polymer elongation. The probability density function (PDF) of polymer end-to-end extensions $R$ in turbulent flows is examined. We demonstrate that if the value of the Lyapunov exponent $λ$ is smaller than the inverse molecular relaxation time $1/τ$ then the PDF has a strong peak at the equilibrium size $R_0$ and a power tail at $R\gg R_0$. This confirms and extends the results of \cite{Lumley72}. There is no essential influence of polymers on the flow in the regime $λτ<1$. At $λ>1/τ$ the majority of molecule…
We present results from a systematic numerical study of decaying turbulence in a dilute polymer solution by using a shell-model version of the FENE-P equations. Our study leads to an appealing definition of drag reduction for the case of decaying turbulence. We exhibit several new results, such as the potential-energy spectrum of the polymer, hitherto unobserved features in the temporal evolution of the kinetic-energy spectrum, and characterize intermittency in such systems. We compare our results with the GOY shell model for fluid turbulence.
We show that viscoelastic plane Poiseuille flow becomes linearly unstable in the absence of inertia, in the limit of high elasticities, for ultra-dilute polymer solutions. While inertialess elastic instabilities have been predicted for curvilinear shear flows, this is the first ever report of a purely elastic linear instability in a rectilinear shear flow. The novel instability continues upto a Reynolds number ($Re$) of $O(1000)$, corresponding to the recently identified elasto-inertial turbulent state believed to underlie the maximum-drag-reduced regime. Thus, for highly elastic ultra-dilute …
The role of polymers additives on the turbulent convective flow of a Rayleigh--Taylor system is investigated by means of direct numerical simulations (DNS) of Oldroyd-B viscoelastic model. The dynamics of polymers elongation follow adiabatically the self-similar evolution of the turbulent mixing layer, and shows the appearance of a strong feedback on the flow which originate a cut off for polymer elongations. The viscoelastic effects on the mixing properties of the flow are twofold. Mixing is appreciably enhanced at large scales (the mixing layer growth-rate is larger than that of the purely N…
A polymer in a turbulent flow undergoes the coil-stretch transition when the Weissenberg number, i.e. the product of the Lyapunov exponent of the flow and the relaxation time of the polymer, surpasses a critical value. The effect of internal friction on the transition is studied by means of Brownian dynamics simulations of the elastic dumbbell model in a homogeneous and isotropic, incompressible, turbulent flow and analytical calculations for a stochastic velocity gradient. The results are explained by adapting the large deviations theory of Balkovsky et al. [Phys. Rev. Lett., 2000, 84, 4765] …
Elasto-inertial turbulence is a new state of turbulence found in flows with polymer additives . The dynamics of turbulence generated and controlled by such additives is investigated from the perspective of the coupling between polymer dynamics and flow structures. Direct numerical simulations of channel flow with Reynolds numbers ranging from 1000 to 6000 (based on the bulk and the channel height) are used to study the formation and dynamics of elastic instabilities and their effects on the flow. The resulting mechanism of interactions between polymer dynamics and the flow helps resolve a long…
The fluids and polymers have different fundamental symmetries. Namely, the Lagrangian relabeling symmetry of fluids is absent for polymers (while the translational and rotational symmetries are still present). This fact results in spontaneous breaking of the relabeling symmetry in fluid turbulence even at a tiny polymer addition. Since helicity conservation in inviscid fluid motions is a consequence of the relabeling symmetry (due to the Noether's theorem) violation of this conservation by the polymer additives results in the strong effects in the distributed chaos. The distributed chaos in tu…
Turbulent channel flow of drag-reducing polymer solutions is simulated in minimal flow geometries. Even in the Newtonian limit, we find intervals of "hibernating" turbulence that display many features of the universal maximum drag reduction (MDR) asymptote observed in polymer solutions: weak streamwise vortices, nearly nonexistent streamwise variations and a mean velocity gradient that quantitatively matches experiments. As viscoelasticity increases, the frequency of these intervals also increases, while the intervals themselves are unchanged, leading to flows that increasingly resemble MDR.
Coherent structures in Newtonian and viscoelastic turbulent planar jets
Okinawa Institute of Science and Technology Graduate University（冲绳科学技术大学院大学）；Universidad Polit{é}cnica de Madrid（马德里理工大学）；Flow Matters Consultancy BV（Flow Matters咨询有限公司）
Mixing in fluids is a rapidly developing field of fluid mechanics \cite{Sreen,Shr,War}, being an important industrial and environmental problem. The mixing of liquids at low Reynolds numbers is usually quite weak in simple flows, and it requires special devices to be efficient. Recently, the problem of mixing was solved analytically for a simple case of random flow, known as the Batchelor regime \cite{Bat,Kraich,Fal,Sig,Fouxon}. Here we demonstrate experimentally that very viscous liquids at low Reynolds number, $Re$. Here we show that very viscous liquids containing a small amount of high mol…
Cellulose nanocrystals (CNC) are naturally-derived nanostructures of growing importance for the production of composites having attractive mechanical properties, and offer improved sustainability over purely petroleum-based alternatives. Fabrication of CNC composites typically involves extrusion of CNC suspensions and gels in a variety of solvents, in the presence of additives such as polymers and curing agents. However, most studies so far have focused on aqueous CNC gels, yet the behavior of CNC-polymer gels in organic solvents is important to their wider processability. Here, we study the r…
We present numerical studies of stretching of Hookean dumbbells in a turbulent Navier-Stokes flow with a linear mean profile, <u_x>=Sy. In addition to the turbulence features beyond the viscous Kolmogorov scale η, the dynamics at the equilibrium extension of the dumbbells significantly below eta is well resolved. The variation of the constant shear rate S causes a change of the turbulent velocity fluctuations on all scales and thus of the intensity of local stretching rate of the advecting flow. The latter is measured by the maximum Lyapunov exponent lambda_1 which is found to increase as λ_1 …
Polymers in a turbulent flow are stretched out by the fluctuating velocity gradient; the stationary probability distribution function (p.d.f.) of extensions $R$ has a power-law tail with an exponent that increases with the Weissenberg number $Wi$, a nondimensional measure of polymer elasticity. This study addresses the following questions: (i) What is the role of the non-Gaussian statistics of the turbulent velocity gradient on polymer stretching? (ii) How does the p.d.f. of $R$ evolve to its asymptotic stationary form? Our analysis is based on simulations of the dynamics of finitely-extensibl…
We address the phenomenon of drag reduction by dilute polymeric additive to turbulent flows, using Direct Numerical Simulations (DNS) of the FENE-P model of viscoelastic flows. It had been amply demonstrated that these model equations reproduce the phenomenon, but the results of DNS were not analyzed so far with the goal of interpreting the phenomenon. In order to construct a useful framework for the understanding of drag reduction we initiate in this paper an investigation of the most important modes that are sustained in the viscoelastic and Newtonian turbulent flows respectively. The modes …
Injection of dilute polymer in a turbulent flow suppresses frictional drag. This challenging and technologically important problem remains primarily unresolved due to the complex nature of the flow. An important factor in the drag reduction is the energy transfer from the velocity field to the polymers. In this paper we quantify this process using energy fluxes, as well as show its universality in diverse flows such as magnetohydrodynamics, quasi-static magnetohydrodynamics, and bubbly turbulence. We show that in such flows, the transfer from kinetic energy to elastic energy leads to a reducti…
In this review, we describe turbulent drag reduction in a variety of flows using a universal framework of energy flux. In a turbulent flow with dilute polymers and magnetic field, the kinetic energy injected at large scales cascades to the velocity field at intermediate scales, as well as to the polymers and magnetic field at all scales. Consequently, the kinetic energy flux, $ Π_u(k) $, is suppressed in comparison to the pure hydrodynamic turbulence. We argue that the suppression of $Π_u(k)$ is an important factor in the reduction of the inertial force $\langle {\bf u \cdot \nabla u} \rangle$…
X-ray particle tracking velocimetry for steady-state rheological characterization: Case study of a complex polymer melt flow in material extrusion additive manufacturing
University of Stuttgart（斯图加特大学）；University of Milan（米兰大学）；CNR – Consiglio Nazionale delle Ricerche, Istituto di Chimica della Materia Condensata e di Tecnologie per l’Energia（意大利国家研究委员会凝聚态材料与能源技术研究所）
Long-chained, viscoelastic surfactant solutions (VES) have been widely employed in the oil and gas industry, particularly in hydraulic fracturing and gravel-packing operations, where turbulence is commonly reached due to high pumping rates. With this motivation, we experimentally investigate the turbulent duct flow of an under-studied class of wormlike micellar solutions that forms a gel at room temperature. The fluid is characterized via rotational rheometry, and the turbulent velocity and Reynolds stress profiles are measured via Laser Doppler Anemometry (LDA). Three surfactant concentration…
