Polymers in a turbulent flow are subject to intense strain, which can cause their scission and thereby limit the experimental study and application of phenomena such as turbulent drag reduction and elastic turbulence. In this paper, we study polymer scission in homogeneous isotropic turbulence, through a combination of stochastic modelling, based on a Gaussian time-decorrelated random flow, and direct numerical simulations (DNSs) with both one-way (passive) and two-way (active) coupling of the polymers and the flow. For the first scission of passive polymers, the stochastic model yields analytical predictions which are found to be in good agreement with results from the DNSs, for the temporal evolution of the fraction of unbroken polymers and the statistics of the survival of polymers. The impact of scission on the dynamics of a turbulent polymer solution is investigated through DNSs with two-way coupling (active polymers). Our results indicate that the reduction of kinetic energy dissipation due to feedback from stretched polymers is an inherently transient effect, which is lost as the polymers breakup. Thus, the overall dissipation-reduction is maximised by an intermediate polymer relaxation time, for which polymers stretch significantly but without breaking too quickly. We also study the dynamics of the polymer fragments which form after scission; these daughter polymers can themselves undergo subsequent, repeated, breakups to produce a hierarchical population of polymers with a range of relaxation times and scission rates.
When injected through a contraction, high molecular weight polymer solutions exhibit a sharp increase of apparent viscosity which originates from stretching polymer chains above a critical extension rate. This chain stretching can also induce polymer scission, which then decreases the extensional viscosity. In practice, the two phenomena are difficult to separate. Moreover, these phenomena are often observed in situation where flow instabilities appear. In order to disentangle the two effects we have measured the pressure-flux relation for polymer solutions passing through a hyperbolic contrac…
The statistics of polymers advected by a turbulent flow are investigated. To limit the polymer lengths above to coil-stretch transition, a FENE-P type relaxation law is used. The turbulence is modeled by a random strain, delta-correlated in time and with Gaussian statistics. The distribution of polymer lengths for both the coiled and stretched states are derived, from which are obtained analytical expressions for the moments of the distribution. The polymer stress on the fluid decreases linearly with the inverse of the Deborah number. The degradation (breaking) of the polymers is also discusse…
We extend the analysis of the friction factor for turbulent pipe flow reported by G. Gioia, P. Chakraborty and N. Goldenfeld (GCG) (G. Gioia and P. Chakraborty, Phys. Rev. Lett. 96, 044502 (2006), N. Goldenfeld, Phys. Rev. Lett. 96, 044503 (2006)) to the case where drag is reduced by polymer additives.
We address the "Additive Equivalence" discovered by Virk and coworkers: drag reduction affected by flexible and rigid rodlike polymers added to turbulent wall-bounded flows is limited from above by a very similar Maximum Drag Reduction (MDR) asymptote. Considering the equations of motion of rodlike polymers in wall-bounded turbulent ensembles, we show that although the microscopic mechanism of attaining the MDR is very different, the macroscopic theory is isomorphic, rationalizing the interesting experimental observations.
The interaction of polymers with small-scale velocity gradients can trigger a coil-stretch transition in the polymers. We analyze this transition within a direct numerical simulation of shear turbulence with an Oldroyd-B model for the polymer. In the coiled state the lengths of polymers are distributed algebraically with an exponent alpha=2 gamma-1/De, where gamma is a characteristic stretching rate of the flow and De the Deborah number. In the stretched state we demonstrate that the length distribution of the polymers is limited by the feedback to the flow.
Drag reduction by polymers in turbulent wall-bounded flows exhibits universal and non-universal aspects. The universal maximal mean velocity profile was explained in a recent theory. The saturation of this profile and the crossover back to the Newtonian plug are non-universal, depending on Reynolds number Re, concentration of polymer $c_p$ and the degree of polymerization $N_p$. We explain the mechanism of saturation stemming from the finiteness of extensibility of the polymers, predict its dependence on $c_p$ and $N$ in the limit of small $c_p$ and large Re, and present the excellent comparis…
The interaction of polymers with turbulent shear flows is examined. We focus on the structure of the elastic stress tensor, which is proportional to the polymer conformation tensor. We examine this object in turbulent flows of increasing complexity. First is isotropic turbulence, then anisotropic (but homogenous) shear turbulence and finally wall bounded turbulence. The main result of this paper is that for all these flows the polymer stress tensor attains a universal structure in the limit of large Deborah number $\De\gg 1$. We present analytic results for the suppression of the coil-stretch …
The existence of drag reduction by polymer additives, well established for wall-bounded turbulent flows, is controversial in homogeneous, isotropic turbulence. To settle this controversy we carry out a high-resolution direct numerical simulation (DNS) of decaying, homogeneous, isotropic turbulence with polymer additives. Our study reveals clear manifestations of drag-reduction-type phenomena: On the addition of polymers to the turbulent fluid we obtain a reduction in the energy dissipation rate, a significant modification of the fluid energy spectrum especially in the deep-dissipation range, a…
We study the physics of turbulent/non-turbulent interface of an isolated turbulent region in dilute polymer solutions and Newtonian fluid. The performance of a FENE-P model with a localized homogeneous forcing is verified using the specially designed experimental setup of a turbulent patch growing in water/dilute polymer solution, without mean shear and far from the walls. The results of the small scale dynamics of vorticity and strain help to reveal the key mechanism of polymer action in turbulent flows without mean shear. Modified degrees of alignment between vorticity, the polymer conformat…
We study the impact of the Peterlin approximation on the statistics of the end-to-end separation of poly- mers in a turbulent flow. The FENE and FENE-P models are numerically integrated along a large number of Lagrangian trajectories resulting from a direct numerical simulation of three-dimensional homogeneous isotropic turbulence. Although the FENE-P model yields results in qualitative agreement with those of the FENE model, quantitative differences emerge. The steady-state probability of large extensions is overesti- mated by the FENE-P model. The alignment of polymers with the eigenvectors …
By tracking small particles in the bulk of an intensely turbulent flow, we show that even a very small concentration of long-chain polymers disrupts the usual turbulent energy cascade. The polymers affect scales much larger than their physical size, from the dissipation range to the inertial range. The effect depends strongly on the polymer concentration. While the dissipative-scale statistics change continuously as the polymer concentration is increased, the inertial-range energy transfer rate is only altered by the polymer additives when the concentration is above a threshold (approximately …
A small amount of polymer additives can cause substantial reduction in the energy dissipation and friction loss of turbulent flow. The problem of polymer-induced drag reduction has attracted continuous attention over the seven decades since its discovery. However, changes in research paradigm and perspectives have triggered a wave of new advancements in the past decade. This review attempts to bring researchers of all levels, from beginners to experts, to the forefront of this area. It starts with a comprehensive coverage of fundamental knowledge and classical findings and theories. It then hi…
Polymers in a turbulent flow are stretched out by the fluctuating velocity gradient; the stationary probability distribution function (p.d.f.) of extensions $R$ has a power-law tail with an exponent that increases with the Weissenberg number $Wi$, a nondimensional measure of polymer elasticity. This study addresses the following questions: (i) What is the role of the non-Gaussian statistics of the turbulent velocity gradient on polymer stretching? (ii) How does the p.d.f. of $R$ evolve to its asymptotic stationary form? Our analysis is based on simulations of the dynamics of finitely-extensibl…
Minute amount of long chain flexible polymer dissolved in a turbulent flow can drastically change flow properties, such as reducing the drag and enhancing mixing. One fundamental riddle is how these polymer additives interact with the eddies of different spatial scales existing in the turbulent flow and in turn alter the turbulence energy transfer. Here we show how turbulent kinetic energy is transferred through deferent scales in the presence of the polymer additives. In particular, we observed experimentally the emerging of a new scaling range, referred to as the elastic range, where increas…
We study properties of dilute polymer solutions which are known to depend strongly on polymer elongation. The probability density function (PDF) of polymer end-to-end extensions $R$ in turbulent flows is examined. We demonstrate that if the value of the Lyapunov exponent $λ$ is smaller than the inverse molecular relaxation time $1/τ$ then the PDF has a strong peak at the equilibrium size $R_0$ and a power tail at $R\gg R_0$. This confirms and extends the results of \cite{Lumley72}. There is no essential influence of polymers on the flow in the regime $λτ<1$. At $λ>1/τ$ the majority of molecule…
A polymer in a turbulent flow undergoes the coil-stretch transition when the Weissenberg number, i.e. the product of the Lyapunov exponent of the flow and the relaxation time of the polymer, surpasses a critical value. The effect of internal friction on the transition is studied by means of Brownian dynamics simulations of the elastic dumbbell model in a homogeneous and isotropic, incompressible, turbulent flow and analytical calculations for a stochastic velocity gradient. The results are explained by adapting the large deviations theory of Balkovsky et al. [Phys. Rev. Lett., 2000, 84, 4765] …
Measurements of heat transport, as expressed by the Nusselt number $Nu$, are reported for turbulent Rayleigh-Bénard convection of water containing up to 120 ppm by weight of poly-[ethylene oxide] with a molecular weight of $4\times10^6$ g/mole. Over the Rayleigh number range $ 5\times 10^9 \alt Ra \alt 7 \times 10^{10}$ $Nu$ is smaller than it is for pure water by up to 10%.
This paper is focused on the fundamental mechanism(s) of viscoelastic turbulence that lead to polymer induced turbulent drag reduction phenomenon. A great challenge in this problem is the computation of viscoelastic turbulent flows, since the understanding of polymer physics is restricted to mechanical models. An effective state-of-the-art numerical method to solve the governing equation for polymers modelled as non-linear springs, without using any artificial assumptions as usual, was implemented here for the first time on a three-dimensional channel flow geometry. The capability of this algo…
This letter confirms the existence of heat transfer enhancement (HTE) and reduction (HTR) in turbulent natural convection with polymer additives. HTE and HTR were numerically predicted by Benzi et al.(PRL, 104, 024502, 2010) in homogenous turbulent convection, but experiments by Ahlers & Nikolaenko(PRL, 104, 034503, 2010) in turbulent natural convection observed HTR only. Using direct numerical simulation of natural convection, the present study reconciles earlier numerical and experimental work on the basis of the dominant role of polymer length in the polymer dynamics in extensional flows.
The modification of dominant coherent structures that extend through the log-region of a drag reduced turbulent boundary layer is studied via examination of two-point correlations from time-resolved particle-image-velocimetry. Measurements were acquired in polymer oceans (uniform concentration) at drag reduction levels corresponding to the low drag reduction regime (< 40%), the high drag reduction (HDR) regime (>40%), and at an intermediate level (46%). The mean velocity profiles and two-point correlations were compared with that of water (Newtonian, DR = 0%). These results show that with incr…
We present an experimental investigation of turbulent drag reduction with flexible and rigid polymer solutions. The flexible polymer is partially hydrolyzed polyacrylamide (HPAM) and the rigid polymer is xanthan gum (XG). The experiments are carried out at low drag reduction ($\%DR < 40$), high drag reduction ($\%DR > 40$) and maximum drag reduction (where the velocity profile $U^+$ roughly matches Virk's asymptote). We compare velocity profiles, streamwise and wall-normal Reynolds stresses and power spectra of streamwise velocity fluctuations measured by Laser Doppler Anemometry (LDA). Our re…
We present direct numerical simulations of turbulent channel flow with passive Lagrangian polymers. To understand the polymer behavior we investigate the behavior of infinitesimal line elements and calculate the probability distribution function (PDF) of finite-time Lyapunov exponents and from them the corresponding Cramer's function for the channel flow. We study the statistics of polymer elongation for both the Oldroyd-B model (for Weissenberg number $\Wi <1$) and the FENE model. We use the location of the minima of the Cramer's function to define the Weissenberg number precisely such that w…
We report measurements of turbulent drag reduction of two different polyelectrolyte solutions: DNA and hydrolyzed Polyacrylamide. Changing the salt concentration in the solutions allows us to change the flexibility of the polymer chains. For both polymers the amount of drag reduction was found to increase with the flexibility. Rheological studies reveal that the elongational viscosity of the solutions increases simultaneously. Hence we conclude that the elongational viscosity is the pertinent macroscopic quantity to describe the ability of a polymer to cause turbulent drag reduction.
We present numerical studies of stretching of Hookean dumbbells in a turbulent Navier-Stokes flow with a linear mean profile, <u_x>=Sy. In addition to the turbulence features beyond the viscous Kolmogorov scale η, the dynamics at the equilibrium extension of the dumbbells significantly below eta is well resolved. The variation of the constant shear rate S causes a change of the turbulent velocity fluctuations on all scales and thus of the intensity of local stretching rate of the advecting flow. The latter is measured by the maximum Lyapunov exponent lambda_1 which is found to increase as λ_1 …
We address the phenomenon of drag reduction by dilute polymeric additive to turbulent flows, using Direct Numerical Simulations (DNS) of the FENE-P model of viscoelastic flows. It had been amply demonstrated that these model equations reproduce the phenomenon, but the results of DNS were not analyzed so far with the goal of interpreting the phenomenon. In order to construct a useful framework for the understanding of drag reduction we initiate in this paper an investigation of the most important modes that are sustained in the viscoelastic and Newtonian turbulent flows respectively. The modes …
We have performed direct numerical simulation of the turbulent flow of a polymer solution in a square duct, with the FENE-P model used to simulate the presence of polymers. First, a simulation at a fixed moderate Reynolds number is performed and its results compared with those of a Newtonian fluid to understand the mechanism of drag reduction and how the secondary motion, typical of the turbulent flow in non-axisymmetric ducts, is affected by polymer additives. Our study shows that the Prandtl's secondary flow is modified by the polymers: the circulation of the streamwise main vortices increas…
Drag reduction, or, what is the same, mean velocity increase in a turbulent flow at a fixed pressure drop through the addition of tiny amounts (several parts per million) of high molecular weight polymers (Thoms effect), is known already for more than sixty years. Rather long ago it was understood that this effect is related to supramolecular structures formed in the flow. Recent experiments by S. Chu, E.S.G. Shaqfeh and their associates, where the motion of supramolecular structures was directly observed, made it possible to understand and quantify the dynamic interaction of the polymeric str…
Injection of dilute polymer in a turbulent flow suppresses frictional drag. This challenging and technologically important problem remains primarily unresolved due to the complex nature of the flow. An important factor in the drag reduction is the energy transfer from the velocity field to the polymers. In this paper we quantify this process using energy fluxes, as well as show its universality in diverse flows such as magnetohydrodynamics, quasi-static magnetohydrodynamics, and bubbly turbulence. We show that in such flows, the transfer from kinetic energy to elastic energy leads to a reducti…
Polymer additives are commonly utilized to manipulate bubbly flows in various applications. Here, we investigate the effects of clean and contaminated bubbles driven upwards (upflow) in Newtonian and viscoelastic turbulent channel flows. Interface-resolved direct numerical simulations are performed to examine sole and combined effects of soluble surfactant and viscoelasticity using an efficient 3D finite-difference/front-tracking method. The incompressible flow equations are solved fully coupled with the FENE-P viscoelastic model and the equations governing interfacial and bulk surfactant conc…
We report experimental measurements of Lagrangian accelerations in the bulk of intense turbulent flows of dilute polymer solutions by following tracer particles with a high-speed optical tracking system. We observed a significant decrease in the acceleration variance in dilute polymer solutions. The shape of the normalized acceleration probability density functions, however, remain the same as in Newtonian water flows. We also observed an increase in the turbulent Lagrangian acceleration autocorrelation time in these dilute polymer solutions.
The role of polymers additives on the turbulent convective flow of a Rayleigh--Taylor system is investigated by means of direct numerical simulations (DNS) of Oldroyd-B viscoelastic model. The dynamics of polymers elongation follow adiabatically the self-similar evolution of the turbulent mixing layer, and shows the appearance of a strong feedback on the flow which originate a cut off for polymer elongations. The viscoelastic effects on the mixing properties of the flow are twofold. Mixing is appreciably enhanced at large scales (the mixing layer growth-rate is larger than that of the purely N…
Turbulence is one of the most fascinating phenomena in nature and one of the biggest challenges for modern physics. It is common knowledge that a flow of a simple, Newtonian fluid is likely to be turbulent, when velocity is high, viscosity is low and size of the tank is large\cite{Landau,Tritt}. Solutions of flexible long-chain polymers are known as visco-elastic fluids\cite{bird}. In our experiments we show, that flow of a polymer solution with large enough elasticity can become quite irregular even at low velocity, high viscosity and in a small tank. The fluid motion is excited in a broad ra…
We study the clustering properties of inertial particles in a turbulent viscoelastic fluid. The investigation is carried out by means of direct numerical simulations of turbulence in the Oldroyd-B model. The effects of polymers on the small scale properties of homogeneous turbulence are considered in relation with their consequences on clustering of particles, both lighter and heavier than the carrying fluid. We show that, depending on particle and flow parameters, polymers can either increase or decrease clustering.
How hydrodynamic interactions alter polymer stretching in turbulence
IITB-Monash Research Academy, Indian Institute of Technology Bombay（印度孟买理工学院-蒙纳士大学联合研究院）；Indian Institute of Technology Bombay（印度孟买理工学院）；Monash University（蒙纳士大学）；Université Côte d’Azur（蔚蓝海岸大学）
The upper bound of polymer drag reduction is identified as a unique transitional state between laminar and turbulent flow corresponding to the onset of the nonlinear breakdown of flow instabilities.
The drag of turbulent flows can be drastically decreased by addition of small amounts of high molecular weight polymers. While drag reduction initially increases with polymer concentration, it eventually saturates to what is known as the maximum drag reduction (MDR) asymptote; this asymptote is generally attributed to the dynamics being reduced to a marginal yet persistent state of subdued turbulent motion. Contrary to this accepted view we will show in the following that for an appropriate choice of parameters polymers can reduce the drag beyond the suggested asymptotic limit, eliminating tur…
In this review, we describe turbulent drag reduction in a variety of flows using a universal framework of energy flux. In a turbulent flow with dilute polymers and magnetic field, the kinetic energy injected at large scales cascades to the velocity field at intermediate scales, as well as to the polymers and magnetic field at all scales. Consequently, the kinetic energy flux, $ Π_u(k) $, is suppressed in comparison to the pure hydrodynamic turbulence. We argue that the suppression of $Π_u(k)$ is an important factor in the reduction of the inertial force $\langle {\bf u \cdot \nabla u} \rangle$…
The flow of fluids in channels, pipes or ducts, as in any other wall-bounded flow (like water along the hulls of ships or air on airplanes) is hindered by a drag, which increases many-folds when the fluid flow turns from laminar to turbulent. A major technological problem is how to reduce this drag in order to minimize the expense of transporting fluids like oil in pipelines, or to move ships in the ocean. It was discovered in the mid-twentieth century that minute concentrations of polymers can reduce the drag in turbulent flows by up to 80%. While experimental knowledge had accumulated over t…
We carry out a direct numerical simulation (DNS) study that reveals the effects of polymers on statistically steady, forced, homogeneous, isotropic fluid turbulence. We find clear manifestations of dissipation-reduction phenomena: On the addition of polymers to the turbulent fluid, we obtain a reduction in the energy dissipation rate, a significant modification of the fluid energy spectrum, especially in the deep-dissipation range, a suppression of small-scale intermittency, and a decrease in small-scale vorticity filaments. We also compare our results with recent experiments and earlier DNS s…
We present experimental and theoretical results addressing the Reynolds number (Re) dependence of drag reduction by sufficiently large concentrations of rod-like polymers in turbulent wall-bounded flows. It is shown that when Re is small the drag is {\em enhanced}. On the other hand when Re increases the drag is reduced and eventually the Maximal Drag Reduction (MDR) asymptote is attained. The theory is shown to be in excellent agreement with experiments, rationalizing and explaining all the universal and the non-universal aspects of drag reduction by rod-like polymers.
We show that viscoelastic plane Poiseuille flow becomes linearly unstable in the absence of inertia, in the limit of high elasticities, for ultra-dilute polymer solutions. While inertialess elastic instabilities have been predicted for curvilinear shear flows, this is the first ever report of a purely elastic linear instability in a rectilinear shear flow. The novel instability continues upto a Reynolds number ($Re$) of $O(1000)$, corresponding to the recently identified elasto-inertial turbulent state believed to underlie the maximum-drag-reduced regime. Thus, for highly elastic ultra-dilute …
Nontrivial steady flows have recently been found that capture the main structures of the turbulent buffer layer. We study the effects of polymer addition on these "exact coherent states" (ECS) in plane Couette flow. Despite the simplicity of the ECS flows, these effects closely mirror those observed experimentally: Structures shift to larger length scales, wall-normal fluctuations are suppressed while streamwise ones are enhanced, and drag is reduced. The mechanism underlying these effects is elucidated. These results suggest that the ECS are closely related to buffer layer turbulence.
We present numerical studies for finitely extensible nonlinear elastic (FENE) dumbbells which are dispersed in a turbulent plane shear flow at moderate Reynolds number. The polymer ensemble is described on the mesoscopic level by a set of stochastic ordinary differential equations with Brownian noise. The dynamics of the Newtonian solvent is determined by the Navier-Stokes equations. Momentum transfer of the dumbbells with the solvent is implemented by an additional volume forcing term in the Navier-Stokes equations, such that both components of the resulting viscoelastic fluid are connected b…
We show that simulations of polymer rheology at a fluctuating mesoscopic scale and at the macroscopic scale where flow instabilities occur can be achieved at the same time with dissipative particle dynamics (DPD) technique.} We model the visco-elasticity of polymer liquids by introducing a finite fraction of dumbbells in the standard DPD fluid. The stretching and tumbling statistics of these dumbbells is in agreement with what is known for isolated polymers in shear flows. At the same time, the model exhibits behaviour reminiscent of drag reduction in the turbulent state: as the polymer fracti…
Turbulent channel flow of drag-reducing polymer solutions is simulated in minimal flow geometries. Even in the Newtonian limit, we find intervals of "hibernating" turbulence that display many features of the universal maximum drag reduction (MDR) asymptote observed in polymer solutions: weak streamwise vortices, nearly nonexistent streamwise variations and a mean velocity gradient that quantitatively matches experiments. As viscoelasticity increases, the frequency of these intervals also increases, while the intervals themselves are unchanged, leading to flows that increasingly resemble MDR.
Coherent structures in Newtonian and viscoelastic turbulent planar jets
Okinawa Institute of Science and Technology Graduate University（冲绳科学技术大学院大学）；Universidad Polit{é}cnica de Madrid（马德里理工大学）；Flow Matters Consultancy BV（Flow Matters咨询有限公司）
Nonlinear traveling waves that are precursors to laminar-turbulent transition and capture the main structures of the turbulent buffer layer have recently been found to exist in all the canonical parallel flow geometries. We study the effect of polymer additives on these "exact coherent states" (ECS), in the plane Poiseuille geometry. Many key aspects of the turbulent drag reduction phenomenon are found, including: delay in transition to turbulence; drag reduction onset threshold; diameter and concentration effects. Furthermore, examination of the ECS existence region leads to a distinct predic…
Mechanical degradation of dilute solutions of polyethylene oxide (PEO) via chain scission was investigated within a turbulent pipe flow. Comparisons of the drag reduction performance with and without degradation were made by matching the onset of drag reduction conditions, which has been shown for PEO to be related to the mean molecular weight. The bulk flow behavior of both the degraded and non-degraded samples were generally consistent with trends observed in the literature, but a subset of conditions showed significant deviation in the slope increment (drag reduction performance) between th…
Using hybrid Direct Numerical Simulation with Langevin dynamics, a comparison is performed between polymer and fiber stress tensors in turbulent flow. The stress tensors are found to be similar, suggesting a common drag reducing mechanism in the onset regime for both flexible polymers and rigid fibers. Since fibers do not have an elastic backbone, this must be a viscous effect. Analysis of the viscosity tensor reveals that all terms are negligible, except the off-diagonal shear viscosity associated with rotation. Based on this analysis, we identify the rotational orientation time as the unifyi…
We investigate the effect of polymer additives on a two-dimensional Kolmogorov flow at very low Reynolds numbers by direct numerical simulations of the Oldroyd-B viscoelastic model. We find that above the elastic instability threshold the flow develops the elastic turbulence regime recently observed in experiments. We observe that both the turbulent drag and the Lyapunov exponent increase with Weissenberg, indicating the presence of a disordered, turbulent-like mixing flow. The energy spectrum develops a power-law scaling range with an exponent close to the experimental and theoretical expecta…
